We extend a field theoretic approach for the investigation of the electronic charge-current density response of crystalline systems to arbitrary applied electromagnetic fields. The approach leads to the introduction of microscopic polarization and magnetization fields, as well as free charge and current densities, the dynamics of which are described by a lattice gauge theory. The spatial averages of such quantities constitute the fields of macroscopic electrodynamics. We implement this formalism to study the orbital electronic response of a class of insulators to applied uniform dc electric and magnetic fields at zero temperature. To first-order in the applied fields, the free charge and current densities vanish; thus the response of the system is characterized by the first-order modifications to the microscopic polarization and magnetization fields. Associated with the dipole moment of the microscopic polarization (magnetization) field is a macroscopic polarization (magnetization), for which we extract various response tensors. We focus on the orbital magnetoelectric polarizability (OMP) tensor, and find the accepted expression as derived from the "modern theory of polarization and magnetization." Since our results are based on the spatial averages of microscopic fields, we can identify the distinct contributions to the OMP tensor from the perspective of this microscopic theory, and we establish the general framework in which extensions to finite frequency can be made.
The orbital motion of electrons in a three-dimensional solid can generate a pseudoscalar magnetoelectric coupling $θ$, a fact we derive for the single-particle case using a recent theory of polarization in weakly inhomogeneous materials. This polarizability $θ$ is the same parameter that appears in the "axion electrodynamics" Lagrangian $Δ{\cal L}_{EM} = (θe^2 / 2 πh) {\bf E} \cdot {\bf B}$, which is known to describe the unusual magnetoelectric properties of the three-dimensional topological insulator ($θ=π$). We compute $θ$ for a simple model that accesses the topological insulator and discu…
We study the response of topological insulator films to strong magnetic and electric fields beyond the linear response theory. As a model, we use the three-dimensional lattice Wilson-Dirac Hamiltonian where we simultaneously introduce both magnetic field through the Peierls substitution and electric field as a potential energy depending on lattice coordinate. We compute the electron energy spectrum by numerically diagonalizing this Hamiltonian and obtain quantized magnetoelectric polarizability. In addition, we find that the magnetoelectric effect vanishes as the film width decreases due to th…
In this paper we develop a fully microscopic theory of the polarizability of excitons in transition metal dichalcogenides. We apply our method to the description of the excitation $2$p dark states. These states are not observable in absorption experiments but can be excited in a pump-probe experiment. As an example we consider $2$p dark states in WSe\textsubscript{2}. We find a good agreement between recent experimental measurements and our theoretical calculations.
A theory of the anomalous and spin Hall effects, based on the space distribution of the current densities, is presented. Spin-orbit coupling gives rise to a space separation of the mass centers, as well as a current density separation of the quasiparticle states having opposite group velocities. It is shown that this microscopic property is essential for existence of both Hall effects.
We study small conducting particles and thin films in an oscillating longitudinal electric field. We find the charge, current, and field distribution in the particle, the polarizability and the electric dipole absorption. We account for Thomas-Fermi screening by adding a Fick's diffusion term to Ohm's law. Alternatively, we describe a particle as a dielectric body with a non-local dielectric constant which is derived in a microscopic linear-response theory. We show that both approaches are equivalent.
It is shown that external magnetic field or magnetization induces electric polarization of microscopic isolated magnetic/non-magnetic hybrid structures due to the spin-dependent electron redistribution and mutual capacity. The magnetoelectric effect can be very strong, for instance the change of electric polarization reaches $100$ $μC/m^{2}$ at a constant magnetic field of only $1.5$ Tesla in the case of $100$ $÷$ $10$ nanometer structures which tightly fill the space, composing a metamaterial. The effect does not require using exotic compounds. Based on the obtained results we suggest a numbe…
We apply a microscopic theory of polarization and magnetization to crystalline insulators at zero temperature and consider the orbital electronic contribution of the linear response to spatially varying, time-dependent electromagnetic fields. The charge and current density expectation values generally depend on both the microscopic polarization and magnetization fields, and on the microscopic free charge and current densities. But contributions from the latter vanish in linear response for the class of insulators we consider. Thus we need only consider the former, which can be decomposed into …
The Ginzburg-Landau free energy of a conventional superconductor coupled to a helimagnet is microscopically derived using functional field integral techniques. We show that the spin texture leads to a Lifshitz invariant in the free energy, which couples the momentum density of the superconducting condensate to the magnetization of the helimagnet. For helimagnets with a conical texture, the Lifshitz invariant yields a spatial modulation of the superconducting phase along the helical wavevector of the magnetic texture. Based on self-consistent numerical calculations, we verify the theoretical fo…
