We articulate confocal microscopy and electron spin resonance to implement spin-to-charge conversion in a small ensemble of nitrogen-vacancy (NV) centers in bulk diamond, and demonstrate charge conversion of neighboring defects conditional on the NV spin state. We build on this observation to show time-resolved NV spin manipulation and ancilla-charge-aided NV spin state detection via integrated measurements. Our results hint at intriguing opportunities in the search for enhanced forms of color-center-based metrology and information processing down to the limit of individual point defects.
We propose a novel scheme to realize electrically controlled quantum memories in the opto- and electro-mechanical (OEM) cavity. Combining this OEM cavity with the mechanism of Electromagnetically Induced Transparency (EIT) we find that the quantum interference, arising from the two optical transitions of the $Λ$ type three-level atomic ensembles, can be manipulated electrically. Numerical calculations show that the probe photon state can be well stored into the atomic spin state by sending an electric current pulse and retrieved with time-reverse symmetry by sending the other current pulse wit…
Storage time extension in photon echoes using optical deshelving via a robust spin state has been investigated for absorption-dependent optical leakage, where an incomplete population transfer, even by a πoptical pulse obviates the phase recovery condition of the deshelving. We analyze an optical depth-dependent echo leakage mechanism in the storage time extended photon echoes for the usage of optical deshelving to photon echo-based quantum memories.
In this article the ability to record, store, and read out the quantum properties of light is studied. The discussion is based on high-speed and adiabatic models of quantum memory in lambda-configuration and in the limit of strong resonance. We show that in this case the equality between efficiency and squeezing ratio, predicted by the simple beamsplitter model, is broken. The requirement of the maximum squeezing in the output pulse should not be accompanied by the requirement of maximum efficiency of memory, as in the beamsplitter model. We have demonstrated a high output pulse squeezing, whe…
Attenuated laser pulses are often employed in place for single photons in order to test the efficiency of the elements of a quantum network. In this work we analyse theoretically the dynamics of storage of an attenuated light pulse (where the pulse intensity is at the single photon level) propagating along a transmission line and impinging on the mirror of a high finesse cavity. Storage is realised by the controlled transfer of the photonic excitations into a metastable state of an atom confined inside the cavity and occurs via a Raman transition with a suitably tailored laser pulse, which dri…
An elementary quantum network operation involves storing a qubit state in an atomic quantum memory node, and then retrieving and transporting the information through a single photon excitation to a remote quantum memory node for further storage or analysis. Implementations of quantum network operations are thus conditioned on the ability to realize such matter-to-light and/or light-to-matter quantum state mappings. Here, we report generation, transmission, storage and retrieval of single quanta using two remote atomic ensembles. A single photon is generated from a cold atomic ensemble at Site …
We study spatial multimode quantum memories based on light storage in extended ensembles of Lambda-type atoms. We show that such quantum light-matter interfaces allow for highly efficient storage of many spatial modes. In particular, forward operating memories possess excellent scaling with the important physical parameters: quadratic scaling with the Fresnel number and even cubic with the optical depth of the atomic ensemble. Thus, the simultaneous use of both the longitudinal and transverse shape of the stored spin wave modes constitutes a valuable and so far overlooked resource for multimod…
Quantum information processed in strongly correlated states of matter can provide built in hardware protection against errors. We may encode information in highly non local degrees of freedom, such as using three dimensional spin lattices for subsystem codes or two dimensional spin lattices for topologically ordered surface codes and measurement based codes. Recently, in [L. Jiang et al., Nature Physics {\bf 4}, 482 (2008)] the authors showed how to manipulate these global degrees of freedom using optical lattices coupled to a bosonic degree of freedom via a cavity. We elaborate on these ideas…
Long-lived optical quantum memories are of great importance for scalable distribution of entanglement over remote networks (e.g. quantum repeaters). Long-lived storage generally relies on storing the optical states as spin excitations since these often exhibit long coherence times. To extend the storage time beyond the intrinsic spin dephasing time one can use dynamical decoupling techniques. However, it has been shown that dynamical decoupling introduces noise in optical quantum memories based on ensembles of atoms. In this article a simple model is proposed to calculate the resulting signal-…
