Quantum interference of "clocks", namely of particles with time-evolving internal degrees of freedom (DOFs), is a promising avenue to test genuine general relativistic effects in quantum systems. The clock acquires which path information while experiencing different proper times on traversing the arms of the interferometer, leading to a drop in its path visibility. We consider scenarios where the clock is subject to environmental noise as it transits through the interferometer. In particular, we develop a generalized formulation of interferometric visibility affected by noise on the clock. We find that, for small noise and small proper time difference between the arms, the noise further reduces the visibility, while in more general situations it can either increase or reduce the visibility. As an example, we investigate the effect of a thermal environment constituted by a single field mode and show that the visibility drops further as the temperature is increased. Additionally, by considering noise models based on standard quantum channels, we show that interferometric visibility can increase or decrease depending on the type of noise and also the time scale and transition probabilities. The quantification of the effect of noise on the visibility -- particularly in the case of a thermal environment paves the way for a better estimate on the expected outcome in an actual experiment.
Metric descriptions of gravitation, among them general relativity as today's established theory, are founded on assumptions summarized by the Einstein equivalence principle (EEP). Its violation would hint at unknown physics and could be a leverage for the development of quantum gravity. Atomic clocks are excellent systems to probe aspects of EEP connected to (proper) time and have evolved into a working horse for tests of local position invariance (LPI). Even though the operational definition of time requires localized and idealized clocks, quantum systems like atoms allow for spatial superpos…
The creation of delocalized coherent superpositions of quantum systems experiencing different relativistic effects is an important milestone in future research at the interface of gravity and quantum mechanics. This could be achieved by generating a superposition of quantum clocks that follow paths with different gravitational time dilation and investigating the consequences on the interference signal when they are eventually recombined. Light-pulse atom interferometry with elements employed in optical atomic clocks is a promising candidate for that purpose, but suffers from major challenges i…
Current attempts to test local position invariance (LPI) compare different clock transition rates with classically exchanged signals. We propose an experimental scheme for the quantum test of LPI: an internal atomic clock interferometer comprising two interfering clocks within one atom. We prepare the atom in a superposition of two clock states and one ground state, which evolves coherently along two quantum clock oscillations into stable internal Ramsey interference patterns. The interference pattern with the shared ground state shows a visibility modulation, which can be interpreted as the b…
We report the first realization of large momentum transfer (LMT) clock atom interferometry. Using single-photon interactions on the strontium ${}^1S_0 - {}^3P_1$ transition, we demonstrate Mach-Zehnder interferometers with state-of-the-art momentum separation of up to $141\,\hbar k$ and gradiometers of up to $81\,\hbar k$. Moreover, we circumvent excited state decay limitations and extend the gradiometer duration to 50 times the excited state lifetime. Because of the broad velocity acceptance of the interferometry pulses, all experiments are performed with laser-cooled atoms at a temperature o…
We discuss quantum variational optimization of Ramsey interferometry with ensembles of $N$ entangled atoms, and its application to atomic clocks based on a Bayesian approach to phase estimation. We identify best input states and generalized measurements within a variational approximation for the corresponding entangling and decoding quantum circuits. These circuits are built from basic quantum operations available for the particular sensor platform, such as one-axis twisting, or finite range interactions. Optimization is defined relative to a cost function, which in the present study is the Ba…
Non-local mass superpositions and optical clock interferometry in atomic ensemble quantum networks
University of Innsbruck（因斯布鲁克大学）；Institute for Quantum Optics and Quantum Information of the Austrian Academy of Sciences（奥地利科学院量子光学和量子信息研究所）；Leibniz Universität Hannover（汉诺威莱布尼茨大学）；JILA, NIST and Department of Physics, University of Colorado（科罗拉多大学JILA、美国国家标准与技术研究院及物理系）；Center for Theory of Quantum Matter, University of Colorado（科罗拉多大学量子物质理论中心）
We theoretically discuss an implementation of a Sagnac interferometer with cold atoms. In contrast to currently existing schemes our protocol does not rely on any free propagation of atoms. Instead it is based on superpositions of fully confined atoms and state-dependent transport along a closed path. Using Ramsey sequences for an atomic clock, the accumulated Sagnac phase is encoded in the resulting population imbalance between two internal (clock) states. Using minimal models for the above protocol we analytically quantify limitations arising from atomic dynamics and finite temperature. We d…
