Zhitong Li, Joseph S. T. Smalley, Ross Haroldson, Dayang Lin, Roberta Hawkins, Abouzar Gharajeh, Jiyoung Moon, Junpeng Hou, Chuanwei Zhang, Walter Hu, Anvar Zakhidov, Qing Gu
A special class of anisotropic media, hyperbolic metamaterials and metasurfaces (HMMs), has attracted much attention in recent years due to its unique abilities to manipulate and engineer electromagnetic waves on the subwavelength scale. Because all HMM designs require metal dielectric composites, the unavoidable metal loss at optical frequencies inspired the development of active HMMs, where gain materials is incorporated to compensate the metal loss. Here, we experimentally demonstrate an active type II HMM that operates at vacuum wavelength near 750 nm on a silicon platform. Different from previous active HMMs operating below 1 μm, the dielectric constituent in our HMM is solely composed of gain medium, by utilizing solution processed and widely tunable metal halide perovskite gain. Thanks to the facile fabrication, tunability and silicon compatibility of our active HMM, this work paves the way towards HMM's integration into on chip components, and eventually, into photonic integrated circuits.
Meta-optics based on optically-resonant dielectric nanostructures is a rapidly developing research field with many potential applications. Halide perovskite metasurfaces emerged recently as a novel platform for meta-optics, and they offer unique opportunities for control of light in optoelectronic devices. Here we employ the generalized Kerker conditions to overlap electric and magnetic Mie resonances in each meta-atom of MAPbBr3 perovskite metasurface and demonstrate broadband suppression of reflection down to 4%. We reveal also that metasurface nanostructuring is also beneficial for the enha…
Lead halide perovskites (MAPbX3) have emerged as promising materials for photovoltaic and optoelectronic devices. However, their exceptional nonlinear properties have not been fully exploited in nanophotonics yet. Herein we fabricate MAPbX3 perovskite metasurfaces and explore their internal nonlinear processes. While both of third-order harmonic generation (THG) and three-photon luminescence are generated, the latter one is less affected by the material loss and has been significantly enhanced by a factor of 60. The corresponding simulation reveals that the improvement is caused by the resonan…
The Rashba effect, i.e., the splitting of electronic spin-polarized bands in the momentum space of a crystal with broken inversion symmetry, has enabled the realization of spin-orbitronic devices, in which spins are manipulated by spin-orbit coupling. In optics, where the helicity of light polarization represents the spin degree of freedom for spin-momentum coupling, the optical Rashba effect is manifested by the splitting of optical states with opposite chirality in the momentum space. Previous realizations of the optical Rashba effect relied on passive devices determining either the propagat…
A spectral splitting, light trapping dielectric metasurface is designed, fabricated and integrated into a four-terminal perovskite/silicon hybrid tandem solar cell to increase the absorption of light close to the bandgap of the perovskite top cell, and enhance transmission of the near-infrared spectral band towards the bottom cell. The metagrating is composed of a hexagonal array of unit cells of 150-nm-tall hydrogenated amorphous silicon trimer nanostructures with dielectric Mie resonances in the 600-800 nm perovskite near-gap region, made using substrate-conformal imprint lithography. By tai…
Emerging immersive visual communication technologies require light sources with complex functionality for dynamic control of polarization, directivity, wavefront, spectrum, and intensity of light. Currently, this is mostly achieved by free space bulk optic elements, limiting the adoption of these technologies. Flat optics based on artificially structured metasurfaces that operate at the sub-wavelength scale are a viable solution, however their integration into electrically driven devices remains challenging. Here we demonstrate a radically new approach of monolithic integration of a dielectric…
Exciton-polaritons, elementary excitations arising from the strong coupling regime between photons and excitons in insulators or semiconductors, represent a promising platform for studying quantum fluids of light and realizing prospective all-optical devices. Among different materials for room temperature polaritonic devices, two-dimensional (2D) layered perovskites have recently emerged as one of the promising candidates thanks to their prominent excitonic features at room temperature. Here we report on the experimental demonstration of exciton-polaritons at room temperature in resonant metas…
Metasurfaces with strongly anisotropic optical properties can support deep subwavelength-scale confined electromagnetic waves (polaritons) that promise opportunities for controlling light in photonic and optoelectronic applications. We develop a mid-infrared hyperbolic metasurface by nanostructuring a thin layer of hexagonal boron nitride supporting deep subwavelength-scale phonon polaritons that propagate with in-plane hyperbolic dispersion. By applying an infrared nanoimaging technique, we visualize the concave (anomalous) wavefronts of a diverging polariton beam, which represent a landmark …