The use of multiplexed atomic quantum memories (MAQM) can significantly enhance the efficiency to establish entanglement in a quantum network. In the previous experiments, individual elements of a quantum network, such as the generation, storage and transmission of quantum entanglement have been demonstrated separately. Here we report an experiment to show the compatibility of these basic operations. Specifically, we generate photon-atom entanglement in a $6\times 5$ MAQM, convert the spin wave to time-bin photonic excitation after a controllable storage time, and then store and retrieve the p…
Quantum states are inherently fragile, making their storage a major concern for many practical applications and experimental tests of quantum mechanics. The field of quantum memories is concerned with how this storage may be achieved, covering everything from the physical systems best suited to the task to the abstract methods that may be used to increase performance. This review concerns itself with the latter, giving an overview of error correction and self-correction, and how they may be used to achieve fault-tolerant quantum computation. The planar code is presented as a concrete example, …
The influence of decoherence on the fidelity of quantum memories for photonic qubits based on dark-state polaritons in atomic ensembles is discussed. It is shown that despite the large entanglement of the collective storage states corresponding to single photons or nonclassical states of light the sensitivity to decoherence does not scale with the number of atoms. This is due to the existence of equivalence classes of storage states corresponding to states with the same number of dark-state polariton excitations but arbitrary excitations in other polariton modes. Several decoherence processes …
For the last decade quantum memories have been intensively studied for potential applications to quantum information and communications using atomic and ionic ensembles. With the importance of a multimode storage capability in quantum memories, on-demand control of reversible inhomogeneous broadening of an optical medium has been broadly investigated recently. However, the photon storage time in these researches is still too short to apply for long-distance quantum communications. In this paper, we demonstrate new physics of spin population decay dependent ultralong photon storage method, wher…
We develop a three-dimensional theory for quantum memories based on light storage in ensembles of Lambda-type atoms, where two long-lived atomic ground states are employed. We consider light storage in an ensemble of finite spatial extent and we show that within the paraxial approximation the Fresnel number of the atomic ensemble and the optical depth are the only important physical parameters determining the quality of the quantum memory. We analyze the influence of these parameters on the storage of light followed by either forward or backward read-out from the quantum memory. We show that f…
We propose a dynamical approach to quantum memories using a synchronous oscillator-cavity model, in which the coupling is shaped in time to provide the optimum interface to a symmetric input pulse. This overcomes the known difficulties of achieving high quantum input-output fidelity with storage times long compared to the input signal duration. Our generic model is applicable to any linear storage medium ranging from a superconducting device to an atomic medium. We show that with temporal modulation of coupling and/or detuning, it is possible to mode-match to time-symmetric pulses that have id…
We propose a dynamical approach to quantum memories using an oscillator-cavity model. This overcomes the known difficulties of achieving high quantum input-output fidelity with storage times long compared to the input signal duration. We use a generic model of the memory response, which is applicable to any linear storage medium ranging from a superconducting device to an atomic medium. The temporal switching or gating of the device may either be through a control field changing the coupling, or through a variable detuning approach, as in more recent quantum memory experiments. An exact calcul…
Cavity assisted quantum memory storage has been proposed [PRA 82, 022310 (2010), PRA 82, 022311 (2010)] for creating efficient (close to unity) quantum memories using weakly absorbing materials. Using this approach we experimentally demonstrate a significant (about 20-fold) enhancement in quantum memory efficiency compared to the no cavity case. A strong dispersion originating from absorption engineering inside the cavity was observed, which directly affect the cavity line-width. A more than 3 orders of magnitude reduction of cavity mode spacing and cavity line-width from GHz to MHz was observ…
