Trapped ions are a promising candidate for large scale quantum computation. Several systems have been built in both academic and industrial settings to implement modestly-sized quantum algorithms. Efficient cooling of the motional degrees of freedom is a key requirement for high-fidelity quantum operations using trapped ions. Here, we present a technique whereby individual ions are used to cool individual motional modes in parallel, reducing the time required to bring an ion chain to its motional ground state. We demonstrate this technique experimentally and develop a model to understand the efficiency of our parallel sideband cooling technique compared to more traditional methods. This technique is applicable to any system using resolved sideband cooling of co-trapped atomic species and only requires individual addressing of the trapped particles.
We report a detailed investigation on near-ground state cooling of one and two trapped atomic ions. We introduce a simple sideband cooling method for confined atoms and ions, using RF radiation applied to bare ionic states in a static magnetic field gradient, and demonstrate its application to ions confined at secular trap frequencies, $ω_z \approx 2π\times 117 $kHz. For a single \ybplus ion, the sideband cooling cycle reduces the average phonon number, $\left\langle\,n\,\right\rangle$ from the Doppler limit to $\left\langle\,n\,\right\rangle =$ 0.30(12). This is in agreement with the theoreti…
Resolved sideband cooling is a standard technique for cooling trapped ions below the Doppler limit to near their motional ground state. Yet, the most common methods for sideband cooling implicitly rely on low Doppler-cooled temperatures and tightly confined ions, and they cannot be optimized for different experimental conditions. Here we introduce a framework which calculates the fastest possible pulsed sideband cooling sequence for a given number of pulses and set of experimental parameters, and we verify its improvement compared to traditional methods using a trapped $^{171}$Yb$^+$ ion. Afte…
We report continuous Raman sideband cooling (CRSC) of a long ion chain to the motional ground state beyond the Lamb-Dicke (LD) regime. By driving multiple sideband transitions simultaneously, we show that nearly all axial modes of a 24-ion chain are cooled to the ground state, with an LD parameter as large as $η= 1.3$, spanning a frequency bandwidth of 4 MHz. Compared to traditional ground-state cooling methods such as pulsed sideband cooling or electromagnetic-induced-transparency (EIT) cooling, our method offers two key advantages: robustness to timing errors; and an ultra-wide bandwidth unl…
We present the results of simulations of optical sideband cooling of atomic ions in a trap with a shallow potential well. In such traps, an ion cannot be Doppler cooled near to the Lamb-Dicke regime ($η^2(2n+1) \ll 1$). Outside the Lamb-Dicke regime, the sideband cooling dynamics are altered by the existence of various Fock states where the cooling becomes very slow. A calcium ion trapped in our Penning trap realises such a situation, hence single stage cooling is inefficient to prepare the ion in the motional ground state. For these systems, it is necessary to study the cooling dynamics in de…
Single neutral atoms trapped in optical tweezers and laser-coupled to Rydberg states provide a fast and flexible platform to generate configurable atomic arrays for quantum simulation. The platform is especially suited to study quantum spin systems in various geometries. However, for experiments requiring continuous trapping, inhomogeneous light shifts induced by the trapping potential and temperature broadening impose severe limitations. Here we show how Raman sideband cooling allows one to overcome those limitations, thus, preparing the stage for Rydberg dressing in tweezer arrays.
