We theoretically explore the RKKY interaction mediated by spin-3/2 quasiparticles in half-Heusler topological semimetals in quasi-two-dimensional geometries. We find that while the Kohn-Luttinger terms gives rise to generalized Heisenberg coupling of the form ${\cal H}_{\rm RKKY} \propto σ_{1,i} {\cal I}_{ij} σ_{2,j}$ with a symmetric matrix ${\cal I}_{ij}$, addition of small antisymmetric linear spin-orbit coupling term leads to Dzyaloshinskii-Moriya (DM) coupling with an antisymmetric matrix ${\cal I}'_{ij}$. We demonstrate that besides the oscillatory dependence on the distance, all coupling strengths strongly depend on the relative orientation of the two impurities with respect to the lattice. This yields a strongly anisotropic behavior for ${\cal I}_{ij}$ such that by only rotating one impurity around another at a constant distance, we can see further oscillations of the RKKY couplings. This unprecedented effect is unique to our system which combines spin-orbit coupling with strongly anisotropic Fermi surfaces. We further find that all of the RKKY terms have two common features: a tetragonal warping in their map of spatial variations, and a complex beating pattern. Intriguingly, all these features survive in all dopings and we see them in both electron- and hole-doped cases. In addition, due to the lower dimensionality combined with the effects of different spin-orbit couplings, we see that only one symmetric off-diagonal term, ${\cal I}_{xy}$ and two DM components ${\cal I}'_{xz}$ and ${\cal I}'_{yz}$ are nonvanishing, while the remaining three off-diagonal components are identically zero. This manifests another drastic difference of RKKY interaction in half-Heusler topological semimetals compared to the electronic systems with spin-1/2 effective description.
We study the RKKY interaction between two magnetic impurities located on the surface of a three-dimensional Dirac semimetal with two Dirac nodes in the band structure. By taking into account both bulk and surface contributions to the exchange interaction between the localized spins, we demonstrate that the surface contribution in general dominates the bulk one at distances larger than the inverse node separation due to a weaker power-law decay. We find a strong anisotropy of the surface term with respect to the spins being aligned along the node separation axis or perpendicular to it. In the m…
We have systematically investigated the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction between two magnetic impurities in Weyl semimetals with arbitrary monopole charge $Q$. We find that the RKKY interaction becomes intrinsically anisotropic for $Q\geq2$, and its dependence on Fermi energy and impurity separation is directly controlled by the monopole charge. With the increase of $Q$, the RKKY interaction becomes more long-ranged and more anisotropic, which makes interesting magnetic orders easier to form and thus may have important applications in spintronics.
We theoretically study the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction between magnetic impurities in both Dirac and Weyl semimetals (SMs). We find that the internode process, as well as the unique three-dimensional spin-momentum locking, has significant influences on the RKKY interaction, resulting in both a Heisenberg and an Ising term, and an additional Dzyaloshinsky-Moriya term if the inversion symmetry is absent. These interactions can lead to rich spin textures and possible ferromagnetism in Dirac and time-reversal symmetry-invariant Weyl SMs. The effect of anisotropic Dirac and Wey…
Ruderman-Kittel-Kasuya-Yosida (RKKY) is an essential long range magnetic interaction between magnetic impurities or magnetic layered structures, the magnitude of which oscillates with the distance ($\mathrm{R}$) between them. We have investigated the RKKY interaction between two magnetic impurities in both time-reversal and inversion symmetry broken Weyl semimetals (WSMs) where the energy dispersion is tilted in momentum space and the momentum of the conduction electron is locked with the pseudo-spin. Two important features are revealed, firstly, at the small tilt limit, we show that the RKKY …
We consider the effective coupling between impurity spins on surfaces of a thin-film Weyl semimetal within Ruderman-Kittel-Kasuya-Yoshida (RKKY) theory. If the spins are on the same surface, their coupling reflects the anisotropy and the spin-momentum locking of the Fermi arcs. By contrast when the spins are on opposite surfaces, their coupling is mediated by the Fermi arcs as well as by bulk states. In this case the coupling is both surprisingly strong and strongly thickness dependent, with a maximum at an optimum thickness. We demonstrate our results using analytical solutions of states in t…
We investigate the response of 3D Luttinger semimetals to localized charge and spin impurities as a function of doping. The strong spin-orbit coupling of these materials strongly influences the Friedel oscillations and RKKY interactions. This can be seen at short distances with an $1/r^4$ divergence of the responses, and anisotropic behavior. Certain of the spin-orbital signatures are robust to temperature, even if the charge and spin oscillations are smeared out, and give an unusual diamagnetic Pauli susceptibility. We compare our results to the experimental literature on the bismuth-based ha…
The Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction has been extensively explored in isotropic Dirac systems with linear dispersion, which typically follows an exponent decaying rate with the impurity distance $R$, i.e., $J\propto 1/R^d$ ($1/R^{2d-1}$) in $d$-dimensional systems at finite (zero) Fermi energy. This fast decay makes it rather difficult to be detected and limits its application in spintronics. Here, we theoretically investigate the influence of anisotropic dispersion on the RKKY interaction, and find that the introduction of non-relativistic dispersion in semi-Dirac semimetals (…
We theoretically investigate the features of Ruderman-Kittel-Kasuya-Yosida (RKKY) exchange interaction between two magnetic impurities, mediated by the interfacial bound states inside a domain wall (DW). The latter separates the two regions with oppositely signed inversion symmetry broken terms in graphene and Weyl semimetal. The DW is modelled by a smooth quantum well which hosts a number of discrete bound states including a pair of gapless, metallic zero-energy modes with opposite chiralities. We find clear signatures of these interfacial chiral bound states in spin response (RKKY exchange i…
Half-Heusler alloy topological semimetal YPtBi is a promising candidate for an efficient spin source material having both large spin Hall angle $θ$$_{SH}$ and high thermal stability. However, high-quality YPtBi thin films with low bulk carrier density are usually grown at 600$°$C, which exceeds the limitation of 400$°$C for back end of line (BEOL) process. Here, we investigate the crystallinity and spin Hall effect of YPtBi thin films grown at lower growth temperature down to 300$°$C. Although $θ$$_{SH}$ degraded with lowering the growth temperature to 300$°$C due to degradation of the crystal…
In this work, we construct a generalized Kane model with a new coupling term between itinerant electron spins and local magnetic moments of anti-ferromagnetic ordering in order to describe the low energy effective physics in a large family of anti-ferromagnetic half-Heusler materials. Topological properties of this generalized Kane model is studied and a large variety of topological phases, including Dirac semimetal phase, Weyl semimetal phase, nodal line semimetal phase, type-B triple point semimetal phase, topological mirror (or glide) insulating phase and anti-ferromagnetic topological insu…
It has recently been demonstrated that various topological states, including Dirac, Weyl, nodal-line, and triple-point semimetal phases, can emerge in antiferromagnetic (AFM) half-Heusler compounds. However, how to determine the AFM structure and to distinguish different topological phases from transport behaviors remains unknown. We show that, due to the presence of combined time-reversal and fractional translation symmetry, the recently proposed second-order nonlinear Hall effect can be used to characterize different topological phases with various AFM configurations. Guided by the symmetry …
Topological materials, such as topological insulators (TIs), have great potential for ultralow power spintronic devices, thanks to their giant spin Hall effect. However, the giant spin Hall angle ($θ_{SH}$ > 1) is limited to a few chalcogenide TIs with toxic elements and low melting points, making them challenging for device integration during the silicon Back-End-of-Line (BEOL) process. Here, we show that by using a half-Heusler alloy topological semi-metal (HHA-TSM), YPtBi, it is possible to achieve both a giant $θ_{SH}$ up to 1.6 and a high thermal budget up to 600$°$C. We demonstrate magne…
The $\mathrm{Co_2}$ family of ferromagnetic Heusler alloys have attracted interest due to their fully spin-polarized nature, making them ideal for applications in spintronic devices. More recently, the existence of room temperature time-reversal-breaking Weyl nodes near the Fermi level was predicted and confirmed in these systems. As a result of the presence of these Weyl nodes, these systems possess a non-zero momentum space Berry curvature that can dramatically influence transport properties such as the anomalous Hall effect. One of these candidate compounds is $\mathrm{Co_2 Ti Ge}$. Recentl…
Recently, abundant transport phenomena characterizing the surface states of Weyl semimetals (WSMs) have been reported. To generate these phenomena, electrons have to complete a closed intersurface orbit. Due to the unavoidable impurities in real materials, this orbit would be destroyed by the impurity scattering, which limits the detection of the surface states in WSMs. Here, we investigate the RKKY interaction between magnetic impurities, solely mediated by a single surface band, in semi-infinite WSMs. It is found that peculiar oscillations and slowly decaying laws of the RKKY interaction can…
Topological materials often exhibit remarkably linear, non-saturating magnetoresistance (LMR), which is both of scientific and technological importance. However, the role of topologically non-trivial states in the emergence of such a behaviour has eluded clear demonstration in experiments. Here, by reducing the coupling between the topological surface states (TSS) and the bulk carriers we controllably tune the LMR behavior in Pt1-xAuxLuSb into distinct plateaus in Hall resistance, which we show arise from a quantum Hall phase. This allowed us to reveal how smearing of the Landau levels, which …
We theoretically study the impacts of linear spin-orbit coupling (SOC) on the Ruderman-Kittel-Kasuya-Yosida interaction between magnetic impurities in two kinds of three-dimensional noncentrosymmetric systems. It has been found that linear SOCs lead to the Dzyaloshinskii-Moriya interaction and the Ising interaction, in addition to the conventional Heisenberg interaction. These interactions possess distinct range functions from three dimensional electron gases and Dirac/Weyl semimetals. In the weak SOC limit, the Heisenberg interaction dominates over the other two interactions in a moderately l…
