Optical frequency combs are one of the most remarkable inventions of the last decades. Originally conceived as the spectral counterpart of the train of short pulses emitted by mode-locked lasers, frequency combs have also been subsequently generated in continuously pumped microresonators, through third-order parametric processes. Quite recently, direct generation of optical frequency combs has been demonstrated in continuous-wave laser-pumped optical resonators with a second-order nonlinear medium inside. Here, we presents a concise introduction to such quadratic combs and the physical mechanism that underlies their formation. We mainly review our recent experimental and theoretical work on formation and dynamics of such quadratic frequency combs. We experimentally demonstrated comb generation in two configurations: a cavity for second harmonic generation, where combs are generated both around the pump frequency and its second harmonic, and a degenerate optical parametric oscillator, where combs are generated around the pump frequency and its sub-harmonic. The experiments have been supported by a thorough theoretical analysis, aimed at modelling the dynamics of quadratic combs, both in frequency and time domains, providing useful insights into the physics of this new class of optical frequency comb synthesizers. Quadratic combs establish a new class of efficient frequency comb synthesizers, with unique features, which could enable straightforward access to new spectral regions and stimulate novel applications.
Driven-dissipative kerr lattices with two-photon driving are experimentally relevant systems known to exhibit a symmetry-breaking phase transition, which belongs to the universality class of the thermal Ising model for the parameter regime studied here. In this work, we perform finite-size scaling of this system as it is quenched to the transition and the dynamical critical exponent is found to be compatible with $z\approx2.18$ corresponding with metropolis dynamics in classical simulations. Furthermore, we show that the Liouvillian gap scales with the same exponent, similar to scaling of the …
A gain-assisted plasmonic waveguide with two detuned resonators is investigated in the plasmon-induced transparency window. Phase map is employed to study power transmittance and group delay for varying gain coefficients and frequency detunings of the two resonators. The gain coefficient for lasing oscillation condition is analytically shown to vary quadratically with the frequency detuning. In the amplification regime below the lasing threshold, the spectrum implies not only large group delay, but also high transmittance and narrow linewidth. This is in contrast to those in the loss-compensat…
We show via numerical simulation that Kerr frequency combs can be generated in a nonlinear resonator characterized with normal group velocity dispersion (GVD). We find the spectral shape of the comb and temporal envelope of the corresponding optical pulses formed in the resonator.
Kerr soliton microcombs have recently emerged as a prominent topic in integrated photonics and enabled new horizons for optical frequency metrology. Kerr soliton microcombs, as its name suggests, are based on the high-order cubic optical nonlinearity. It is desirable to exploit quadratic photonic materials, namely Pockels materials, for soliton generation and on-chip implementation of 1f-2f comb self-referencing. Such quadratically-driven solitons have been theoretically proposed, but have not yet been observed in a nanophotonic platform despite of recent progresses in quadratic comb generatio…
We report on the experimental demonstration of a tunable monolithic optical frequency comb generator. The device is based on the four-wave mixing in a crystalline calcium fluoride whispering gallery mode resonator. The frequency spacing of the comb is given by an integer number of the free spectral range of the resonator. We select the desired number by tuning the pumping laser frequency with respect to the corresponding resonator mode. We also observe interacting optical combs and high-frequency hyperparametric oscillation, depending on the experimental conditions. A potential application of …
We propose a scheme for the generation of a robust stationary squeezed state of a mechanical resonator in a quadratically coupled optomechanical system, driven by a pulsed laser. The intracavity photon number presents periodic intense peaks suddenly stiffening the effective harmonic potential felt by the mechanical resonator. These "optical spring kicks" tend to squeeze the resonator position, and due to the interplay with fluctuation-dissipation processes one can generate a stationary state with more than 13 dB of squeezing even starting from moderately "pre-cooled" initial thermal states.
