Extinction strain rate (ESR) and laminar flame speed (LFS) are fundamental properties of a fuel/air mixture that are often utilized as scaling parameters in turbulent combustion. While LFS at atmospheric and elevated pressures are extensively investigated, experimental measurements of ESR with counterflow premixed flames are very limited for flame instability often occurs near extinction, especially at high pressures. Due to the scarcity of ESR measurements, most combustion kinetic models are mainly validated and optimized against LFS. However, it is questionable whether the controlling reactions are the same for ESR and LFS such that those models are also valid for predicting ESR. This work quantifies the kinetic similarities between ESR and LFS by analyzing their kinetic sensitivity directions. The direction is represented by a unit vector composed of the normalized sensitivity of ESR or LFS to the rate constant for each elemental reaction. Consequently, the similarity between the two directions is measured by the inner product of the corresponding unit vectors. The sensitivity directions of ESR and LFS are found parallel for various fuels, equivalence ratios, and pressures. Furthermore, sensitivity directions at various strain rates are also similar for the maximum temperature, local temperature at various locations in the flame coordinate, and ESR in counterflow premixed flames. These findings suggest that LFS and ESR are similarly effective as the target for constraining and optimizing rate constants in kinetic models. In addition, the independence of the sensitivity directions on the strain rate also enables us to perform uncertainty quantification for turbulent flames with a wide range of strain rates based on the kinetic sensitivity of ESR and LFS.
This paper presents a flame-height correlation for laminar to transition-to-turbulent regime diffusion flames. Flame-height measurements are obtained by means of numerical and experimental studies in which three high definition cameras were employed to take frontal, lateral and 45° angled images simultaneously. The images were analysed using an image-processing algorithm to determine the flame-height through indirect measurement. To locate an overall chemical-flame-length, numerical simulations were conducted with the unsteady Reynolds-Averaged Navier-Stokes technique. The eddy-dissipation mod…
Laminar premixed flame profiles of methane/air free flames and strained flames at different fuel/air ratios and strain rates are analysed using detailed chemistry with Lewis numbers equal to one. It is shown that the detailed chemistry flame profiles of progress variables CO2+CO and H2O+H2 in canonically stretched coordinates can be fitted accurately by a slight generalization of recently proposed analytical presumed flame profiles over a wide range of fuel/air ratios through adaptation of a single model parameter. Strained flame profiles can be reproduced using an additional linear coordinate…
This study aims to build a theoretical model to describe the ignition process of spherical spray flame laden with fuel droplets under overall fuel-lean condition. Two characteristic fronts are introduced to reveal where the evaporation starts and ends in the ignition process. The results demonstrate that the flame has been strengthened with extra fuel droplet adding while the minimum ignition energy (MIE) is decreased. The evolution of the two evaporation fronts in the flame kernel and propagating branches has also be revealed coupled with the evaporation zone length.
Hydrogen-enrichment of conventional natural gas mixtures is an actively-explored strategy for reducing pollutant emissions from combustion. This study investigates the effect of hydrogen enrichment on the unsteady flame response to perturbations, with a view to understanding the implications for thermoacoustic stability. The Level Set Approach for kinematically tracking the flame front was applied to a laminar conical premixed methane / hydrogen / air flame subjected to 2D incompressible velocity perturbations. For hydrogen enrichment levels ranging from 0% to 80% by volume, the resulting unst…
Reported in the paper are results of unsteady three-dimensional direct numerical simulations of laminar and turbulent, lean hydrogen-air, complex-chemistry flames propagating in forced turbulence in a box. To explore the eventual influence of thermo-diffusive instability of laminar flames on turbulent burning velocity, (i) a critical length scale Λn that bounds regimes of unstable and stable laminar combustion is numerically determined by gradually decreasing the width Λ of computational domain until a stable laminar flame is obtained and (ii) simulations of turbulent flames are performed by v…