We experimentally demonstrate a new interferometry paradigm: a self-interfering clock. We split a clock into two spatially separated wave packets, and observe an interference pattern with a stable phase showing that the splitting was coherent, i.e., the clock was in two places simultaneously. We then make the clock wave packets "tick" at different rates to simulate a proper time lag. The entanglement between the clock's time and its path yields "which path" information, which affects the visibility of the clock's self-interference. By contrast, in standard interferometry, time cannot yield "wh…
This paper is divided into three parts. In the first (section 1), we demonstrate that all of quantum mechanics can be derived from the fundamental property that the propagation of a matter wave packet is described by the same gravitational and kinematic time dilation that applies to a clock. We will do so in several steps, first deriving the Schroedinger equation for a nonrelativistic particle without spin in a weak gravitational potential, and eventually the Dirac equation in curved space-time describing the propagation of a relativistic particle with spin in strong gravity. In the second par…
Bayesian Frequency Metrology with Optimal Ramsey Interferometry in Optical Atomic Clocks
Institute for Theoretical Physics and Institute for Gravitational Physics (Albert-Einstein-Institute), Leibniz University Hannover（汉诺威莱布尼茨大学理论物理研究所与引力物理研究所（爱因斯坦研究所））
Gravitational time dilation in quantum clock interferometry with entangled multi-photon states and quantum memories
Humboldt-Universität zu Berlin（柏林洪堡大学）；ZARM, Unversität Bremen（不来梅大学ZARM中心）；Vienna Center for Quantum Science and Technology, Atominstitut, TU Wien（维也纳量子科学与技术中心，原子物理研究所，维也纳工业大学）
Atom interferometry on optical clock transitions is being pursued for numerous long-baseline experiments both terrestrially and for future space missions. Crucial to meeting these experiments' required sensitivities is the implementation of large momentum transfer ($>$10$^3\hbar k$). Here we show that to sequentially apply such a large momentum via $π$ pulses places stringent requirements on the frequency noise of the interferometry laser, finding that the linewidth is required to be considerably lower than has previously been suggested. This is due to imperfect pulse fidelity in the presence …
Clocks play a special role at the interface of general relativity and quantum mechanics. We analyze a clock-interferometry thought experiment and go on to theoretically derive and experimentally test a complementarity relation for quantum clocks in the context of the gravitational time lag. We study this relation in detail and discuss its application to various types of quantum clocks.
This article is based on the talk with the same title at the Blaubeuren meeting. First we discuss briefly the importance of time and time keeping, explaining the basic functioning of clocks in general and atomic clocks in particular, which rely on Ramsey interferometry. The usefulness of cold atoms is discussed as well as their limits in Bose-Einstein condensates. An alternative that we study is a different cold-atom regime: the Tonks-Girardeau (TG) gas of tightly confined and strongly interacting bosons. The TG gas is reviewed and then generalized for two-level atoms. Finally, we explore the …
A new generation of atomic sensors using ultra-narrow optical clock transitions and composite pulses are pushing quantum engineering control to a very high level of precision for applied and fundamental physics. Here, we propose a new version of Ramsey-Bordé interferometry introducing arbitrary composite laser pulses with tailored pulse duration, Rabi field, detuning and phase-steps. We explore quantum metrology below the $10^{-18}$ level of fractional accuracy by a fine tuning control of light excitation parameters protecting ultra-narrow optical clock transitions against residual light-shift…
We present a Ramsey-type atom interferometer operating with an optically trapped sample of 10^6 Bose-condensed Rb-87 atoms. The optical trap allows us to couple the |F =1, mF =0>\rightarrow |F =2, mF =0> clock states using a single photon 6.8GHz microwave transition, while state selective readout is achieved with absorption imaging. Interference fringes with contrast approaching 100% are observed for short evolution times. We analyse the process of absorption imaging and show that it is possible to observe atom number variance directly, with a signal-to-noise ratio ten times better than the at…
We investigate general properties of optical interferometry in stationary spacetimes and apply the obtained results focusing on quantum-optical experiments in near-Earth environments. We provide a rigorous expression for the {gravitationally induced} phase difference and adapt the parametrized post-Newtonian formalism for calculations of polarization rotation. We investigate two optical versions of the Colella-Overhauser-Werner experiment and show that the phase difference is independent of the post-Newtonian parameter $γ$, making it a possible candidate for an optical test of the Einstein equ…
A novel quantum time dilation effect is shown to arise when a clock moves in a quantum superposition of two relativistic velocities. This effect is argued to be measurable using existing atomic interferometry techniques, potentially offering a new test of relativistic quantum theory.