We calculate the temperature dependent long-range magnetic coupling in the presence of dilute concentrations of random magnetic impurities in chiral multilayer two-dimensional semimetals, i.e., undoped intrinsic multilayer graphene. Assuming a carrier-mediated indirect RKKY exchange interaction among the well-separated magnetic impurities with the itinerant carriers mediating the magnetic interaction between the impurities, we investigate the magnetic properties of intrinsic multilayer graphene using an effective chiral Hamiltonian model. We find that due to the enhanced density of states in t…
The noncentrosymmetric Half Heusler compound YPtBi exhibits superconductivity below a critical temperature T_c = 0.77 K with a zero-temperature upper critical field H_c2(0) = 1.5 T. Magnetoresistance and Hall measurements support theoretical predictions that this material is a topologically nontrivial semimetal having a surprisingly low positive charge carrier density of 2 x 10^18 cm^-3. Unconventional linear magnetoresistance and beating in Shubnikov-de Haas oscillations point to spin-orbit split Fermi surfaces. The sensitivity of magnetoresistance to surface roughness suggests a possible con…
Topological semimetals can be classified by the connectivity and dimensionality of the band cross- ing in momentum space. The band crossings of a Dirac, Weyl, or an unconventional fermion semimet- al are 0D points, whereas the band crossings of a nodal-line semimetal are 1D closed loops. Here we propose that the presence of perpendicular crystalline mirror planes can protect 3D band crossings characterized by nontrivial links such as a Hopf link or a coupled-chain, giving rise to a variety of new types of topological semimetals. We show that the nontrivial winding number protects topolog- ical…
We investigate topological Cooper pairing, including gapless Weyl and fully gapped class DIII superconductivity, in a three-dimensional doped Luttinger semimetal. The latter describes effective spin-3/2 carriers near a quadratic band touching and captures the normal-state properties of the 227 pyrochlore iridates and half-Heusler alloys. Electron-electron interactions may favor non-$s$-wave pairing in such systems, including even-parity $d$-wave pairing. We argue that the lowest energy $d$-wave pairings are always of complex (e.g., $d + i d$) type, with nodal Weyl quasiparticles. This implies …
Pure spin currents carry information in quantum spintronics and could play an essential role in the next generation low-energy-consumption electronics. Here we theoretically predict that the magnetic field can induce a quantum spin current without a concomitant charge current in metals without time reversal symmetry $\mathcal{T}$ and inversion symmetry $\mathcal{P}$ but respect the combined $\mathcal{PT}$ symmetry. It is governed by the magnetic moment of the Bloch states on the Fermi surface, and can be regarded as a spinful generalization of the gyrotropic magnetic effect in $\mathcal{P}$-br…
Large intrinsic anomalous Hall effect (AHE) due to the Berry curvature in magnetic topological semimetals is attracting enormous interest due to its fundamental importance and technological relevance. Mechanisms resulting in large intrinsic AHE include diverging Berry curvature in Weyl semimetals, anticrossing nodal rings or points of non-trivial bands, and noncollinear spin structures. Here we show that a half-topological semimetal (HTS) state near a topological critical point can provide a new mechanism for driving an exceptionally large AHE. We reveal this through a systematic experimental …
We compute the effects of electronic interactions on gapless spin-3/2 excitations that in a noninteracting system emerge at a bi-quadratic touching of Kramers degenerate valence and conduction bands, known as Luttinger semimetal. This model can describe the low-energy physics of HgTe, gray-Sn, 227 pyrochlore iridates and half-Heuslers. For the sake of concreteness we only consider the short-range components of the Coulomb interaction. By combining mean-field analysis with a renormalization group (RG) calculation, we construct multiple cuts of the global phase diagram of interacting spin-3/2 fe…
The half-Heusler rare-earth intermetallic GdPtBi has recently gained attention due to peculiar magnetotransport phenomena that have been associated with the possible existence of Weyl fermions, thought to arise from the crossings of spin-split conduction and valence bands. On the other hand, similar magnetotransport phenomena observed in other rare-earth intermetallics have often been attributed to the interaction of itinerant carriers with localized magnetic moments stemming from the $4f$-shell of the rare-earth element. In order to address the origin of the magnetotransport phenomena in GdPt…
Recently, the notion of topological phases of matter has been extended to higher-order incarnations, supporting gapless modes on even lower dimensional boundaries, such as corners and hinges. We here identify a collection of cubic spin-3/2 fermions with biquadratic touching of Kramers degenerate valence and conduction bands as a platform to strain-engineer higher-order topological (HOT) phases: external uniaxial strain gives birth to a HOT Dirac semimetal or an insulator, depending on its sign, featuring topological \emph{hinge} modes in the strain direction. The insulator in fact exhibits \em…