Nonlinear Kerr micro-resonators have enabled fundamental breakthroughs in the understanding of dissipative solitons, as well as in their application to optical frequency comb generation. However, the conversion efficiency of the pump power into a soliton frequency comb typically remains below a few percent. We introduce a hybrid Mach-Zehnder ring resonator geometry, consisting of a micro-ring resonator embedded in an additional cavity with twice the optical path length of the ring. The resulting interferometric back coupling enables to achieve an unprecedented control of the pump depletion: pu…
Optical frequency combs have recently been demonstrated in micro--resonators through nonlinear Kerr processes. Investigations in the past few years provided better understanding of micro--combs and showed that spectral span and mode locking are governed by cavity spectrum and dispersion. While various cavities provide unique advantages, dispersion engineering has been reported only for planar waveguides. In this Letter, we report a resonator design that combines dispersion control, mode crossing free spectrum, and ultra--high quality factor. We experimentally show that as the dispersion of a M…
Experiments and theoretical modeling yielded significant progress towards understanding of Kerr-effect induced optical frequency comb generation in microresonators. However, the simultaneous interaction of hundreds or thousands of optical comb frequencies with the same number of resonator modes leads to complicated nonlinear dynamics that are far from fully understood. An important prerequisite for modeling the comb formation process is the knowledge of phase and amplitude of the comb modes as well as the detuning from their respective microresonator modes. Here, we present comprehensive measu…
We experimentally study the factors that influence the span in frequency combs derived from the crystalline whispering gallery mode resonators. We observe that cavity dispersion plays an important role in generation of combs by cascaded four wave mixing process. We observed combs from the resonators with anomalous dispersion and nearly zero dispersion at the pump wavelength. In addition, the comb generation efficiency is found to be affected by the crossing of modes of different families. The influence of Raman gain is discussed as well as the role of cavity diameter and pump power. Copyright …
Aluminum nitride has been shown to possess both strong Kerr nonlinearity and electro-optic Pockels effect. By combining these two effects, here we demonstrate on-chip reversible on/off switching of the optical frequency comb generated by an aluminum nitride microring resonator. We optimize the design of gating electrodes and the underneath resonator structure to effectively apply electric field without increasing the optical loss. The switching of the comb is monitored by measuring one of the frequency comb peaks while varying the electric field. The controlled comb electro-optic response is i…
We show that scattering-based interaction among nearly degenerate optical modes is the key factor in low threshold generation of Kerr frequency combs in nonlinear optical resonators possessing small group velocity dispersion (GVD). The mode interaction is capable of producing drastic change in the local GVD, resulting in either a significant reduction or increase of the oscillation threshold. It is also responsible for the majority of observed combs in resonators characterized with large normal GVD. We present results of our numerical simulations as well as supporting experimental data.
We demonstrate a novel mode locked ultrafast laser, based on an integrated high-Q micr-oring resonator. Our scheme exhibits stable operation of two slightly shifted spectral optical comb replicas. It generates a highly monochromatic radiofrequency modulation of 60MHz on a 200GHz output pulse train, with a linewidth < 10kHz
The influence of Raman scattering and higher order dispersions on solitons and frequency comb generation in silica microring resonators is investigated. The Raman effect introduces a threshold value in the resonator quality factor above which the frequency locked solitons can not exist and, instead, a rich dynamics characterized by generation of self-frequency shift- ing solitons and dispersive waves is observed. A mechanism of broadening of the Cherenkov radiation through Hopf instability of the frequency locked solitons is also reported.
Aluminum nitride is an appealing nonlinear optical material for on-chip wavelength conversion. Here we report optical frequency comb generation from high quality factor aluminum nitride micro-ring resonators integrated on silicon substrates. By engineering the waveguide structure to achieve near-zero dispersion at telecommunication wavelengths and optimizing the phase matching for four-wave mixing, frequency combs are generated with a single wavelength continuous-wave pump laser. The Kerr coefficient (n2) of aluminum nitride is further extracted from our experimental results.
