A semiconductor quantum dot (QD) embedded within an optical microcavity is a system of fundamental importance within quantum information processing. The optimization of quantum coherence is crucial in such applications, requiring an in-depth understanding of the relevant decoherence mechanisms. We provide herein a critical review of prevalent theoretical treatments of the QD-cavity system coupled to longitudinal acoustic phonons, comparing predictions against a recently obtained exact solution. Within this review we consider a range of temperatures and exciton-cavity coupling strengths. Predictions of the polaron Nakajima-Zwanzig (NZ) and time-convolutionless (TCL) master equations, as well as a variation of the former adapted for adiabatic continuous wave excitation (CWE), are compared against an asymptotically exact solution based upon Trotter's decomposition (TD) theorem. The NZ and TCL implementations, which apply a polaron transformation to the Hamiltonian and subsequently treat the exciton-cavity coupling to second order, do not offer a significant improvement accuracy relative to the polaron transformation alone. The CWE adaptation provides a marked improvement, capturing the broadband features of the absorption spectrum (not present in NZ and TCL implementations). We attribute this difference to the effect of the Markov approximation, and particularly its unsuitability in pulsed excitation regime. Even the CWE adaptation, however, breaks down in the regime of high temperature ($50K$) and strong exciton-cavity coupling ($g \gtrsim 0.2$ meV). The TD solution is of comparable computational complexity to the above-mentioned master equation approaches, yet remains accurate at higher temperatures and across a broad range of exciton-cavity coupling strengths (at least up to $g=1.5$ meV).
We study phonon-assisted dephasing in optically excited semiconductor quantum dots within the frameworks of the independent Boson model and optimal control. Using a realistic description for the quantum dot states and the phonon coupling, we demonstrate that such dephasing has a drastic impact on the coherent optical response. We employ optimal control theory to search for control strategies that allow to fight decoherence, and show that appropriate tailoring of laser pulses allows a complete control of the optical excitation despite the phonon dephasing.
Polaron dephasing processes are investigated in InAs/GaAs dots using far-infrared transient four wave mixing (FWM) spectroscopy. We observe an oscillatory behaviour in the FWM signal shortly (< 5 ps) after resonant excitation of the lowest energy conduction band transition due to coherent acoustic phonon generation. The subsequent single exponential decay yields long intraband dephasing times of 90 ps. We find excellent agreement between our measured and calculated FWM dynamics, and show that both real and virtual acoustic phonon processes are necessary to explain the temperature dependence of…
We present the theory and numerical evaluations of the backscattering rate determined by acceptor holes or Mn spins in HgTe and (Hg,Mn)Te quantum wells in the quantum spin Hall regime. The role of anisotropic s-p and sp-d exchange interactions, Kondo coupling, Luttinger liquid effects, precessional dephasing, and bound magnetic polarons is quantified. The determined magnitude and temperature dependence of conductance are in accord with experimental results for HgTe and (Hg,Mn)Te quantum wells.
We use an on-chip superconducting resonator as a sensitive meter to probe the properties of graphene double quantum dots at microwave frequencies. Specifically, we investigate the charge dephasing rates in a circuit quantum electrodynamics architecture. The dephasing rates strongly depend on the number of charges in the dots, and the variation has a period of four charges, over an extended range of charge numbers. Although the exact mechanism of this fourfold periodicity in dephasing rates is an open problem, our observations hint at the fourfold degeneracy expected in graphene from its spin a…
We present a semi-analytic and asymptotically exact solution to the problem of phonon-induced decoherence in a quantum dot-microcavity system. Particular emphasis is placed on the linear polarization and optical absorption, but the approach presented herein may be straightforwardly adapted to address any elements of the exciton-cavity density matrix. At its core, the approach combines Trotter's decomposition theorem with the linked cluster expansion. The effects of the exciton-cavity and exciton-phonon couplings are taken into account on equal footing, thereby providing access to regimes of co…
Systems in the dispersive regime of cavity quantum electrodynamics (QED) are approaching the limits of validity of the dispersive approximation. We present a model which takes into account nonlinear corrections to the dressing of the atom by the field. We find that in the presence of pure dephasing, photons populating the cavity act as a heat bath on the atom, inducing incoherent relaxation and excitation. These effects are shown to reduce the achievable signal-to-noise ratio in cavity QED realizations where the atom is measured indirectly through cavity transmission and in particular in circu…
The time evolution of a quantum dot exciton in Coulomb interaction with wetting layer carriers is treated using an approach similar to the independent boson model. The role of the polaronic unitary transform is played by the scattering matrix, for which a diagrammatic, linked cluster expansion is available. Similarities and differences to the independent boson model are discussed. A numerical example is presented.