We demonstrate phase locking of two ultraviolet laser sources by modulating a fundamental infrared laser with 4th-order sidebands using an electro-optic modulator and phase locking of one sideband to a second fundamental infrared laser. Subsequent sum frequency generation and second harmonic generation successfully translates the frequency offset to the ultraviolet domain. The phase lock at 139 GHz is confirmed through stimulated Raman transitions for thermometry of $^9$Be$^+$ ions confined in a cryogenic Penning trap. This technique might be used for sideband cooling of single $^9$Be$^+$ ions…
Doppler and sideband cooling are long standing techniques that have been used together to prepare trapped atomic ions in their ground state of motion. In this paper we study how these techniques can be extended to cool both radial modes of motion of a single ion in a Penning trap. We numerically explore the prerequisite experimental parameters for efficient Doppler cooling in the presence of an additional oscillating electric field to resonantly couple the radial modes. The simulations are supported by experimental data for a single $^{40}$Ca$^+$ ion Doppler cooled to $\sim$100 phonons in both…
We demonstrate resolved sideband laser cooling of a single 40Ca+ ion in a macroscopic linear radio frequency trap with a radial diagonal electrode spacing of 7 mm and an rf drive frequency of just 3.7 MHz. For an oscillation frequency of 585 kHz along the rf-field-free axis, a ground state population of 99+-1% has been achieved, corresponding to a temperature of only 6 microkelvin. For several oscillation frequencies in the range 285 - 585 kHz, heating rates below one motional quantum per second have been measured at room temperature. The lowest measured heating power is about an order of magn…
A method of sideband Raman cooling to the vibrational ground state of the $m=0$ Zeeman sublevel in a far-detuned two-dimensional optical lattice is proposed. In our scheme, the Raman coupling between vibrational manifolds of the adjacent Zeeman sublevels is shifted to the red sideband due to the ac Stark effect induced by a weak pump field. Thus, cooling and optical pumping to $m=0$ is achieved by purely optical means with coplanar cw laser beams. The optical lattice and cooling parameters are estimated in the framework of simple theoretical models. An application of the transverse sideband co…
We clarify the optimal conditions for the protocol of Raman sideband cooling (RSC) of a single atom confined with a tightly focused far-off-resonant optical dipole trap (optical tweezers). The protocol ultimately pursues cooling to a three-dimensional ground state of the confining potential. We show that the RSC protocol has to fulfil a set of critical requirements for the parameters of cooling beams and the excitation geometry to be effective in a most general three-dimensional confguration and for an atom, having initial temperature between the recoil and the Doppler bounds. We perform a num…
We report the laser cooling of a single $^{40}\text{Ca}^+$ ion in a Penning trap to the motional ground state in one dimension. Cooling is performed in the strong binding limit on the 729-nm electric quadrupole $S_{1/2}\leftrightarrow D_{5/2}$ transition, broadened by a quench laser coupling the $D_{5/2}$ and $P_{3/2}$ levels. We find the final ground state occupation to be $98\pm1\%$. We measure the heating rate of the trap to be very low with $\dot{\bar{n}}\approx 0.3\pm0.2\textrm{s}^{-1}$ for trap frequencies from $150-400\textrm{kHz}$, consistent with the large ion-electrode distance.
We theoretically propose and experimentally demonstrate the use of motional sidebands in a trapped ensemble of $^{87}$Rb atoms to engineer tunable long-range XXZ spin models. We benchmark our simulator by probing a ferromagnetic to paramagnetic dynamical phase transition in the Lipkin-Meshkov-Glick (LMG) model, a collective XXZ model plus additional transverse and longitudinal fields, via Rabi spectroscopy. We experimentally reconstruct the boundary between the dynamical phases, which is in good agreement with mean-field theoretical predictions. Our work introduces new possibilities in quantum…
