Photon absorption in a semiconductor produces bright excitons that recombine very fast into photons. We here show that in a quantum dot set close to a p-doped reservoir, this absorption can produce a dark duo, i.e., an electron-hole pair that does not emit light. This unexpected effect relies on the fact that the wave function for a hole leaks out of a finite-barrier dot less than for electron. This difference can render the positively charged trio unstable in the dot by tuning the applied bias voltage in a field-effect device. The unstable trio that would result from photon absorption in a positively charged dot, has to eject one of its two holes. The remaining duo can be made dark with a probability close to 100% after a few pumping cycles with linearly polarized photons, in this way engineering long-lived initial states for quantum information processing.
Semiconductor quantum dots are considered to be the leading venue for fabricating on-demand sources of single photons. However, the generation of long-lived dark excitons imposes significant limits on the efficiency of these sources. We demonstrate a technique that optically pumps the dark exciton population and converts it to a bright exciton population, using intermediate excited biexciton states. We show experimentally that our method considerably reduces the DE population while doubling the triggered bright exciton emission, approaching thereby near-unit fidelity of quantum dot depletion.
In a recent experiment [A. Donarini et al., Nat Comms 10, 381 (2019)], electronic transport through a carbon nanotube quantum dot was observed to be suppressed by the formation of a quantum-coherent ``dark state''. In this paper we consider theoretically the counting statistics and waiting-time distribution of this dark-state-limited transport. We show that the statistics are characterised by giant super-Poissonian Fano factors and long-tailed waiting-time distributions, both of which are signatures of the bistability and extreme electron bunching caused by the dark state.
We present a phenomenological model to consider the effect of shape symmetry breaking on the optical properties of self-assembled quantum dots. We compare between quantum dots with two-fold rotational and two reflections ($C_{2v}$) symmetry and quantum dots in which this symmetry is reduced by perturbation to one reflection only ($C_{s}$). We show that this symmetry reduction drastically affects the optical activity of the dark exciton. In symmetric quantum dots, one of the dark exciton eigenstate is totally dark and the other, due to heavy- and light-hole mixing, has a small dipole moment pol…
Formation of excitonic states in quantum dots of nitride based III-V semiconductors GaN and AlN including coulomb and exchange interactions are investigated. Dark exciton formation is found to occur for both GaN quantum dots(QDs) with wurtzite structure having positive crystal field splitting and GaN and AlN QDs with zero crystal field splitting with a transition from dark to bright exciton at about 40Å. In wurtzite AlN QDs with negative crystal field splitting the splitting between the dark and bright excitonic states is very small and vanishes at about 15Å.
We study an impact of the fine structure of the heavy--hole ground state exciton confined in semiconductor quantum dots on the photoluminescence polarization dynamics solving the relevant system of the rate equations. The presence of the dark excitons is usually ignored and the polarization decay is assumed to be caused by direct transitions within the radiative doublet. We demonstrate that in strongly confined quantum dots the dark excitons, which are energetically well below the bright excitons, have actually a decisive effect on the polarization dynamics due to their persistent nature. The …
Because of their weak coupling to the electromagnetic field dark excitons in semiconductor quantum dots possess extremely long lifetimes, which makes them attractive candidates for quantum information processing. On the other hand, preparation and manipulation of dark states is challenging, because commonly used optical excitation mechanisms are not applicable. We propose a new, efficient mechanism for the deterministic preparation of the dark exciton exploiting the application of a tilted magnetic field and the optical excitation with a chirped, i.e., frequency modulated, laser pulse.
We use an atomistic model to consider the effect of shape symmetry breaking on the optical properties of self-assembled InAs/GaAs quantum dots. In particular, we investigate the energy level structure and optical activity of the lowest energy excitons in these nanostructures. We compare between quantum dots with two-fold rotational and two reflections (C2v) symmetry and quantum dots in which this symmetry was reduced to one reflection only (Cs) by introducing a facet between the quantum dots and the host material. We show that the symmetry reduction mostly affects the optical activity of the d…
We consider theoretically the transport through the double quantum dot structure of the recent experiment of C. Payette {\it et al.} [Phys. Rev. Lett. {\bf 102}, 026808 (2009)] and calculate stationary current and shotnoise. Three-level mixing gives rise to a pronounced current suppression effect, the character of which charges markedly with bias direction. We discuss these results in connexion with the dark states of coherent population trapping in quantum dots.