Quantum memories are a crucial element towards efficient quantum protocols. In the continuous variables domain, such memories need to have near unity efficiencies. Moreover, one needs to store complex quantum states exhibiting negative Wigner functions after storage. We report the implementation of an all optical quantum memory: the storage of single and two-photon Fock states with high fidelities has been realized. The Wigner functions of the reconstructed states shows negativity after $\sim 0.75~μs$ and $\sim 0.61~μs$ respectively for the single-photon and two-photon Fock states. This is, to…
Inspired by recent developments in the control and manipulation of quantum dot nuclear spins, which allow for the transfer of an electron spin state to the surrounding nuclear-spin ensemble for storage, we propose a quantum repeater scheme that combines individual quantum dot electron spins and nuclear-spin ensembles, which serve as spin-photon interfaces and quantum memories respectively. We consider the use of low-strain quantum dots embedded in high-cooperativity optical microcavities. Quantum dot nuclear-spin ensembles allow for the long-term storage of entangled states, and heralded entan…
Quantum memories are a crucial technology for enabling large-scale quantum networks through synchronisation of probabilistic operations. Such networks impose strict requirements on quantum memory, such as storage time, retrieval efficiency, bandwidth, and scalability. On- and off-resonant ladder protocols on warm atomic vapour platforms are promising candidates, combining efficient high-bandwidth operation with low-noise on-demand retrieval. However, their storage time is severely limited by motion-induced dephasing caused by the broad velocity distribution of atoms comprising the vapour. In t…
We demonstrate the storage and manipulation of narrowband heralded single photons from a cavity-enhanced spontaneous parametric downconversion (SPDC) source in the atomic quantum memory based on electromagnetically induced transparency. We show that nonclassical correlations are preserved between the heralding and the retrieved photons after storage process. By varying the intensity of the coupling field during retrieval process, we further demonstrate that the waveform or bandwidth of the single photons can be manipulated and the nonclassical correlation between the photon pairs can be even e…
Solid-state impurity spins with optical control are currently investigated for quantum networks and repeaters. Among these, rare-earth-ion doped crystals are promising as quantum memories for light, with potentially long storage time, high multimode capacity, and high bandwidth. However, with spins there is often a tradeoff between bandwidth, which favors electronic spin, and memory time, which favors nuclear spins. Here, we present optical storage experiments using highly hybridized electron-nuclear hyperfine states in $^{171}$Yb$^{3+}$:Y$_2$SiO$_5$, where the hybridization can potentially of…
Quantum memories with long storage times are key elements in long-distance quantum networks. The atomic frequency comb (AFC) memory in particular has shown great promise to fulfill this role, having demonstrated multimode capacity and spin-photon quantum correlations. However, the memory storage times have so-far been limited to about one millisecond, realized in a Eu${}^{3+}$ doped Y${}_2$SiO${}_5$ crystal at zero applied magnetic field. Motivated by studies showing increased spin coherence times under applied magnetic field, we developed a AFC spin-wave memory utilizing a weak 15 mT magnetic…
Photon loss in optical fibers prevents long-distance distribution of quantum information on the ground. Quantum repeater is proposed to overcome this problem, but the communication distance is still limited so far because of the system complexity of the quantum repeater scheme. Alternative solutions include transportable quantum memory and quantum-memory-equipped satellites, where long-lived optical quantum memories are the key components to realize global quantum communication. However, the longest storage time of the optical memories demonstrated so far is approximately 1 minute. Here, by em…
Improving Entanglement Resilience in Quantum Memories with Error-Detection-Based Distillation
School of Electrical Engineering, Korea University（韩国大学电气工程学院）；Quantum Network Research Center, Korea Institute of Science and Technology Information（韩国科学技术信息研究院量子网络研究中心）
A novel method of multi-bit quantum optical data storage is presented, where the storage time can be lengthened far beyond the spin phase-decay time in a reversible spin inhomogeneous system excited by consecutive resonant Raman optical data pulses. The ultralong storage time is obtained by an optical population locking mechanism of modified rephasing process. This gives potentials to quantum repeaters utilizing quantum memories for long distance quantum communications, in which ultralong storage time plays a major role.
