Cubic chiral magnets, such as Cu$_{2}$OSeO$_{3}$, exhibit a variety of non-collinear spin textures, including a trigonal lattice of spin whirls, so-called skyrmions. Using magnetic resonant elastic x-ray scattering (REXS) on a crystalline Bragg peak and its magnetic satellites while exciting the sample with magnetic fields at GHz frequencies, we probe the ferromagnetic resonance modes of these spin textures by means of the scattered intensity. Most notably, the three eigenmodes of the skyrmion lattice are detected with large sensitivity. As this novel technique, which we label REXS-FMR, is carried out at distinct positions in reciprocal space, it allows to distinguish contributions originating from different magnetic states, providing information on the precise character, weight and mode mixing as a prerequisite of tailored excitations for applications.
We report chirality-induced current-in-plane magnetoresistance (CIP-MR) in chiral molecule/ferromagnetic metal bilayer at room temperature. The previously reported chiralityinduced current-perpendicular-to-plane magnetoresistance (CPP-MR) originates from the chiral induced spin-selectivity (CISS) effect that needs charge-current passing through the molecule. In contrast, the observed CIP-MR in the present study requires no bias charge current through the molecule. The temperature dependence of CIP-MR suggests thermally induced spin-polarization in the chiral molecules is the key for the observ…
The sustainable society requires the recycling of rare metals. Rare earth Nd is one of rare metals, accompanying huge consumption especially in Nd-Fe-B magnets. Although the wet process using acid is in practical use in the in-plant recycle of sludge, higher selectivity between Nd and Fe at room temperature is desired. We have proposed a pretreatment of corrosion before the dissolution into HCl and the oxalic acid precipitation. The corrosion produces $γ$-FeOOH and a Nd hydroxide, which have high selectivity for HCl solution at room temperature. Nd can be recovered as Mn$_{2}$O$_{3}$-type Nd$_…
We demonstrate selective excitation of a spin wave mode in a ferromagnetic (Ga,Mn)As film by picosecond strain pulses. For a certain range of magnetic fields applied in the layer plane only a single frequency is detected for the magnetization precession. We explain this selectivity of spin mode excitation by the necessity of spatial matching of magnon and phonon eigenfunctions, which represents a selection rule analogous to momentum conservation for magnon-phonon interaction in bulk ferromagnetic materials.
The magnetization characteristic in a permalloy thin strip is investigated by electrically measuring the anisotropic magnetoresistance and ferromagnetic resonance in in-plane and out-of-plane configurations. Our results indicate that the magnetization vector can rotate in the film plane as well as out of the film plane by changing the intensity of external magnetic field of certain direction. The magnetization characteristic can be explained by considering demagnetization and magnetic anisotropy. Our method can be used to obtain the demagnetization factor, saturated magnetic moment and the mag…
We investigate the magnetization dynamics through the magnetoimpedance effect in ferromagnetic NiFe/Cu/Co films. We observe that the magnetoimpedance response is dependent on the thickness of the non-magnetic Cu spacer material, a fact associated to the kind of the magnetic interaction between the ferromagnetic layers. Thus, we present an experimental study on asymmetric magnetoimpedance in ferromagnetic films with biphase magnetic behavior and explore the possibility of tuning the linear region of the magnetoimpedance curves around zero magnetic field by varying the thickness of the non-magne…
Magnetic proximity effect between topological insulator (TI) and ferromagnetic insulator (FMI) is considered to have great potential in spintronics. However, a complete determination of interfacial magnetic structure has been highly challenging. We theoretically investigate the interlayer exchange coupling of two FMIs separated by a TI thin film, and show that the particular electronic states of the TI contributing to the proximity effect can be directly identified through the coupling behavior between two FMIs, together with a tunability of coupling constant. Such FMI/TI/FMI structure not onl…
Ferromagnetic vortices deliver robust out-of-plane magnetization at extremely small scales. Their handling and creation therefore has high potential to become a necessary ingredient for future data storage technologies in order to keep up with the pace of growing information density demands. In this study we show that by using one step nanolithography method, we are able to create ferromagnetic vortex lattices in thin nickel films. The necessary control of the magnetic stray field at the domain edges was achieved by actively modifying the ferromagnetic thin film anisotropic properties at nanom…
