Laser-Induced Transient Magnons in Sr3Ir2O7 Throughout the Brillouin Zone
D. G. Mazzone, D. Meyers, Y. Cao, J. G. Vale, C. D. Dashwood, Y. Shi, A. J. A. James, N. J. Robinson, J. Q. Lin, V. Thampy, Y. Tanaka, A. S. Johnson, H. Miao, R… 展开作者
D. G. Mazzone, D. Meyers, Y. Cao, J. G. Vale, C. D. Dashwood, Y. Shi, A. J. A. James, N. J. Robinson, J. Q. Lin, V. Thampy, Y. Tanaka, A. S. Johnson, H. Miao, R. Wang, T. A. Assefa, J. Kim, D. Casa, R. Mankowsky, D. Zhu, R. Alonso-Mori, S. Song, H. Yavas, T. Katayama, M. Yabashi, Y. Kubota S. Owada, J. Liu, J. Yang, R. M. Konik, I. K. Robinson, J. P. Hill, D. F. McMorrow, M. Forst, S. Wall, X. Liu, M. P. M. Dean
备注：
6 pages, 4 figures, not including supplemental material; accepted in PNAS
Although ultrafast manipulation of magnetism holds great promise for new physical phenomena and applications, targeting specific states is held back by our limited understanding of how magnetic correlations evolve on ultrafast timescales. Using ultrafast resonant inelastic x-ray scattering we demonstrate that femtosecond laser pulses can excite transient magnons at large wavevectors in gapped antiferromagnets, and that they persist for several picoseconds which is opposite to what is observed in nearly gapless magnets. Our work suggests that materials with isotropic magnetic interactions are preferred to achieve rapid manipulation of magnetism.
Inelastic neutron scattering is used to measure spin excitations in fully deuterated single crystal samples of the strong-leg antiferromagnetic S=1/2 spin ladder compound (C$_7$H$_{10}$N)$_2$CuBr$_4$. Sharp resolution-limited magnons are observed across the entire one-dimensional Brillouin zone. The results validate the previously proposed {\it symmetric} spin ladder model and provide a reliable estimate of the relevant exchange interactions.
We use a neutron spin-echo method with $μ$eV resolution to determine the lifetimes of spin waves in the prototypical antiferromagnet MnF$_2$ over the entire Brillouin zone. A theory based on the interaction of magnons with longitudinal spin fluctuations provides an excellent, parameter-free description of the data, except at the lowest momenta and temperatures. This is surprising, given the prominence of alternative theories based on magnon-magnon interactions in the literature. The results and technique open up a new avenue for the investigation of fundamental concepts in magnetism. The techn…
The spectral distribution of parametrically excited dipole-exchange magnons in an in-plane magnetized epitaxial film of yttrium-iron garnet was studied by means of frequency- and wavevector-resolved Brillouin light scattering spectroscopy. The experiment was performed in a parallel pumping geometry where an exciting microwave magnetic field was parallel to the magnetizing field. It was found that for both dipolar and exchange spectral areas parallel pumping excites the lowest volume magnon modes propagating in the film plane perpendicularly to the magnetization direction. In order to interpret…
Due to the small photon momentum, optical spectroscopy commonly probes magnetic excitations only at the center of the Brillouin zone; however, there are ways to override this restriction. In the case of the distorted kagome quantum magnet Y-kapellasite, Y$_3$Cu$_9$(OH)$_{19}$Cl$_8$, under scrutiny here, the magnon density of states can be accessed over the entire Brillouin zone through three-center magnon excitations. This mechanism is aided by the three different magnetic sublattices and strong short-range correlations in the distorted kagome lattice. The results of THz time-domain experiment…
Non-Reciprocal Zone Boundary Magnon Propagation in Cu$_2$OSeO$_3$
Institut Laue-Langevin (ILL)（朗之万研究所）；Max-Planck-Institut für Festkörperforschung（马克斯·普朗克固体研究所）；Technische Universität München (TUM)（慕尼黑工业大学）；Jülich Centre for Neutron Science (JCNS)（朱利希中子科学中心）；Forschungsneutronenquelle Heinz-Maier-Leibnitz (FRM-II)（海因茨·迈尔-莱布尼茨研究用中子源）；Munich Center for Quantum Science and Technology (MCQST)（慕尼黑量子科学与技术中心）；Zentrum für QuantumEngineering (ZQE)（量子工程中心）
Using time-of-flight and triple-axis inelastic neutron spectroscopy, we determine spin wave excitations throughout the Brillouin zone for ferromagnetic manganites La$_{1-x}$Ca$_x$MnO$_3$ ($x=0.25,0.3$) in their low temperature metallic states. While spin wave excitations in the long wavelength limit (spin stiffness $D$) have similar values for both compounds, the excitations near the Brillouin zone boundary of La$_{0.7}$Ca$_{0.3}$MnO$_3$ are considerable softened in all symmetry directions compared to that of La$_{0.75}$Ca$_{0.25}$MnO$_3$. A Heisenberg model with the nearest neighbor and the f…
Inelastic neutron scattering has been used to study the magneto-elastic excitations in the multiferroic manganite hexagonal YMnO$_3$. An avoided crossing is found between magnon and phonon modes close to the Brillouin zone boundary in the $(a,b)$-plane. Neutron polarization analysis reveals that this mode has mixed magnon-phonon character. An external magnetic field along the $c$-axis is observed to cause a linear field-induced splitting of one of the spin wave branches. A theoretical description is performed, using a Heisenberg model of localized spins, acoustic phonon modes and a magneto-ela…
Temperature and magnetic field dependent polarized Brillouin spectra of CuGeO_3 are reported. In addition to a bound singlet state at 30 cm^{-1}, a new feature has been observed at 18 cm^{-1}. This feature is interpreted in terms of a novel three-magnon light scattering process between excited triplet states.