Motional ground state cooling and internal state preparation are important elements for quantum logic spectroscopy (QLS), a class of quantum information processing. Since QLS does not require the high gate fidelities usually associated with quantum computation and quantum simulation, it is possible to make simplifying choices in ion species and quantum protocols at the expense of some fidelity. Here, we report sideband cooling and motional state detection protocols for $^{138}$Ba$^+$ of sufficient fidelity for QLS without an extremely narrowband laser or the use of a species with hyperfine str…
We investigate quantum control of a single atom in an optical tweezer trap created by a tightly focused optical beam. We show that longitudinal polarization components in the dipole trap arising from the breakdown of the paraxial approximation give rise to significant internal-state decoherence. We show that this effect can be mitigated by appropriate choice of magnetic bias field, enabling Raman sideband cooling of a single atom close to its three-dimensional ground state in an optical trap with a beam waist as small as $w=900$ nm. We achieve vibrational occupation numbers of $\bar{n}_r = 0.0…
Sideband cooling is a popular method for cooling atoms to the ground state of an optical trap. Applying the same method to molecules requires a number of challenges to be overcome. Strong tensor Stark shifts in molecules cause the optical trapping potential, and corresponding trap frequency, to depend strongly on rotational, hyperfine and Zeeman state. Consequently, transition frequencies depend on the motional quantum number and there are additional heating mechanisms, either of which can be fatal for an effective sideband cooling scheme. We develop the theory of sideband cooling in state-dep…
We propose a novel cooling scheme for realising single photon sideband cooling on particles trapped in a state-dependent optical potential. We develop a master rate equation from an ab-initio model and find that in experimentally feasible conditions it is possible to drastically reduce the average occupation number of the vibrational levels by applying a frequency sweep on the cooling laser that sequentially cools all the motional states. Notably, this cooling scheme works also when a particle experiences a deeper trap in its internal ground state than in its excited state, a condition for whi…
We present a single solid-state laser system to cool, coherently manipulate and detect $^{25}$Mg$^+$ ions. Coherent manipulation is accomplished by coupling two hyperfine ground state levels using a pair of far-detuned Raman laser beams. Resonant light for Doppler cooling and detection is derived from the same laser source by means of an electro-optic modulator, generating a sideband which is resonant with the atomic transition. We demonstrate ground-state cooling of one of the vibrational modes of the ion in the trap using resolved-sideband cooling. The cooling performance is studied and disc…
We demonstrate 3D microwave projection sideband cooling of trapped, neutral atoms. The technique employs state-dependent potentials that enable microwave photons to drive vibration-number reducing transitions. The particular cooling sequence we employ uses minimal spontaneous emission, and works even for relatively weakly bound atoms. We cool 76% of atoms to their 3D vibrational ground states in a site-resolvable 3D optical lattice.
We utilize the dark state in a Λ-type three-level system to cool an ensemble of 85Rb atoms in an optical lattice [Morigi et al., Phys. Rev. Lett. 85, 4458 (2000)]. The common suppression of the carrier transition of atoms with different vibrational frequencies allows them to reach a subrecoil temperature of 100 nK after being released from the optical lattice. A nearly zero vibrational quantum number is determined from the time-of-flight measurements and adiabatic expansion process. The features of sideband cooling are examined in various parameter spaces. Our results show that dark-state side…
We report on the first realization of sub-Doppler laser cooling of 39K atoms using degenerate 3D Raman sideband cooling. We take advantage of the well-resolved excited hyperfine states on the D1 optical transition to produce spin polarized samples with $1.4 \times 10^8$ atoms at temperatures of 1.8 $μ$K. The phase-space densities are $\geq 10^{-4}$, which significantly improves the initial conditions for a subsequent evaporative cooling step. The presented cooling technique using the D1 line can be adapted to other atomic species and is applicable to high-resolution imaging schemes in far off-…