Ferromagnet-ferroelectric-metal superlattices are proposed to realize the large room-temperature magnetoelectric effect. Spin dependent electron screening is the fundamental mechanism at the microscopic level. We also predict an electric control of magnetization in this structure. The naturally broken inversion symmetry in our tri-component structure introduces a magnetoelectric coupling energy of $P M^2$. Such a magnetoelectric coupling effect is general in ferromagnet-ferroelectric heterostructures, independent of particular chemical or physical bonding, and will play an important role in th…
We discuss the problem of equilibrium spin currents in ferromagnets with inhomogeneous magnetization. Using simple microscopic models we explain the physical origin of equilibrium spin currents. Next we derive the equilibrium spin current from the Hamiltonian with a gauge field associated with local rotations in the spin space. Several examples of magnetic systems are studied in details, and the persistent spin current is found to exist in the ground state of these systems. We also demonstrate the possibility to measure the equilibrium spin current using the magnetoelectrically induced electri…
Composite multiferroics, heterostructures of ferromagnetic (FM) and ferroelectric (FE) materials, are characterized by a remarkable magnetoelectric effect at the interface. Previous work has supported the ferromagnetic structure with magnetic spins and the ferroelectric with pseudospins which act as electric dipoles in a microscopic model, coupled with a magnetoelectric interaction [J. Appl. Phys. 118, 124109 (2015)]. In this work, by solving the stochastic Landau-Lifshitz-Gilbert equation, the electric-field-induced magnetization switching in a twisted boundary condition has been studied, and…
The orbital magnetoelectric effect (OME) generically refers to the appearance of an orbital magnetization induced by an applied electric field. Here, we show that nanoribbons of transition metal dichalcogenides (TMDs) with zigzag (ZZ) edges may exhibit a sizeable OME activated by an electric field applied along the ribbons' axis. We examine nanoribbons extracted from a monolayer (1L) and a bilayer (2L) of MoS$_2$ in the trigonal (H) structural phase. Transverse profiles of the induced orbital angular momentum accumulations are calculated to first order in the longitudinally applied electric fi…
Magnetoelectric flat band induced by a $\sqrt{3}\times\sqrt{3}$ charge density wave in monolayer CrSe$_2$
Universidade de Santiago de Compostela（圣地亚哥-德孔波斯特拉大学）；Instituto de Materiais iMATUS, Universidade de Santiago de Compostela（圣地亚哥-德孔波斯特拉大学iMATUS材料研究所）；International Iberian Nanotechnology Laboratory (INL)（伊比利亚纳米技术国际实验室）；Center for Research in Biological Chemistry and Molecular Materials CIQUS, Universidade de Santiago de Compostela（圣地亚哥-德孔波斯特拉大学CIQUS生物化学与分子材料研究中心）；Aalto University（阿尔托大学）；Donostia International Physics Center (DIPC)（多诺斯蒂亚国际物理中心）；IKERBASQUE, Basque Foundation for Science（巴斯克科学基金会 IKERBASQUE）
We study the interaction between a topological insulator nanoparticle and a quantum dot subject to an applied electric field. The electromagnetic response of the topological insulator is derived from axion electrodynamics in the quasistatic approximation. Localized modes are quantized in terms of dipolar bosonic modes, which couples dipolarly to the quantum dot. Hence, we treat the hybrid as a two-level system interacting with a single bosonic mode, where the coupling strength encodes the information concerning the nontrivial topology of the nanoparticle. The interaction of the hybrid with the…
We present a general microscopic first-principles method to study the Coulomb-interaction-mediated heat transfer in the near field. Using the nonequilibrium Green's function formalism, we derive Caroli formulas for heat transfers between materials with translational invariance. The central physical quantities are the screened Coulomb potential and the spectrum function of polarizability. Within the random phase approximation, we calculate the polarizability using the linear response density functional theory and obtain the screened Coulomb potential from a retarded Dyson equation. We show that…
Quantum Geometric Origin of Nonlinear Current Induced Orbital Magnetization
University of Macau（澳门大学）；Great Bay University（大湾区大学）；Great Bay Institute for Advanced Study（大湾区高等研究院）；Fudan University（复旦大学）；Max Planck Institute for Chemical Physics of Solids（马克斯·普朗克固体化学物理研究所）；University of Science and Technology of China（中国科学技术大学）；The Hong Kong Polytechnic University（香港理工大学）
We investigate a valleytronic device based on graphene with charge separation at different sublattices and correspondingly at nonequivalent valleys. We characterize the maximality condition of valley polarization and investigate the parameters and conditions upon which we can coherently control the carriers and store data via valley degree of freedom. The valley polarization is controlled by the amplitude as well as the carrier envelope phase of the pulse and the curvature of the electron trajectory in the reciprocal space. When strong field excitation is taken into account, the optical select…
The recently predicted topological magnetoelectric effect and the response to an electric charge that mimics an induced mirror magnetic monopole are fundamental attributes of topological states of matter with broken time reversal symmetry. Using a SQUID-on-tip, acting simultaneously as a tunable scanning electric charge and as ultrasensitive nanoscale magnetometer, we induce and directly image the microscopic currents generating the magnetic monopole response in a graphene quantum Hall electron system. We find a rich and complex nonlinear behavior governed by coexistence of topological and non…
