A new regime in the interaction of a two-colour ($ω$,$2ω$) laser with a nanometre-scale foil is identified, resulting in the emission of extremely intense, isolated attosecond pulses - even in the case of multi-cycle lasers. For foils irradiated by lasers exceeding the blow-out field strength (i.e. capable of fully separating electrons from the ion background), the addition of a second harmonic field results in the stabilization of the foil up to the blow-out intensity. This is then followed by a sharp transition to transparency that essentially occurs in a single optical cycle. During the transition cycle, a dense, nanometre-scale electron bunch is accelerated to relativistic velocities and emits a single, strong attosecond pulse with a peak intensity approaching that of the laser field.
Doppler harmonic generation of a high-power laser on a relativistic plasma mirror is a promising path to produce bright attosecond light bursts. Yet, a major challenge has been to find a way to generate isolated attosecond pulses, better suited to timed-resolved experiments, rather than trains of pulses. A promising technique is the attosecond lighthouse effect, which consists in imprinting different propagation directions to successive attosecond pulses of the train, and then spatially filtering one pulse in the far field. However, in the relativistic regime, plasma mirrors get curved by the …
Relativistic surface high harmonics have been considered a unique source for the generation of intense isolated attosecond pulses in the extreme ultra-violet (XUV) and X-ray spectral range. However, its experimental realization is still a challenging task requiring identification of the optimum conditions for the generation of isolated attosecond pulses as well as their temporal characterization. Here, we demonstrate measurements in both directions. Particularly, we have made a first step towards the temporal characterization of the emitted XUV radiation by adapting the attosecond streak camer…
The creation of attosecond pulses via laser-plasma interaction has been a subject of great scientific interest for more than three decades. This process is investigated by using particle-in-cell simulation with varying the plasma and laser parameters. The steepness of the density gradient at the plasma-vacuum interface is examined to see how this parameter affects the high-order harmonic generations and isolated-attosecond pulse creation. The optimal density gradient lengths $L$ are explored within the relativistic oscillating mirror mechanism. Although the ideal gradient lengths for the full …
Sub-10-attosecond pulses with half-cycle electric fields provide exceptional options to detect and manipulate electrons in the atomic timescale. However, the availability of such pulses is still challenging. Here, we propose a method to generate isolated sub-10-attosecond half-cycle pulses based on a cascade process naturally happening in plasma. A 100s-attosecond pulse is first generated by shooting a moderate overdense plasma with a one-cycle femtosecond pulse. After that, the generated attosecond pulse cascadedly produce a sub-10-attosecond half-cycle pulse in the transmission direction by …
Half-cycle picosecond pulses have been produced from thin photo-conductors, when applying an electric field across the surface and switching on conduction by a short laser pulse. Then the transverse current in the wafer plane emits half-cycle pulses in normal direction, and pulses of 500 fs duration and 1e6 V/m peak electric field have been observed. Here we show that single half-cycle pulses of 50 as duration and up to 1e13 V/m can be produced when irradiating a double foil target by intense few-cycle laser pulses. Focused onto an ultra-thin foil, all electrons are blown out, forming a unifor…
The explosion in attosecond technology has opened the gate to investigating many unexplored areas which require ultrahigh spatial and temporal resolution. In the area of nuclear physics, using gamma-rays with ultrahigh resolution in time and space will help to investigate intra-nuclear dynamics in an unprecedentedly explicit way. However, the generation of ultrahigh brilliance attosecond gamma-ray pulses with current-generation laser facilities has not been reported. In this letter, we propose a novel method to generate high charge (~1nC) attosecond (<200 attosecond) electron bunch by the near…
A method to generate an intense isolated few-cycle attosecond XUV pulse is demonstrated using particle-in-cell simulations. When a tailored laser pulse with a sharp edge irradiates a foil target, a strong transverse net current can be excited, which emits a few-cycle XUV pulse from the target rear side. The isolated pulse is ultrashort in the time domain with a duration of several hundred attoseconds. It also has a narrow bandwidth in the spectral domain compared to other XUV sources of high-order harmonics. It has most energy confined around the plasma frequency and no low-harmonic orders bel…
A proposal for a novel source of isolated attosecond XUV -- soft X-ray pulses with a well controlled carrier-envelope phase difference (CEP) is presented in the framework of nonlinear Thomson-backscattering. Based on the analytic solution of the Newton-Lorentz equations, the motion of a relativistic electron is calculated explicitly, for head-on collision with an intense fs laser pulse. By using the received formulae, the collective spectrum and the corresponding temporal shape of the radiation emitted by a mono-energetic electron bunch can be easily computed. For certain suitable and realisti…
