arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 2001.00368cond-mat.mtrl-sciphysics.app-ph
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基于热辐射效应的纳米片导热系数测量

Thermal Conductivity Measurements in Nanosheets via Bolometric Effect

Onur Çakıroğlu, Naveed Mehmood, Mert Miraç Çiçek, Aizimaiti Aikebaier, Hamid Reza Rasouli, Engin Durgun, T. Serkan Kasırga

摘要:

纳米尺度材料的热导率测量技术需要制造非常复杂的设备,或者其适用性仅限于一类材料。发现具有高热敏性的新方法是广泛使用热导率测量表征材料性能所必需的。我们提出并证明了一种简单的非破坏性的方法,具有优越的热灵敏度,测量面内的热导率的纳米片和纳米线使用的热效应。该方法利用激光束加热在具有电接触的纳米材料的悬浮部分上产生温度梯度,该温度梯度小至开尔文的几分之一。由于激光照射引起的局部温度升高会改变器件的电阻,这可以精确测量。然后,使用热导率作为拟合参数,将该电阻变化用于提取沿纳米材料的温度分布。我们测量了V2 O3纳米片的热导率,以验证该方法的适用性,并发现与文献非常吻合。此外,我们首次测量了金属2 H-TaS 2的热导率,并进行了从头计算来支持我们的测量。最后,我们讨论了半导体纳米片的方法的适用性和WS 2和二硫化钼薄片进行测量。

英文摘要:

Thermal conductivity measurement techniques for materials with nanoscale dimensions require fabrication of very complicated devices or their applicability is limited to a class of materials. Discovery of new methods with high thermal sensitivity are required for the widespread use of thermal conductivity measurements in characterizing materials properties. We propose and demonstrate a simple non-destructive method with superior thermal sensitivity to measure the in-plane thermal conductivity of nanosheets and nanowires using the bolometric effect. The method utilizes laser beam heating to create a temperature gradient, as small as a fraction of a Kelvin, over the suspended section of the nanomaterial with electrical contacts. Local temperature rise due to the laser irradiation alters the electrical resistance of the device, which can be measured precisely. This resistance change is then used to extract the temperature profile along the nanomaterial using thermal conductivity as a fitting parameter. We measured the thermal conductivity of V2O3 nanosheets to validate the applicability of the method and found an excellent agreement with the literature. Further, we measured the thermal conductivity of metallic 2H-TaS2 for the first time and performed ab initio calculations to support our measurements. Finally, we discussed the applicability of the method on semiconducting nanosheets and performed measurements on WS2 and MoS2 thin flakes.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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