A combined experimental and numerical investigation of partially premixed laminar methane-air flames undergoing side-wall quenching (SWQ) is performed. A well-established SWQ burner is adapted to allow the seeding of the main flow with additional gaseous products issued from a (secondary) wall inlet close to the flame's quenching point. First, the characteristics of the partially premixed flame that quenches at the wall are assessed using planar laser-induced fluorescence measurements of the OH radical, and a corresponding numerical simulation with fully-resolved transport and chemistry is con…
The non-monotonic profile of temperature is to be considered in the context of combustion inside tubes or thermonuclear flames, which may accelerates to become detonation waves. This transition is known as deflagration-to-detonation transition. Focusing on this point, we extend the study of adiabatic flames, which assumes zero temperature gradient at the burned-side edge of a flame front, to the case of non-zero temperature gradient by introducing compression zone behind the front. Such a treatment has been performed in the previous work based on the ignition temperature approximation. In that…
The effects of initial pressure and temperature on the laminar burning speed of n-hexane-air mixtures were investigated experimentally and numerically. The spherically expanding flame technique with a nonlinear extrapolation procedure was employed to measure the laminar burning speed at atmospheric and sub-atmospheric pressures and at nominal temperatures ranging from 296 to 422 K. The results indicated that the laminar burning speed increases as pressure decreases and as temperature increases. The predictions of three reaction models taken from the literature were compared with the experiment…
We study the effect of thermal noise on the propagation speed of a planar flame. We show that this out of equilibrium greatly amplifies the effect of thermal noise to yield macroscopic reductions in the flame speed over what is predicted by the noise-free model. Computations show that noise slows the flame significantly. The flame is modeled using Navier Stokes equations with appropriate diffusive transport terms and chemical kinetic mechanism of hydrogen/oxygen. Thermal noise is modeled within the continuum framework using a system of stochastic partial differential equations, with transport …
This paper presents an experimental methodology to measure the height of the flame using convolution image processing and statistical analysis. The experimental setup employs a burner with four circularly arranged nozzles. Six different volumetric fuel flows were employed, and flame images were captured from three different visualization planes utilizing a three high-definition camera array, a thermal imaging camera and an image-processing algorithm. The flame height was indirectly measured using pixel quantification and conversion through a reference length. Although the fuel flow was the mos…
The mixing process of multiple jets of liquefied petroleum gas and air in a diffusion flame is numerically analysed. The case study considers a four-port array burner where the fuel is injected by four peripheral nozzles and mixed with the surrounding air. Simulations are conducted with the Reynolds-Averaged Navier-Stokes technique, and the turbulence effect is modelled with the realizable k-e model. In addition, the eddy dissipation model is implemented to calculate the effect of the turbulent chemical reaction rate. Results show that the essential mixture mechanism occurs within a flame cone…
Three-dimensional laminar flow structures with mixing, chemical reaction, normal strain, and shear strain qualitatively representative of turbulent combustion at the small scales are analyzed. A mixing layer is subjected to counterflow in the transverse y- and z-directions. Both non-reactive and reactive flows are examined. Reduction of the three-dimensional boundary-layer equations to a one-dimensional similar form is obtained allowing for heat and mass diffusion with variations in density and properties. In steady configurations, a set of ODEs governs the three velocity components as well as…
We study the dynamics and properties of a turbulent flame, formed in the presence of subsonic, high-speed, homogeneous, isotropic Kolmogorov-type turbulence in an unconfined system. Direct numerical simulations are performed with Athena-RFX, a massively parallel, fully compressible, high-order, dimensionally unsplit, reactive-flow code. A simplified reaction-diffusion model represents a stoichiometric H2-air mixture. The system being modeled represents turbulent combustion with the Damkohler number Da = 0.05 and with the turbulent velocity at the energy injection scale 30 times larger than the…