Much progress, both experimentally and theoretically, has recently been made towards optical frequency comb generation from continuously pumped second-order nonlinear systems. Here, we present the first observations towards finding an integrated solution for such a system, using a titanium indiffused lithium niobate waveguide resonator. These results are compared to recently developed theory for equivalent systems. The system is seen to exhibit strong instabilities, which require further investigation in order to fully determine the suitability of this platform for stable optical frequency com…
We develop a theory of optical frequency comb generation in ultra-compact Surface Nanoscale Axial Photonic (SNAP) bottle microresonators, employing the nonlinear interaction of whispering gallery modes which are confined along an optical fiber with nanoscale radius variation. We predict that a SNAP microresonator with a few-$μ$m radius can generate a frequency comb with an ultra-fine sub-GHz spectral spacing, which would require traditional ring resonators of $cm$ radius. We identify regimes of stable or quasi-periodic comb dynamics due to soliton excitation, and also show that special enginee…
We developed a frequency-domain model describing optical frequency-comb generation in optical resonators with second- and third-order nonlinearities. Compared with time-domain models, our model in principle allows one to express the cavity dispersion accurately, avoiding the dispersion being truncated beyond a certain order. Moreover, the frequency-domain model can readily include frequency dependence of system parameters, such as the linear absorption and the cavity coupling ratio. To demonstrate the validity of our model, we numerically simulated quadratic combs in a singly resonant second-h…
An optical comb is shown to arise from a whispering gallery mode resonator pumped by two optical frequencies. Two externally excited modes couple due to Kerr nonlinearity to initially empty modes and give rise to new frequency components. This thresholdles process is much more efficient than the previously reported single-pump four-wave mixing. As a result, a few milliwatt pump is sufficient to generate strong secondary fields, that efficiently generate higher-order frequency components and so on, in a cascade process leading to an optical comb.
We report a novel geometry for OPOs based on nonlinear microcavity resonators. This approach relies on a self-locked scheme that enables OPO emission without the need for thermal locking of the pump laser to the microcavity resonance. By exploiting a CMOS-compatible microring resonator, we achieve oscillation with a complete absence of shutting down, or self-terminating behavior, a very common occurrence in externally pumped OPOs. Further, this scheme consistently produces very wide bandwidth (>300nm, limited by our experimental set-up) combs that oscillate at a spacing of the FSR of the micro…
We demonstrate a photonic RF Hilbert transformer for broadband microwave in-phase and quadrature-phase generation based on an integrated frequency optical comb, generated using a nonlinear microring resonator based on a CMOS compatible, high-index contrast, doped-silica glass platform. The high quality and large frequency spacing of the comb enables filters with up to 20 taps, allowing us to demonstrate a quadrature filter with more than a 5-octave (3 dB) bandwidth and an almost uniform phase response.
We show that both the power and repetition rate of a frequency comb generated in a nonlinear ring resonator, pumped with continuous wave (cw) coherent light, are modulated. The modulation is brought about by the interaction of the cw background with optical pulses excited in the resonator, and occurs in resonators with nonzero high-order chromatic dispersion and wavelength-dependent quality factor. The modulation frequency corresponds to the detuning of the pump frequency from the eigenfrequency of the pumped mode in the resonator.
