There is renewed interest in using the coherence between beams generated in separate down-converter sources for new applications in imaging, spectroscopy, microscopy and optical coherence tomography (OCT). These schemes make use of continuous wave (CW) pumping in the low parametric gain regime, which produces frequency correlations, and frequency entanglement, between signal-idler pairs generated in each single source. But can induced coherence still be observed if there is no frequency correlation, so the biphoton wavefunction is factorable? We will show that this is the case, and this might be an advantage for OCT applications. High axial resolution requires a large bandwidth. For CW pumping this requires the use of short nonlinear crystals. This is detrimental since short crystals generate small photon fluxes. We show that the use of ultrashort pump pulses allows improving axial resolution even for long crystal that produce higher photon fluxes.
In this work we study the spatio-temporal correlations of photons produced by spontaneous parametric down conversion. In particular, we study how the waists of the detection and pump beams impact on the spectral bandwidth of the photons. Our results indicate that this parameter is greatly affected by the spatial properties of the detection beam, while not as much by the pump beam. This allows for a simple experimental implementation to control the bandwidth of the biphoton spectra, which only entails modifying the optical configuration to collect the photons. Moreover, we have performed Hong-O…
In this work we present a simple method to reconstruct the complex spectral wavefunction of a biphoton, and hence gain complete information about the spectral and temporal properties of a photon pair. The technique, which relies on quantum interference, is applicable to biphoton states produced with a monochromatic pump when a shift of the pump frequency produces a shift in the relative frequencies contributing to the biphoton. We demonstrate an example of such a situation in type-II parametric down-conversion (SPDC) allowing arbitrary paraxial spatial pump and detection modes. Moreover, our t…
We consider a double Gaussian approximation to describe the wavefunction of twin photons (also called a biphoton) created in a nonlinear crystal via a type-I spontaneous parametric downconversion (SPDC) process. We find that the wavefunction develops a Gouy phase while it propagates, being dependent of the two-photon correlation through the Rayleigh length. We evaluate the covariance matrix and show that the logarithmic negativity, useful in quantifying entanglement in Gaussian states, although Rayleigh-dependent, does not depend on the propagation distance. In addition, we show that the two-p…
We describe spontaneous parametric down-conversion experiments in which induced coherence across two coupled interferometers results in high-visibility single-photon interference. Opening additional photon channels allows "which-path" information and reduces the visibility of the singlephoton interference, but results in nearly perfect visibility when photons are counted in coincidence. A simplified theoretical model accounts for these complementary observations and attributes them directly to the relations among the vacuum fields at the different crystals.
We theoretically propose a biphoton entanglement-enhanced multidimensional spectroscopic technique as a probe for the dissipative polariton dynamics in the ultrafast regime. It is applied to the cavity-confined monomeric photosynthetic complex that represents a prototypical multi-site excitonic quantum aggregate. The proposed technique is shown to be particularly sensitive to inter-manifold polariton coherence between the two and one-excitation subspaces. It is demonstrated to be able to monitor the dynamical role of cavity-mediated excitonic correlations, and dephasing in the presence of phon…
As a tutorial to the spatial aspects of Spontaneous Parametric Downconversion (SPDC), we present a detailed first-principles derivation of the transverse correlation width of photon pairs in degenerate collinear SPDC. This width defines the size of a biphoton birth zone, the region where the signal and idler photons are likely to be found when conditioning on the position of the destroyed pump photon. Along the way, we discuss the quantum-optical calculation of the amplitude for the SPDC process, as well as its simplified form for nearly collinear degenerate phase matching. Following this, we …
Coherence can be induced or stimulated in parametric down-conversion using two or three crystals when, for example, the idler modes of the crystals are aligned. Previous experiments with induced coherence [Phys. Rev. Lett. 114, 053601 (2015)] focused on which-path information and the role of vacuum fields in realizing complementarity via reduced visibility in single-photon interference. Here we describe experiments comparing induced and stimulated coherence. Different single-photon interference experiments were performed by blocking one of the pump beams in a three-crystal setup. Each counted …
The observation of the Hanbury Brown and Twiss (HBT) effect with thermal light marked the birth of quantum optics. All the thermal sources considered to date did not feature quantum signatures of light, as they consisted of independent emitters that emit uncorrelated photons. Here, we propose and demonstrate an incoherent light source based on phase-randomized spatially entangled photons, which we coin thermal biphotons. We show that in contrast to thermal light, the width of the HBT peak for thermal biphotons is determined by their correlations, leading to violation of the Siegert relation an…
We analyze the quantum-state purity of heralded single photons produced from frequency-anti-correlated biphotons. We find that the quantum-state purity in time-frequency domain depends strongly on the response time uncertainty of the trigger-photon detector that heralds the generation of its paired photon. If the trigger response time is much shorter than the two-photon coherence time, the time-frequency quantum-state purity of heralded single photons approaches unity and the heralded single photon is in a nearly pure state. If the trigger response time is much longer than the two-photon coher…
We investigate spontaneous four wave mixing (SFWM) in a single-channel side-coupled integrated spaced sequence of resonators (SCISSOR). Analytic expressions for the number of photon pairs generated, as well as the biphoton wave function (joint spectral amplitude) describing the pairs, are derived and numerically computed for different pump pulse durations and numbers of ring resonators. In the limit of a long input pump pulse, we show a strong analogy between super-linear scaling of generation efficiency with respect to the number of rings in the structure and Dicke superradiance. More general…
