On-chip realization of complex photonic functionalities is essential for further progress in planar integrated nanophotonics, especially when involving nonclassical light sources such as quantum emitters (QEs). Hybrid plasmonic nanocircuits integrated with QEs have been attracting considerable attention due to the prospects of significantly enhancing QE emission rates and miniaturizing quantum nanophotonic components. Spin-orbit interactions on subwavelength scales have been increasingly explored in both conventional and quantum nanophotonics for realization and utilization of the spin-dependent flow of light. Here, we propose and realize a dielectric-loaded plasmonic nanocircuit consisting of an achiral spin-orbit coupler for unidirectional routing of pump radiation into branched QE-integrated waveguides. We demonstrate experimentally the circular-polarization controlled coupling of 532-nm pump laser light into polymer-loaded branched waveguides followed by the excitation of spatially separated (by a distance of ~ 10 μm) QEs, nanodiamonds, with multiple nitrogen vacancy centres, that are embedded in and efficiently coupled to the corresponding waveguides. The realization of on-chip spin-orbit controlled excitation of different QEs coupled to branched waveguides opens new avenues for designing complex quantum plasmonic nanocircuits exploiting the spin degree of freedom within chiral quantum nanophotonics.
On-chip manipulating and controlling the temporal and spatial evolution of light is of crucial importance for information processing in future planar integrated nanophotonics. The spin and orbital angular momentum of light, which can be treated independently in classical macroscopic geometrical optics, appear to be coupled on subwavelength scales. We use spin-orbit interactions in a plasmonic achiral nano-coupler to unidirectionally excite surface plasmon polariton modes propagating in seamlessly integrated plasmonic slot waveguides. The spin-dependent flow of light in the proposed nanophotoni…
Plasmon resonant arrays or meta-surfaces shape both the incoming optical field and the local density of states for emission processes. They provide large regions of enhanced emission from emitters and greater design flexibility than single nanoantennas. This makes them of great interest for engineering optical absorption and emission. Here we study the coupling of a single quantum emitter, a self-assembled semiconductor quantum dot, to a plasmonic meta-surface. We investigate the influence of the spectral properties of the nanoantennas and the position of the emitter in the unit cell of the st…
Metal nanoantennas enable the manipulation of light emission and detection at the single photon level by confining light into very small volumes. Emitters coupled to these plasmonic structures are thus ideal candidates for usage in quantum information technology. However, controllably and reproducibly placing quantum emitters into nanocavities has been challenging due to the sizes of the systems involved. Here, we investigate the trapping dynamics of single emitters into nanocavities via optical gradient forces by using single-molecule super-resolution imaging and tracking. We show that molecu…
Realizing strong coupling between a single quantum emitter (QE) and an optical cavity is of crucial importance in the context of various quantum optical applications. While Rabi splitting of single quantum emitters coupled to high-Q diffraction limited cavities have been reported in numerous configurations, attaining single emitter Rabi splitting with a plasmonic nanostructure is still elusive. Here, we establish the analytical condition for strong coupling between a single QE and a plasmonic nanocavity and apply it to study various plasmonic arrangements that were shown to enable Rabi splitti…
Nanoscale pulsed light is highly desirable in nano-integrated optics. In this letter, we obtained femtosecond pulses with THz repetition frequency via the strong coupling between quantum emitters (QEs) and plasmonic resonators. Our structure consists of a V-groove (VG) plasmonic resonator and a nanowire embedded with two-level QEs. The influences of the incident light intensity and QE number density on the transmission response for this hybrid system are investigated through semi-classical theory and simulation. It is found that the transmission response can be modulated to the pulse form. The…
A new concept for second-harmonic generation (SHG) in an optical nanocircuit is proposed. We demonstrate both theoretically and experimentally that the symmetry of an optical mode alone is sufficient to allow SHG even in centro-symmetric structures made of centro-symmetric material. The concept is realized using a plasmonic two-wire transmission-line (TWTL), which simultaneously supports a symmetric and an anti-symmetric mode. We first confirm the generated second-harmonics belong only to the symmetric mode of the TWTL when fundamental excited modes are either purely symmetric or anti-symmetri…