We demonstrate evidence for a radiative recombination channel of dark excitons in self-assembled quantum dots. This channel is due to a light hole admixture in the excitonic ground state. Its presence was experimentally confirmed by a direct observation of the dark exciton photoluminescence from a cleaved edge of the sample. The polarization resolved measurements revealed that a photon created from the dark exciton recombination is emitted only in the direction perpendicular to the growth axis. Strong correlation between the dark exciton lifetime and the in-plane hole g-factor enabled us to sh…
We here propose a mechanism to teleport electrons between quantum dots through the transformation of a virtual bright exciton into a dark exciton. This mechanism relies on the interactions of two composite bosons: a pair of electrons with opposite spins, trapped in two dots and an electron-hole pair in a free exciton coupled to an unabsorbed pump pulse, which makes it ``bright'' but virtual. This bright exciton first turns ``dark'' by dropping its electron and stealing the trapped electron with opposite spin through an exchange Coulomb process with the trapped pair. In a second step, the dark …
A promising method to investigate dark exciton transitions in quantum dots is presented. The optical recombination of the dark exciton is allowed when the exciton state is coupled with an individual magnetic impurity (manganese ion). It is shown that the efficient radiative recombination is possible when the exchange interaction with the magnetic ion is accompanied by a mixing of the heavy-light hole states related to an in-plane anisotropy of the quantum dot. It is also shown that the dark exciton recombination is an efficient channel of manganese spin orientation.
Quantum dots are arguably one of the best platforms for optically accessible spin based qubits. The paramount demand of extended qubit storage time can be met by using quantum-dot-confined dark exciton: a longlived electron-hole pair with parallel spins. Despite its name the dark exciton reveals weak luminescence that can be directly measured. The origins of this optical activity remain largely unexplored. In this work, using the atomistic tight-binding method combined with configuration-interaction approach, we demonstrate that atomic-scale randomness strongly affects oscillator strength of d…
In semiconductor quantum dots the coupling to the environment, i.e. to phonons, plays a crucial role for optical state preparation. We analyze the phonon impact on two methods for a direct optical preparation of the dark exciton, which is enabled by a tilted magnetic field: the excitation with a chirped laser pulse and the excitation with a detuned pulse. Our study reveals that for both methods phonons either do not impede the proposed mechanism or are even useful by widening the parameter range where a dark state preparation is possible due to phonon-assisted dark exciton preparation. In view…
We present a transport setup of coupled quantum dots that enables the creation of spatially separated spin-entangled two-electron dark states. We prove the existence of an entangled transport dark state by investigating the system Hamiltonian without coupling to the electronic reservoirs. In the transport regime the entangled dark state which corresponds to a singlet has a strongly enhanced Fano factor compared to the dark state which corresponds to a mixture of the triplet states. Furthermore we calculate the concurrence of the occupying electrons to show the degree of entanglement in the tra…
We consider the transport through a system of three coupled quantum dots in a perpendicular magnetic field. At zero field, destructive interference can trap an electron in a dark state -- a coherent superposition of dot states that completely blocks current flow. The magnetic field can disrupt this interference giving rise to oscillations in the current and its higher-order statistics as the field is increased. These oscillations have a period of either the flux-quantum or half the flux-quantum, depending on the dot geometry. We give results for the stationary current and for the shotnoise and…
Excitons in alloyed nanowire quantum dots have unique spectra as shown here using atomistic calculations. The bright exciton splitting is triggered solely by alloying and despite cylindrical quantum dot shape reaches over $15~μ$eV, contrary to previous theoretical predictions, however, in line with experimental data. This splitting can however be tuned by electric field to go below $1$~$μ$eV threshold. The dark exciton optical activity is also strongly affected by alloying reaching notable $1/3500$ fraction of the bright exciton and having large out-of-plane polarized component.
We propose a scheme to induce weak-light nonlinearity in a double quantum dot. The scheme positively utilizes locality and dissipation of an external auxiliary system. As a plausible setup, we consider a complex system in which a localized plasmon field from a metallic nanotip couples with only one of the coupled quantum dots. The perturbative calculation with respect to the light intensity shows that, even by a sufficiently weak light, a dipole-forbidden two-exciton NOON state is prepared as the steady state. This result can be explained by combining the two factors: decoherence-induced quant…
We study transport through a triple quantum dot in a triangular geometry with applied bias such that both singly- and doubly- charged states participate. We describe the formation of electronic dark states -- coherent superpositions that block current flow -- in the system, and focus on the formation of a two-electron dark state. We discuss the conditions under which such a state forms and describe the signatures that it leaves in transport properties such as the differential conductance and shotnoise.