Understanding the multiferroic coupling is one of the key issues in the feld of multiferroics. As shown here theoretically, the ferromagnetic resonance (FMR) renders possible an access to the magnetoelectric coupling coefficient in composite multiferroics. This we evidence by a detailed analysis and numerical calculations of FMR in an unstrained chain of BaTiO3 in the tetragonal phase in contact with Fe, including the effect of depolarizing field. The spectra of the absorbed power in FMR are found to be sensitive to the orientation of the interface electric polarization and to an applied stati…
Graphene has been predicted to develop a magnetic moment by proximity effect when placed on a ferromagnetic film, a promise that could open exciting possibilities in the fields of spintronics and magnetic data recording. In this work, we study in detail the interplay between the magnetoresistance of graphene and the magnetization of an underlying ferromagnetic insulating film. A clear correlation between both magnitudes is observed but we find, through a careful modelling of the magnetization and the weak localization measurements, that such correspondence can be explained by the effects of th…
Interplay between Exchange Interaction and Magnetic Shape Anisotropy of ferromagnetic nanoparticles in a non-magnetic matrix for rare-earth-free permanent magnets
The asymmetry of the modal profiles for dipole-exchange spin waves propagating in in-plane magnetized ferromagnetic films at a right angle to the applied magnetic field has been investigated theoretically. It was found that in the large-magnetic moment ferromagnetic metallic films with typical thicknesses 10-60 nm the fundamental mode of the spectrum is localized at the surface opposite to the surface of localization of the exchange-free Damon-Eshbach surface wave. This anomalous localization of the wave does not affect the non-reciprocity of spin wave excitation by microstrip and coplanar tra…
Magnetic fingerprint in a ferromagnetic wire: Spin torque diode effect and induction of the DC voltage spectrum inherent in the wire under application for RF current
Chiral Spinterfaces as an Overlooked Component of the Chiral-Induced Spin Selectivity Effect
Chemnitz University of Technology（开姆尼茨工业大学）；Research Center for Materials, Architectures and Integration of Nanomembranes (MAIN)（纳米膜材料、架构与集成研究中心）；Eindhoven University of Technology（埃因霍温理工大学）
Chiral molecule-induced contributions to ferromagnetic resonance
Helmholtz-Zentrum Dresden–Rossendorf（德累斯顿-罗森多夫亥姆霍兹中心）；Universidad Técnica Federico Santa María（费德里科·圣玛丽亚技术大学）；Universität Duisburg–Essen（杜伊斯堡-埃森大学）；Chemnitz University of Technology（开姆尼茨工业大学）；Adam Mickiewicz University（亚当·密茨凯维奇大学）
Ability to tailor the nature of the magnetic coupling between two ferromagnetic electrodes can enable the realization of new spintronics device systems. This paper discusses our finding that deposition of an ultrathin tantalum (Ta) on the NiFe top electrode reversed the nature of inter-ferromagnetic electrode coupling. We observed that the deposition of ~ 5 nm Ta on the top of a magnetic tunnel junction with Ta( 2 nm)/Co(5 nm)/NiFe (5 nm)/AlOx( 2 nm)/NiFe (10-15 nm) configuration changed the magnetic coupling between two ferromagnetic electrodes from antiferromagnetic to ferromagnetic. We inve…
Spin wave scattering in the right angle ferromagnetic cross was measured. Shape anisotropy defined magnetization ground states at zero biasing magnetic fields. Scattering of the spin waves in the center of ferromagnetic cross is strongly dependent on the amplitude and angle of the biasing magnetic field. Micromagnetic simulations indicate that low in-plane biasing magnetic fields rotate the magnetization of the cross center while the arms stay axially magnetized due to the shape anisotropy. We discuss effect of biasing magnetic fields on the spin wave scattering and approaches to an effective …
A coplanar waveguide shorted in one end is proposed, designed, and implemented successfully to measure the properties of magnetic thin films as a part of the vector network analyzer ferromagnetic resonance (VNA-FMR) spectroscopy set-up. Its simple structure, potential applications and easy installation inside the cryostat chamber made it advantageous especially for low-temperature measurements. It provides a wide band of frequencies in the gigahertz range essential for FMR measurements. Our spectroscopy set-up with short-circuited coplanar waveguide has been used to extract Gilbert damping coe…
We study the enhancement of the magnetic transition temperature $T_c$ due to incident light in ferromagnetic semiconductors such as EuS. The photoexcited carriers mediate an extra ferromagnetic interaction due to the coupling with the localized magnetic moments. The Hamiltonian consists of a Heisenberg model for the localized moments and an interaction term between the photoexcited carriers and the localized moments. The model predicts a small enhancement of the transition temperature in semi-quantitative agreement with the experiments.