Influences of reaction zone thickening and local extinctions on the burning rate of extremely turbulent hydrogen-enriched methane-air flames are investigated using simultaneous planar laser-induced fluorescence of formaldehyde molecule and hydroxyl radical as well as separate stereoscopic particle image velocimetry techniques. Karlovitz numbers upto 76 are examined. It is shown that, by increasing the turbulence intensity, the preheat and reaction zone thicknesses can increase to values that are, respectively, 6.3 and 4.9 of the corresponding laminar flames. Broadening of these zones for inten…
(Abridged) Direct numerical simulations of the interaction of a premixed flame with driven, subsonic, homogeneous, isotropic, Kolmogorov-type turbulence in an unconfined system are used to study the mechanisms determining the turbulent flame speed, S_T, in the thin reaction zone regime. High intensity turbulence is considered with the r.m.s. velocity 35 times the laminar flame speed, S_L, resulting in the Damkohler number Da = 0.05. Here we show that: (1) The flame brush has a complex internal structure, in which the isosurfaces of higher fuel mass fractions are folded on progressively smaller…
Comprehensive knowledge of local flame displacement speed, $S_d$, in turbulent premixed flames is crucial towards the design and development of hydrogen fuelled next-generation engines. Premixed hydrogen-air flames are characterized by significantly higher laminar flame speed compared to other conventional fuels. Furthermore, in the presence of turbulence, $S_d$ is enhanced much beyond its corresponding unstretched, planar laminar value $S_L$. In this study, the effect of high Karlovitz number ($Ka$) turbulence on density-weighted flame displacement speed, $\widetilde{S_d}$, in a H$_2$-air fla…
HiPrFlame-An ab initio based real-fluid modeling approach for high-pressure combustion-I. Rationale, methodology, and application to laminar premixed flames
G-equations are level-set type Hamilton-Jacobi partial differential equations modeling propagation of flame front along a flow velocity and a laminar velocity. In consideration of flame stretching, strain rate may be added into the laminar speed. We perform finite difference computation of G-equations with the discretized strain term being monotone with respect to one-sided spatial derivatives. Let the flow velocity be the time-periodic cellular flow (modeling Rayleigh-Bénard advection), we compute the turbulent flame speeds as the asymptotic propagation speeds from a planar initial flame fron…
Uncovering flame physics with machine learning: application to the reaction rate in hydrogen flames
University of Edinburgh（爱丁堡大学）；RWTH Aachen University（亚琛工业大学）；Vrije Universiteit Brussel（布鲁塞尔自由大学）；Brussels Institute for Thermal-Fluid Systems and Clean Energy (BRITE), VUB-ULB（布鲁塞尔热流体系统与清洁能源研究所（BRITE），布鲁塞尔自由大学-布鲁塞尔大学）；University of Cambridge（剑桥大学）；University of Southampton（南安普顿大学）
The present work reports on the numerical investigation of NOx in three turbulent piloted diffusion flames of different levels of extinction. The study involves two-dimensional axisymmetric modeling of combustion in these flames with fairly detailed chemistry, i.e. GRI 3.0 mechanism. The main focus of the study is to analyze the effects of the two different combustion model approaches, such as infinitely fast chemistry based unsteady flamelet and finite rate chemistry based EDC, in predicting the NOx formation in three piloted methane jet flames (Sandia D, E, and F). The EDC approach is able t…
We, herein, present a new model based on the framework of synchronization to describe a thermoacoustic system and capture the multiple bifurcations that such a system undergoes. Instead of applying flame describing function to depict the unsteady heat release rate as the flame's response to acoustic perturbation, the new model considers the acoustic field and the unsteady heat release rate as a pair of nonlinearly coupled damped oscillators. By varying the coupling strength, multiple dynamical behaviors, including limit cycle oscillation, quasi-periodic oscillation, strange nonchaos, and chaos…
An a priori analysis of a DNS database of turbulent lean premixed methane flames is presented considering the relative effects of turbulence and LES filtering, along with a potential modelling approach for LES with finite-rate chemistry. The leading-order effect was found to be due to the filter operation; flame response to turbulence was a secondary effect, and manifested primarily as an increase in standard deviations about conditional means. It was found that the radicals O, H and OH were less impacted by the filter than other high-temperature radicals, which were significantly reduced in m…