We present an analytic and numerical study for realizing single photon sideband cooling in an ultracold sample of fermionic Lithium trapped in a periodic optical potential. We develop an analytical model and obtain a master equation for the bound level populations. The cooling sequence is simulated both with a laser at a fixed frequency and with a frequency sweep. Finally, a Monte Carlo simulation is performed taking into account the full hyperfine spectrum of $^6\!$Li. We find that a gas of $^6\!$Li atoms loaded from a Magneto-Optical trap into a deep optical lattice can be cooled down to a $…
We report cooling of a single neutral atom to its three-dimensional vibrational ground state in an optical tweezer. After employing Raman sideband cooling for tens of milliseconds, we measure via sideband spectroscopy a three-dimensional ground-state occupation of ~90%. We further observe coherent control of the spin and motional state of the trapped atom. Our demonstration shows that an optical tweezer, formed simply by a tightly focused beam of light, creates sufficient confinement for efficient sideband cooling. This source of ground-state neutral atoms will be instrumental in numerous quan…
Laser cooling of atoms usually necessitates several laser frequencies. Alkaline atoms, for example, are cooled by two lasers with a frequency difference in the Gigahertz range. This gap cannot be closed with simple shifting techniques. Here, we present a method of generating sidebands at 6.6 GHz by modulating the current of a tapered amplifier which is seeded by an unmodulated master laser. The sidebands enable trapping of 1.1*10^9 Rubidium 87 atoms in a chip-based magneto-optical trap. Compared to the direct modulation of the master laser, this method allows for an easy implementation, a fast…
We use Rabi spectroscopy to explore the low-energy excitation spectrum of a finite-temperature Bose gas of rubidium atoms across the phase transition to a Bose-Einstein condensate (BEC). To record this spectrum, we coherently drive the atomic population between two spin states. A small relative displacement of the spin-specific trapping potentials enables sideband transitions between different motional states. The intrinsic non-linearity of the motional spectrum, mainly originating from two-body interactions, makes it possible to resolve and address individual excitation lines. Together with s…
Trapping lithium with a big number in a simplified experimental setup has difficulties and challenges today. In this paper, we experimentally demonstrate the enhancement of \textsuperscript{6}Li trapping efficiency in a three-dimensional magneto-optical trap (3D MOT) by using the multiple-sideband cooling in a two-dimensional magneto-optical trap (2D MOT). To improve the number of trapped atoms, we broaden the cooling light spectrum to 102 MHz composed of seven frequency components and then trap atoms with a number of $6.0\times10^8$ which is about 4 times compared to that in the single-freque…
We report on the implementation of degenerate Raman sideband cooling of $^{40}$K atoms. The scheme incorporates a 3D optical lattice, which confines the atoms and drives the Raman transitions. The optical cooling cycle is closed by two optical pumping beams. The wavelength of the laser beams forming the lattice is close to the D$_2$ atomic transition, while the optical pumping is operated near the D$_1$ transition. With this cooling method, we achieve temperature of $\sim$$1μ$K of a cloud with $\sim$$10^7$ atoms. This corresponds to a phase space density of $\ge$$10^{-3}$. Moreover, the fermio…
We perform quantum logic spectroscopy (QLS) on $^{27}$Al$^+$ ion $^1$S$_0$ - $^3$P$_1$ transition, which is an important step toward the QLS based $^{27}$Al$^+$ ion optical clock. As a precondition of QLS, both the stretch (STR) mode and the common (COM) mode of the $^{27}$Al$^+$ and $^{25}$Mg$^+$ ions pair are cooled to the vibrational ground state by Raman sideband cooling. The mean phonon number is measured to be 0.10(1) for the STR mode and 0.01(1) for the COM mode, respectively. The heating rate is evaluated to be 13(3) phonons/s for the STR mode and 5.5(1) phonons/s for the COM mode.