The dark exciton state in semiconductor quantum dots constitutes a long-lived solid-state qubit which has the potential to play an important role in implementations of solid-state based quantum information architectures. In this work, we exploit deterministically fabricated QD microlenses with enhanced photon extraction, to optically prepare and readout the dark exciton spin and observe its coherent precession. The optical access to the dark exciton is provided via spin-blockaded metastable biexciton states acting as heralding state, which are identified deploying polarization-sensitive spectr…
Incoherent pumping in quantum dots (QDs) can create a biexciton state through two paths: via the formation of bright or dark exciton states. The latter, dark-pumping, path is shown to enhance the probability of two-photon simultaneous emission, and hence increase $g^{(2)}(0)$ by a factor $\propto 1/γ_S$, due to the slow spin relaxation rate $γ_S$ in QDs. The existence of the dark path is shown to impose a limitation on the single photon (SP) emission process, especially in nanocavities which exhibit a large exciton-cavity coupling and a Purcell enhancement for fast quantum telecommunications.
Several important proposals to use semiconductor quantum dots in quantum information technology rely on the control of the dark exciton ground states, such as dark exciton based qubits with a $μ$s life time. In this paper, we present an efficient way to occupy the dark exciton ground state by a single short laser pulse. The scheme is based on an optical excitation with a longitudinal field component featured by, e.g., radially polarized beams or certain Laguerre-Gauss or Bessel beams. Utilizing this component, we show within a configuration interaction approach that high-energy exciton states …
We theoretically investigate the spectrum of the fluorescence from triple quantum-dot molecules and demonstrate that it is possible to use tunneling to induce dark states. Unlike the atomic system, in quantum-dot molecules we can use tunneling to create the dark states and control fluorescence emission, requiring no coupling lasers. And interesting features such as quenching and narrowing of the fluorescence can be obtained. We also explain the spectrum with the transition properties of the dressed states generated by the coupling of the laser and the two tunneling. The quenching of the fluore…
Electron, hole, and exciton states of multishell CdS/HgS/CdS quantum-dot quantum well nanocrystals are determined by use of a multiband theory that includes valence-band mixing, modeled with a 6-band Luttinger-Kohn Hamiltonian, and nonparabolicity of the conduction band. The multiband theory correctly describes the recently observed dark-exciton ground state and the lowest, optically active, bright-exciton states. Charge separation in pair states is identified. Previous single-band theories could not describe these states or account for charge separation.
When a detuned and strong laser pulse acts on an optical transition, a Stark shift of the corresponding energies occurs. We analyze how this optical Stark effect can be used to prepare and control the dark exciton occupation in a semiconductor quantum dot. The coupling between the bright and dark exciton states is facilitated by an external magnetic field. Using sequences of laser pulses, we show how the dark exciton and different superposition states can be prepared. We give simple analytic formulas, which yield a good estimate for optimal preparation parameters. The preparation scheme is qui…
We demonstrate that the cycling between internal states of quantum dots during fluorescence blinking can be used to tune the near-field coupling with a sharp tip. In particular, the balance between tip-induced field enhancement and energy transfer depends explicitly on the intrinsic quantum yield of the quantum dot. Our measurements show that for internal states with low quantum yield, energy transfer is strongly suppressed in favor of field enhancement, and explicitly demonstrate that suppressed blinking of quantum dots near metal surfaces is due to fast energy transfer.
