Large water Cherenkov detectors have been successfully used for decades in high- and low-energy particle physics. Nevertheless, detecting neutrons remains a challenge for such detectors since a neutron capture on a hydrogen atom doesn't release a sufficient amount of gamma energy to be observed efficiently. The use of gadolinium in the form of soluble salts has been explored extensively to remedy this issue, as gadolinium exhibits both a very large neutron capture cross section and a subsequent high-energy gamma cascade. However, in order for large gadolinium-loaded detectors to operate stably over long time periods, water optical transparency must be maintained by in situ purification. New methods have been developed involving band-pass molecular filtering. While these methods are very successful, they are expensive and consume considerable power and space as they seek to minimize loss of gadolinium while removing other impurities. For smaller detectors where some gadolinium loss can be tolerated, a less expensive way to do this is very desirable. In this paper, we describe the design, development and testing of a system used to purify the gadolinium-loaded water in the 26-ton ANNIE neutrino detector.
We report on the production and characterization of liquid scintillators for the detection of electron antineutrinos by the Daya Bay Reactor Neutrino Experiment. One hundred eighty-five tons of gadolinium-loaded (0.1% by mass) liquid scintillator (Gd-LS) and two hundred tons of unloaded liquid scintillator (LS) were successfully produced from a linear-alkylbenzene (LAB) solvent in six months. The scintillator properties, the production and purification systems, and the quality assurance and control (QA/QC) procedures are described.
In this study, simulation-based design and optimization studies of a gadolinium loaded segmented plastic scintillator detector are presented for monitoring applications of nuclear reactors in Turkey using antineutrinos. For the first time in the literature, a multivariate analysis technique is introduced to suppress cosmic background for such a reactor antineutrino detector.
Monitoring of high energy cosmic ray neutrons is of particular interest for cosmic ray water Cherenkov detectors as intense bundles of delayed neutrons have been found to arrive after the initial passage of a high energy air shower. In this paper we explore the possibility of building large-area high-energy neutron monitors using gadolinium-loaded Water Cherenkov Detectors (WCDs). GEANT4 simulations of photon production in WCDs are used to estimate the maximum detection efficiency for a hypothetical system. Requiring a series of neutron induced gamma ray flashes distributed over an extended pe…
The new Super-Kamiokande-Gadolinium (SK-Gd) project is an upgrade of the Super-Kamiokande (SK) detector. In the SK-Gd project, 0.2\% Gd$_2$(SO$_4$)$_3$ is loaded into the 50 kton water tank of the SK. One of the main purposes of the project is to discover Supernova Relic Neutrinos. Neutrino measurements and proton decay searches will also be performed in the SK-Gd. In order to measure solar neutrinos with a low energy threshold of $\sim$3.5 MeV in the SK-Gd, the main radioactive contaminations, $^{238}$U and $^{232}$Th, in Gd$_2$(SO$_4$)$_3{\cdot}$8H$_2$O, should be minimized before loading. O…
Scintillator doped with a high neutron-capture cross-section material can be used to detect neutrons via their resulting gamma rays. Examples of such detectors using liquid scintillator have been successfully used in high-energy physics experiments. However, a liquid scintillator can leak and is not as amenable to modular or complex shapes as a solid scintillator. Polystyrene-based scintillators from a variety of gadolinium compounds with varying concentrations were polymerized in our laboratory. The light output, emission spectra, and attenuation length of our samples were measured and light …
A new experiment, which is called as NEOS (NEutrino Oscillation at Short baseline), is proposed on the site of Hanbit reactors at Yonggwang, South Korea, to investigate a reactor antineutrino anomaly. A homogeneous NEOS detector having a 1000-L target volume has been constructed and deployed at the tendon gallery ~25 m away from the reactor core. A linear alkylbenzene (LAB) is used as a main base solvent of the NEOS detector. Furthermore, a di-isopropylnaphthalene (DIN) is added to improve the light output and pulse shape discrimination (PSD) ability. The ratio of LAB to DIN is 90:10. PPO (3 g…
Antineutrino detectors are practical, non-intrusive tools capable of remotely monitoring the activity of nuclear reactors. Here we explore the sensitivity of the Super-Kamiokande water-Cherenkov detector, following gadolinium loading, to antineutrinos from a nuclear reactor complex at a distance of approximately 190 km. The livetimes required to observe the two currently operating cores in the reactor complex depend on the activity of other reactors in the vicinity, as well as on estimates of detection efficiency and background rates. Under reasonable assumptions, we find that gadolinium-loade…