Halide perovskites belong to an important family of semiconducting materials with unique electronic properties that enable a myriad of applications, especially in photovoltaics and optoelectronics. Their optical properties, including photoluminescence quantum yield, are affected and notably enhanced at crystal imperfections where the symmetry is broken and the density of states increases. These lattice distortions can be introduced through structural phase transitions, allowing charge gradients to appear near the interfaces between phase structures. In this work, we demonstrate controlled mult…
Hyperbolic metasurfaces based on van der Waals (vdW) materials support propagation of extremely anisotropic polaritons towards nanoscale light compression and manipulation, and thus has great potential in the applications of planar hyperlens, nanolasing, quantum optics and ultrasensitive infrared spectroscopy. Two-dimensional hexagonal boron nitride (h-BN) as a vdW metasurface can manipulate the propagation of hyperbolic polaritons at the level of single atomic layers, possessing higher degree of field confinement and lower losses than the conventional media. However, active manipulation of hy…
Auxiliary nanostructures introduce additional flexibility into optomechanical manipulation schemes. Metamaterials and metasurfaces capable to control electromagnetic interactions at the near-field regions are especially beneficial for achieving improved spatial localization of particles, reducing laser powers required for trapping, and for tailoring directivity of optical forces. Here, optical forces acting on small particles situated next to anisotropic substrates, are investigated. A special class of hyperbolic metasurfaces is considered in details and is shown to be beneficial for achieving…
Meta-optics based on optically resonant all-dielectric structures is a rapidly developing research area driven by its potential applications for low-loss efficient metadevices. Active, light-emitting subwavelengh nanostructures and metasurfaces are of a particular interest for meta-optics, as they offer unique opportunities for novel types of compact light sources and nanolasers. Recently, the study of halide perovskites has attracted an enormous attention due to their exceptional optical and electrical properties. As a result, this family of materials can provide a prospective platform for mo…
Since the invention of the laser, adoption of new gain media and device architectures has provided solutions to a variety of applications requiring specific power, size, spectral, spatial, and temporal tunability. Here we introduce a fundamentally new type of tunable semiconductor laser based on a phase-change perovskite metasurface that acts simultaneously as gain medium and optical cavity. As a proof of principle demonstration, we fabricate a subwavelength-thin perovskite metasurface supporting bound states in the continuum (BICs). Upon the perovskite structural phase transitions, both its r…
Achieving electrical injection of exciton-polaritons, half-light, half-matter quasiparticles arising from the strong coupling between photonic and excitonic resonances, is a crucial milestone to scale up polaritonic devices such as optical computers, quantum simulators and inversionless lasers. Here we present a new approach to achieve strong coupling between electrically injected excitons and photonic bound states in the continuum of a dielectric metasurface monolithically patterned in the channel of a light-emitting transistor. Exciton-polaritons are generated by coupling electrically inject…
Advances in graphene plasmonics offer numerous opportunities for enabling the design and manufacture of a variety of nanoelectronics and other exciting optical devices. However, due to the limitation of material properties, its operating frequency cannot drop to the microwave range. In this work, a new concept of microwave equivalent graphene based on the ultrathin monolayer plasmonic metasurface is proposed and demonstrated. Based on this concept, elliptical and hyperbolic dispersion can be theoretically obtained by stacking the equivalent graphene metasurfaces periodically. As proofs of the …
Retroreflectors that can accurately redirect the incident wave in free space back along its original channel provide unprecedented opportunities for light manipulation in wireless communication. However, to the best of our knowledge, the existing methods of designing retroreflectors suffer from either the bulky size, narrow angular bandwidth, or time-consuming post-processing. Here, a scheme of designing ultrathin and all-angle retroreflectors based on hyperbolic plasmonic metasurfaces is proposed and experimentally demonstrated. The physical mechanism underlying this scheme is the high-effici…
Moving metasurfaces support guided waves exhibiting unusual optical properties, including strong anisotropy, nonreciprocity, and hyperbolic dispersion. However, for these phenomena to be noticeable, high speeds are typically required, challenging their practical implementation. Here, we show a viable route towards the realization of one-way hyperbolic propagation in metasurfaces placed synthetically in motion through traveling-wave space-time modulation. In addition to non-reciprocal hyperbolic propagation, the proposed time-modulation scheme induces additional exotic opportunities for nanopho…
We reveal the existence of a new type of surface electromagnetic waves supported by hyperbolic metasurfaces, described by a conductivity tensor with an indefinite signature. We demonstrate that the spectrum of the hyperbolic metasurface waves consists of two branches corresponding to hybrid TE-TM waves with the polarization that varies from linear to elliptic or circular depending on the wave frequency and propagation direction. We analyze the effect of losses of the surface waves and derive the corresponding analytical asymptotic expressions.
