The postulate of the existence of a jamming phase diagram (Liu and Nagel, Nature 396, 21 EP (1998aa)) provides a theoretical basis for the classification of a wide range of amorphous solids (colloidal, molecular and emulsion glasses, colloidal and polymer gels, foams and granular matter) on the basis of whether these materials are in the jammed or unjammed state. Whilst such simple classification is appealing, it fails to capture that the criterion of rigidity of such amorphous solids may be defined with respect to a particular deformation orientation or mode (i.e. shear, extrusion, consolidation). We consider this problem via the consolidation of strong colloidal gels, and find that the critical transitions during the consolidation of a strong colloidal gel (as indicated by maxima and minima in the relative normal stress difference) correspond directly to directed, frictional and non-frictional rigidity percolation. These results indicate a hierarchy of directed, jammed states during consolidation of such amorphous solids, and a direct link between particle-scale interactions and macroscopic collective behaviour of these systems driven far from equilibrium
Using molecular dynamics simulations, we study the steady shear flow of dense assemblies of anisotropic spherocylindrical particles of varying aspect ratios. Comparing frictionless and frictional particles we discuss the specific role of frictional inter-particle forces for the rheological properties of the system. In the frictional system we evidence a shear-thickening regime, similar to that for spherical particles. Furthermore, friction suppresses alignment of the spherocylinders along the flow direction. Finally, the jamming density in frictional systems is rather insensitive to variations…
We study the nature of the frictional jamming transition within the framework of rigidity percolation theory. Slowly sheared frictional packings are decomposed into rigid clusters and floppy regions with a generalization of the pebble game including frictional contacts. We discover a second-order transition controlled by the emergence of a system-spanning rigid cluster accompanied by a critical cluster size distribution. Rigid clusters also correlate with common measures of rigidity. We contrast this result with frictionless jamming, where the rigid cluster size distribution is noncritical.
Simulations are used to study the steady shear rheology of dense suspensions of frictional particles exhibiting discontinuous shear thickening and shear jamming, in which finite-range cohesive interactions result in a yield stress. We develop a constitutive model that combines yielding behavior and shear thinning at low stress with the frictional shear thickening at high stresses, in good agreement with the simulation results. This work shows that there is a distinct difference between solids below the yield stress and in the shear-jammed state, as the two occur at widely separated stress leve…
By generalizing a geometric argument for frictionless spheres, a model is proposed for the jamming density $ϕ_J$ of mechanically stable packings of bidisperse, frictional spheres. The monodisperse, $μ_s$-dependent jamming density $ϕ_J^{\mathrm{mono}}(μ_s)$ is the only input required in the model, where $μ_s$ is the coefficient of friction. The predictions of the model are validated by robust estimates of $ϕ_J$ obtained from computer simulations of up to $10^7$ particles for a wide range of $μ_s$, and size ratios up to 40:1. Although $ϕ_J$ varies nonmonotonically with the volume fraction of sma…
The role of friction coefficient, $μ$, on the jamming properties of disordered, particle packings is studied using computer simulations. Compressed, soft-sphere packings are brought towards the jamming transition - the point where a packing loses mechanical stability - by decreasing the packing fraction. The values of the packing fraction at the jamming transition, $ϕ^μ_{c}$, gradually decrease from the random close packing point for zero friction, to a value coincident with random loose packing as the friction coefficient is increased over several orders of magnitude. This is accompanied by a…
The critical rheology of sheared frictional granular materials near jamming transition is numer- ically investigated. It is confirmed that there exist a true critical density which characterizes the onset of the yield stress, and two fictitious critical densities which characterize the scaling laws of rheological properties. We find the existence of a hysteresis loop between two of the critical densities for each friction coefficient. It is noteworthy that the critical scaling law for frictionless jamming transition seems to be still valid even for frictional jamming despite using fictitious c…
In stark contrast to the jamming of frictionless hard-sphere (hard-disk if in two dimensions) packings, the critical jamming of frictional packings is much more elusive and still under intense debate. Here we show that frictional hard-disk packings self-organize near a critical jamming state when subjected to quasi-static steady-state cyclic shear, displaying scale-free fluctuations in particle velocity fields as characterized by the power spectra $E(k)\propto k^{-α}$ for both longitudinal and transverse modes in wavevector space, with $α\approx2.0\pm0.15$, and the nearly flat spectra $E(ω)\pr…
While frictionless spheres at jamming are isostatic, frictional spheres at jamming are not. As a result, frictional spheres near jamming do not necessarily exhibit an excess of soft modes. However, a generalized form of isostaticity can be introduced if fully mobilized contacts at the Coulomb friction threshold are considered as slipping contacts. We show here that, in this framework, the vibrational density of states (DOS) of frictional discs exhibits a plateau when the generalized isostaticity line is approached. The crossover frequency to elastic behavior scales linearly with the distance f…
We measure the displacement response of a frictional multicontact interface between identical polymer glasses to a biased shear force oscillation. We evidence the existence, for maximum forces close below the nominal static threshold, of a jamming creep regime governed by an ageing-rejuvenation competition acting within the micrometer-sized contacting asperities. Quantitative analysis of the creep curves suggests that another such mechanism might be at work within the nanometer-thick adhesive junctions.
