The multi-scale computational method of combining first-principles calculation and finite element electromagnetic simulations is used to study plasmon-enhanced interlayer charge transfer (ICT) exciton of 2D lateral and van der Waals MoS2/WS2 heterostructure with 2H phase. The weak ICT excitons are observed in the 2H lateral and van der Waals MoS$_2$/WS$_2$ heterostructures. Theoretical results reveal the physical principle of plexciton resulting from strong coupling between plasmonic and ICT exciton. The weak CT exciton can be strongly enhanced by metal plasmon, can provide a new way to observe the weak CT exciton. Our results can promote deeper understanding of the plexciton resulting from strong coupling interaction between plasmon and exciton of lateral and van der Waals heterostructures.
We show that the optical force exerted on a finite size chiral sphere by a surface plasmon mode has a component along a direction perpendicular to the plasmon linear momentum. We reveal how this chiral lateral force, pointing in opposite directions for opposite enantiomers, stems from an angular-to-linear crossed momentum transfer involving the plasmon transverse spin angular momentum density and mediated by the chirality of the sphere. Our multipolar approach allows us discussing the inclusion of the recoil term in the force on a small sphere taken in the dipolar limit and observing sign inve…
We investigate lateral recoil forces exerted on nanoparticles located near plasmonic platforms with in-plane nonreciprocal response. To this purpose, we first develop a comprehensive theoretical framework based on the Lorentz force within the Rayleigh approximation combined with nonreciprocal Green's functions and then derive approximate analytical expressions to model lateral recoil forces, demonstrating their explicit dependence on the dispersion relation of the system and unveiling the mechanisms that govern them. In particular, a dominant lateral recoil force component appears due to the m…
Lateral two-dimensional (2D) transitional metal dichalcogenide (TMD) heterostructures have recently attracted a wide attention as promising materials for optoelectronic nanodevices. Due to the nanoscale width of lateral heterojunctions, the study of their optical properties is challenging and requires using subwavelength optical characterization techniques. We investigated the photoresponse of a lateral 2D WSe2/MoSe2 heterostructure using tip-enhanced photoluminescence (TEPL) with nanoscale spatial resolution and with picoscale tip-sample distance dependence. We demonstrate the observation of …
We study theoretically the influence of the surface plasmon excitation on the Goos-Hänchen lateral shift of a $p$-polarized Gaussian beam incident obliquely on a dielectric-metal bilayer in the Otto configuration. We find that the lateral shift depends sensitively on the thickness of the metal layer and the width of the incident beam, as well as on the incident angle. Near the incident angle at which surface plasmons are excited, the lateral shift changes from large negative values to large positive values as the thickness of the metal layer increases through a critical value. For wide inciden…
The negative shifts seen by Wang and Zhu are not due to the excitation of surface plasmons but to leaky modes of the slab propagating backward. Provided the characteristics of the LHM slab are chosen correctly, it is shown that a leaky surface plasmon can actually be excited using the KR configuration.
The ability to create high-quality lateral p-n junctions at nanometer length scales is essential for the next generation of two-dimensional (2D) electronic and plasmonic devices. Using a charge-transfer heterostructure consisting of graphene on $α$-RuCl$_3$, we conduct a proof-of-concept study demonstrating the existence of intrinsic nanoscale lateral p-n junctions in the vicinity of graphene nanobubbles. Our multi-pronged experimental approach incorporates scanning tunneling microscopy (STM) and spectroscopy (STS) and scattering-type scanning near-field optical microscopy ($\textit{s}$-SNOM) …
The hybrid modes incorporating surface phonon polariton (SPhP) modes in boron nitride nanotubes (BNNTs) and surface plasmon polariton (SPP) modes in graphene monolayers are theoretically studied. The combination of the 1D BNNTs and 2D graphene monolayer further improves the modal characteristics with electrical tunability. Superior to the graphene monolayers, the proposed heterostructures supports single mode transmission with lateral optical confinement. The modal characteristics can be shifted from SPP-like toward SPhP-like. Both the figure of merit and field enhancement of hybrid modes are …
The plasmon-mediated manipulation of light-matter interaction in two-dimensional atomically transition-metal dichalcogenides (TMDs) critically depends on the design of plasmonic nanostructures to achieve the maximum optical field in TMDs. Here, a metal-isolator-metal Salisbury-type perfect absorber was fabricated to serve as a generator of the localized surface plasmons. The significant photoluminescence (PL) enhancement up to 60-fold was observed experimentally in the monolayer (ML) MoS2 on the top of this gold plasmonic hybrid nanostructures. Furthermore, the PL linear polarization can appro…
Photonic integrated circuits are an enabling technology in modern communications systems. The continually increasing demands for higher-speed and lower operating power devices have resulted in the continued impetus to shrink photonic components. In this work, we demonstrate a primitive nanophotonic integrated circuit element composed of a single silver nanowire and single-layer molybdenum disulfide (MoS2) flake. We show that nanowire plasmons can excite MoS2 photoluminescence via direct plasmon-to-exciton conversion along the wire and plasmon-to-photon-to-exciton conversion at the MoS2-covered…