We theoretically propose a scheme to perform rotation sensing in a Whispering-gallery-mode resonator setup. With the assistance of a large detuned two-level atom, which induces the effective coupling between clockwise and counterclockwise propagating modes in the resonator, we realize an effective interferometry with SU(2) algebraic structure. By studying the quantum Fisher information of the system, we find that the estimate accuracy for the angular velocity of the rotation can achieve and even break the Heisenberg limit in linear and nonlinear setup, respectively. The high performance of qua…
Quantum signatures of proper time in optical ion clocks
Stevens Institute of Technology（史蒂文斯理工学院）；University of Waterloo（滑铁卢大学）；National Institute of Standards and Technology（美国国家标准与技术研究院）；Colorado State University（科罗拉多州立大学）；Stockholm University（斯德哥尔摩大学）
A wide variety of positioning and ranging procedures are based on repeatedly sending electromagnetic pulses through space and measuring their time of arrival. This paper shows that quantum entanglement and squeezing can be employed to overcome the classical power/bandwidth limits on these procedures, enhancing their accuracy. Frequency entangled pulses could be used to construct quantum positioning systems (QPS), to perform clock synchronization, or to do ranging (quantum radar): all of these techniques exhibit a similar enhancement compared with analogous protocols that use classical light. Q…
We demonstrate quantum coherent control of a single electron spin in a NV center in diamond using the Landau-Zener-Stuckelberg interferometry at room temperature. Interference pattern is observed oscillating as a function of microwave frequency. The decays in the visibility of the interference are well explained by numerical simulation which includes the thermal fluctuations of the nuclear bath which shows that Landau-Zener-Stuckelberg interferometry can be used for probing electron spin decoherence processes.
Massachusetts Institute of Technology（麻省理工学院）；Scuola Superiore Meridionale（南方高等学院）；Istituto Nazionale di Fisica Nucleare (INFN)（意大利国家核物理研究所）；Università degli Studi di Napoli Federico II（那不勒斯费德里科二世大学）；Research Laboratory of Electronics, Massachusetts Institute of Technology（麻省理工学院电子研究实验室）；University of the Basque Country UPV/EHU（巴斯克大学）
We quantify the impact of spatio-temporally correlated Gaussian quantum noise on frequency estimation by Ramsey interferometry. While correlations in a classical noise environment can be exploited to reduce uncertainty relative to the uncorrelated case, we show that quantum noise environments with frequency asymmetric spectra generally introduce additional sources of uncertainty due to uncontrolled entanglement of the sensing system mediated by the bath. For the representative case of collective noise from bosonic sources, and experimentally relevant collective spin observables, we find that t…
Exponential enhancement of sensitivity in Ramsey interferometry with optically thick ensemble of atoms
Kazan Quantum Center, Kazan National Research Technical University n.a. A.N. Tupolev-KAI（喀山量子中心，喀山国立研究技术大学（A.N. 图波列夫-CAI））；Department of Physics, McGill University（麦吉尔大学物理系）
A new class of atomic interferences using ultra-narrow optical transitions are pushing quantum engineering control to a very high level of precision for a next generation of sensors and quantum gate operations. In such context, we propose a new quantum engineering approach to Ramsey-Bordé interferometry introducing multiple composite laser pulses with tailored pulse duration, Rabi field amplitude, frequency detuning and laser phase-step. We explore quantum metrology with hyper-Ramsey and hyper-Hahn-Ramsey clocks below the $10^-18$ level of fractional accuracy by a fine tuning control of light …
We consider the conditioning of the timeless solution to the Wheeler-DeWitt equation by a predefined matter clock state in the simple scenario of de Sitter universe. The resulting evolution of the geometrodynamical degree of freedom with respect to clock time is characterized by the "Berry connection" of the reduced geometrodynamical space, which relies on the coupling of the clock with the geometry. When the connection vanishes, the standard Schrödinger equation is obtained for the geometry with respect to clock time. When one considers environment-induced decoherence in the semi-classical li…
