M. J. Jacquet, T. Boulier, F. Claude, A. Maitre, E. Cancellieri, C. Adrados, A. Amo, S. Pigeon, Q. Glorieux, A. Bramati, E. Giacobino
备注：
Accepted for publication in Philosophical Transactions of the Royal Society A: special issue on Analogue Gravity. V3 with some typos corrected and amended abstract
Analogue gravity enables the study of fields on curved spacetimes in the laboratory. There are numerous experimental platforms in which amplification at the event horizon or the ergoregion has been observed. Here, we demonstrate how optically generating a defect in a polariton microcavity enables the creation of one- and two-dimensional, transsonic fluid flows. We show that this highly tuneable method permits the creation of sonic horizons. Furthermore, we present a rotating geometry akin to the water-wave bathtub vortex. These experiments usher-in the possibility of observing stimulated as well as spontaneous amplification by the Hawking, Penrose and Zeld'ovich effects in fluids of light.
We demonstrate generation of chiral modes -- vortex flows with fixed handedness in exciton-polariton quantum fluids. The chiral modes arise in the vicinity of exceptional points (non-Hermitian spectral degeneracies) in an optically-induced resonator for exciton polaritons. In particular, a vortex is generated by driving two dipole modes of the non-Hermitian ring resonator into degeneracy. Transition through the exceptional point in the space of the system's parameters is enabled by precise manipulation of real and imaginary parts of the closed-wall potential forming the resonator. As the syste…
Exciton-polaritons have been shown to be an optimal system in order to investigate the properties of bosonic quantum fluids. We report here on the observation of dark solitons in the wake of engineered circular obstacles and their decay into streets of quantized vortices. Our experiments provide a time-resolved access to the polariton phase and density, which allows for a quantitative study of instabilities of freely evolving polaritons. The decay of solitons is quantified and identified as an effect of disorder-induced transverse perturbations in the dissipative polariton gas.
We study the quantum hydrodynamical features of exciton-polaritons flowing circularly in a ring-shaped geometry. We consider a resonant-excitation scheme in which the spinor polariton fluid is set into motion in both components by spin-to-orbital angular momentum conversion. We show that this scheme allows to control the winding number of the fluid, and to create two circulating states differing by two units of the angular momentum. We then consider the effect of a disorder potential, which is always present in realistic nanostructures. We show that a smooth disorder is efficiently screened by…
We report the formation of a macroscopic coherent state emerging from colliding polariton fluids. Four lasers with random relative phases, arranged in a square, pump resonantly a planar microcavity, creating four coherent polariton fluids propagating toward each other. When the density (interactions) increases, the four fluids synchronise and the topological excitations (vortex or soliton) disappear to form a single superfluid.
Quantum effects of fields on curved spacetimes may be studied in the laboratory thanks to quantum fluids. Here we use a polariton fluid to study the Hawking effect, the correlated emission from the quantum vacuum at the acoustic horizon. We show how out-of-equilibrium physics affects the dispersion relation, and hence the emission and propagation of correlated waves: the fluid properties on either side of the horizon are critical to observing the Hawking effect. We find that emission may be optimised by supporting the phase and density of the fluid upstream of the horizon in a regime of optica…
We theoretically investigate how the presence of a reservoir of incoherent excitations affects the superfluidity properties of resonantly driven polariton fluids. While in the absence of reservoir the two cases of a defect moving in a fluid at rest and of a fluid flowing against a static defect are linked by a formal Galilean transformation, here the reservoir defines a privileged reference frame attached to the semiconductor structure and causes markedly different features between the two settings. The consequences on the critical velocity for superfluidity are highlighted and compared to exp…
We use a one-dimensional polariton fluid in a semiconductor microcavity to explore the rich nonlinear dynamics of counter-propagating interacting Bose fluids. The intrinsically driven-dissipative nature of the polariton fluid allows to use resonant pumping to impose a phase twist across the fluid. When the polariton-polariton interaction energy becomes comparable to their kinetic energy, linear interference fringes transform into a train of solitons. A novel type of bistable behavior controlled by the phase twist across the fluid is experimentally evidenced.