Large hydrocarbon fuels are used for ground and air transportation and will be for the foreseeable future. Despite their extensive use, turbulent combustion of large hydrocarbon fuels, remains relatively poorly understood and difficult to predict. A key parameter when burning these fuels is the turbulent consumption speed; the velocity at which fuel and air are consumed through a turbulent flame front. Such information can be useful as a model input parameter and for validation of modeled results. In this study, turbulent consumption speeds were measured for three jet-like fuels using a premix…
This study investigates the effects of curvature on the local heat release rate and mixture fraction during turbulent flame-wall interaction of a lean dimethyl ether/air flame using a fully resolved simulation with a reduced skeletal chemical reaction mechanism and mixture-averaged transport. The region in which turbulent flame-wall interaction affects the flame is found to be restricted to a wall distance less than twice the laminar flame thickness. In regions without heat losses, heat release rate and curvature, as well as mixture fraction and curvature, are negatively correlated, which is i…
Given the need to develop zero-carbon combustors for power and aircraft engine applications, $S_d$ of a turbulent premixed flame, especially for H$_2$-air, is of immediate interest. The present study investigates 3D DNS cases of premixed H$_2$-air turbulent flames at varied pressures for different $Re_t$ and $Ka$ with detailed chemistry to theoretically model $S_d$ at negative curvatures. Prior studies at atmospheric pressure showed $\widetilde{S_d}$ to be enhanced significantly over $S_L$ at large negative $κ$ due to flame-flame interactions. 1D simulations of an imploding cylindrical H$_2$-a…
Despite the high technical relevance of early flame kernel development for the reduction of cycle-to-cycle variations in spark ignition engines, there is still a need for a better fundamental understanding of the governing in-cylinder phenomena in order to enable resilient early flame growth. To isolate the effects of small- and large-scale turbulent flow motion on the young flame kernel, a three-dimensional DNS database has been designed to be representative for engine part load conditions. The analysis is focussed on flame displacement speed and flame area in order to investigate effects of …
Shock flame interactions are fundamental problems in many combustion applications ranging from flame acceleration to flame control in supersonic propulsion applications. The present paper seeks to quantify the rate of deformation of the flame surface and burning velocity caused by the interaction and to clarify the underlying mechanisms. The interaction of a single shock wave with a cellular flame in a Hele-Shaw shock tube configuration was studied experimentally, numerically, and theoretically. A mixture of stoichiometric hydrogen-air at sub-atmospheric pressure was chosen such that large cel…
A series of Direct Numerical Simulations (DNS) of lean methane/air flames was conducted in order to investigate the enhancement of the turbulent flame speed and modifications to the reaction layer structure associated with the systematic increase of the integral scale of turbulence $l$ while the Karlovitz number and the Kolmogorov scale are kept constant. Four turbulent slot jet flames are simulated at increasing Reynolds number and up to $Re \approx 22000$, defined based on the bulk velocity, slot width, and the reactants' properties. The turbulent flame speed $S_T$ is evaluated locally at se…
This paper experimentally analyzes the simultaneous influence of heat release and coherent vortex structures on the transfer of kinetic energy across scales around the laminar flame thickness $δ^0_\mathrm{L}$ in a turbulent premixed swirl flame and a non-reacting swirl flow. High-resolution tomographic particle image velocimetry and formaldehyde planar laser induced fluorescence measurements are used to obtain 3D velocity fields and estimates of the progress variable and density fields. The kinetic energy transfer across a filter scale of $Δ= 1.5 δ^0_\mathrm{L}$ was then quantified using physi…
In the present work we compare reliability of several most widely used reduced detailed chemical kinetic schemes for hydrogen-air and hydrogen-oxygen combustible mixtures. The validation of the schemes includes detailed analysis of 0D and 1D calculations and comparison with experimental databases containing data on induction time, equilibrium temperature, composition of the combustion products, laminar flame speed and the flame front thickness at different pressures. 1D calculations are carried out using the full gasdynamical system for compressible viscous thermal conductive multicomponent mi…
Nonlinear responses of the premixed V-flame subjected to dual-frequency disturbances
Beihang University（北京航空航天大学）；Beijing Institute of Control Engineering（北京控制工程研究所）；Imperial College London（伦敦帝国学院）；Research Institute of Aero-Engine, Beihang University（北京航空航天大学航空发动机研究院）；Hangzhou International Innovation Institute, Beihang University（北京航空航天大学杭州国际创新院）