On-chip frequency comb generations enable compact broadband sources for spectroscopic sensing and precision spectroscopy. Recent microcomb studies focus on infrared spectral regime and have difficulty in accessing visible regime. Here, we demonstrate comb-like visible frequency line generation through second, third harmonic, and sum frequency conversion of a Kerr comb within a high Q aluminum nitride microring resonator pumped by a single telecom laser. The strong power enhancement, in conjunction with the unique combination of Pockels and Kerr optical nonlinearity of aluminum nitride, leads t…
Kerr nonlinearity based frequency combs and solitons have been generated from on-chip optical microresonators with high quality factors and global or local anomalous dispersion. However, fabrication of such resonators usually requires materials and/or processes that are not standard in semiconductor manufacturing facilities. Moreover, in certain frequency regimes such as visible and ultra-violet, the large normal material dispersion makes it extremely difficult to achieve anomalous dispersion. Here we present a concentric racetrack-shaped resonator that achieves anomalous dispersion in a 300 n…
We establish an exact partial differential equation to model Kerr comb generation in whispering-gallery mode resonators. This equation is a variant of the Lugiato-Lefever equation that includes higher-order dispersion and nonlinearity. This spatio-temporal model, whose main variable is the total intracavity field, is significantly more suitable than the modal expansion approach for the theoretical understanding and the numerical simulation of wide-span combs. It allows us to explore pulse formation in which a large number of modes interact cooperatively. This versatile approach can be straight…
Microcombs -- optical frequency combs generated in coherently-driven nonlinear microresonators -- have attracted significant attention over the last decade. The ability to generate two such combs in a single resonator device has in particular enabled a host of applications from spectroscopy to imaging. Concurrently, novel comb generation techniques such as synchronous pulsed driving have been developed to enhance the efficiency and flexibility of microcomb generation. Here we report on the first experimental demonstration of dual-microcomb generation via synchronous pulsed pumping of a single …
Deformed square resonators with the flat sides replaced by circular sides are proposed and demonstrated to enhance mode Q factors and adjust transverse mode intervals using the regular ray dynamic analysis and numerical simulations. Dual-transverse-mode emissions due to the ultrahigh-Q factors with different wavelength intervals are realized experimentally for AlGaInAs/InP circular-side square microlasers, and the stationary condition of the dual-mode emission is satisfied because the high-Q confined modes have totally different mode numbers. Furthermore, optical frequency combs are generated …
Direct optical frequency Comb Spectroscopy (DCS) is proving to be a fundamental tool in many areas of science and technology thanks to its unique performance in terms of ultra-broadband, high-speed detection and frequency accuracy, allowing for high-fidelity mapping of atomic and molecular energy structure. Here we present a novel DCS approach based on a scanning Fabry-Perot micro-cavity resonator (SMART) providing a simple, compact and accurate method to resolve the mode structure of an optical frequency comb. The SMART approach, while drastically reducing system complexity, allows for a stra…
Optical whispering gallery mode (WGM) resonators have been very attracting platforms for versatile Kerr frequency comb generations. We report a systematic study on the material dispersion of various optical materials that are capable of supporting quality factors above $10^9$. Using an analytical approximation of WGM resonant frequencies in disk resonators, we investigate the effect of the geometry and transverse mode order on the total group-velocity dispersion ($GVD$). We demonstrate that the major radii and the radial mode indices play an important role in tailoring the $GVD$ of WGM resonat…
Starting from the infinite-dimensional Ikeda map, we derive an extended temporal Lugiato-Lefever equation that may account for the effects of the conjugate electromagnetic fields (also called `negative frequency fields'). In the presence of nonlinearity in a ring cavity, these fields lead to new forms of modulational instability and resonant radiations. Numerical simulations based on the new extended Lugiato-Lefever model show that the negative-frequency resonant radiations emitted by ultrashort cavity solitons can impact Kerr frequency comb formation in externally pumped temporal optical cavi…
Kerr microresonators driven in the normal dispersion regime typically require the presence of localized dispersion perturbations, such as those induced by avoided mode crossings, to initiate the formation of optical frequency combs. In this work, we experimentally demonstrate that this requirement can be lifted by driving the resonator with a pulsed pump source. We also show that controlling the desynchronization between the pump repetition rate and the cavity free-spectral range (FSR) provides a simple mechanism to tune the center frequency of the output comb. Using a fiber mini-resonator wit…
Frequency comb generation in microresonators at visible wavelengths has found applications in a variety of areas such as metrology, sensing, and imaging. To achieve Kerr combs based on four-wave mixing in a microresonator, dispersion must be in the anomalous regime. In this work, we demonstrate dispersion engineering in a microbubble resonator (MBR) fabricated by a two-CO$_2$ laser beam technique. By decreasing the wall thickness of the MBR down to 1.4 $μ$m, the zero dispersion wavelength shifts to values shorter than 764 nm, making phase matching possible around 765 nm. With the optical \text…
Photonic integrated circuits that exploit nonlinear optics in order to generate and process signals all-optically have achieved performance far superior to that possible electronically - particularly with respect to speed. We review the recent achievements based in new CMOS-compatible platforms that are better suited than SOI for nonlinear optics, focusing on radio frequency (RF) and microwave based applications that exploit micro-resonator based frequency combs. We highlight their potential as well as the challenges to achieving practical solutions for many key applications. These material sy…
We demonstrate that whispering gallery mode resonators can be utilized to generate optical frequency combs based on four wave mixing process at virtually any frequency that lies in the transparency window of the resonator host material. We show theoretically how the morphology of the resonator can be engineered to produce a family of spectrally equidistant modes with anomalous group velocity dispersion appropriate for the comb generation. We present experimental results for a frequency comb centered at 794 nm to support our theoretical findings.