We propose a phase diagram for the shear flow of dry granular particles in two dimensions based on simulations and a phenomenological Landau-theory for a nonequilibrium first order phase transition. Our approach incorporates both frictional as well as frictionless particles. The most important feature of the frictional phase diagram is re-entrant flow and a critical jamming point at finite stress. In the frictionless limit the regime of re-entrance vanishes and the jamming transition is continuous with a critical point at zero stress. The jamming phase diagrams derived from the model agree wit…
Dense suspension of particles in a liquid exhibit rich, non-Newtonian behaviors such as shear thickening and shear jamming. Shear thickening is known to be enhanced by increasing the particles' frictional interactions and also by making their shape more anisotropic. For shear jamming, however, only the role of interparticle friction has been investigated, while the effect of changing particle shape has so far not been studied systematically. To address this we here synthesize smooth silica particles and design the particle surface chemistry to generate strong frictional interactions such that …
The granular jamming transition is experimentally investigated in a two-dimensional system of frictional, bi-dispersed disks subject to quasi-static, uniaxial compression at zero granular temperature. Currently accepted results show the jamming transition occurs at a critical packing fraction $ϕ_c$. In contrast, we observe the first compression cycle exhibits {\it fragility} - metastable configuration with simultaneous jammed and un-jammed clusters - over a small interval in packing fraction ($ϕ_1 < ϕ< ϕ_2$). The fragile state separates the two conditions that define $ϕ_c$ with an exponential …
The non-equilibrium transition from a fluid-like state to a disordered solid-like state, known as the jamming transition, occurs in a wide variety of physical systems, such as colloidal suspensions and molecular fluids, when the temperature is lowered or the density increased. Shear stress, as temperature, favors the fluid-like state, and must be also considered to define the system 'jamming phase diagram' [1-4]. Frictionless athermal systems [1], for instance, can be described by the zero temperature plane of the jamming diagram in the temperature, density, stress space. Here we consider the …
We study agitated frictional disks in two dimensions with the aim of developing a scaling theory for their diffusion over time. As a function of the area fraction $ϕ$ and mean-square velocity fluctuations $\langle v^2\rangle$ the mean-square displacement of the disks $\langle d^2\rangle$ spans 4-5 orders of magnitude. The motion evolves from a subdiffusive form to a complex diffusive behabvior at long times. The statistics of $\langle d^n\rangle$ at all times are multiscaling, since the probability distribution function (pdf) of displacements has very broad wings. Even where a diffusion consta…
The formation of self-organised structures that resist shear deformation have been discussed in the context of shear jamming and thickening[1-3], with frictional forces playing a key role. However, shear induces geometric features necessary for jamming even in frictionless packings[4]. We analyse conditions for jamming in such assemblies by solving force and torque balance conditions for their contact geometry. We demonstrate, and validate with frictional simulations, that the isostatic condition for mean contact number Z = D + 1 (for spatial dimension D = 2, 3) holds at jamming for both finit…
A wide variety of interacting particle assemblies driven by an external force are characterized by a transition between a blocked and a moving phase. The origin of this deblocking transition can be traced back to the presence of either external quenched disorder, or of internal constraints. The first case belongs to the realm of the depinning transition, which, for example, is relevant for flux-lines in type II superconductors and other elastic systems moving in a random medium. The second case is usually included within the so-called jamming scenario observed, for instance, in many glassy mat…
Using numerical simulations we examine the velocity fluctuations of a probe particle driven with constant force through a two-dimensional disordered assembly of disks which has a well-defined jamming point J at a density of ϕ_J=0.843. As ϕincreases toward ϕ_J, the average velocity of the probe particle decreases and the velocity fluctuations show an increasingly intermittent or avalanchelike behavior. When the system is within a few percent of the jamming density, the velocity distributions are exponential, while when the system is less than a percent away from jamming, the velocity distributi…
We report a joint experimental and theoretical investigation of cyclic training of amorphous frictional granular assemblies, with special attention to memory formation and retention. Measures of dissipation and compactification are introduced, culminating with a proposed scaling law for the reducing dissipation and increasing memory. This scaling law is expected to be universal, insensitive to the details of the elastic and frictional interactions between the granules.