function of the CEP, we observe a transition from a modulated to a continuous SHHG spectrum, indicating the transition from double to high-contrast isolated attosecond pulse emission. Single shot-acquisitions of XUV spectral continua support isolated attosecond pulses with isolation degrees between 10 and 50 for the majority of the driving pulse CEPs, which represents a significant improvement in terms of isolation degree as well as repetition rate over previous results obtained with 2-cycle drivers at 10-Hz. 2D Particle-in-cell simulations corroborate this interpretation and predict percent-l…
We develop an analytical model for ultraintense attosecond pulse emission in the highly relativistic laser-plasma interaction. In this model, the attosecond pulse is emitted by a strongly compressed electron layer around the instant when the layer transverse current changes the sign and its longitudinal velocity approaches the maximum. The emitted attosecond pulse has a broadband exponential spectrum and a stabilized constant spectral phase $ψ(ω)=\pmπ/2-ψ_{A_m}$. The waveform of the attosecond pulse is also given explicitly, to our knowledge, for the first time. We validate the analytical mode…
Generation of Isolated Collimated Polarized $γ$-ray Beams via Spatiotemporal Optical Vortex Modulation
State Key Laboratory of Ultra-Intense Laser Science and Technology, Shanghai Institute of Optics and Fine Mechanics (SIOM), Chinese Academy of Sciences (CAS)（中国科学院上海光学精密机械研究所）；Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences（中国科学院大学材料科学与光电技术学院）；Laboratory of Zhongyuan Light, School of Physics, Zhengzhou University（郑州大学物理学院中原之光实验室）；State Key Laboratory of Dark Matter Physics, Key Laboratory for Laser Plasmas (MoE), School of Physics and Astronomy, Shanghai Jiao Tong University（上海交通大学物理与天文学院激光等离子体教育部重点实验室暗物质物理国家重点实验室）
Laser-plasma electron accelerators can be used to produce high-intensity X-rays, as electrons accelerated in wakefields emit radiation due to betatron oscillations.Such X-ray sources inherit the features of the electron beam; sub-femtosecond electron bunches produce betatron sources of the same duration, which in turn allow probing matter on ultrashort time scales. In this paper we show, via Particle-in-Cell simulations, that attosecond electron bunches can be obtained using low-energy, ultra-short laser beams both in the self-injection and the controlled injection regimes at low plasma densit…
High harmonic generation by relativistically intense laser pulses from overdense plasma layers is surveyed. High harmonics are generated in form of (sub-)attosecond pulses when the plasma surface rebounds towards the observer with relativistic velocity. Different cases are considered. The "relativistically oscillating mirror" (ROM) model, describing the most typical case, is analyzed in detail. The resulting harmonic spectrum is usually a power law with the exponent -8/3 [baeva2006relativistic], but possible exceptions due to "higher order γ-spikes" are considered. It is shown that under certa…
The birth of attosecond light sources is expected to inspire a breakthrough in ultrafast optics, which may extend human real-time measurement and control techniques into atomic-scale electronic dynamics. For applications, it is essential to obtain a single attosecond pulse of high intensity, large photon energy and short duration. Here we show that single 100-terawatt attosecond X-ray light pulse with intensity ${1\times10^{21}}\textrm{W}/\textrm{cm}^{ 2}$ and duration ${7.9} \textrm{as}$ can be produced by intense laser irradiation on a capacitor-nanofoil target composed of two separate nanof…
We present a scheme for amplifying an extreme-ultraviolet (XUV) seed isolated attosecond pulse via stimulated Raman scattering of a pulse-train pump. At sufficient seed and pump intensity, the amplification is nonlinear, and the amplitude of the seed pulse can reach that of the pump, one order of magnitude higher than the initial seed amplitude. In the linear amplification regime, we find that the spectral signature of the pump pulse train is imprinted on the spectrum of the amplified seed pulse. Since the spectral signature is imprinted with its frequency downshifted by the plasma frequency, …
Sources of intense, ultra-short electromagnetic pulses enable applications such as attosecond pulse generation, control of electron motion in solids and the observation of reaction dynamics at the electronic level. For such applications both high-intensity and carrier envelope phase~(CEP) tunability are beneficial, yet hard to obtain with current methods. In this work we present a new scheme for generation of isolated CEP-tunable intense sub-cycle pulses with central frequencies that range from the midinfrared to the ultraviolet. It utilizes an intense laser pulse which drives a wake in a plas…
Ultrafast extreme ultraviolet (XUV) sources with a controllable polarization state are powerful tools for investigating the structural and electronic as well as the magnetic properties of materials. However, such light sources are still limited to only a few free-electron laser facilities and, very recently, to high-order harmonic generation from noble gases. Here we propose and numerically demonstrate a laser-plasma scheme to generate bright XUV pulses with fully controlled polarization. In this scheme, an elliptically-polarized laser pulse is obliquely incident on a plasma surface, and the r…