Light-pulse atom interferometers constitute powerful quantum sensors for inertial forces. They are based on delocalised spatial superpositions and the combination with internal transitions directly links them to atomic clocks. Since classical tests of the gravitational redshift are based on a comparison of two clocks localised at different positions under gravity, it is promising to explore whether the aforementioned interferometers constitute a competitive alternative for tests of general relativity. Here we present a specific geometry which together with state transitions leads to a scheme t…
We minimize the stray electric field in a linear Paul trap quickly and accurately, by applying interferometry pulse sequences to a trapped ion optical qubit. The interferometry sequences are sensitive to the change of ion equilibrium position when the trap stiffness is changed, and we use this to determine the stray electric field. The simplest pulse sequence is a two-pulse Ramsey sequence, and longer sequences with multiple pulses offer a higher precision. The methods allow the stray field strength to be minimized beyond state-of-the-art levels, with only modest experimental requirements. Usi…
Parameter Estimation from Amplitude Collapse in Correlated Matter-Wave Interference
Technische Universität Darmstadt（达姆施塔特工业大学）；Helmholtz Forschungsakademie Hessen für FAIR (HFHF), GSI Helmholtzzentrum für Schwerionenforschung（黑森FAIR亥姆霍兹研究院，GSI重离子研究中心）
Interferometry with Heisenberg limited phase resolution may play an important role in the next generation of atomic clocks, gravitational wave detectors, and in quantum information science. For experimental implementations the robustness of the phase resolution is crucial since any experimental realization will be subject to imperfections. In this article we study the robustness of phase reconstruction with two number states as input subject to fluctuations in the state preparation. We find that the phase resolution is insensitive to fluctuations in the total number of particles and robust aga…
Sensing and measurement tasks in severely adverse conditions such as loss, noise and dephasing can be improved by illumination with quantum states of light. Previous results have shown a modest reduction in the number of measurements necessary to achieve a given precision. Here, we compare three illumination strategies for estimating the relative phase in a noisy, lossy interferometer. When including a common phase fluctuation in the noise processes, we show that using an entangled probe achieves an advantage in parameter estimation precision that scales with the number of entangled modes. Thi…
Usually, decoherence is generated from the coupling with an outer environment. However, a macroscopic object generically possesses its own environment in itself, namely the complicated dynamics of internal degrees of freedom. We address a question: when and how the internal dynamics decohere interference of the center of mass motion of a macroscopic object. We will also show that weak localization of a macroscopic object in disordered potentials can be destroyed by such decoherence.
Atomic clocks can measure the gravitational redshift predicted by general relativity with great accuracy and for height differences as little as 1 cm. All existing experiments, however, involve the comparison of two independent clocks at different locations rather than a single clock in a delocalized quantum superposition. Here we present an interferometry scheme employing group-II-type atoms, such as Sr or Yb, capable of measuring the gravitational time dilation in a coherent superposition of atomic wave packets at two different heights. In contrast to other recent proposals, there is no need…
The use of real clocks and measuring rods in quantum mechanics implies a natural loss of unitarity in the description of the theory. We briefly review this point and then discuss the implications it has for the measurement problem in quantum mechanics. The intrinsic loss of coherence allows to circumvent some of the usual objections to the measurement process as due to environmental decoherence.