We have performed spectroscopic measurements of a superconducting qubit dispersively coupled to a nonlinear resonator driven by a pump microwave field. Measurements of the qubit frequency shift provide a sensitive probe of the intracavity field, yielding a precise characterization of the resonator nonlinearity. The qubit linewidth has a complex dependence on the pump frequency and amplitude, which is correlated with the gain of the nonlinear resonator operated as a small-signal amplifier. The corresponding dephasing rate is found to be close to the quantum limit in the low-gain limit of the am…
Superconducting electrical circuits can be used to study the physics of cavity quantum electrodynamics (QED) in new regimes, therefore realizing circuit QED. For quantum information processing and quantum optics, an interesting regime of circuit QED is the dispersive regime, where the detuning between the qubit transition frequency and the resonator frequency is much larger than the interaction strength. In this paper, we investigate how non-linear corrections to the dispersive regime affect the measurement process. We find that in the presence of pure qubit dephasing, photon population of the…
In this work we develop a semi-analytical variational ansatz to study the properties of few photon excitations interacting with a collection of quantum emitters in regimes that go beyond the rotating wave approximation. This method can be used to approximate both the static and dynamical properties of a superconducting qubit in an open transmission line, including the spontaneous emission spectrum and the resonances in scattering experiments. The approximations are quantitatively accurate for rather strong couplings, as shown by a direct comparison to Matrix-Product-State numerical methods, an…
We analyze the backaction of homodyne detection and photodetection on superconducting qubits in circuit quantum electrodynamics. Although both measurement schemes give rise to backaction in the form of stochastic phase rotations, which leads to dephasing, we show that this can be perfectly undone provided that the measurement signal is fully accounted for. This result improves upon that of Phys. Rev. A, 82, 012329 (2010), showing that the method suggested can be made to realize a perfect two-qubit parity measurement. We propose a benchmarking experiment on a single qubit to demonstrate the met…
We observe measurement-induced qubit state mixing in a transmon qubit dispersively coupled to a planar readout cavity. Our results indicate that dephasing noise at the qubit-readout detuning frequency is up-converted by readout photons to cause spurious qubit state transitions, thus limiting the nondemolition character of the readout. Furthermore, we use the qubit transition rate as a tool to extract an equivalent flux noise spectral density at f ~ 1 GHz and find agreement with values extrapolated from a $1/f^α$ fit to the measured flux noise spectral density below 1 Hz.
The influence of electron--phonon interactions on the dynamics of a quantum dot coupled to a photonic cavity mode is investigated using a nonequilibrium Green's function approach. Within a polaron frame, the self-consistent-Born approximation is used to treat the phonon-assisted scattering processes between the quantum dot polaron and the cavity. Two-time correlators of the quantum dot-cavity system are calculated by solving the Kadanoff-Baym equations, giving access to photon spectra and photon indistinguishability. The non-Markovian nature of the interaction with the phonon bath is shown to …
When mobile impurities are introduced and coupled to a Fermi sea, new quasiparticles known as Fermi polarons are formed. There are two interesting, yet drastically different regimes of the Fermi polaron problem: (I) the attractive polaron (AP) branch, connected to pairing phenomena spanning the crossover from BCS superfluidity to the Bose-Einstein condensation of molecules; and (II) the repulsive branch (RP), which underlies the physics responsible for Stoner's itinerant ferromagnetism. Here, we study Fermi polarons in two dimensional systems, where many questions and debates regarding their n…
A Lorentz invariant version of a mass-gap graphene-like planar quantum electrodynamics, the parity-preserving $U(1)\times U(1)$ massive QED$_3$, exhibits attractive interaction in low-energy electron-polaron--electron-polaron $s$-wave scattering, favoring quasiparticles bound states, the $s$-wave bipolarons.