The spectral-temporal correlation and the correlation time of a biphoton wavepacket generated in the process of parametric down-conversion (PDC), is of great importance for a broad range of quantum experiments. We utilise an integrated PDC source to generate biphotons with different types of spectral-temporal correlations and probe their respective correlation times. The outcomes confirms that the correlation time is independent of the coherence time of the pump light, and it is only determined by the waveguide length and its dispersion properties. Furthermore, we investigate the properties of…
Interference of two beams produced at separate biphoton sources was first observed more than two decades ago. The phenomenon, often called "induced coherence without induced emission", has recently gained attention after its applications to imaging, spectroscopy, and measuring biphoton correlations have been discovered. The sources used in the corresponding experiments are nonlinear crystals pumped by laser light. The use of a laser pump makes the occurrence of induced (stimulated) emission unavoidable and the effect of stimulated emission can be observed in the joint detection rate of the two…
Quantum entanglement is an integral part of quantum optics and has been exploited in areas such as computation, cryptography and metrology. The entanglement between photons can be present in various degrees of freedom (DOFs), and even the simplest bi-partite systems can occupy a large Hilbert space. Therefore, it is desirable to exploit this multi-dimensional space for various quantum applications by fully controlling the properties of the entangled photons in multiple DOFs. While current entangled-photon sources are capable of generating entanglement in one or more DOFs, there is currently a …
We study the ground state properties of the one-dimensional extended Hubbard model at half-filling from the perspective of its particle reduced density matrix. We focus on the reduced density matrix of $2$ fermions and perform an analysis of its quantum correlations and coherence along the different phases of the model. Specifically, we study its (i) entanglement entropy, (ii) $\ell_1$ norm of coherence, (iii) irreducible two-body cumulant matrix and (iv) entanglement spectrum. Our results show that these different properties are complementary to each other depending on the phase of the system…
Many-body densities and correlation functions are of paramount importance for understanding quantum many-body physics. Here, we present a method to compute them; our approach is general and based on the action of bosonic or fermionic annihilation field operators on the many-body wavefunction. We analyze $N = 6$ quasi-one-dimensional harmonically-trapped bosons with weak to strong contact interaction strength up to the Tonks-Girardeau limit with infinite repulsion using the MultiConfigurational Time-Dependent Hartree method for indistinguishable particles (MCTDH-X). We compare our MCTDH-X solut…
Quantum coherent light-matter interactions have been at the forefront of scientific interest since the fundamental predictions of Einstein and the later work of Rabi. Direct observation of quantum coherent interactions entails probing the electronic wavefunction which requires that the electronic state of the matter does not de-phase during the measurement, a condition that can be satisfied by lengthening the coherence time or by shortening the observation time. The short de-phasing time in semiconductors has dictated that all coherent effects reported to date have been recorded directly only …
Engineering and studying few-electron states in ballistic conductors is a key step towards understanding entanglement in quantum electronic systems. In this Letter, we introduce the intrinsic two-electron coherence of an electronic source in quantum Hall edge channels and relate it to two-electron wavefunctions and to current noise in an Hanbury Brown--Twiss interferometer. Inspired by the analogy with photon quantum optics, we propose to measure the intrinsic two-electron coherence of a source using low-frequency current correlation measurements at the output of a Franson interferometer. To i…
Single-molecule sensitivity of nuclear magnetic resonance (NMR) and angstrom resolution of magnetic resonance imaging (MRI) are the highest challenges in magnetic microscopy. Recent development in dynamical-decoupling- (DD) enhanced diamond quantum sensing has enabled single-nucleus NMR and nanoscale NMR. Similar to conventional NMR and MRI, current DD-based quantum sensing utilizes the frequency fingerprints of target nuclear spins. The frequency fingerprints by their nature cannot resolve different nuclear spins that have the same noise frequency or differentiate different types of correlati…
In this article, we propose a method to realize the "delayed choice experiment" using ultra-cold atoms. Here we attempt to probe the "welcher-Weg" information without collapsing the wavefunction of the atom. This experiment consists of components built around proven techniques that are put together in novel configuration to preserve the coherence of the system during the measurement. The Ramsey interference is used to establish the wave nature of the atom and the particle nature of the atom is probed by detecting its internal state by performing a nondemolition measurement using an ultra-high …
Coherence-induced deep thermalization transition in random permutation quantum dynamics
National University of Singapore（新加坡国立大学）；The University of Texas at Austin（德克萨斯大学奥斯汀分校）；Centre for Quantum Technologies, National University of Singapore（新加坡国立大学量子技术中心）
This PhD thesis is dedicated to the study of the interplay between symmetries of quantum states and their self-similar properties. It consists of three connected threads of research: polynomial invariants for multiphoton states, visualization schemes for quantum many-body systems and a complex networks approach to quantum walks on a graph. First, we study the problem of which many-photon states are equivalent up to the action of passive linear optics. We prove that it can be converted into the problem of equivalence of two permutation-symmetric states, not necessarily restricted to the same op…
Frequency Detuning and Interference-Induced Bohmian Chaos in a Two-Dimensional Anisotropic Harmonic Oscillator
Centre of Foundation Studies in Science of Universiti Putra Malaysia (ASPutra), Universiti Putra Malaysia (UPM)（博特拉大学科学基础研究中心）；Institute for Mathematical Research (INSPEM) Universiti Putra Malaysia (UPM)（博特拉大学数学研究所）；Department of Physics, Faculty of Science, Universiti Putra Malaysia (UPM)（博特拉大学理学院物理系）；Department of Applied Physics, Faculty of Science and Technology Universiti Kebangsaan Malaysia (UKM)（马来西亚国立大学科技与理学院应用物理系）