Characterising elementary excitations in quantum fluids is essential to study collective effects within. We present an original angle-resolved coherent probe spectroscopy technique to study the dispersion of these excitation modes in a fluid of polaritons under resonant pumping. Thanks to the unprecedented spectral and spatial resolution, we observe directly the low-energy phononic behaviour and detect the negative-energy modes, i.e. the \textit{ghost branch}, of the dispersion relation. In addition, we reveal narrow spectral features precursory of dynamical instabilities due to the intrinsic …
Exciton-polaritons in semiconductor microcavities constitute the archetypal realization of a quantum fluid of light. Under coherent optical drive, remarkable effects such as superfluidity, dark solitons or the nucleation of hydrodynamic vortices have been observed. These phenomena can be all understood as a specific manifestation of collective excitations forming on top of the polariton condensate. In this work, we performed a Brillouin scattering experiment to measure their dispersion relation $ω(\mathbf{k})$ directly. The result, such as a speed of sound which is apparently twice too low, ca…
In resonantly pumped polariton superfluids we recently explored a new regime based on the bistability of the polariton system to enhance the propagation of polariton fluids up to macroscopic distances. This technique together with an all-optical imprinting method allowed the generation and control of various topological excitations such as quantized vortices and dark solitons. The flexibility and scalability of the new experimental scheme opens the way to the systematic study of quantum turbulence in driven dissipative quantum fluids of light. In this article we review the basic working princi…
We investigate the propagation and scattering of polaritons in a planar GaAs microcavity in the linear regime under resonant excitation. The propagation of the coherent polariton wave across an extended defect creates phase and intensity patterns with identical qualitative features previously attributed to dark and half-dark solitons of polaritons. We demonstrate that these features are observed for negligible nonlinearity (i.e., polariton-polariton interaction) and are, therefore, not sufficient to identify dark and half-dark solitons. A linear model based on the Maxwell equations is shown to…
Atomically thin transition metal dichalcogenides (TMDs) possess a number of properties that make them attractive for realizing room-temperature polariton devices. An ideal platform for manipulating polariton fluids within monolayer TMDs is that of Bloch surface waves, which confine the electric field to a small volume near the surface of a dielectric mirror. Here we demonstrate that monolayer tungsten disulfide ($\text{WS}_2$) can sustain Bloch surface wave polaritons (BSWPs) with a Rabi splitting of 43 meV and propagation constants reaching 33 $μ$m. In addition, we evidence strong polariton-p…
Exciton-polaritons constitute a unique realization of a quantum fluid interacting with its environment. Using Selenide based microcavities, we exploit this feature to warm up a polariton condensate in a controlled way and monitor its spatial coherence. We determine directly the amount of heat picked up by the condensate by measuring the phonon-polariton scattering rate and comparing it with the loss rate. We find that upon increasing the heating rate, the spatial coherence length decreases markedly, while localized phase structures vanish, in good agreement with a stochastic mean field theory.…
Motivated by recent experiments, we theoretically analyze the flow past an obstacle of a one-dimensional "quantum fluid of light" which is resonantly driven, and exhibits bistability. The flow is found to abruptly change several times when the fluid velocity or the obstacle potential strength are increased. In contrast to the cases of usual fluids and superfluids, the transitions take place between stationary states. They involve the fluid bistability in an essential way. Remarkably, at the transitions points, the fluid in the obstacle wake lies in the unstable intermediate density state.
Spinorial or multi-component Bose-Einstein condensates may sustain fractional quanta of circulation, vorticant topological excitations with half integer windings of phase and polarization. Matter-light quantum fluids, such as microcavity polaritons, represent a unique test bed for realising strongly interacting and out-of-equilibrium condensates. The direct access to the phase of their wavefunction enables us to pursue the quest of whether half vortices ---rather than full integer vortices--- are the fundamental topological excitations of a spinor polariton fluid. Here, we are able to directly…
We study exciton-polariton nonlinear optical fluids in a high momentum regime for the first time. Defects in the fluid develop into dark solitons whose healing length decreases with increasing density. We deduce interaction constants for continuous wave polaritons an order of magnitude larger than with picosecond pulses. Time dependent measurements show a 100ps time for the buildup of the interaction strength suggesting a self-generated excitonic reservoir as the source of the extra nonlinearity. The experimental results agree well with a model of coupled photons, excitons and the reservoir.