Detailed properties of resonance fluorescence from a single quantum dot in a micropillar cavity are investigated, with particular focus on emission coherence in dependence on optical driving field power and detuning. Power-dependent series over a wide range could trace characteristic Mollow triplet spectra with large Rabi splittings of $|Ω| \leq 15$ GHz. In particular, the effect of dephasing in terms of systematic spectral broadening $\propto Ω^2$ of the Mollow sidebands is observed as a strong fingerprint of excitation-induced dephasing. Our results are in excellent agreement with prediction…
Motivated by recent experiments, we analyse the phonon-assisted steady-state gain of a microwave field driving a double quantum-dot in a resonator. We apply the results of our companion paper, which derives the complete set of fourth-order Lindblad dissipators using Keldysh methods, to show that resonator gain and loss are substantially affected by dephasing-assisted dissipative processes in the quantum-dot system. These additional processes, which go beyond recently proposed polaronic theories, are in good quantitative agreement with experimental observations
Recent breakthroughs in quantum-dot circuit-quantum-electrodynamics (circuit-QED) systems are important both from a fundamental perspective and from the point of view of quantum photonic devices. However, understanding the applications of such setups as potential thermoelectric diodes and transistors has been missing. In this paper, via the Keldysh nonequilibrium Green's function approach, we show that cavity-coupled double quantum-dots can serve as excellent quantum thermoelectric diodes and transistors. Using an enhanced perturbation approach based on polaron-transformations, we find non-mon…
We propose an analog quantum simulator for the Holstein molecular-crystal model based on a superconducting circuit QED system in the dispersive regime. By varying the driving field on the superconducting resonators, one can readily access both the adiabatic and anti-adiabatic regimes of this model. Strong e-ph coupling required for small-polaron formation can also be reached. We show that small-polaron state of arbitrary quasimomentum can be generated by applying a microwave pulse to the resonators. We also show that significant squeezing in the resonator modes can be achieved in the polaron-c…
We investigate the influence of electron-phonon interactions on the dynamical properties of a quantum-dot-cavity QED system. We show that non-Markovian effects in the phonon reservoir lead to strong changes in the dynamics, arising from photon-assisted dephasing processes, not present in Markovian treatments. A pronounced consequence is the emergence of a phonon induced spectral asymmetry when detuning the cavity from the quantum-dot resonance. The asymmetry can only be explained when considering the polaritonic quasi-particle nature of the quantum-dot-cavity system. Furthermore, a temperature…
We study the resonance fluorescence spectra of a driven quantum dot placed inside a high $Q$ semiconductor cavity and interacting with an acoustic phonon bath. The dynamics is calculated using a time-convolutionless master equation obtained in the polaron frame. We demonstrate pronounced spectral broadening of the Mollow sidebands through cavity-emission which, for small cavity-coupling rates, increases quadratically with the Rabi frequency. However, for larger cavity coupling rates, this broadening dependence is found to be more complex. This field-dependent Mollow triplet broadening is prima…
We investigate the power-dependent photoluminescence spectra from a strongly coupled quantum dot-cavity system using a quantum master equation technique that accounts for incoherent pumping, pure dephasing, and fermion or boson statistics. Analytical spectra at the one-photon correlation level and the numerically exact multi-photon spectra for fermions are presented. We compare to recent experiments on a quantum dot-micropiller cavity system and show that an excellent fit to the data can be obtained by varying only the incoherent pump rates in direct correspondence with the experiments. Our th…
Circuit cavity quantum electrodynamics (QED) is proving to be a powerful platform to implement quantum feedback control schemes due to the ability to control superconducting qubits and microwaves in a circuit. Here, we present a simple and promising quantum feedback control scheme for deterministic generation and stabilization of a three-qubit $W$ state in the superconducting circuit QED system. The control scheme is based on continuous joint Zeno measurements of multiple qubits in a dispersive regime, which enables us not only to infer the state of the qubits for further information processin…
We study coherent transport through a double quantum dot. Its two electronic leads induce electronic matter and energy transport and a phonon reservoir contributes further energy exchanges. By treating the system-lead couplings perturbatively, whereas the coupling to vibrations is treated non-perturbatively in a polaron-transformed frame, we derive a thermodynamic consistent low-dimensional master equation. When the number of phonon modes is finite, a Markovian description is only possible when these couple symmetrically to both quantum dots. For a continuum of phonon modes however, also asymm…
We study the decoherence of a superconducting qubit due to the dispersive coupling to a damped harmonic oscillator. We go beyond the weak qubit-oscillator coupling, which we associate with a phase Purcell effect, and enter into a strong coupling regime, with qualitatively different behavior of the dephasing rate. We identify and give a physicaly intuitive discussion of both decoherence mechanisms. Our results can be applied, with small adaptations, to a large variety of other physical systems, e. g. trapped ions and cavity QED, boosting theoretical and experimental decoherence studies.