Controlled manipulation, storage and retrieval of quantum information is essential for quantum communication and computing. Quantum memories for light, realized with cold atomic samples as the storage medium, are prominent for their high storage efficiencies and lifetime. We demonstrate the controlled transport of stored light over 1:2 mm in such a storage system and show that the transport process and its dynamics only have a minor effect on the coherence of the storage. Extending the presented concept to longer transport distances and augmenting the number of storage sections will allow for …
Multiplexed quantum memories capable of storing and processing entangled photons are essential for the development of quantum networks. In this context, we demonstrate the simultaneous storage and retrieval of two entangled photons inside a solid-state quantum memory and measure a temporal multimode capacity of ten modes. This is achieved by producing two polarization entangled pairs from parametric down conversion and mapping one photon of each pair onto a rare-earth-ion doped (REID) crystal using the atomic frequency comb (AFC) protocol. We develop a concept of indirect entanglement witnesse…
Spectral and temporal mode matching are required for the efficient interaction of photons and quantum memories. In our previous work, we proposed a new route to spectrally compress broadband photons to achieve spectral mode matching with narrowband memories, using a linear, time-variant optical cavity based on rapid switching of input coupling. In this work, we extend our approach to attain temporal mode matching as well by exploiting the time-variation of output coupling of the cavity. We numerically analyze the mode matching and loss performance of our time-varying cavity and present a possi…
Long-lived quantum memories are essential components of a long-standing goal of remote distribution of entanglement in quantum networks. These can be realized by storing the quantum states of light as single-spin excitations in atomic ensembles. However, spin states are often subjected to different dephasing processes that limit the storage time, which in principle could be overcome using spin-echo techniques. Theoretical studies have suggested this to be challenging due to unavoidable spontaneous emission noise in ensemble-based quantum memories. Here we demonstrate spin-echo manipulation of …
Future multi-photon applications of quantum optics and quantum information science require quantum memories that simultaneously store many photon states, each encoded into a different optical mode, and enable one to select the mapping between any input and a specific retrieved mode during storage. Here we show, with the example of a quantum repeater, how to employ spectrally-multiplexed states and memories with fixed storage times that allow such mapping between spectral modes. Furthermore, using a Ti:Tm:LiNbO3 waveguide cooled to 3 Kelvin, a phase modulator, and a spectral filter, we demonstr…
Scalable quantum information processing critically depends on the capability of storage of a quantum state. In particular, a long-lived storable and retrievable quantum memory for single excitations is of crucial importance to the atomic-ensemble-based long-distance quantum communication. Although atomic memories for classical lights and continuous variables have been demonstrated with milliseconds storage time, there is no equal advance in the development of quantum memory for single excitations, where only around 10 $μ$s storage time was achieved. Here we report our experimental investigatio…
We investigate theoretically the coupling of a cavity mode to a continuous distribution of emitters. We discuss the influence of the emitters inhomogeneous broadening on the existence and on the coherence properties of the polaritonic peaks. We find that their coherence depends crucially on the shape of the distribution and not only on its width. Under certain conditions the coupling to the cavity protects the polaritonic states from inhomogeneous broadening, resulting in a longer storage time for a quantum memory based on emitters ensembles. When two different ensembles of emitters are couple…
We introduce a general scheme to realize perfect storage of quantum information in systems of interacting qubits. This novel approach is based on {\it global} external controls of the Hamiltonian, that yield time-periodic inversions in the dynamical evolution, allowing a perfect periodic quantum state recontruction. We illustrate the method in the particularly interesting and simple case of spin systems affected by XY residual interactions with or without static imperfections. The global control is achieved by step time-inversions of an overall topological phase of the Aharonov-Bohm type. Such…