We study the stability of a multicomponent exciton-polariton fluid under resonant excitation within the linear response approximation of a generalized Gross-Pitaevskii equation. We show that, two spatially homogeneous and independently tunable pumping lasers produce, for the same values of the system parameters, up to three stable solutions. Three-stability is understood by noting that the cavity can be either little or highly populated and, in this second case, the largest part of the population lies in either one of the two components. Moreover, we show that easily tunable multistable hyster…
We present the theoretical prediction of spontaneous rotating vortex rings in a parametrically driven quantum fluid of polaritons -- coherent superpositions of coupled quantum well excitons and microcavity photons. These rings arise not only in the absence of any rotating drive, but also in the absence of a trapping potential, in a model known to map quantitatively to experiments. We begin by proposing a novel parametric pumping scheme for polaritons, with circular symmetry and radial currents, and characterize the resulting nonequilibrium condensate. We show that the system is unstable to spo…
If a quantum fluid is driven with enough angular momentum, at equilibrium the ground state of the system is given by a lattice of quantised vortices whose density is prescribed by the quantization of circulation. We report on the first experimental study of the Feynman-Onsager relation in a non-equilibrium polariton fluid, free to expand and rotate. Upon initially imprinting a lattice of vortices in the quantum fluid, we track the vortex core positions on picosecond time scales. We observe an accelerated stretching of the lattice and an outward bending of the linear trajectories of the vortice…
Monopoles are magnetic charges, point-like sources of magnetic field. Contrary to electric charges they are absent in Maxwell's equations and have never been observed as fundamental particles. Quantum fluids such as spinor Bose-Einstein condensates have been predicted to show monopoles in the form of excitations combining phase and spin topologies. Thanks to its unique spin structure and the direct optical control of the fluid wavefunction, an ideal system to experimentally explore this phenomenon is a condensate of exciton-polaritons in a semiconductor microcavity. We use this system to creat…
We study the linear response of a coherently driven polariton fluid in the pump-only configuration scattering against a point-like defect and evaluate analytically the drag force exerted by the fluid on the defect. When the system is excited near the bottom of the lower polariton dispersion, the sign of the interaction-renormalised pump detuning classifies the collective excitation spectra in three different categories [C. Ciuti and I. Carusotto, physica status solidi (b) 242, 2224 (2005)]: linear for zero, diffusive-like for positive, and gapped for negative detuning. We show that both cases …
Seeing macroscopic quantum states directly remains an elusive goal. Particles with boson symmetry can condense into such quantum fluids producing rich physical phenomena as well as proven potential for interferometric devices [1-10]. However direct imaging of such quantum states is only fleetingly possible in high-vacuum ultracold atomic condensates, and not in superconductors. Recent condensation of solid state polariton quasiparticles, built from mixing semiconductor excitons with microcavity photons, offers monolithic devices capable of supporting room temperature quantum states [11-14] tha…
Topological defects such as quantized vortices are one of the most striking manifestations of the superfluid nature of Bose-Einstein condensates and typical examples of quantum mechanical phenomena on a macroscopic scale. Here we demonstrate the formation of a lattice of vortex-antivortex pairs and study, for the first time, its properties in the non-linear regime at high polarion-density where polariton-polariton interactions dominate the behaviour of the system. In this work first we demonstrate that the array of vortex-antivortex pairs can be generated in a controllable way in terms of size…
Polariton Fluids as Quantum Field Theory Simulators on Tailored Curved Spacetimes
Laboratoire Kastler Brossel, Sorbonne Université, CNRS, ENS-Université PSL, Collège de France（卡斯勒-布罗塞尔实验室，索邦大学，法国国家科学研究中心，巴黎高等师范学院-巴黎文理研究大学，法兰西公学院）；Department of Physics and Astronomy, Louisiana State University（路易斯安那州立大学物理与天文系）
We consider two concentric rings formed by bosonic condensates of exciton-polaritons. A circular superfluid flow of polaritons in one of the rings can be manipulated by acting upon the second annular polariton condensate. The complex coupling between the rings with different topological charges triggers nucleation of stable Josephson vortices (JVs) which are revealed as topological defects of the angular dependence of the relative phase between rings. Being dependent on the coupling strength, the structure of the JV governs the difference of the mean angular momenta of the inner and the outer …