Discontinuous shear-thickening in dense suspensions naturally emerges from the activation of frictional forces by shear flow in non-Brownian systems close to jamming. Yet, this physical picture is incomplete as most experiments study soft colloidal particles subject to thermal fluctuations. To characterise discontinuous shear-thickening in colloidal suspensions we use computer simulations to provide a complete description of the competition between athermal jamming, frictional forces, thermal motion, particle softness, and shear flow. We intentionally neglect hydrodynamics, electrostatics, lub…
Pressure-imposed rheometry is used to examine the influence of surface roughness on the rheology of immersed and dry frictional spheres in the dense regime. The quasi-static value of the effective friction coefficient is not significantly affected by particle roughness while the critical volume fraction at jamming decreases with increasing roughness. These values are found to be similar in immersed and dry conditions. Rescaling the volume fraction by the maximum volume fraction leads to collapses of rheological data on master curves. The asymptotic behaviors are examined close to the jamming t…
Solids are distinguished from fluids by their ability to resist shear. In traditional solids, the resistance to shear is associated with the emergence of broken translational symmetry as exhibited by a non-uniform density pattern, which results from either minimizing the energy cost or maximizing the entropy or both. In this work, we focus on a class of systems, where this paradigm is challenged. We show that shear-driven jamming in dry granular materials is a collective process controlled solely by the constraints of mechanical equilibrium. We argue that these constraints lead to a broken tra…
Amorphous packings of frictionless, spherical particles are isostatic at jamming onset, with the number of constraints (contacts) equal to the number of degrees of freedom. Their structural and mechanical properties are controlled by the interparticle contact network. In contrast, amorphous packings of frictional particles are typically hyperstatic at jamming onset. We perform extensive numerical simulations in two dimensions of the geometrical asperity (GA) model for static friction, to further investigate the role of isostaticity. In the GA model, interparticle forces are obtained by summing…
We study granular suspensions under a variety of extensional deformations and simple shear using numerical simulations. The viscosity and Trouton's ratio (the ratio of extensional to shear viscosity) are computed as functions of solids volume fraction $ϕ$ close to the limit of zero inertia. Suspensions of frictionless particles follow a Newtonian Trouton's ratio for $ϕ$ all the way up to $ϕ_0$, a universal jamming point that is independent of deformation type. In contrast, frictional particles lead to a deformation-type-dependent jamming fraction $ϕ_m$, which is largest for shear flows. Trouto…
We present extensive computational results for the effective temperature, defined by the fluctuation-dissipation relation between the mean square displacement and the average displacement of grains, under the action of a weak, external perturbation, of a sheared, bi-disperse granular packing of compressible spheres. We study the dependence of this parameter on the shear rate and volume fractions, the type of particle and the observable in the fluctuation-dissipation relation. We find the same temperature for different tracer particles in the system. The temperature becomes independent on the s…
We show that in slowly generated 2d packings of frictional spheres, a significant fraction of the friction forces lies at the Coulomb threshold - for small pressure p and friction coefficient mu, about half of the contacts. Interpreting these contacts as constrained leads to a generalized concept of isostaticity, which relates the maximal fraction of fully mobilized contacts and contact number. For p->0, our frictional packings approximately satisfy this relation over the full range of mu. This is in agreement with a previous conjecture that gently built packings should be marginal solids at j…
Packings of macroscopic granular chains capture some of the essential aspects of molecular polymer systems and have been suggested as a paradigm to understand the physics on a molecular scale. However, here we demonstrate that the interparticle friction $μ$ in granular chain packings, which has no counterpart in polymer systems, leads to a nontrivial yielding and rheological response. Based on discrete element simulations we study the nonlinear rheology of random packings of granular chains under large amplitude oscillatory shear. We find that the maximum stress and the penetration depth of th…