Electromagnetically induced transparency (EIT) and Autler-Townes splitting (ATS) are similar,but different quantum optical phenomena: EIT results from a Fano interference, whereas ATS is described by the AC-Stark effect. Likewise, despite their close resemblance, light-storage techniques based on the EIT memory protocol and the recently-proposed ATS memory protocol (E. Saglamyurek et al. Nature Photonics 12, 2018) are distinct: the EIT protocol relies on adiabatic elimination of absorption, whereas the ATS protocol is based on absorption. In this article, we elaborate on the distinction betwee…
Inhomogeneously broadened spin ensembles play an important role in present-day implementation of hybrid quantum processing architectures. When coupled to a resonator such an ensemble may serve as a multi-mode quantum memory for the resonator field, and by employing spin-refocusing techniques the quantum memory time can be extended to the coherence time of individual spins in the ensemble. In the present paper we investigate such a memory protocol capable of storing an unknown resonator-field state, and we examine separately the various constituents of the protocol: the storage and read-out par…
We report an optical memory in a rare earth doped crystal with long storage times, up to 20 ms, together with an optical bandwidth of 1.5 MHz. This is obtained by transferring optical coherences to nuclear spin coherences, which were then protected against environmental noise by dynamical decoupling. With this approach, we achieved a 33 fold increase in spin wave storage time over the intrinsic spin coherence lifetime. Comparison between different decoupling sequences indicates that sequences insensitive to initial spin coherence increase retrieval efficiency. Finally, an interference experime…
We introduce a general scheme to realize perfect quantum state reconstruction and storage in systems of interacting qubits. This novel approach is based on the idea of controlling the residual interactions by suitable external controls that, acting on the inter-qubit couplings, yield time-periodic inversions in the dynamical evolution, thus cancelling exactly the effects of quantum state diffusion. We illustrate the method for spin systems on closed rings with XY residual interactions, showing that it enables the massive storage of arbitrarily large numbers of local states, and we demonstrate …
Quantum memories capable of storing single photons are essential building blocks for quantum information processing, enabling the storage and transfer of quantum information over long distances. Devices operating at room temperature can be deployed on a large scale and integrated into existing photonic networks, but so far warm quantum memories have been susceptible to noise at the single photon level. This problem is circumvented in cold atomic ensembles, but these are bulky and technically complex. Here we demonstrate controllable, broadband and efficient storage and retrieval of weak cohere…
Light storage, the controlled and reversible mapping of photons onto long-lived states of matter [1], enables memory capability in optical quantum networks [2-6]. Prominent storage media are warm alkali gases due to their strong optical coupling and long-lived spin states [7,8]. In a dense gas, the random atomic collisions dominate the lifetime of the spin coherence, limiting the storage time to a few milliseconds [9,10]. Here we present and experimentally demonstrate a storage scheme that is insensitive to spin-exchange collisions, thus enabling long storage times at high atomic densities. Th…
Quantum memories for quantum communication need to be able to store photons for an extended time and then to release them on demand. This can be achieved in atomic frequency comb ensemble based quantum memories by control pulses that transfer the excitation to and from long-lived spin states. However, such pulses can give rise to coherent and incoherent noise due to their interaction with the memory ensemble. In this article, we experimentally demonstrate the ability to switch off the coherent noise from such control pulses during the echo emission in a spin-wave quantum memory, using the line…
We report on a source of heralded narrowband (3MHz) single photons compatible with solid-state spin-wave quantum memories based on praseodymium doped crystals. Widely non-degenerate narrow-band photon pairs are generated using cavity enhanced down conversion. One photon from the pair is at telecom wavelengths and serves as heralding signal, while the heralded single photon is at 606nm, resonant with an optical transition in Pr:YSO. The source offers a heralding efficiency of 28% and a generation rate exceeding 2000 pairs/mW in a single-mode. The single photon nature of the heralded field is co…
Quantum memories are indispensible for establishing a long-distance quantum network. High-dimensional quantum memories enable a higher channel capacity compared to a quantum memory working in a two-dimensional space, and have a lower requirement for storage lifetime in the field of quantum coomunication. The photonic transverse spatial modes such as Laguerra-Gaussian modes orbital angular momentum (OAM) are ideal candidates for encoding high-dimensional information, because it can form an infinite-dimensional Hilbert space. Although the faithful storage of an OAM qubit or qutrit has been reali…