Demand to use gadolinium (Gd) in detectors is increasing in the field of elementary particle physics, especially neutrino measurements and dark matter searches. Large amounts of Gd are used in these experiments. Therefore, to access the impacts of Gd onto the environments, it is becoming important to measure the baseline concentrations of Gd in the environments. The measurement of the baseline concentrations, however, is not easy due to interferences by other elements. In this paper, a method for measuring the concentrations of rare earth elements including Gd is proposed. In the method, an in…
We report on the design and performance of the LUX-ZEPLIN (LZ) "Screener", a small liquid scintillator detector consisting of $\approx 23$ kg of LAB-based gadolinium-loaded liquid scintillator (GdLS) to be used in the LZ Outer Detector. The Outer Detector will be filled with 17.3 tonnes of GdLS and will surround the central liquid xenon time projection chamber of LZ. Its primary function will be to veto neutron single-scatter events in the liquid xenon which could mimic a WIMP dark matter signal. To meet the requirements for the Outer Detector, the radioimpurity levels in the GdLS must be kept…
Chemical extraction using a molecular recognition resin named "Empore Radium Rad Disk" was developed to improve sensitivity for the low concentration of radium (Ra). Compared with the previous method, the extraction process speed was improved by a factor of three and the recovery rate for $^{226}$Ra was also improved from 81$\pm$4% to $>$99.9%. The sensitivity on the 10$^{-1}$ mBq level was achieved using a high purity germanium detector. This improved method was applied to determine $^{226}$Ra in Gd$_2$(SO$_4$)$_3{\cdot}$8H$_2$O which will be used in the Super-Kamiokande Gadolinium project. T…
High-purity germanium (HPGe) detectors are widely used for the measurement of the low concentrated radioactivities. For the Super-Kamiokande-Gadolinium project, the concentration of radium in Gd$_2$(SO$_4$)$_3{\cdot}$8H$_2$O is determined by using HPGe detectors. The amount of the sample is generally limited by the size of the sample space of a HPGe detector. This leads the limitation of the detector efficiency. A new method of chemical extraction using the molecular recognition resin was developed to minimize this problem. Using the developed method, radium could be extracted from Gd$_2$(SO$_…
Over the course of several decades, organic liquid scintillators have formed the basis for successful neutrino detectors. Gadolinium-loaded liquid scintillators provide efficient background suppression for electron antineutrino detection at nuclear reactor plants. In the Double Chooz reactor antineutrino experiment, a newly developed beta-diketonate gadolinium-loaded scintillator is utilized for the first time. Its large scale production and characterization are described. A new, light yield matched metal-free companion scintillator is presented. Both organic liquids comprise the target and "G…
The STEREO experiment measures the electron antineutrino spectrum emitted in a research reactor using the inverse beta decay reaction on H nuclei in a gadolinium loaded liquid scintillator. The detection is based on a signal coincidence of a prompt positron and a delayed neutron capture event. The simulated response of the neutron capture on gadolinium is crucial for the comparison with data, in particular in the case of the detection efficiency. Among all stable isotopes, $^{155}$Gd and $^{157}$Gd have the highest cross sections for thermal neutron capture. The excited nuclei after the neutro…
The Accelerator Neutrino Neutron Interaction Experiment (ANNIE) is designed to serve as a test bed for new detector technologies in future water and liquid scintillator based neutrino experiments. Located on the Booster Neutrino Beam at Fermilab, ANNIE will be the first gadolinium-loaded water Cherenkov detector on a neutrino beam and will provide high statistics measurements of neutron yields from neutrino interactions in water. It is also the first particle physics application of the new photosensor technology: Large Area Picosecond Photodetectors (LAPPDs). With single photon time resolution…
Neutron multiplicity measurement in muon capture on oxygen nuclei in the Gd-loaded Super-Kamiokande detector
Kamioka Observatory, Institute for Cosmic Ray Research, University of Tokyo（东京大学宇宙线研究所神冈观测站）；Kavli Institute for the Physics and Mathematics of the Universe (WPI), The University of Tokyo Institutes for Advanced Study, University of Tokyo（东京大学前沿研究机构宇宙物理与数学研究 Kavli 研究所（WPI））
Design and development of optical modules for the BUTTON-30 detector
University of Edinburgh（爱丁堡大学）；University of Michigan（密歇根大学）；Lawrence Livermore National Laboratory（劳伦斯利弗莫尔国家实验室）；University of Pennsylvania（宾夕法尼亚大学）；University of Warwick（华威大学）；University of Liverpool（利物浦大学）；United Kingdom National Nuclear Laboratory（英国国家核实验室）；University of Sheffield（谢菲尔德大学）；STFC（科学与技术设施委员会）；Brookhaven National Laboratory（布鲁克海文国家实验室）；University of Florida（佛罗里达大学）
In order to improve Super-Kamiokande's neutron detection efficiency and to thereby increase its sensitivity to the diffuse supernova neutrino background flux, 13 tons of $\rm Gd_2(\rm SO_4)_3\cdot \rm 8H_2O$ (gadolinium sulfate octahydrate) was dissolved into the detector's otherwise ultrapure water from July 14 to August 17, 2020, marking the start of the SK-Gd phase of operations. During the loading, water was continuously recirculated at a rate of 60 m$^3$/h, extracting water from the top of the detector and mixing it with concentrated $\rm Gd_2(\rm SO_4)_3\cdot \rm 8H_2O$ solution to creat…