Control of nonlinear response of nanostructures via path interference effects, i.e. Fano resonances, has been studied extensively. In such materials, a frequency conversion process which takes place near a hot spot has been considered. Here, we study a different case. The frequency conversion process takes place along the body of a nonlinear crystal. Metal nanoparticle-quantum emitter dimers control the down-conversion process, taking place throughout the crystal body, via introducing interfering conversion paths. Dimers behave as interaction centers. We show that a 2 order of magnitude enhanc…
Control of nonlinear response of nanostructures via path interference effects, i.e., Fano resonances, has been studied extensively. In such studies, a frequency conversion process takes place near a hot spot. Here, we study the case where the frequency conversion process takes place \textit{along the body of a nonlinear crystal}. Metal nanoparticle-quantum emitter dimers control the down-conversion process, taking place throughout the crystal body, via introducing interfering conversion paths. Dimers behave as interaction centers. We show that a 2 orders of magnitude enhancement is possible, o…
We investigate the impact of the dipole-active modes formed via the mode-mixing of the dipole mode with higher-order surface plasmon modes of a nanoegg on the radiative decay rate and quantum yield of an excited molecule near the nanoegg. The Purcell factor, rate of power dissipation by the emitter, antenna efficiency of the nanoegg, as well as quantum yield enhancement of the emitter, were studied using the quasistatic approximation and the semiclassical theory of radiation, following the Gersten-Nitzan and Ford-Weber approaches. Compared to the concentric nanoshell, we show that the dielectr…
The present work deals with a theoretical research on the emission and radiation properties of a dipole emitter source close to a dimer graphene plasmonic antenna. Modification of the radiation and the quantum efficiencies resulting from varying the position of the emitter and the orientation of its dipole moment are calculated by using a rigorous electromagnetic method based on Green's second identity. Large enhancements in the emission and the radiation of the emitter occur due to the coupling with the antenna surface plasmons in the spectral region from 4THz to 15THz. Our results show that …
Strong coupling of plasmonic excitations and dipolar emitters, such as organic molecules, have been studied extensively in the last years. The questions whether strong coupling can be achieved with a single molecule only and how this is unambiguously proven are still under debate. A critical issue of plasmonic in contrast to photonic systems is additional excitonic line broadening, which is often neglected when modeling such systems. This has led to too optimistic design predictions or incorrect interpretation of ambiguous experimental data, for example in models relying on Maxwell solvers wit…
Herein we report on our studies of radiative and non-radiative interaction between an individual quantum emitter and an anisotropic plasmonic nanostructure: a gold nanotriangle. Our theoretical and three-dimensional electromagnetic simulation studies highlight an interesting connection between: dipole-orientation of the quantum emitter, anisotropy of the plasmonic nanostructure and, radiative and non-radiative energy transfer processes between the emitter and the plasmonic geometry. For the out of plane orientation of quantum emitter, the total decay rate and non-radiative decay rate was found…
Single-emitter plasmonic patch antennas are room-temperature deterministic single photon sources, which exhibit highly accelerated and directed single photon emission. However, for efficient operation these structures require three-dimensional nanoscale deterministic control of emitter positioning within the device, which is a demanding task, esp. when emitter damage during fabrication is a major concern. To overcome this limitation, our deterministic room-temperature in situ optical lithography protocol uses spatially modulated light to position a plasmonic structure non-destructively on any …
Plasmonic waveguides are key elements in nanophotonic devices serving as optical interconnects between nanoscale light sources and detectors. Multimode operation in plasmonic two-wire transmission lines promises important degrees of freedom for near-field manipulation and information encoding. However, highly confined plasmon propagation in gold nanostructures is typically limited to the near-infrared region due to ohmic losses, excluding all visible quantum emitters from plasmonic circuitry. Here, we report on top-down fabrication of complex plasmonic nanostructures in single-crystalline silv…
Plasmonic antennas are attractive optical structures for many applications in nano and quantum technologies. By providing enhanced interaction between a nanoemitter and light, they efficiently accelerate and direct spontaneous emission. One challenge, however, is the precise nanoscale positioning of the emitter in the structure. Here we present a laser etching protocol that deterministically positions a single colloidal CdSe/CdS core/shell quantum dot emitter inside a subwavelength plasmonic patch antenna with three-dimensional nanoscale control. By exploiting the properties of metal-insulator…