Plasmon-Enhanced Second-Harmonic Generation in Atomically Thin Crystalline Silver Nanostructures
ICFO–Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology（ICFO-光子科学研究所，巴塞罗那科学技术研究院）；University of Vienna, Faculty of Physics, Vienna Center for Quantum Science and Technology (VCQ)（维也纳大学物理学院，维也纳量子科学与技术中心）；Center for Nanophotonics, NWO Institute AMOLF（纳米光子学中心，NWO AMOLF研究所）；Department of Physics, Dokuz Eylül University（德古兹埃勒大学物理系）；Centro de Física de Materiales CSIC-UPV/EHU and Materials Physics Center（CSIC-巴斯克国立大学物质物理学中心和材料物理中心）
Strong interactions between surface plasmons in ultra-compact nanocavities and excitons in two dimensional materials have attracted wide interests for its prospective realization of polariton devices at room temperature. Here, we propose a continuous transition from weak coupling to strong coupling between excitons in MoS2 monolayer and highly localized plasmons in ultra-compact nanoantenna. The nanoantenna is assembled by a silver nanocube positioned over a gold film and separated by a dielectric spacer layer. We observed a 1570-fold enhancement in the photoluminescence at weak coupling regim…
Hybrid systems of excitons strongly coupled to localized surface plasmons supported by metallic nanoparticles define a new approach to control light-matter interactions. Here, we report exciton-plasmon coupling in two-dimensional (2D) semiconductors, such as MoS2 and WS2, hybridized with silver nanoparticles. Prominent photoluminescence enhancement in monolayer MoS2 was observed with localized surface plasmon resonance (LSPR) tuned to the exciton resonance. By tuning the excitation energy, the contributions from near field enhancement and radiative emission rate enhancement via Purcell effect …
A surface plasmon resonance imaging biosensor based on $\text{MoS}_2$ deposited on Aluminium substrate is designed for high imaging sensitivity and detection accuracy. The proposed biosensor exhibits better performance than graphene-based biosensor in the near-infrared regime. A high imaging sensitivity of more than 970 $\text{RIU}^{-1}$ is obtained at the wavelength of 1540 nm. The effect of aluminium thickness, number of $\text{MoS}_2$ layers and the refractive index of sensing layer are investigated to obtain an optimized design for high sensor performance. In addition, the sensor performan…
We demonstrate strong exciton-plasmon coupling in silver nanodisk arrays integrated with monolayer MoS2 via angle-resolved reflectance microscopy spectra of the coupled system. Strong exciton-plasmon coupling is observed with the exciton-plasmon coupling strength up to 58 meV at 77 K, which also survives at room temperature. The strong coupling involves three types of resonances: MoS2 excitons, localized surface plasmon resonances (LSPRs) of individual silver nanodisks and plasmonic lattice resonances of the nanodisk array. We show that the exciton-plasmon coupling strength, polariton composit…
Molybdenum disulfide (MoS2) monolayers have attracted much attention for their novel optical properties and efficient light-matter interactions. When excited by incident laser, the optical response of MoS2 monolayers was effectively modified by elementary photo-excited excitons owing to their large exciton binding energy, which can be facilitated for the optical-controllable exciton-plasmon interactions. Inspired by this concept, we experimentally investigated active light control of surface plasmon resonance (SPR) in MoS2-Ag hybrid nanostructures. The white light spectra of SPR were gradually…
Plasmon decay via the surface or interface is a critical process for practical energy conversion and plasmonic catalysis. However, the relationship between plasmon damping and the coupling between the plasmon and 2D materials is still unclear. The spectral splitting due to plasmon-exciton interaction impedes the conventional single-particle method to evaluate the plasmon damping rate by the spectral linewidth directly. Here, we investigated the interaction between a single gold nanorod (GNR) and 2D materials using the single-particle spectroscopy method assisted with in situ nanomanipulation t…
The advance in designing arrays of ultrathin two-dimensional optical nano-resonators, known as metasurfaces, is currently enabling a large variety of novel flat optical components. The remarkable control over the electromagnetic fields offered by this technology can be further extended to the active regime in order to manipulate the light characteristics in real-time. In this contribution, we couple the excitonic resonance of atomic thin MoS2 monolayers with gap-surface-plasmon (GSP) metasurfaces, and demonstrate selective enhancement of the exciton-plasmon polariton emissions. We further demo…
Here, we experimentally demonstrate an Indium Tin Oxide (ITO) Mach-Zehnder interferometer heterogeneously integrated in silicon photonics. The phase shifter section is realized in a novel lateral MOS configuration, which, due to favorable electrostatic overlap, leads to efficient modulation (VπL = 63 Vum). This is achieved by (i) selecting a strong index changing material (ITO) and (ii) improving the field overlap as verified by the electrostatic field lines. Furthermore, we show that this platform serves as a building block in an endfire silicon photonics optical phased array (OPA) with a hal…