Multi-phonon physics is an emerging field that serves as a test bed for fundamental quantum physics and several applications in metrology, on-chip communication, among others. Quantum acoustic cavities or resonators are devices that are being used to study multi-phonon phenomena both theoretically and experimentally. In particular, we study a system consisting of a semiconductor quantum dot pumped by a driving laser, and coupled to an acoustic cavity. This kind of systems has proven to yield interesting multi-phonon phenomena, but the description of the quantum dot has been limited to a two-le…
Illumination of atoms by resonant lasers can pump electrons into a coherent superposition of hyperfine levels which can no longer absorb the light. Such superposition is known as dark state, because fluorescent light emission is then suppressed. Here we report an all-electric analogue of this destructive interference effect in a carbon nanotube quantum dot. The dark states are a coherent superposition of valley (angular momentum) states which are decoupled from either the drain or the source leads. Their emergence is visible in asymmetric current-voltage characteristics, with missing current s…
We study the spin-polarized transport through a triple quantum dot molecule weakly coupled to ferromagnetic leads. The analysis is performed by means of the real-time diagrammatic technique including up to the second order of perturbation expansion with respect to the tunnel coupling. The emphasis is put on the impact of dark states on spin-resolved transport characteristics. It is shown that the interplay of coherent population trapping and cotunneling processes results in a highly nontrivial behavior of the tunnel magnetoresistance, which can take negative values. Moreover, a super-Poissonia…
Towards Quantum-Dot Detectors as Barcodes for Dark Matter Interactions
Czech Technical University in Prague（布拉格捷克理工大学）；Stockholm University（斯德哥尔摩大学）；The Oskar Klein Centre for Cosmoparticle Physics（奥斯卡·克莱因宇宙粒子物理中心）；Massachusetts Institute of Technology（麻省理工学院）；The Pennsylvania State University（宾夕法尼亚州立大学）；Princeton University（普林斯顿大学）；C.N. Yang Institute for Theoretical Physics, Stony Brook University（纽约州立大学石溪分校陈省身理论物理研究所）；Friedrich-Alexander-Universität Erlangen-Nürnberg（埃尔朗根-纽伦堡大学）
Optically active quantum dots, for instance self-assembled InGaAs quantum dots, are potentially excellent single photon sources. The fidelity of the single photons is much improved using resonant rather than non-resonant excitation. With resonant excitation, the challenge is to distinguish between resonance fluorescence and scattered laser light. We have met this challenge by creating a polarization-based dark-field microscope to measure the resonance fluorescence from a single quantum dot at low temperature. We achieve a suppression of the scattered laser exceeding a factor of 10^7 and backgr…
In photoluminescence spectra of symmetric [111] grown GaAs/AlGaAs quantum dots in longitudinal magnetic fields applied along the growth axis we observe in addition to the expected bright states also nominally dark transitions for both charged and neutral excitons. We uncover a strongly non-monotonous, sign changing field dependence of the bright neutral exciton splitting resulting from the interplay between exchange and Zeeman effects. Our theory shows quantitatively that these surprising experimental results are due to magnetic-field-induced \pm 3/2 heavy-hole mixing, an inherent property of …
We investigate the dynamical purification of maximally entangled electron states by transport through coupled quantum dots. Under resonant ac driving and coherent tunneling, even-parity Bell states perform Rabi oscillations that decouple from the environment, leading to a dark state. The two electrons remain spatially separated, one in each quantum dot. We propose configurations where this effect will prove as antiresonances in transport spectroscopy experiments.
We report on high-resolution photoluminescence (PL) and photocurrent (PC) spectroscopies of a single self-assembled InAs/GaAs quantum dot (QD) embedded in an n-i-Schottky device with an applied magnetic field in Faraday and Voigt geometries. The single-QD PC spectrum of neutral exciton (X$^0$) is obtained by sweeping the bias-dependent X$^0$ transition energy to achieve resonance with a fixed narrow-bandwidth laser through quantum-confined Stark effect. With a magnetic field applied in Faraday geometry, the diamagnetic effect and the Zeeman splitting of X$^0$ are observed both in PL and PC spe…
We demonstrate that the quantum dot-confined dark exciton forms a long-lived integer spin solid state qubit which can be deterministically on-demand initiated in a pure state by one optical pulse. Moreover, we show that this qubit can be fully controlled using short optical pulses, which are several orders of magnitude shorter than the life and coherence times of the qubit. Our demonstrations do not require an externally applied magnetic field and they establish that the quantum dot-confined dark exciton forms an excellent solid state matter qubit with some advantages over the half-integer spi…
We investigate sequential tunneling through a multilevel quantum dot confining multiple electrons, in the regime where several channels are available for transport within the bias window. By analyzing solutions to the master equations of the reduced density matrix, we give general conditions on when the presence of a second transport channel in the bias window quenches transport through the quantum dot. These conditions are in terms of distinct tunneling anisotropies which may aid in explaining the occurrence of negative differential conductance in quantum dots in the nonlinear regime.