Particles suspended in a Newtonian fluid raise the viscosity and also generally give rise to a shear-rate dependent rheology. In particular, pronounced shear thickening may be observed at large solid volume fractions. In a recent article (R. Seto, R. Mari, J. F. Morris, and M. M. Denn., Phys. Rev. Lett., 111:218301, 2013) we have considered the minimum set of components to reproduce the experimentally observed shear thickening behavior, including Discontinuous Shear Thickening (DST). We have found frictional contact forces to be essential, and were able to reproduce the experimental behavior b…
Multi-phase flows encountered in nature or in industry, exhibit non trivial rheological properties, that can be understood better thanks to model materials and appropriate rheometers. Here, we use model unsaturated granular materials: assemblies of frictional spherical particles bonded by a small quantity of a wetting liquid, over a rough inclined plane. Our results show steady uniform flows for a wide range of parameters (the inclination angle and the mass flow-rate). A theoretical model, based on the Mohr-Coulomb yield criterion extended to inertial flows: $τ$ = $τ$c + $μ$(I)P, in which $τ$c…
We compare the structural and mechanical properties of mechanically stable (MS) packings of frictional disks in two spatial dimensions (2D) generated with isotropic compression and simple shear protocols from discrete element modeling (DEM) simulations. We find that the average contact number and packing fraction at jamming onset are similar (with relative deviations $< 0.5\%$) for MS packings generated via compression and shear. In contrast, the average stress anisotropy $\langle {\hat Σ}_{xy} \rangle = 0$ for MS packings generated via isotropic compression, whereas $\langle {\hat Σ}_{xy} \ra…
The shear modulus of jammed frictional granular materials with the harmonic repulsive interaction under an oscillatory shear is numerically investigated. It is confirmed that the storage modulus, the real part of the shear modulus, for frictional grains with sufficiently small strain amplitude $γ_0$ discontinuously emerges at the jamming transition point. The storage modulus for small $γ_0$ differs from that of frictionless grains even in the zero friction limit, while they are almost identical with each other for sufficiently large $γ_0$, where the transition becomes continuous. The stress-st…
We report recent results of molecular dynamics simulations of frictional athermal particles at constant volume fraction and constant applied shear stress, focusing on a range of control parameters where the system first flows, but then jams after a time tjam. On decreasing the volume fraction, the mean jamming time diverges, while its sample fluctuations become so large that the jamming time probability distribution P(tjam) becomes a power-law. We obtain an insight on the origin of this phenomenology focusing on the flowing regime, which is characterized by the presence of a clear correlation …
Jammed states of frictional granular systems can be induced by shear strain at densities below the isostatic jamming density ($ϕ_c$). It remains unclear, however, how much friction affects this so-called shear-jamming. Friction appears in two ways in this type of experiment: friction between particles, and friction between particles and the base on which they rest. Here, we study how particle-bottom friction, or basal friction, affects shear jamming in quasi-two dimensional experiments. In order to study this issue experimentally, we apply simple shear to a disordered packing of photoelastic d…
The jamming transition is accompanied by a rich phenomenology, such as hysteresis or non-local effects, which is still not well understood. Here we experimentally investigate a model frictionless granular layer flowing down an inclined plane, as a way to disentangle generic collective effects from those arising from frictional interactions. We find that thin frictionless granular layers are devoid of hysteresis, yet the layer stability is increased as it gets thinner. Rheological laws obtained for different layer thicknesses can be collapsed into a unique master curve, supporting that non-loca…
We present experimental results on the shape of arches that block the outlet of a two dimensional silo. For a range of outlet sizes, we measure some properties of the arches such as the number of particles involved, the span, the aspect ratio, and the angles between mutually stabilizing particles. These measurements shed light on the role of frictional tangential forces in arching. In addition, we find that arches tend to adopt an aspect ratio (the quotient between height and half the span) close to one, suggesting an isotropic load. The comparison of the experimental results with data from nu…