Hyperbolic propagation offers exciting opportunities in nanophotonics, from sub-diffraction imaging to enhanced local density of states. This transport regime is typically induced by strong modulation of conductivity, i.e., with alternating metallic and dielectric material properties. Here, we analyze a moving impedance surface, showing that suitably tailored homogeneous metasurfaces can support one-way hyperbolic propagation when in motion, adding non-reciprocity to hyperbolic propagation phenomena, and without suffering from nonlocal effects stemming from discretization or finite granularity…
Exciton-polaritons are mixed light-matter excitations that result from the strong coupling regime between an active excitonic material and photonic resonances. Harnessing these hybrid excitations provides a rich playground to explore fascinating fundamental features, such as out-of-equilibrium Bose-Einstein condensation and quantum fluids of light, as well as novel mechanisms to be exploited in optoelectronic devices. Here, we investigate experimentally the formation of exciton-polaritons arising from the mixing between hybrid inorganic-organic perovskite excitons and an optical Bound state In…
Dyakonov surface wave existing at the interface with anisotropy offers a promising way of guiding light in two-dimension with almost no loss. However, predicted decades ago, the experimental demonstration of the Dyakonov surface wave seems always challenging for the weak anisotropic indices from the natural materials. Here we experimentally demonstrated a Dyakonov surface wave mode propagating in a hyperbolic metasurface at the visible frequency. Dyakonov surface waves at the two surfaces of the metasurface can be supported simultaneously by the hyperbolic anisotropy and form a Dyakonov typed …
Recent advances in twistronics of low-dimensional materials, such as bilayer graphene and transition-metal dichalcogenides, have enabled a plethora of unusual phenomena associated with moiré physics. However, several of these effects require demanding manipulation of superlattices at the atomic scale, such as the careful control of rotation angle between two closely spaced atomic lattices. Here, we study moiré hyperbolic plasmons in pairs of hyperbolic metasurfaces (HMTSs), unveiling analogous phenomena at the mesoscopic scale. HMTSs are known to support confined surface waves collimated towar…
Plasmonic hyperbolic metasurfaces have emerged as an effective platform for manipulating the propagation of light. Here, confined modes on arrays of silver nanoridges that exhibit hyperbolic dispersion are used to demonstrate and model a super-resolution imaging technique based on structured illumination microscopy. A spatial resolution of ~75 nm at 458 nm is demonstrated, which is 3.1 times better than an equivalent diffraction limited image. This work emphasizes the ability to engineer the properties of confined optical modes and to leverage those characteristics for applications in imaging.…
We propose the optical trapping of Rayleigh particles using tailored anisotropic and hyperbolic metasurfaces illuminated with a linearly polarized Gaussian beam. This platform permits to engineer optical traps at the beam axis with a response governed by nonconservative and giant recoil forces coming from the directional excitation of ultra-confined surface plasmons during the light scattering process. Compared to optical traps set over bulk metals, the proposed traps are broadband in the sense that can be set with beams oscillating at any frequency within the wide range in which the metasurfa…
The in-plane negative refraction of high-momentum (i.e., high-k) photonic modes could enable many applications such as imaging and hyperlensing in a planar platform at deep-subwavelength scales. However, its practical implementation in experiments remains elusive so far. Here we propose a class of hyperbolic metasurfaces, which is characterized by an anisotropic magnetic sheet conductivity and can support the in-plane ultrahigh-k magnetic designer polaritons. Based on such metasurfaces, we report the first experimental observation of the all-angle negative refraction of designer polaritons at …