We study theoretically the cooling of an ensemble of nuclear spins coupled to the spin of a localized electron in a quantum dot. We obtain a master equation for the state of the nuclear spins interacting with a sequence of polarized electrons that allows us to study quantitatively the cooling process including the effect of nuclear spin coherences, which can lead to ``dark states'' of the nuclear system in which further cooling is inhibited. We show that the inhomogeneous Knight field mitigates this effect strongly and that the remaining dark state limitations can be overcome by very few shift…
Exciton luminescence of a CdSe quantum dot (QD) inserted in a ZnSe nanowire is strongly influenced by the dark exciton states. Because of the small size of these QDs (2-5nm), exchange interaction between hole and electron is highly enhanced and we measured large energy splitting between bright and dark exciton states ($ΔE\in [4, 9.2 ]$ meV) and large spin flip rates between these states. Statistics on many QDs showed that this splitting depends on the QD size. Moreover, we measured an increase of the spin flip rate to the dark states with increasing energy splitting. We explain this observatio…
The population dynamics of dark and bright excitons in (In,Ga)As/GaAs quantum dots is studied by two-color pump-probe spectroscopy in an external magnetic field. With the field applied in Faraday geometry and at T<20 K, the dark excitons decay on a ten nanoseconds time scale unless the magnetic field induces a resonance with a bright exciton state. At these crossings their effective lifetime is drastically shortened due to spin flips of either electron or hole by which the dark excitons are converted into bright ones. Due to the quasielastic character we attribute the origin of these flips to …
Realizing perfect two-photon entanglement from quantum dots has been a long-standing scientific challenge. It is generally thought that the nuclear spins limit the entanglement fidelity through spin flip dephasing processes. However, this assumption lacks experimental support. Here, we show dephasing-free two-photon entanglement from an Indium rich single quantum dot comprising of nuclear spin 9/2 when excited quasi-resonantly. This remarkable finding is based on a perfect match between our entanglement measurements with our model that assumes no dephasing and takes into account the detection …
Optical studies of a bright exciton provide only limited information about the hole anisotropy in a quantum dot. In this work we present a universal method to study heavy hole anisotropy using a dark exciton in a moderate in-plane magnetic field. By analysis of the linear polarization of the dark exciton photoluminescence we identify both isotropic and anisotropic contributions to the hole g-factor. We employ this method for a number of individual self-assembled CdTe/ZnTe quantum dots, demonstrating a variety of behaviors of in-plane hole g-factor: from almost fully anisotropic to almost isotr…
Quantum dots are arguably the best interface between matter spin qubits and flying photonic qubits. Using quantum dot devices to produce joint spin-photonic states requires the electronic spin qubits to be stored for extended times. Therefore, the study of the coherence of spins of various quantum dot confined charge carriers is important both scientifically and technologically. In this study we report on spin relaxation measurements performed on five different forms of electronic spin qubits confined in the very same quantum dot. In particular, we use all optical techniques to measure the spi…
We discuss the spectral lineshapes of N quantum dots in strong coupling with the single mode of a microcavity. Nontrivial features are brought by detuning the emitters or probing the direct exciton emission spectrum. We describe dark states, quantum nonlinearities, emission dips and interferences and show how these various effects may coexist, giving rise to highly peculiar lineshapes.
Graphene-based photodetectors have shown responsivities up to 10$^8$A/W and photoconductive gains up to 10$^{8}$ electrons per photon. These photodetectors rely on a highly absorbing layer in close proximity of graphene, which induces a shift of the graphene chemical potential upon absorption, hence modifying its channel resistance. However, due to the semi-metallic nature of graphene, the readout requires dark currents of hundreds of $μ$A up to mA, leading to high power consumption needed for the device operation. Here we propose a novel approach for highly responsive graphene-based photodete…
We demonstrate the suppression of nuclear spin fluctuations in an InAs quantum dot and measure the timescales of the spin narrowing effect. By initializing for tens of milliseconds with two continuous wave diode lasers, fluctuations of the nuclear spins are suppressed via the hole assisted dynamic nuclear polarization feedback mechanism. The fluctuation narrowed state persists in the dark (absent light illumination) for well over one second even in the presence of a varying electron charge and spin polarization. Enhancement of the electron spin coherence time (T2*) is directly measured using c…
We investigate the strong coupling regime of a self-assembled quantum dot in a tunable microcavity with dark-field laser spectroscopy. The high quality of the spectra allows the lineshapes to be analyzed revealing subtle quantum interferences. Agreement with a model calculation is achieved only by including exciton dephasing which reduces the cooperativity from a bare value of 9.0 to the time-averaged value 5.5. In the pursuit of high cooperativity, besides a high-Q and low mode-volume cavity, we demonstrate that equal efforts need to be taken towards lifetime-limited emitter linewidths.
