We derive a general criterion for determining the onset of superradiant phase transition in electronic bands coupled to a cavity field, with possibly electron-electron interactions. For longitudinal superradiance in 2D or genuine 1D systems, we prove that it is always prevented, thereby extending existing no-go theorems. Instead, a superradiant phase transition can occur to a nonuniform transverse cavity field and we give specific examples in non-interacting models, either through Fermi surface nesting or parabolic band touching. Investigating the resulting time-reversal symmetry breaking superradiant states, we find in the former case Fermi surface lifting down to four Dirac points on a square lattice model, with topologically protected zero-modes, and in the latter case topological bands with non-zero Chern number on an hexagonal lattice.
Hybrid photonic-plasmonic nanostructures allow one to engineer coupling of quantum emitters and cavity modes accounting for the direct coherent and environment mediated dissipative pathways. Using generalized plasmonic Dicke model, we explore the non-equilibrium phase diagram with respect to these interactions. The analysis shows that their interplay results in the extension of the superradiant and regular lasing states to the dissipative coupling regime and an emergent lasing phase without population inversion having boundary with the superradiant and normal states. Calculated photon emission…
Bismuth-chalchogenides are model examples of three-dimensional topological insulators. Their ideal bulk-truncated surface hosts a single spin-helical surface state, which is the simplest possible surface electronic structure allowed by their non-trivial $\mathbb{Z}_2$ topology. They are therefore widely regarded ideal templates to realize the predicted exotic phenomena and applications of this topological surface state. However, real surfaces of such compounds, even if kept in ultra-high vacuum, rapidly develop a much more complex electronic structure whose origin and properties have proved co…
Spontaneous Symmetry Breaking of Cavity Vacuum and Emergent Gyrotropic Effects in Embedded moiré Superlattices
New Cornerstone Science Lab, Department of Physics, The University of Hong Kong（香港大学新Cornerstone科学实验室物理系）；HK Institute of Quantum Science & Technology, University of Hong Kong（香港大学香港量子科学与技术研究所）；Institute of Applied Physics and Materials Engineering, University of Macau（澳门大学应用物理与材料工程研究所）
We study the influence of the proximity-induced pairing on electronic version of the Dicke effect in a heterostructure, comprising three quantum dots vertically coupled between the metallic and superconducting leads. We discuss a feasible experimental procedure for detecting the narrow/broad (subradiant/superradiant) contributions by means of the subgap Andreev spectroscopy. In the Kondo regime and for small energy level detuning the Dicke effect is manifested in the differential conductance.
Different channels over which electrons scatter between parts of the Fermi surface are the key to various electronic quantum matters, such as superconductivity and density waves. We consider an effective model in higher dimensions where each of the two pockets in the original model maps to (the Landau levels of) two Dirac fermions. We discover an emergent channel when two Dirac fermions from different pairs annihilate, where the presence of a strong density wave is essential. We support our analysis with numerical calculations on model examples in the vicinity of ferromagnetic and antiferromag…
Visualizing Electronic Structure of Twisted Bilayer MoTe2 in Devices
University of Oxford（牛津大学）；University of Washington（华盛顿大学）；Lawrence Berkeley National Laboratory（劳伦斯伯克利国家实验室）；National Institute for Materials Science（国立材料研究所）
The effective low-energy excitations in a metallic or semimetallic crystalline system (i.e. electronic quasiparticles) always have a finite spatial extent. It is self-evident but virtually unexplored how the associated internal degrees of freedom manifest themselves in the quasiparticle response. Here, we investigate this question by illuminating an intimate connection between the theory of nonlinear response and the equations of motion of classical deformable bodies. This connection establishes that nth-order response in an external perturbation corresponds to nth-order derivatives of the qua…
Emergent electronic insulating states in a one-dimensional moiré superlattice
Zhejiang University（浙江大学）；The University of Osaka（大阪大学）；Dalian University（大连大学）；Inha University（仁荷大学）；National Institute for Materials Science (NIMS)（国立材料研究所）；Stony Brook University（石溪大学）
Twisted van der Waals bilayers provide an ideal platform to study the electron correlation in solids. Of particular interest is the 30 degree twisted bilayer honeycomb lattice system, which possesses an incommensurate Moire pattern and uncommon electronic behaviors may appear due to the absence of phase coherence. Such system is extremely sensitive to further twist and many intriguing phenomena will occur. In this work, we show that due to the twist induced spatial inhomogeneity of interlayer coupling, there emerges an U(1) gauge field in magnetic transition-metal dichalcogenides (TMD) bilayer…