The eigenmodes of unstable canonical optical resonators possess fractal structure in their transverse intensity cross-sections [Karman et al., Nature 402, 138 (1999)]. In one particular plane, the magnified self-conjugate plane, this structure can be explained in terms of a combination of imaging and diffraction [Courtial and Padgett, PRL 85, 5320 (2000)]. Here we show that this combination of imaging and diffraction simultaneously occurs in the longitudinal direction, resulting in three-dimensional self-similar fractal structure around the centre of the magnified self-conjugate plane.
A necessary condition for generation of bright soliton Kerr frequency combs in microresonators is to achieve anomalous group velocity dispersion (GVD) for the resonator modes. This condition is hard to implement in visible as well as ultraviolet since the majority of optical materials are characterized with large normal GVD in these wavelength regions. We overcome this challenge by borrowing ideas from strongly dispersive coupled systems in solid state physics and optics. We show that photonic compound ring resonators can possess large anomalous GVD at any desirable wavelength, even if each in…
An external-cavity diode laser is reported with ultralow noise, high power coupled to a fiber, and fast tunability. These characteristics enable the generation of an optical frequency comb in a silica micro-resonator with a single-soliton state. Neither an optical modulator nor an amplifier was used in the experiment. This demonstration greatly simplifies the soliton generation setup and represents a significant step forward to a fully integrated soliton comb system.
Using the Lugiato-Lefever model, we analyze the effects of third order chromatic dispersion on the existence and stability of dark and bright soliton Kerr frequency combs in the normal dispersion regime. While in the absence of third order dispersion only dark solitons exist over an extended parameter range, we find that third order dispersion allows for stable dark and bright solitons to coexist. Reversibility is broken and the shape of the switching waves connecting the top and bottom homogeneous solutions is modified. Bright solitons come into existence thanks to the generation of oscillati…
We experimentally demonstrate stimulated four-wave mixing in two linearly uncoupled integrated Si$_3$N$_4$ micro-resonators. In our structure the resonance combs of each resonator can be tuned independently, with the energy transfer from one resonator to the other occurring in the presence of a nonlinear interaction. This method allows flexible and efficient on-chip control of the nonlinear interaction, and is readily applicable to other third-order nonlinear phenomena.