We investigate the behavior of a circuit QED device when the resonator is initially populated with a mesoscopic coherent field. The strong coupling between the cavity and the qubit produces an entangled state involving mesoscopic quasi-pointer states with respect to cavity dissipation. The overlap of the associated field components results in collapse and revivals for the Rabi oscillation. Although qubit relaxation and dephasing do not preserve these states, a simple analytical description of the dissipative dynamics of the circuit QED device including cavity relaxation as well as qubit dissip…
We develop a theoretical framework to describe the scattering of photons against a two-level quantum emitter with arbitrary correlated dephasing noise. This is particularly relevant to waveguide-QED setups with solid-state emitters, such as superconducting qubits or quantum dots, which couple to complex dephasing environments in addition to the propagating photons along the waveguide. Combining input-output theory and stochastic methods, we predict the effect of correlated dephasing in single-photon transmission experiments with weak coherent inputs. We discuss homodyne detection and photon co…
We describe a scheme for the efficient generation of microwave photon pairs by parametric downconversion in a superconducting transmission line resonator coupled to a Cooper pair box serving as an artificial atom. By properly tuning the first three levels with respect to the cavity modes, the down-conversion probability may become higher than in the most efficient schemes for optical photons. We show this by numerically simulating the dissipative quantum dynamics of the coupled cavity-box system and discuss the effects of dephasing and relaxation. The setup analyzed here might form the basis f…
We present an off-resonant excitation scheme that realizes pronounced stationary inversion in a two level system. The created inversion exploits a cavity-assisted two photon resonance to enhance the multi-photon regime of nonlinear cavity QED and survives even in a semiconductor environment, where the cavity decay rate is comparable to the cavity-dot coupling rate. Exciton populations of greater than 0.75 are obtained in the presence of realistic decay and pure dephasing. Quantum trajectory simulations and quantum master equation calculations help elucidate the underlying physics and delineate…
We use a quasi Hamiltonian formalism to describe the dissipative dynamics of a circuit QED qubit that is affected by several fluctuating two level systems with a 1/f noise power spectrum. The qubit-resonator interactions are described by the Jaynes Cummings model. We argue that the presence of pure dephasing noise in such a qubit-resonator system will also induce an energy relaxation mechanism via a fluctuating dipole coupling term. This random modulation of the coupling is seen to lead to rich physical behavior. For non-Markovian noise, the coupling can either worsen or alleviate decoherence …
We reveal the existence of polariton soliton solutions in the array of weakly coupled optical cavities, each containing an ensemble of interacting qubits. An effective complex Ginzburg-Landau equation is derived in the continuum limit taking into account the effects of cavity field dissipation and qubit dephasing. We have shown that an enhancement of the induced nonlinearity can be achieved by two order of the magnitude with a negative interaction strength which implies a large negative qubit-field detuning as well. Bright solitons are found to be supported under perturbations only in the uppe…
The strong coupling limit of cavity quantum electrodynamics (QED) implies the capability of a matter-like quantum system to coherently transform an individual excitation into a single photon within a resonant structure. This not only enables essential processes required for quantum information processing but also allows for fundamental studies of matter-light interaction. In this work we demonstrate strong coupling between the charge degree of freedom in a gate-detuned GaAs double quantum dot (DQD) and a frequency-tunable high impedance resonator realized using an array of superconducting quan…
We propose an approach for studying quantum information and performing high resolution spectroscopy of rotational states of trapped molecular ions using an on-chip superconducting microwave resonator. Molecular ions have several advantages over neutral molecules. Ions can be loaded into deep (1 eV) RF traps and are trapped independent of the electric dipole moment of their rotational transition. Their charge protects them from motional dephasing and prevents collisional loss, allowing 1 s coherence times when used as a quantum memory, with detection of single molecules possible in <10 ms. An a…