Magnon linewidth of La_1.2 Sr_1.8 Mn_2 O_7 near the Brillouin zone boundary is investigated from both theoretical and experimental points of view. Abrupt magnon broadening is ascribed to a strong magnon-phonon coupling. Magnon broadening observed in cubic perovskite manganites is also discussed.
In order to study the magnetic excitation behaviors in colossal magnetoresistance manganites, a magnon-phonon interacting system is investigated. Sudden broadening of magnon linewidth is obtained when a magnon branch crosses over an optical phonon branch. Onset of the broadening is approximately determined by the magnon density of states. Anomalous magnon damping at the brillouine zone boundary observed in low Curie temperature manganites is explained.
Understanding spin excitations and their connection to unconventional superconductivity have remained a central issue since the discovery of the cuprates. Direct measurement of the dynamical spin structure factor in the parent compounds can provide key information on important interactions relevant in the doped regime, and variations in the magnon dispersion have been linked closely to differences in crystal structure between families of cuprate compounds. Here, we elucidate the relationship between spin excitations and various controlling factors thought to be significant in high-$T_c$ materi…
Recently, based on the refined crystal structure of Pr0.6Ca0.4MnO3 from neutron diffraction, Daoud-Aladine et al.[PRL89,97205(2002)] have proposed a new ground state structure for the half-doped manganites R0.5Ca0.5MnO3, where R is a trivalent ion like Bi,La,Pr,Sm or Y. Their proposal describes the CE magnetic structure attributed to these materials as an arrangement of dimers along the ferromagnetic Mn zig-zag chains that form it. However, the dimers' proposal is in conflict with the Goodenough-Kanamori-Anderson rules, which give a coherent description of many transition metal insulating comp…
Understanding the nature of the excitation spectrum in quantum spin liquids is of fundamental importance, in particular for the experimental detection of candidate materials. However, current theoretical and numerical techniques have limited capabilities, especially in obtaining the dynamical structure factor, which gives a crucial characterization of the ultimate nature of the quantum state and may be directly assessed by inelastic neutron scattering. In this work, we investigate the low-energy properties of the $S=1/2$ Heisenberg model on the triangular lattice, including both nearest-neighb…
In electronic topological Dirac semimetals the conduction and valence bands touch at discrete points in the Brillouin zone and form Dirac cones. They are robust against spin-orbit interaction (SOI) and protected by crystal symmetries. They can be driven to different topological phases by breaking the symmetries. In the low-temperature quantum magnetic systems the magnon dispersions have similar band structures as the electron dispersions, but with positive definite energies. In these magnetic systems SOI manifests in the form of the Dzyaloshinskii-Moriya interaction (DMI). In this Communicatio…
We present the detailed inelastic neutron scattering measurements of the noncollinear antiferromagnet Mn$_3$Ge. Time-of-flight and triple-axis spectroscopy experiments were conducted at the temperature of 6~K, well below the high magnetic ordering temperature of 370~K. The magnetic excitations have a 5-meV gap and display an anisotropic dispersive mode reaching $\simeq 90$~meV at the boundaries of the magnetic Brillouin zone. The spectrum at the zone center shows two additional excitations that demonstrate characteristics of both magnons and phonons. The \textit{ab initio} lattice-dynamics cal…
Weyl nodes have been experimentally realized in photonic, electronic, and phononic crystals. However, magnonic Weyl nodes are yet to be seen experimentally. In this paper, we propose Weyl magnon nodes in noncoplanar stacked frustrated kagome antiferromagnets, naturally available in various real materials. Most crucially, the Weyl nodes in the current system occur at the lowest excitation and possess a topological (anomalous) thermal Hall effect, therefore they are experimentally accessible at low temperatures due to the population effect of bosonic quasiparticles. In stark contrast to other ma…