We report on realization of an efficient triply-resonant coupling between two long lived optical modes and a high frequency surface acoustic wave (SAW) mode of the same monolithic crystalline whispering gallery mode resonator. The coupling results in an opto-mechanical oscillation and generation of a monochromatic SAW. A strong nonlinear interaction of this mechanical mode with other equidistant SAW modes leads to mechanical hyper-parametric oscillation and generation of a SAW pulse train and associated frequency comb in the resonator. We visualized the comb observing the modulation of the mod…
Optical frequency combs (OFCs) at Mid-Infrared (MIR) wavelengths are essential for applications in precise spectroscopy, gas sensing and molecular fingerprinting, because of its revolutionary precision in both wavelength and frequency domain. The microresonator-based OFCs make a further step towards practical applications by including such high precision in a compact and cost-effective package. However, dispersion engineering is still a challenge for the conventional chi-3 micro-ring resonators and a MIR pump laser is required. Here we develop a different platform of a chi-2 optical superlatti…
A systematic dispersion engineering approach is presented toward designing a III-Nitride micro-resonator for a blue/UV frequency comb. The motivation for this endeavor is to fill the need for compact, coherent, multi-wavelength photon sources that can be paired with, e.g., the $^{171}{\textrm{Yb}}^{+}$ ion in a photonic integrated chip for optical sensing, time-keeping, and quantum computing applications. The challenge is to overcome the normal material dispersion exhibited by the otherwise ideal i.e., low-loss and large-Kerr-coefficient) AlGaN family of materials, as this is a prerequisite fo…
We present a technique to improve the slow-light performance of a side-coupled spaced sequence of resonators (SCISSOR) combined with a stimulated Brillouin scattering (SBS) gain medium in optical fiber. We evaluate device performance of SCISSOR-only and SCISSOR + SBS systems for different numbers of cascaded resonators from 1 to 70 using two different data fidelity metrics including eye-opening and mutual information. A practical system design is demonstrated by analyzing its performance in terms of fractional delay, power transmission, and data fidelity. We observe that the results from the t…
A novel zero-order resonator has been designed by an optical surface transformation (OST) method. The resonator proposed here has many novel features. Firstly, the mode volume can be very small (e.g. in the subwavelength scale). Secondly, the resonator is open (no reflecting walls are utilized) and resonant effects can be found in a continuous spectrum (i.e. a continuum of eigenmodes). Thirdly, we only need one homogenous medium to realize the proposed resonator. The shape of the resonator can be a ring structure of arbitrary shape. In addition to the natural applications (e.g. optical storage…
Optical frequency combs generated in normally dispersive Kerr microresonators have been observed to correspond to dark temporal structures, and theoretically explained as interlocked switching waves (also known as domain walls or fronts). The time-domain dynamics that underpin the formation of this type of frequency combs has however so far eluded direct experimental observation. Here we use a closely related system - a synchronously driven optical fibre ring resonator - to experimentally study the dynamics of deterministically excited switching waves. We measure the switching wave velocities …
Mode interaction in silicon nitride micro-resonators is investigated. We provide clear experimental evidence of mode interaction between two family modes and mode interaction is demonstrated to be the cause of the comb generation in resonators with normal dispersion.
Cavity opto-mechanics enabled radiation-pressure coupling between optical and mechanical modes of a micro-mechanical resonator gives rise to dynamical backaction, enabling amplification and cooling of mechanical motion. Due to a combination of large mechanical oscillations and necessary saturation of amplification, the noise floor of the opto-mechanical resonator increases, rendering it ineffective at transducing small signals, and thereby cooling another mechanical resonance of the system. Here we show amplification of one mechanical resonance in a micro-mechanical ring resonator while simult…
We demonstrate the elements of a coupled-resonator optical waveguide in a side-coupled Fabry-Pérot configuration, and show that the coupling rate between adjacent waveguides can be widely tuned through the thermo-optic effect. The device is linearly scalable and can be combined with other integrated devices, with applications as an optical delay line or as a key element in a cavity-QED based quantum simulator.
We derive a general theory of linear coupling and Kerr nonlinear coupling between modes of dielectric optical resonators from first principles. The treatment is not specific to a particular geometry or choice of mode basis, and can therefore be used as a foundation for describing any phenomenon resulting from any combination of linear coupling, scattering and Kerr nonlinearity, such as bending and surface roughness losses, geometric backscattering, self- and cross-phase modulation, four-wave mixing, third-harmonic generation and Kerr frequency comb generation. The theory is then applied to a t…
We are reporting that the Lugiato-Lefever equation describing the frequency comb generation in ring resonators with the localized pump and loss terms also describes the simultaneous nonlinear resonances leading to the multistability of nonlinear modes and coexisting solitons that are associated with the spectrally distinct frequency combs.
On-chip optical resonators have the promise of revolutionizing numerous fields including metrology and sensing; however, their optical losses have always lagged behind their larger discrete resonator counterparts based on crystalline materials and flowable glass. Silicon nitride (Si3N4) ring resonators open up capabilities for optical routing, frequency comb generation, optical clocks and high precision sensing on an integrated platform. However, simultaneously achieving high quality factor and high confinement in Si3N4 (critical for nonlinear processes for example) remains a challenge. Here, …