We investigate the influence of the electron-phonon interaction on the decay dynamics of a quantum dot coupled to an optical microcavity. We show that the electron-phonon interaction has important consequences on the dynamics, especially when the quantum dot and cavity are tuned out of resonance, in which case the phonons may add or remove energy leading to an effective non-resonant coupling between quantum dot and cavity. The system is investigated using two different theoretical approaches: (i) a second-order expansion in the bare phonon coupling constant, and (ii) an expansion in a polaron-…
We study the fundamental limit on single-photon indistinguishability imposed by decoherence due to phonon interactions in semiconductor quantum dot-cavity QED systems. Employing an exact diagonalization approach we find large differences compared to standard methods. An important finding is that short-time non-Markovian effects limit the maximal attainable indistinguishability. The results are explained using a polariton picture that yields valuable insight into the phonon-induced dephasing dynamics.
We theoretically study measurement induced-dephasing of a superconducting qubit in the circuit QED architecture and compare the results to those obtained experimentally by Schuster {\it et al.}, [Phys. Rev. Lett. 94, 123602 (2005)]. Strong coupling of the qubit to the resonator leads to a significant ac-Stark shift of the qubit transition frequency. As a result, quantum fluctuations in the photon number populating the resonator cause dephasing of the qubit. We find good agreement between the predicted line shape of the qubit spectrum and the experimental results. Furthermore, in the strong dis…
We present a comprehensive theoretical study of the resonance fluorescence spectra of an exciton-driven quantum dot (QD) placed inside a high-$Q$ semiconductor cavity and interacting with an acoustic phonon bath. We derive a quantum master equation (ME) in the polaron frame which includes exciton-phonon and exciton-cavity coupling to all orders. This work details and extends the theory used in a recent issue of {\em Physical Review Letters} (C. Roy and S. Hughes 2011: Phys. Rev. Lett. {\bf 106} 247403) to describe the QD Mollow triplet in the regime of semiconductor cavity-QED. Here we introdu…
We present a theoretical study of a superconducting charge qubit dispersively coupled to a transmission line resonator. Starting from a master equation description of this coupled system and using a polaron transformation, we obtain an exact effective master equation for the qubit. We then use quantum trajectory theory to investigate the measurement of the qubit by continuous homodyne measurement of the resonator out-field. Using the same porlaron transformation, a stochastic master equation for the conditional state of the qubit is obtained. From this result, various definitions of the measur…
Quantum state transfer into a memory, state shuttling over long distances via a quantum bus, and high-fidelity readout are important tasks for quantum technology. Realizing these tasks is challenging in the presence of realistic couplings to an environment. Here, we introduce and assess protocols that can be used in cavity QED to perform high-fidelity quantum state transfer and fast quantum nondemolition qubit readout through Hamiltonian engineering. We show that high-fidelity state transfer between a cavity and a single qubit can be performed, even in the limit of strong dephasing due to inho…
Understanding large-scale interacting quantum matter requires dealing with the huge number of quanta that are produced by scattering even a few particles against a complex quantum object. Prominent examples are found from high energy cosmic ray showers to the optical or electrical driving of degenerate Fermi gases. We tackle this challenge in the context of many-body quantum optics, as motivated by the recent developments of circuit quantum electrodynamics at ultrastrong coupling. The issue of particle production is addressed quantitatively with a simple yet powerful concept rooted in the quan…
We study the propagation of photons in a one-dimensional environment consisting of two non-interacting species of photons frustratingly coupled to a single spin-1/2. The ultrastrong frustrated coupling leads to an extreme mixing of the light and matter degrees of freedom, resulting in the disintegration of the spin and a breakdown of the "dressed-spin", or polaron, description. Using a combination of numerical and analytical methods, we show that the elastic response becomes increasingly weak at the effective spin frequency, showing instead an increasingly strong and broadband response at high…