Plasmonic waveguides offer the unique possibility to confine light far below the diffraction limit. Past room temperature experiments of single quantum emitters coupled to such waveguides have mainly focused on efficient channelling of the spontaneous emission into waveguide modes after a linear optical excitation. However, only the simultaneous interaction of the emitter with multiple plasmonic fields would lead to functionality in a plasmonic circuit. Here, we demonstrate the nonlinear optical interaction of a single molecule and propagating plasmons. An individual terrylene diimide (TDI) mo…
Strong coupling between a single quantum emitter and an electromagnetic mode is one of the key effects in quantum optics. In the cavity QED approach to plasmonics, strongly coupled systems are usually understood as single-transition emitters resonantly coupled to a single radiative plasmonic mode. However, plasmonic cavities also support non-radiative (or "dark") modes, which offer much higher coupling strengths. On the other hand, realistic quantum emitters often support multiple electronic transitions of various symmetry, which could overlap with higher order plasmonic transitions -- in the …
Plasmonic nano-objects have shown great potential in enhancing biological and chemical sensing, light harvesting and energy transfer, and optical and quantum computing to name a few. Therefore, an extensive effort has been vested in optimizing plasmonic systems and exploiting their field enhancement properties. Super-resolution imaging with quantum dots (QDs) is a promising method to probe plasmonic near-fields, but is hindered by the distortion of the emission intensity and radiation pattern. Here we investigate the interaction between QDs and 'L-shaped' gold nanoantennas, and demonstrate bot…
The collective spontaneous emission of two point-dipole emitters near a plasmonic core-shell nanosphere is theoretically investigated. Based on the expansion of mode functions in vector spherical harmonics, we derive closed analytical expressions for both the cooperative decay rate and the dipole-dipole interaction strength associated with two point dipoles close to a sphere. Considering a plasmonic nanoshell containing a linearly amplifying medium inside the core, the second-order correlation function for the two emitters shows that it is possible to tune the photon emission, selecting either…
The emerging field of plasmonics can lead to enhanced light matter interactions at extremely nanoscale regions. Plasmonic (metallic) devices promise to efficiently control both classical and quantum properties of light. Plasmonic waveguides are usually used to excite confined electromagnetic modes at the nanoscale that can strongly interact with matter. The analysis of these nanowaveguides exhibits similarities with their low frequency microwave counterparts. In this article, we review ways to study plasmonic nanostructures coupled to quantum optical emitters from a classical electromagnetic p…
We theoretically demonstrate the generation and radiation of coherent nanoplasmons powered by a single three-level quantum emitter on a plasmonic nanoresonator. By pumping the three-level emitter in a Raman configuration, we show a pathway to achieve macroscopic accumulation of nanoplasmons due to stimulated emission in the nanoresonator despite their fast relaxation. Thanks to the antenna effect of the nanoresonator, the system acts as an efficient and bright nanoscopic coherent light source with a photon emission rate of hundreds of Terahertz and could be realized with solid-state emitters a…
The modified radiative and non-radiative states due to the weak coupling of an emitter with other resonant objects (Purcell effect), can be recast as a quantum interference of the paths of the photon that define the classical scattering and absorption by the object. When the coupling is stronger, additional paths representing the (Rabi oscillations or) possible re-absorption of the photon from the excited object, by the emitter at ground-state, have to be included in the quantum interference. The effect of these additional Rabi paths of the photon on the radiative states and the efficiency of …
Optical cavities can enhance and control light-matter interactions. This has recently been extended to the nanoscale, and with single emitter strong coupling regime even at room temperature using plasmonic nano-cavities with deep sub-diffraction-limited mode volumes. However, with emitters in static nano-cavities, this limits the ability to tune coupling strength or to couple different emitters to the same cavity. Here, we present tip-enhanced strong coupling (TESC) spectroscopy, imaging, and control. Based on a nano-cavity formed between a scanning plasmonic antenna-tip and the substrate, by …
Hybrid plasmonic nanoemitters based on the combination of quantum dot emitters (QD) and plasmonic nanoantennas open up new perspectives in the control of light. However, precise positioning of any active medium at the nanoscale constitutes a challenge. Here, we report on the optimal overlap of antenna's near-field and active medium whose spatial distribution is controlled via a plasmon-triggered 2-photon polymerization of a photosensitive formulation containing QDs. Au nanoparticles of various geometries are considered. The response of these hybrid nano-emitters is shown to be highly sensitive…