We propose an approach to cool a mechanical resonator (MR) via quantum interference in a triple quantum dot (TQD) capacitively coupled to the MR. The TQD connected to three electrodes is an electronic analog of a three-level atom in $Λ$ configuration. The electrons can tunnel from the left electrode into one of the two dots with lower-energy states, but can only tunnel out from the higher-energy state at the third dot to the right electrode. When the two lower-energy states are tuned to be degenerate, an electron in the TQD can be trapped in a superposition of the degenerate states called the …
We demonstrate the extension of coherence between all four two-electron spin ground states of an InAs quantum dot molecule (QDM) via non-local suppression of nuclear spin fluctuations in both constituent quantum dots (QDs), while optically addressing only the upper QD transitions. Long coherence times are revealed through dark-state spectroscopy as resulting from nuclear spin locking mediated by the exchange interaction between the QDs. Lineshape analysis provides the first measurement of the quieting of the Overhauser field distribution correlating with reduced nuclear spin fluctuations.
We theoretically analyze the carrier capture and distribution among the available energy levels of a symmetric semiconductor quantum dot under continuous-wave excitation resonant with the barrier energy levels. At low temperature all the dot level-occupations but one decrease monotonically with energy. The uncovered exception, corresponding to the second (dark) energy level, displays a steady-state carrier density exceeding that of the lowest level more than a factor two. The root cause is not radiative recombination before relaxation to lower energy levels, but at the opposite, carrier trappi…
The theory of exciton coupling to photons and LO phonons in quantum dots (QDs) and quantum-dot molecules (QDMs) is presented. Resonant-round trips of the exciton between the ground (bright) and excited (dark or bright) states mediated by the LO-phonon alter the decay time and yield the Rabi oscillation. The initial distributions of the population in the ground and the excited states dominate the oscillating amplitude and frequency. This property provides a detectable signature to the information stored in a qubit made from QD or QDM for a wide range of temperature T. Our results presented here…
The thermoelectric effect in a quantum dot (QD) attached to two leads in the presence of microwave fields is studied by using the Keldysh nonequilibrium Green function technique. When the microwave is applied only on the QD and in the linear-response regime, the main peaks in the thermoelectric figure of merit and the thermopower are found to decrease, with the emergence of a set of photon-induced peaks. Under this condition the microwave field can not generate heat current or electrical bias voltage. Surprisingly, when the microwave field is applied only to one (bright) lead and not to the ot…
We propose an approach for achieving ground-state cooling of a nanomechanical resonator (NAMR) capacitively coupled to a triple quantum dot (TQD). This TQD is an electronic analog of a three-level atom in $Λ$ configuration which allows an electron to enter it via lower-energy states and to exit only from a higher-energy state. By tuning the degeneracy of the two lower-energy states in the TQD, an electron can be trapped in a dark state caused by destructive quantum interference between the two tunneling pathways to the higher-energy state. Therefore, ground-state cooling of an NAMR can be achi…
We present a theoretical model describing the photo-electrical response of a system composed of quantum dots embedded in a dielectric matrix. The model is based on the non-coherent rate equations and the Transfer Hamiltonian formalism. The self charge was included. Within this methodology, the response of the system only depends on fundamental material parameters and its geometry. Transport through several quantum dot configurations was simulated obtaining current-voltage curves in dark and illuminating conditions for three different scenarios: single one quantum dot and two quantum dots in pa…
Taking into account the tetrahedral shape of a quantum dot quantum well (QDQW) when describing excitonic states, phonon modes and the exciton-phonon interaction in the structure, we obtain within a non-adiabatic approach a quantitative interpretation of the photoluminescence (PL) spectrum of a single CdS/HgS/CdS QDQW. We find that the exciton ground state in a tetrahedral QDQW is bright, in contrast to the dark ground state for a spherical QDQW.
We present a theoretical study of the collective optical effects which can occur in groups of three and four quantum dots. We define conditions for stable subradiant (dark) states, rapidly decaying superradiant states,and spontaneous trapping of excitation. Each quantum dot is treated like a two-level system. The quantum dots are though realistic, meaning that they may have different transition energies and dipole moments. The dots interact via a short-range coupling which allows excitation transfer across the dots, but conserves the total population. We calculate the time evolution of single-…
We investigate the interplay between long-range and direct photon-assisted transport in a triple quantum dot chain where local ac voltages are applied to the outer dots. We propose the phase difference between the two ac voltages as an external parameter, which can be easily tuned to manipulate the current characteristics. For gate voltages in phase opposition we find quantum destructive interferences analogous to the interferences in closed-loop undriven triple dots. As the voltages oscillate in phase, interferences between multiple paths give rise to dark states. Those totally cancel the cur…