Reports of emergent conductivity, superconductivity, and magnetism at oxide interfaces have helped to fuel intense interest in their rich physics and technological potential. Here we employ magnetic force microscopy to search for room-temperature magnetism in the well-studied LaAlO3/SrTiO3 system. Using electrical top gating to deplete electrons from the oxide interface, we directly observe an in-plane ferromagnetic phase with sharply defined domain walls. Itinerant electrons, introduced by a top gate, align antiferromagnetically with the magnetization, at first screening and then destabilizin…
Artifical superlattice (SL) potentials have been employed extensively for band structure engineering of two-dimensional (2D) Dirac electron gas in graphene. While such engineered electronic band structures can modify optical or plasmonic properties of graphene, an emergent polaritonic behavior beyond weak perturbative effects (e.g. anisotropic Drude weights) has not been reported. Here, we show that an extreme modulation of one-dimensional (1D) SL potentials in monolayer graphene deforms the underlying Dirac band dispersion and introduces ladder-like energy levels near the Fermi surface, which…
It is highly desirable to combine recent advances in the topological quantum phases with technologically relevant materials. Chromium dioxide (CrO2) is a half-metallic material, widely used in high-end data storage applications. Using first principles calculations, we show via interfacial orbital design that a novel class of half semi-metallic Dirac electronic phase emerges at the interface CrO2 with TiO2 in both thin film and superlattice configurations, with four spin-polarized Dirac points in momentum-space (k-space) band structure. When the spin and orbital degrees of freedom are allowed t…
The electronic band structure of iron pnictides exhibits four Dirac cones, which are due to crystal symmetry and orbital bonding orientation. This hallmark signature presents the pnictide family as an ideal candidate in the search for quasi-two-dimensional topological crystalline insulators. In this report, we explore interaction-induced topological phases which cannot be described by conventional local order parameters. Based on a model Hamiltonian our symmetry analysis shows that sponta- neous novel topological phases may be realized in compounds with tetragonal crystal field symmetry, where…
Scanning tunnelling microscopy and break-junction experiments realize metallic and molecular nanocontacts that act as ideal one-dimensional channels between macroscopic electrodes. Emergent nanoscale phenomena typical of these systems encompass structural, mechanical, electronic, transport, and magnetic properties. This Review focuses on the theoretical explanation of some of these properties obtained with the help of first-principles methods. By tracing parallel theoretical and experimental developments from the discovery of nanowire formation and conductance quantization in gold nanowires to…
We report on quantum capacitance measurements of high quality, graphite- and hexagonal boron nitride encapsulated Bernal stacked trilayer graphene devices. At zero applied magnetic field, we observe a number of electron density- and electrical displacement-tuned features in the electronic compressibility associated with changes in Fermi surface topology. At high displacement field and low density, strong trigonal warping gives rise to emergent Dirac gullies centered near the corners of the hexagonal Brillouin and related by three fold rotation symmetry. At low magnetic fields of $B=1.25$~T, th…
Relativistic spin-orbit interaction drastically modifies electronic band and endows emergent functionalities. One of the example is the Rashba effect. In noncentrosymmetric systems such as interface and polar materials, the electronic band is spin-splitted depending on the momentum direction owing to the spin-orbit interaction, which is useful for the electric manipulation of spin current. Similar relativistic band-modification is also emergent for spin wave (magnon) in magnetic materials. The asymmetric magnon band dispersion induced by the Dzyaloshinskii-Moriya interaction, which is antisymm…
The realization of equilibrium superradiant quantum phases (photon condensates) in a spatially-uniform quantum cavity field is forbidden by a "no-go" theorem stemming from gauge invariance. We here show that the no-go theorem does not apply to spatially-varying quantum cavity fields. We find a criterion for its occurrence that depends solely on the static, non-local orbital magnetic susceptibility $χ_{\rm orb}(q)$, of the electronic system (ES) evaluated at a cavity photon momentum $\hbar q$. Only 3DESs satisfying the Condon inequality $χ_{\rm orb}(q)>1/(4π)$ can harbor photon condensation. Fo…