Transverse spin angular momentum is an inherent feature of evanescent waves which may have applications in nanoscale optomechanics, spintronics, and quantum information technology due to the robust spin-directional coupling. Here we analyze a local spin angular momentum density of hybrid surface waves propagating along anisotropic hyperbolic metasurfaces. We reveal that, in contrast to bulk plane waves and conventional surface plasmons at isotropic interfaces, the spin of the hybrid surface waves can be engineered to have an arbitrary angle with the propagation direction. This property allows …
Hyperbolic polaritons in van der Waals materials and metamaterial heterostructures provide unprecedented control over light-matter interaction at the extreme nanoscale. Here, we propose a concept of type-I hyperbolic metasurface supporting highly-squeezed magnetic designer polaritons, which act as magnetic analogues to hyperbolic polaritons in the hexagonal boron nitride (h-BN) in the first Reststrahlen band. Comparing with the natural h-BN, the size and spacing of the metasurface unit cell can be readily scaled up (or down), allowing for manipulating designer polaritons in frequency and in sp…
Metasurfaces offer the potential to control light propagation at the nanoscale for applications in both free-space and surface-confined geometries. Existing metasurfaces frequently utilize metallic polaritonic elements with high absorption losses, and/or fixed geometrical designs that serve a single function. Here we overcome these limitations by demonstrating a reconfigurable hyperbolic metasurface comprising of a heterostructure of isotopically enriched hexagonal boron nitride (hBN) in direct contact with the phase-change material (PCM) vanadium dioxide (VO2). Spatially localized metallic an…
Highly confined surface waves present unique opportunities to enhance light interactions with localized emitters or molecules. Hyperbolic dispersion in metasurfaces allows us to tailor and manipulate surface waves, enhancing the local density of states over broad bandwidths. So far, propagation on this platform was mainly studied in planar geometries, which facilitates the analysis but somehow limits the realm of possibilities. Here we show that "wrapping" hyperbolic metasurfaces into tubes may greatly enrich the wave propagation dynamics along their axis. This system shows strong interaction …
Polaritons, coupled excitations of photons and dipolar matter excitations, can propagate along anisotropic metasurfaces with either hyperbolic or elliptical dispersion. At the transition from hyperbolic to elliptical dispersion (corresponding to a topological transition), various intriguing phenomena are found, such as an enhancement of the photonic density of states, polariton canalization and hyperlensing. Here we investigate theoretically and experimentally the topological transition and the polaritonic coupling of deeply subwavelength elements in a uniaxial infrared-phononic metasurface, a…
Optical antennas made out of materials with hyperbolic dispersion is an alternative approach to realizing efficient subwavelength scatterers and may overcome limitations imposed by plasmonic and all-dielectric designs. Recently emerged natural hyperbolic material hexagonal boron nitride supports phonon-polariton excitations with low optical losses and high anisotropy. Here we study scattering properties of the hyperbolic-medium (HM) antennas, and in particular, we consider a combination of two types of the particles - HM bars and silicon spheres - arranged in a periodic array. We analyze excit…
Hyperbolic phonon polaritons (HPhPs) are generated when infrared photons couple to polar optic phonons in anisotropic media, confining long-wavelength light to nanoscale volumes. However, to realize the full potential of HPhPs for infrared optics, it is crucial to understand propagation and loss mechanisms on substrates suitable for applications from waveguiding to infrared sensing. In this paper, we employ scattering-type scanning near-field optical microscopy (s-SNOM) and nano-Fourier transform infrared (FTIR) spectroscopy, in concert with analytical and numerical calculations, to elucidate …