Jamming crossovers occur at zero temperature in assemblies of particles interacting via finite range repulsive potentials, when on increasing the density particles make contacts with those of subsequent coordination shells. Density anomalies, including an increased diffusivity upon isothermal compression and a negative thermal expansion coefficient, are the finite temperature signatures of the jamming crossovers. In this manuscript we show that the jamming crossovers are correlated to an increase of the non affine response of the system to density changes, and clarify that jammed systems evolv…
We use 2D numerical simulations to study dense suspensions of non-Brownian hard particles using the Critical Load Model (CLM) under constant confining pressures. This simple model shows discontinuous shear thickening (DST) as the tangential forces get activated upon increased shear stresses. By parameterizing a simple binary system of frictional and non-frictional particles of different proportions we show that the jamming packing fraction, at which the viscosity diverges, is controlled by the fraction of frictional contacts. The viscosity of dense suspensions can thereby be expressed as a fun…
We find that in simulations of quasi-statically sheared frictional disks, the shear jamming transition can be characterized by an abrupt jump in the number of force bearing contacts between particles. This mechanical coordination number increases discontinuously from $Z = 0$ to $Z \gtrsim d +1$ at a critical shear value $γ_c$, as opposed to a smooth increase in the number of geometric contacts. This is accompanied by a diverging timescale $τ^*$ that characterizes the time required by the system to attain force balance when subjected to a perturbation. As the global shear $γ$ approaches the cri…
Dense suspensions of hard particles in a liquid can exhibit strikingly counter-intuitive behavior, such as discontinuous shear thickening (DST) [1-8] and reversible shear jamming (SJ) into a state with finite yield stress [9-13]. Recent studies identified a stress-activated crossover from hydrodynamic interactions to frictional particle contacts to be key for these behaviors [2-4, 6-8, 10, 14]. However, many suspensions exhibit only DST and not SJ. Here we show that particle surface chemistry can play a central role in creating conditions that allow for SJ. We find the system's ability to form…
The rotational Brownian motion of colloidal spheres in dense suspensions reflects local hydrodynamics and friction, both key to non-linear rheological phenomena such as shear-thickening and jamming, and transport in crowded environments, including intracellular migration and blood flow. To fully elucidate the role of rotational dynamics experimentally, it is crucial to measure the translational and rotational motion of all spheres simultaneously. Here, we develop compositionally uniform colloidal spheres with an off-centre, fully embedded core with a different fluorophore to the particle body,…
The mixing of a powder of 10-50μm primary particles into a liquid to form a dispersion with the highest possible solid content is a common industrial operation. Building on recent advances in the rheology of such 'granular dispersions', we study a paradigmatic example of such powder incorporation: the conching of chocolate, in which a homogeneous, flowing suspension is prepared from an inhomogeneous mixture of particulates, triglyceride oil and dispersants. Studying the rheology of a simplified formulation, we find that the input of mechanical energy and staged addition of surfactants combine …
We use computer simulations to study the microscopic dynamics of an athermal assembly of soft particles near the fluid-to-solid, jamming transition. Borrowing tools developed to study dynamic heterogeneity near glass transitions, we discover a number of original signatures of the jamming transition at the particle scale. We observe superdiffusive, spatially heterogeneous, and collective particle motion over a characteristic scale which displays a surprising non-monotonic behavior across the transition. In the solid phase, the dynamics is an intermittent succession of elastic deformations and p…
We review the physics of jamming from the theoretical, experimental and numerical perspectives. We summarize the mean-field theory of jamming and the marginally stable solid phase, with particular emphasis on the connection with the Replica Symmetry Breaking theory of glasses. We report validations of the mean-field theory of jamming from experimental and numerical studies of critical behaviors near the transition. In particular, we describe the physics of jamming of frictionless, spherical particles, as well as more recent work on jamming of frictionless, non-spherical particles and frictiona…
