Controlling the electromagnetic helicity and directionality of the light scattered by dielectric particles is paramount to a variety of phenomenology of interest in all-dielectric optics and photonics. In this Letter, we show that the conservation of the electromagnetic helicity in the scattering by high-index dielectric Mie spheres can be used as a probe of pure-multipolar spectral regions, particularly, of dipolar nature, beyond its presumed spectral interval. This finding reveals that the dipolar behavior is not necessarily limited to small particles, in striking contrast to the current state of the art. Interestingly, we demonstrate that the optimum forward light scattering condition, predicted for a particular nano-sphere in the limit of small particle, is fulfilled in fact at a fixed x size parameter for an infinite number of refractive indexes
A classical way for exploring the scattering behavior of a small sphere is to approximate Mie coefficients with a Taylor series expansion. This ansatz delivered a plethora of insightful results, mostly for small spheres supporting localized plasmonic resonances. However, many scattering aspects are still uncharted, especially with regards to magnetic resonances. Here, an alternative system ansatz is proposed based on the Padé approximants for the Mie coefficients. The result reveal the existence of a self-regulating radiative damping mechanism for the first magnetic resonance and new general r…
Generation of an ultra-bright, deterministic, solid-state single photon source with high photon collection rate is an imperative requirement for quantum technologies. In this direction, various nanophotonic systems coupled with single quantum emitters are being implemented, but results in low decay rate enhancement and MHz photon collection rate. Here, we unravel coherent superposition of excited Mie-scattering moments in a dipolar antenna, coupled with a single nitrogen-vacancy (NV-) center, to achieve bright single photon source with GHz collection rate. Such balancing of Mie-scattering mome…
By combining analytical and numerical approaches, we study resonantly enhanced second-harmonic generation (SHG) by individual high-index dielectric nanoparticles made of centrosymmetric materials. Considering both bulk and surface nonlinearities, we describe second-harmonic nonlinear scattering from a silicon nanoparticle optically excited in the vicinity of the magnetic and electric dipolar resonances. We discuss the contributions of different nonlinear sources, and the effect of the low-order optical Mie modes on the characteristics of the generated far-field. We demonstrate that the multipo…
Tailored multipolar optical trapping with higher-order structured light
The Institute of Optics, University of Rochester（罗切斯特大学光学研究所）；Department of Physics, University of Rochester（罗切斯特大学物理系）；Center for Coherence and Quantum Optics, University of Rochester（罗切斯特大学相干与量子光学中心）
We review three different approaches for the calculation of electromagnetic multipoles, namely the Cartesian primitive multipoles, the Cartesian irreducible multipoles and the spherical multipoles. We identify the latter as the best suited to describe the scattering of electromagnetic radiation, as exemplified for an amorphous silicon sphere. These multipoles are then used to calculate the optical force acting on semiconductor, dielectric or metallic particles in a wide wavelength range, from the dipolar down to the Mie regimes.
The imaginary Poynting momentum (IPM) of light has been captivated an unusual origin of optomechanical effects on dipolar magnetoelectric particles, but yet observed in experiments. Here, we report, for the very first time, a whole family of high-order IPM forces for not only magnetoelectric but also generic Mie particles, assisted with their excited higher multipoles within. Such optomechanical phenomena derive from a nonlinear contribution of the IPM to the optical force, and can be remarkable even when the incident IPM is small. We observe the high-order optomechanics in a structured light …
Besides purely academic interest, giant field enhancement within subwavelength particles at light scattering of a plane electromagnetic wave is important for numerous applications ranging from telecommunications to medicine and biology. In this paper, we experimentally demonstrate the enhancement of the intensity of the magnetic field in a high-index dielectric cylinder at the proximity of the dipolar Mie resonances by more than two orders of magnitude for both the TE and TM polarizations of the incident wave. We present a complete theoretical explanation of the effect and show that the phenom…
All-dielectric resonant nanophotonics is a rapidly developing research field driven by its exceptional application potential for low-loss nanoscale metadevices. The tight confinement of the local electromagnetic fields and interferences in resonant photonic nanostructures can boost many optical effects, thus offering novel opportunities for the subwavelength control of light-matter-interactions. Active, light-emitting nanoscale structures are of particular interest, as they offer unique opportunities for novel types of light sources and nanolasers. Here, we review the latest advances in this r…
The exciting properties of high index dielectric nanoparticles exhibiting both electric and magnetic Mie resonances are nowadays paving the way towards efficient light manipulation at the nanoscale. A commonly disregarded peculiarity of light scattering by Mie particles is their ability to extract angular momentum from the incident electromagnetic field. In this work, we have investigated numerically and analytically the angular momentum transfer from a circularly polarized plane wave to the transversely scattered field generated by a high index cube. Therefore, the tangential components of th…
Featured with a plethora of electric and magnetic Mie resonances, high index dielectric nanostructures offer a versatile platform to concentrate light-matter interactions at the nanoscale. By integrating unique features of far-field scattering control and near-field concentration from radiationless anapole states, here, we demonstrate a giant photothermal nonlinearity in single subwavelength-sized silicon nanodisks. The nanoscale energy concentration and consequent near-field enhancements mediated by the anapole mode yield a reversible nonlinear scattering with a large modulation depth and a b…
We investigate electromagnetic scattering of normally irradiated gyrotropic, magneto-optical core-shell cylinders using Lorenz-Mie theory. A general expression for time-averaged electromagnetic energy inside a coated gyroelectric and gyromagnetic scatterer is derived. Using realistic material parameters for a silica core and InSb shell, we calculate the stored electromagnetic energy and the scattering anisotropy. We show that the application of an external magnetic field along the cylinder axis induces a drastic decrease in electromagnetic absorption in a frequency range in the terahertz, wher…