In this paper we discuss, within the Gross--Pitaevskii framework, superfluidity, soliton nucleation, and instabilities in a non-equilibrium polariton fluid injected by a spatially localized and continuous-wave coherent pump and flowing against a defect located outside the pump spot. In contrast to equilibrium condensates, the steady-state solutions of the driven-dissipative equations in this specific geometry hardly show a clean superfluid flow around the defect and rather feature a crossover from shallow to deep soliton-like perturbation. This is explained in terms of the properties of one-di…
In a recent preprint (arXiv:1401.1128v1) Cilibrizzi and co-workers report experiments and simulations showing the scattering of polaritons against a localised obstacle in a semiconductor microcavity. The authors observe in the linear excitation regime the formation of density and phase patterns reminiscent of those expected in the non-linear regime from the nucleation of dark solitons. Based on this observation, they conclude that previous theoretical and experimental reports on dark solitons in a polariton system should be revised. Here we comment why the results from Cilibrizzi et al. take p…
Quantum vortices, the quantized version of classical vortices, play a prominent role in superfluid and superconductor phase transitions. However, their exploration at a particle level in open quantum systems has gained considerable attention only recently. Here we study vortex pair interactions in a resonant polariton fluid created in a solid-state microcavity. By tracking the vortices on picosecond time scales, we reveal the role of nonlinearity, as well as of density and phase gradients, in driving their rotational dynamics. Such effects are also responsible for the split of composite spin-v…
We study Bogoliubov excitations of a spinor Bose Einstein condensate in a honeycomb periodic potential, in the presence of a Zeeman field and of a spin-orbit coupling specific for photonic systems, which is due to the energy splitting between TE and TM polarized eigenstates. We also consider spin-anisotropic interactions typical for cavity polaritons. We show that the non-trivial topology of the single particle case is also present for the interacting system. At low condensate density, the topology of the single-particle bands is transferred to the bogolon dispersion. At a critical value, the …
Quantum simulations are one of the pillars of quantum technologies. These simulations provide insight in fields as varied as high energy physics, many-body physics, or cosmology to name only a few. Several platforms, ranging from ultracold-atoms to superconducting circuits through trapped ions have been proposed as quantum simulators. This article reviews recent developments in another well established platform for quantum simulations: polaritons in semiconductor microcavities. These quasiparticles obey a nonlinear Schrödigner equation (NLSE), and their propagation in the medium can be underst…
Rotation of a container holding a viscous fluid forms a vortex which grows with increasing angular velocity. A superfluid, however, is intrinsically different from these normal fluids because its rotation is quantized. Even if a container of superfluid is rotating, the fluid itself remains still until a critical velocity is reached. Beyond the critical velocity, all the particles conspire to suddenly pick up an angular momentum of $\hbar$ each and forms a quantized vortex. As a result, a superfluid is known to increase its rotation by a total angular momentum of $N\hbar$. In this letter, we sh…
Quantum fluids of light are realized in semiconductor microcavities by exciton-polaritons, solid-state quasi-particles with a light mass and sizeable interactions. Here, we use the microscopic analogue of oceanographic techniques to measure the excitation spectrum of a thermalised polariton condensate. Increasing the fluid density, we demonstrate the transition from a free-particle parabolic dispersion to a linear, sound-like Goldstone mode characteristic of superfluids at equilibrium. Notably, we show that excitations are created with a definite direction with respect to the condensate, analo…
The quest of utilizing neutral particles to simulate the behaviour of charged particles in a magnetic field makes the generation of artificial magnetic field of great interest. The previous and the only proposal for the production of synthetic magnetic field for the dark state polaritons in electromagnetically induced transparency invokes the mechanical rotation of a sample. Here, we put forward an optical scheme to generate effective gauge potentials for stationary-light polaritons. 5To demonstrate the capabilities of our approach, we present recipes for having dark state polaritons in degene…
Phase frustration in periodic lattices is responsible for the formation of dispersionless flat bands. The absence of any kinetic energy scale makes flat band physics critically sensitive to perturbations and interactions. We report here on the experimental investigation of the nonlinear dynamics of cavity polaritons in the gapped flat band of a one-dimensional Lieb lattice. We observe the formation of gap solitons with quantized size and very abrupt edges, signature of the frozen propagation of switching fronts. This type of gap solitons belongs to the class of truncated Bloch waves, and had o…