The Stark shift due to blackbody radiation (BBR) is the key factor limiting the performance of many atomic frequency standards, with the BBR environment inside the clock apparatus being difficult to characterize at a high level of precision. Here we demonstrate an in-vacuum radiation shield that furnishes a uniform, well-characterized BBR environment for the atoms in an ytterbium optical lattice clock. Operated at room temperature, this shield enables specification of the BBR environment to a corresponding fractional clock uncertainty contribution of $5.5 \times 10^{-19}$. Combined with uncert…
We provide a self-contained quantum description of the interference produced by macromolecules diffracted by a grating, with particular reference to fullerene interferometry experiments. We analyze the processes inducing loss of coherence consisting in beam preparation (collimation setup and thermal spread of the wavelengths of the macromolecules) and in environmental disturbances. The results show a good agreement with experimental data published by Zeilinger's group and highlight the analogy with optics. Our analysis gives some hints for planning future experiments.
A two-slit interference of a massive particle in the presence of environment induced decoherence is theoretically analyzed using a fully quantum mechanical calculation. The Markovian Master equation, derived from coupling the particle to a harmonic-oscillator heat bath, is used to obtain exact solutions which show the existence of an interference. Interestingly, decoherence does not affect the pattern, but only leads to a reduction in the fringe visibility.
Ramsey interferometry is routinely used in quantum metrology for the most sensitive measurements of optical clock frequencies. Spontaneous decay to the electromagnetic vacuum ultimately limits the interrogation time and thus sets a lower bound to the optimal frequency sensitivity. In dense ensembles of two-level systems the presence of collective effects such as superradiance and dipole-dipole interaction tends to decrease the sensitivity even further. We show that by a redesign of the Ramsey-pulse sequence to include different rotations of individual spins that effectively fold the collective…
We propose to test the theory of continuous spontaneous localization (CSL) in an all-optical time-domain Talbot-Lau interferometer for clusters with masses exceeding 1000000 amu. By assessing the relevant environmental decoherence mechanisms, as well as the growing size of the particles relative to the grating fringes, we argue that it will be feasible to test the quantum superposition principle in a mass range excluded by recent estimates of the CSL effect.
Recently it was shown that by means of an STM it is experimentally possible to stimulate clock transitions between the singlet and the non-magnetic triplet state of a Heisenberg-coupled spin dimer (Bae et al., Science Advances 4, eaau4159). This leads to more strongly protected clock transitions while ordinary ones only provide first-order protection against magnetic noise. However, large decoherence times of clock like states normally refer to ensembles of spins which do not dephase. In the cited experiment only one single dimer is manipulated and not an ensemble. For this reason we simulate …
We show that Feynman's Clock construction, in which the time-evolution of a closed quantum system is encoded as a ground state problem, can be extended to open quantum systems. In our formalism, the ground states of an ensemble of non-Hermitian Feynman Clock Hamiltonians yield stochastic trajectories, which unravel the evolution of a Lindblad master equation. In this way, one can use Feynman's Clock not only to simulate the evolution of a quantum system, but also it's interaction with an environment such as a heat bath or measuring apparatus. A simple numerical example of a two-level atom unde…
We present a novel continuous dynamical decoupling scheme for the construction of a robust qubit in a three-level system. By means of a clock transition adjustment, we first show how robustness to environmental noise is achieved, while eliminating drive-noise, to first-order. We demonstrate this scheme with the spin sub-levels of the NV-centre's electronic ground state. By applying drive fields with moderate Rabi frequencies, the drive noise is eliminated and an improvement of 2 orders of magnitude in the coherence time is obtained compared to the pure dephasing time. We then show how the cloc…
A three-body quantum correlation is calculated for two particles reflecting from a mirror. Correlated interference, a consequence of conservation of energy and momentum, occurs for states in which the order of reflection is indeterminate. The resulting quantum joint probability density function exhibits interference with diverse characteristics, depending on the coherence lengths of the substates. Marginal probability density functions can contain information about the quantum nature of all three bodies, even if only one particle is measured. Microscopic particles reflecting from a mesoscopic …