The structural properties of static, jammed packings of monodisperse spheres in the vicinity of the jamming transition are investigated using large-scale computer simulations. At small wavenumber $k$, we argue that the anomalous behavior in the static structure factor, $S(k) \sim k$, is consequential of an excess of low-frequency, collective excitations seen in the vibrational spectrum. This anomalous feature becomes more pronounced closest to the jamming transition, such that $S(0) \to 0$ at the transition point. We introduce an appropriate dispersion relation that accounts for these phenomen…
A consensus is emerging that discontinuous shear thickening (DST) in dense suspensions marks a transition from a flow state where particles remain well separated by lubrication layers, to one dominated by frictional contacts. We show here that reasonable assumptions about contact proliferation predict two distinct types of DST in the absence of inertia. The first occurs at densities above the jamming point of frictional particles; here the thickened state is completely jammed and (unless particles deform) cannot flow without inhomogeneity or fracture. The second regime shows strain- rate hyste…
The phenomenon of shear-induced jamming is a factor in the complex rheological behavior of dense suspensions. Such shear-jammed states are fragile, i.e., they are not stable against applied stresses that are incompatible with the stress imposed to create them. This peculiar flow-history dependence of the stress response is due to flow-induced microstructures. To examine jammed states realized under constant shear stress, we perform dynamic simulations of non-Brownian particles with frictional contact forces and hydrodynamic lubrication forces. We find clear signatures that distinguish these fr…
Amorphous materials as diverse as foams, emulsions, colloidal suspensions and granular media can jam into a rigid, disordered state where they withstand finite shear stresses before yielding. Here we review the current understanding of the transition to jamming and the nature of the jammed state for disordered packings of particles that act through repulsive contact interactions and are at zero temperature and zero shear stress. We first discuss the breakdown of affine assumptions that underlies the rich mechanics near jamming. We then extensively discuss jamming of frictionless soft spheres. …
We analyze the isotropic compaction of assemblies composed of soft pentagons interacting through classical Coulomb friction via numerical simulations. The effect of the initial particle shape is discussed by comparing packings of pentagons with packings of soft circular particles. We characterize the evolution of the packing fraction, the elastic modulus, and the microstructure (particle rearrangement, connectivity, contact force and particle stress distributions) as a function of the applied stresses. Both systems behave similarly; the packing fraction increases and tends asymptotically to a …
Amorphous packings of spheres have been intensely investigated in order to understand the mechanical and flow behaviour of dense granular matter, and to explore universal aspects of the transition from fluid to structurally arrested or jammed states. Considerable attention has recently been focussed on anisotropic packings of frictional grains generated by shear deformation leading to shear jamming, which occurs below the jamming density for isotropic packings of frictionless grains. With the aim of disentangling the role of shear deformation induced structures and friction in generating shear…
The effect of increasing structural disorder on the distribution of contact forces P(f), inside three dimensional particle assemblies is systematically studied using computer simulations of model granular packings. Starting from a face-centred cubic array, where all contact forces are identical, an increasing number of defects is introduced into the assembly, after which the system is then allowed to relax into a new mechanically stable state. Three distinct protocols for imposing disorder are compared. A quantitative measure of the disorder is obtained from distributions of the coordination n…
We investigate the rheology of granular materials via molecular dynamics simulations of homogeneous, simple shear flows of soft, frictional, noncohesive spheres. In agreement with previous results for frictionless particles, we observe three flow regimes existing in different domains of particle volume fraction and shear rate, with all stress data collapsing upon scaling by powers of the distance to the jamming point. Though this jamming point is a function of the interparticle friction coefficient, the relation between pressure and strain rate at this point is found to be independent of frict…