In this work we experimentally demonstrate for the first time spontaneous generation of two-dimensional exciton-polariton X-waves. X-waves belong to the family of localized packets, which are capable of sustaining their shape with no spreading even in the linear regime. This allows to keep the packet shape and size for very low densities and very long times compared, for instance, to soliton waves, which always necessitate a nonlinearity to compensate the diffusion. Here we exploit the polariton nonlinearity and unique structured dispersion, comprising both positive- and negative-mass curvatur…
We study the Bose polaron problem in a nonequilibrium setting, by considering an impurity embedded in a quantum fluid of light realized by exciton-polaritons in a microcavity, subject to a coherent drive and dissipation on account of pump and cavity losses. We obtain the polaron effective mass, the drag force acting on the impurity, and determine polaron trajectories at a semiclassical level. We find different dynamical regimes, originating from the unique features of the excitation spectrum of driven-dissipative polariton fluids, in particular a non-trivial regime of acceleration against the …
By imaging single-shot realizations of an organic polariton quantum fluid, we observe the long-sought dynamical instability of non-equilibrium condensates. Without any free parameters, we find an excellent agreement between the experimental data and a numerical simulation of the open-dissipative Gross-Pitaevskii equation, which allows us to draw several important conclusions about the physics of the system. We find that the reservoir dynamics are in the strongly nonadiabatic regime, which renders the complex Ginzburg-Landau description invalid. The observed transition from stable to unstable f…
In inflationary cosmology, the rapid expansion of the early universe resulted in the spontaneous production of cosmological particles from vacuum fluctuations, observable today in the cosmic microwave background anisotropies. The analogue of cosmological particle creation in a quantum fluid could provide insight, but an observation has not yet been achieved. Here we report the spontaneous creation of analogue cosmological particles in the laboratory, using a quenched 3-dimensional quantum fluid of light. We observe acoustic peaks in the density power spectrum, in close quantitative agreement w…
The phenomenon of stable persistent currents is central to the studies of superfluidity in a range of physical systems. While all of the previous theoretical studies of superfluid flows in annular geometries concentrated on conservative systems, here we extend the stability analysis of persistent currents to open-dissipative exciton-polariton superfluids. By considering an exciton-polariton condensate in an optically-induced annular trap, we determine stability conditions for an initially imposed flow with a non-zero orbital angular momentum. We show, theoretically and numerically, that the sy…
We present a simple method to compensate for losses in a polariton superfluid. Based on a weak support field, it allows for an extended propagation of a resonantly driven polariton superfluid at a minimal energetic cost. Moreover, this setup based on optical bistability, leads to a significant release of the phase constraint imposed by the resonant driving. This release, together with the macroscopic polariton propagation, offers a unique opportunity to study the hydrodynamics of topological excitations of polariton superfluids such as quantized vortices and dark solitons. We numerically study…
Acoustic Black Holes in a Shock-Wave Exciton-Polariton Condensate
Moscow Center for Advanced Studies（莫斯科高等研究中心）；Zhejiang Normal University（浙江师范大学）；Zhejiang Institute of Photoelectronics（浙江光电子研究所）；St. Petersburg State University（圣彼得堡国立大学）
The dynamics of sound in a fluid is intrinsically nonlinear. We derive the consequences of this fact for the analogue gravitational field experienced by sound waves, by first describing generally how the nonlinearity of the equation for phase fluctuations back-reacts onto the definition of the background providing the effective space-time metric. Subsequently, we use the the analytical tool of Riemann invariants in one-dimensional motion to derive source terms of the effective gravitational field stemming from nonlinearity. Finally, we show that the consequences of nonlinearity we derive can b…
Half-integer topological defects in polariton condensates can be regarded as magnetic charges, with respect to built-in effective magnetic fields present in microcavities. We show how an integer topological defect can be separated into a pair of half-integer ones, paving the way towards flows of magnetic charges: spin currents or magnetricity. We discuss the corresponding experimental implementation within microwires (with half-solitons) and planar microcavities (with half-vortices).
A quantum fluid passing an obstacle behaves differently from a classical one. When the flow is slow enough, the quantum gas enters a superfluid regime and neither whirlpools nor waves form around the obstacle. For higher flow velocities, it has been predicted that the perturbation induced by the defect gives rise to the turbulent emission of quantised vortices and to the nucleation of solitons. Using an interacting Bose gas of exciton-polaritons in a semiconductor microcavity, we report the transition from superfluidity to the hydrodynamic formation of oblique dark solitons and vortex streets …