In order to use a collection of trapped ions for experiments where a well defined preparation of vibrational states is necessary, all vibrational modes have to be cooled to ensure precise and repeatable manipulation of the ions' quantum states. A method for simultaneous sideband cooling of all axial vibrational modes is proposed. By application of a magnetic field gradient the absorption spectrum of each ion is modified such that sideband resonances of different vibrational modes coincide. The ion string is then irradiated with monochromatic electromagnetic radiation, in the optical or microwa…
We report our experiment on sideband cooling with two Raman transitions in a $Λ$ configuration that allows selective coherent population trapping (CPT) of the motional ground state. The cooling method is applied to $^{87}$Rb atoms in a circularly-polarized one-dimensional optical lattice. Owing to the vector polarizability, the vibration frequency of a trapped atom depends on its Zeeman quantum number, and CPT resonance for a pair of bound states in the $Λ$ configuration depends on their vibrational quantum numbers. We call this scheme motion-selective coherent population trapping (MSCPT) and …
Quantum Beam-Splitter Cooling and Thermometry in Large Trapped-Ion Crystals
Indian Institute of Technology Madras（印度马德拉斯理工学院）；Center for Quantum Information, Communication and Computing, Indian Institute of Technology Madras（印度马德拉斯理工学院量子信息、通信与计算中心）
We demonstrate a general method for state detection of trapped ions that can be applied to a large class of atomic and molecular species. We couple a "spectroscopy" ion (Al+) to a "control" ion (Mg+) in the same trap and perform state detection through off-resonant laser excitation of the spectroscopy ion that induces coherent motion. The motional amplitude, dependent on the spectroscopy ion state, is measured either by time-resolved photon counting, or by resolved sideband excitations on the control ion. The first method provides a simplified way to distinguish "clock" states in Al+, which av…
We present a new electro-optic modulation technique that enables a single laser diode to realize a cold-atom source and a quantum inertial sensor based on matter-wave interferometry. Using carrier-suppressed dual single-sideband modulation, an IQ modulator generates two optical sidebands from separate radio-frequency (rf) signals. These sidebands are controlled independently in frequency, phase, and power using standard rf components. Our laser source exhibits improved rejection of parasitic sidebands compared to those based on phase modulators, which generate large systematic shifts in atom i…
We experimentally realize an enhanced Raman control scheme for neutral atoms that features an intrinsic suppression of the two-photon carrier transition, but retains the sidebands which couple to the external degrees of freedom of the trapped atoms. This is achieved by trapping the atom at the node of a blue detuned standing wave dipole trap, that acts as one field for the two-photon Raman coupling. The improved ratio between cooling and heating processes in this configuration enables a five times lower fundamental temperature limit for resolved sideband cooling. We apply this method to perfor…
We report enhanced three-dimensional degenerated Raman sideband cooling (3D DRSC) of caesium (Cs) atoms in a standard single-cell vapour-loading magneto-optical trap. Our improved scheme involves using a separate repumping laser and optimized lattice detuning. We load $1.5 \times 10^7$ atoms into the Raman lattice with a detuning of -15.5 GHz (to the ground F = 3 state). Enhanced 3D DRSC is used to cool them from 60 $μ$K to 1.7 $μ$K within 12 ms and the number of obtained atoms is about $1.2 \times 10^7$. A theoretical model is proposed to simulate the measured number of trapped atoms. The res…
We analyze the optomechanics of an atomic Bose-Einstein condensate interacting with the optical lattice inside a laser-pumped optical cavity and subject to a uniform bias force such as gravity. An atomic wave packet in a tilted lattice undergoes Bloch oscillations; in a cavity the backaction of the atoms on the light leads to a time-dependent modulation of the intracavity lattice at the Bloch frequency. When the Bloch frequency is on the order of the cavity damping rate we find transport of the atoms either up or down the lattice. The transport dynamics can be interpreted as a manifestation of…
This book chapter gives an introduction to, and an overview of, methods for cooling trapped ions. The main addressees are researchers entering the field. It is not intended as a comprehensive survey and historical account of the extensive literature on this topic. We present the physical ideas behind several cooling schemes, outline their mathematical description, and point to relevant literature useful for a more in-depth study of this topic.
