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arXiv 2004.09850cond-mat.str-el

二维准周期海森堡反铁磁体的光学观测

Optical observation of quasiperiodic Heisenberg antiferromagnets in two dimensions

Takashi Inoue, Shoji Yamamoto

AI总结:

本文通过Shastry-Shraiman拉曼散射理论计算二维彭罗斯晶格海森堡反铁磁体的磁拉曼光谱,利用不同偏振光分离各不可约表示,并揭示A2模式可直接探测自旋手性涨落,为双磁振子散射提供理论解释。

摘要:

我们计算了二维彭罗斯晶格上海森堡反铁磁体的磁拉曼光谱。我们遵循强关联哈伯德系统中拉曼散射的Shastry-Shraiman表述,得到了二阶和四阶有效拉曼算符。二阶拉曼强度来自E2模式,并且在偏振矢量任意旋转下保持不变。四阶拉曼强度包含A1和A2模式以及E2模式,因此表现出强烈的偏振依赖性。特别是,A2模式强度直接探测动力学自旋手性涨落。利用线偏振光和圆偏振光,我们可以从观测中分别提取每一个不可约表示。我们进一步讨论了磁振子-磁振子相互作用对磁拉曼散射的影响。我们的理论为双磁振子散射过程提供了合理的解释。

英文摘要:

We calculate magnetic Raman spectra of Heisenberg antiferromagnets on the two-dimensional Penrose lattice. We follow the Shastry-Shraiman formulation of Raman scattering in a strongly correlated Hubbard system and obtain the second- and fourth-order effective Raman operators. The second-order Raman intensity comes from the E2 mode, and it is invariant under an arbitrary rotation of polarization vectors. The fourth-order Raman intensities consist of A1 and A2, as well as E2, modes and therefore yield strong polarization dependence. In particular, the A2 mode intensity directly detects the dynamical spin-chirality fluctuations. Employing linearly and circularly polarized lights, we can separately extract every irreducible representation from the observations. We further discuss effects of magnon-magnon interactions on the magnetic Raman scattering. Our theory provides a reasonable explanation for the two-magnon scattering process.

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