Using semiclassical method combined with stereographic projection approach, we investigate the magnetic dynamics of the skyrmion crystal (SkX), formed in planar ferromagnet with both Dzyaloshinskii-Moriya interaction and uniform magnetic field. The topologically non-trivial ground state of SkX is described in stereographic projection by the complex valued function with simple poles at skyrmions' positions. We use the earlier proposed ansatz for this ground state function in the form of the sum of individual skyrmions. The dynamics follows from the second variation of the classical action. Nume…
The frustrated pyrochlore magnet Yb$_2$Ti$_2$O$_7$ has the remarkable property that it orders magnetically, but has no propagating magnons over wide regions of the Brillouin zone. Here we use inelastic neutron scattering to follow how the spectrum evolves in cubic-axis magnetic fields. At high fields we observe in addition to dispersive magnons also a two-magnon continuum, which grows in intensity upon reducing the field and overlaps with the one-magnon states at intermediate fields leading to strong renormalization of the dispersion relations, and magnon decays. Using heat capacity measuremen…
Field-induced quasi-bound state within the two-magnon continuum of a square-lattice Heisenberg antiferromagnet
KTH Royal Institute of Technology（皇家理工学院）；Ecole Polytechnique Fédérale de Lausanne (EPFL)（洛桑联邦理工学院）；University of Tennessee, Knoxville（田纳西大学诺克斯维尔分校）；Paul Scherrer Institute（保罗谢尔研究所）；Technical University of Munich（慕尼黑工业大学）；Novo Nordisk A/S（诺和诺德公司）；Technical University of Denmark（丹麦技术大学）；Rutherford Appleton Laboratory（卢瑟福阿普尔顿实验室）；Royal Holloway University of London（伦敦大学皇家霍洛威学院）；University of Bern（伯尔尼大学）
The two-magnon problem for the frustrated XXZ spin-1/2 Heisenberg Hamiltonian and external magnetic fields exceeding the saturation field Bs is considered. We show that the problem can be exactly mapped onto an effective tight-binding impurity problem. It allows to obtain explicit exact expressions for the two-magnon Green's functions for arbitrary dimension and number of interactions. We apply this theory to a quasi-one dimensional helimagnet with ferromagnetic nearest neighbor J1 < 0 and antiferromagnetic next-nearest neighbor J2 > 0 interactions. An outstanding feature of the excitation spe…
We study the field dependence of the antiferromagnetic spin-1/2 Heisenberg model on the square lattice by means of exact diagonalizations. In a first part, we calculate the spin-wave velocity, the spin-stiffness, and the magnetic susceptibility and thus determine the microscopic parameters of the low-energy long-wavelength description. In a second part, we present a comprehensive study of dynamical spin correlation functions for magnetic fields ranging from zero up to saturation. We find that at low fields, magnons are well defined in the whole Brillouin zone, but the dispersion is substantial…
We investigated the doping dependence of magnetic excitations in the lightly doped cuprate La2-xSrxCuO4 via combined studies of resonant inelastic x-ray scattering (RIXS) at the Cu L3-edge and theoretical calculations. With increasing doping, the magnon dispersion is found to be essentially unchanged, but the spectral width broadens and the spectral weight varies differently at different momenta. Near the Brillouin zone center, we directly observe bimagnon excitations which possess the same energy scale and doping dependence as previously observed by Raman spectroscopy. They disperse weakly in…
Curvilinear magnonic crystal based on 3D hierarchical nanotemplates
Helmholtz-Zentrum Dresden-Rossendorf e.V.（德累斯顿罗森多夫亥姆霍兹中心）；Université Sorbonne Paris Nord（索邦巴黎北大学）；University of California, Santa Cruz（加州大学圣克鲁兹分校）；Leibniz Institute for Solid State and Materials Research（莱布尼兹固体与材料研究所）
We study the roton-like dip in the magnon dispersion at the boundary of the Brillouin zone in the isotropic S=1/2 Heisenberg quantum antiferromagnet. This high-energy feature is sometimes seen as indication of a fractionalization of the magnons to spinons. In this article, we provide evidence that the description of the dip in terms of magnons can be improved significantly by applying more advanced evaluation schemes. In particular, we illustrate the usefulness of the application of the principle of minimal sensitivity in varied perturbation theory. Thereby, we provide an example for the appli…