All-electrical dephasing-protected spin qubits in altermagnets
Consejo Superior de Investigaciones Científicas (CSIC)（西班牙高等科学研究委员会）；Quantum Advanced Research Center (QuARC)（量子先进研究中心）；Instituto de Ciencia de Materiales de Madrid (ICMM)（马德里材料科学研究所）；Nordita（北欧理论天体物理学研究所）；KTH Royal Institute of Technology（瑞典皇家理工学院）；Stockholm University（斯德哥尔摩大学）
Chip-based cavity quantum electrodynamics (QED) devices consisting of a self-assembled InAs quantum dot (QD) coupled to a high quality factor GaAs microdisk cavity are coherently probed through their optical channel using a fiber taper waveguide. We highlight one particularly important aspect of this all-fiber measurement setup, which is the accuracy to which the optical coupling level and optical losses are known relative to typical free-space excitation techniques. This allows for precise knowledge of the intracavity photon number and measurement of absolute transmitted and reflected signals…
Polarized cross-correlation spectroscopy on a quantum dot charged with a single hole shows the sequential emission of photons with common circular polarization. This effect is visible without magnetic field, but becomes more pronounced as the field along the quantization axis is increased. We interpret the data in terms of electron dephasing in the X+ state caused by the Overhauser field of nuclei in the dot. We predict the correlation timescale can be increased by accelerating the emission rate with cavity-QED.
We present both experimental and theoretical investigations of a laser-driven quantum dot (QD) in the dressed-state regime of resonance fluorescence. We explore the role of phonon scattering and pure dephasing on the detuning-dependence of the Mollow triplet and show that the triplet sidebands may spectrally broaden or narrow with increasing detuning. Based on a polaron master equation approach which includes electron-phonon interaction nonperturbatively, we derive a fully analytical expression for the spectrum. With respect to detuning dependence, we identify a crossover between the regimes o…
We provide a self-contained review of master equation approaches to modelling phonon effects in optically driven self-assembled quantum dots. Coupling of the (quasi) two-level excitonic system to phonons leads to dissipation and dephasing, the rates of which depend on the excitation conditions, intrinsic properties of the QD sample, and its temperature. We describe several techniques, which include weak-coupling master equations that are perturbative in the exciton-phonon coupling, as well as those based on the polaron transformation that can remain valid for strong phonon interactions. We add…
Photonic states of superconducting microwave cavities controlled by transmon ancillas provide a platform for encoding and manipulating quantum information. A key challenge in scaling up the platform is the requirement to communicate on demand the information between the cavities. It has been recently demonstrated that a tunable bilinear interaction between two cavities can be realized by coupling them to a bichromatically-driven transmon ancilla, which allows swapping and interfering the multi-photon states of the cavities [Gao et al., Phys. Rev. X 8, 021073(2018)]. Here, we explore both theor…
We study entanglement dynamics in a system consisting of a qubit dispersively coupled to a finite-temperature, dissipative, driven oscillator. We show that there are two generic ways to generate entanglement: one can entangle the qubit either with the phase or the amplitude of the oscillator's motion. Using an exact solution of the relevant quantum master equation, we study the robustness of both these kinds of entanglement against the effects of dissipation and temperature; in the limit of zero temperature (but finite damping), a simple analytic expression is derived for the logarithmic negat…
Electron-phonon coupling in semiconductor quantum dots plays a significant role in determining the optical properties of excited excitons, especially the spectral nature of emitted photons. This paper presents a comprehensive theory and analysis of emission spectra from artificial atoms or quantum dots coupled to structured photon reservoirs and acoustic phonons, when excited with incoherent pump fields. As specific examples of structured reservoirs, we chose a Lorentzian cavity and a coupled cavity waveguide, which are of current experimental interest. For the case of optical cavities, we dir…
Cavity Control of Strongly Correlated Electrons Beyond Resonant Coupling
RWTH Aachen University（亚琛工业大学）；Max Planck Institute for the Structure and Dynamics of Matter（物质结构与动力学马普研究所）；Max Planck Institute for the Physics of Complex Systems（复杂系统物理马普研究所）