Spin-dependent optical potentials allow us to use microwave radiation to manipulate the motional state of trapped neutral atoms (Förster et al. 2009 Phys. Rev. Lett. 103, 233001). Here, we discuss this method in greater detail, comparing it to the widely-employed Raman sideband coupling method. We provide a simplified model for sideband cooling in a spin-dependent potential, and we discuss it in terms of the generalized Lamb-Dicke parameter. Using a master equation formalism, we present a quantitative analysis of the cooling performance for our experiment, which can be generalized to other exp…
A mixed system of cooled and trapped, ions and atoms, paves the way for ion assisted cold chemistry and novel many body studies. Due to the different individual trapping mechanisms, trapped atoms are significantly colder than trapped ions, therefore in the combined system, the strong binary ion$-$atom interaction results in heat flow from ions to atoms. Conversely, trapped ions can also get collisionally heated by the cold atoms, making the resulting equilibrium between ions and atoms intriguing. Here we experimentally demonstrate, Rubidium ions (Rb$^+$) cool in contact with magneto-optically …
We demonstrate the enhancement and optimization of a cold strontium atomic beam from a two-dimensional magneto-optical trap (2D-MOT) transversely loaded from a collimated atomic beam by adding a sideband frequency to the cooling laser. The parameters of the cooling and sideband beams were scanned to achieve the maximum atomic beam flux and compared with Monte Carlo simulations. We obtained a 2.3 times larger, and 4 times brighter, atomic flux than a conventional, single-frequency 2D-MOT, for a given total power of 200 mW. We show that the sideband-enhanced 2D-MOT can reach the loading rate per…
We control the relative coupling strength of carrier and first order motional sideband interactions of a trapped ion by placing it in a resonant optical standing wave. Our configuration uses the surface of a microfabricated chip trap as a mirror, avoiding technical challenges of in-vacuum optical cavities. Displacing the ion along the standing wave, we show a periodic suppression of the carrier and sideband transitions with the cycles for the two cases $180^\circ$ out of phase with each other. This technique allows for suppression of off-resonant carrier excitations when addressing the motiona…
We investigate the temporal dynamics of Doppler cooling of an initially hot single trapped atom in the weak binding regime using a semiclassical approach. We develop an analytical model for the simplest case of a single vibrational mode for a harmonic trap, and show how this model allows us to estimate the initial energy of the trapped particle by observing the fluorescence rate during the cooling process. The experimental implementation of this temperature measurement provides a way to measure atom heating rates by observing the temperature rise in the absence of cooling. This method is techn…
We experimentally demonstrate microwave control of the motional state of a trapped ion placed in a state-dependent potential generated by a running optical lattice. Both the optical lattice depth and the running lattice frequency provide tunability of the spin-motion coupling strength. The spin-motional coupling is exploited to demonstrate sideband cooling of a Yb171 ion to the ground state of motion.
Since the advent of atom laser-cooling, trapping or cooling natural molecules has been a long standing and challenging goal. Here, we demonstrate a method for laser-trapping molecules that is radically novel in its configuration, in its underlined physical dynamics and in its outcomes. It is based on self-optically spatially-nanostructured high pressure molecular hydrogen confined in hollow-core photonic-crystal-fibre. An accelerating molecular-lattice is formed by a periodic potential associated with Raman saturation except for a 1-dimentional array of nanometer wide and strongly-localizing s…
We report Raman sideband cooling of a single sodium atom to its three-dimensional motional ground state in an optical tweezer. Despite a large Lamb-Dicke parameter, high initial temperature, and large differential light shifts between the excited state and the ground state, we achieve a ground state population of $93.5(7)$% after $53$ ms of cooling. Our technique includes addressing high-order sidebands, where several motional quanta are removed by a single laser pulse, and fast modulation of the optical tweezer intensity. We demonstrate that Raman sideband cooling to the 3D motional ground st…
We report the electromagnetically-induced-transparency (EIT) cooling of a large trapped $^{171}$Yb$^+$ ion chain to the quantum ground state. Unlike conventional EIT cooling, we engage a four-level tripod structure and achieve fast sub-Doppler cooling over all motional modes. We observe simultaneous ground-state cooling across the complete transverse mode spectrum of up to $40$ ions, occupying a bandwidth of over $3$ MHz. The cooling time is observed to be less than $300\,μ$s, independent of the number of ions. Such efficient cooling across the entire spectrum is essential for high-fidelity qu…
We combine near--deterministic preparation of a single atom with Raman sideband cooling, to create a push button mechanism to prepare a single atom in the motional ground state of tightly focused optical tweezers. In the 2D radial plane, we achieve a large ground state fidelity for the entire procedure (loading and cooling) of $\sim$0.73, while the ground state occupancy is $\sim$0.88 for realizations with a single atom present. For 1D axial cooling, we attain a ground state fraction of $\sim$0.52. The combined 3D cooling provides a ground state population of $\sim$0.11. Our Raman sideband coo…