The present article concludes that a ferromagnetic sample could be considered like a paramagnetic system where the role of magnetic moments plays magnetic domains. Based on this conclusion and taking into account presence of an anisotropic field the formula which describes magnetization dependence on the external magnetic field is derived. Expressions for a remanent magnetization and a coercive force are presented. The new parameter to characterize a magnetic stiffness of a material is introduced. A physical expression for a dynamic magnetic susceptibility as a function of material's character…
In the present work a detailed thermodynamic consideration for the magnetic free energy of the composite material consisting of the ferromagnetic powder particles embedded into a polymer matrix is given. We estimate their magnetostatic interaction energy and its dependence on the microscopic distribution of the magnetization and the magnetic field in the composite material. We also define the hydrostatic component of the mechanical force developed and the volume change effect caused by the magnetostatic interactions in such composites.
Both magnetic-resonance damping and the giant magnetoresistance effect have been predicted to be strongly affected by the local density of states in thin ferromagnetic films. We employ the antiferromagnetic coupling between Co and Gd to provide a spontaneous change from parallel to antiparallel alignment of two Co films. A sharp increase in magnetic damping accompanies the change from parallel to antiparallel alignment, analogous to resistivity changes in giant magnetoresistance.
Magnetic Tunnel Junction devices find use in several applications based on the exploitation of the Spin-Transfer Torque phenomenon. The Ferromagnetic Resonance curve is a key characteristic of any Magnetic Tunnel Junctions. It is usually characterized both experimentally and numerically by performing a lot of measurements of the magnetic response to a sinusoidal field or current. Here we propose the use of a chirp signal as excitation signal to reconstruct the Ferromagnetic resonance curve with a single measurement/simulation. A micromagnetic comparison of the proposed method with the traditio…
We carefully investigated the ferromagnetic coupling in the as-grown and annealed ferromagnetic semiconductor GaMnAs/AlGaMnAs bilayer devices. We observed that the magnetic interaction between the two layers strongly affects the magnetoresistance of the GaMnAs layer with applying out of plane magnetic field. After low temperature annealing, the magnetic easy axis of the AlGaMnAs layer switches from out of plane into in-plane and the interlayer coupling efficiency is reduced from up to 0.6 to less than 0.4. However, the magnetic coupling penetration depth for the annealed device is twice that o…
We investigate the dynamic magnetic response of ferromagnetic flexible NiFe/Ta and FeCuNbSiB/Ta multilayers under external stress. We explore the possibility of handling magnetic anisotropy and dynamic magnetic response of flexible magnetostrictive nanostructures. We quantify the sensitivity of the multilayers under external stress by calculating the ratio $|Δ\textrm{MI}|/|Δ\barσ|$ and show that considerable values can be reached by tuning the magnetic field, frequency, magnetostriction constant, and external stress. The results reveal possibilities of application of flexible magnetostrictive …
The authors have investigated magnetic domain wall induced capacitance variation as a tool for the detection of magnetic reversal in magnetic nanowires for in-plane (NiFe) and out-of-plane (Co/Pd) magnetization configurations. The switching fields in the capacitance measurements match with that of the magnetoresistance measurements in the opposite sense. The origin of the magnetocapacitance has been attributed to magnetoresistance. This magnetocapacitance detection technique can be useful for magnetic domain wall studies.
Chiral-Induced Spin Selectivity Effect in a 1 nm Thin 1,1'-Binaphthyl-2,2'-diyl Hydrogenphosphate Self-Assembled Monolayer on Nickel Oxide
Technical University of Darmstadt（达姆施塔特工业大学）；Technical University of Munich（慕尼黑工业大学）；Weizmann Institute of Science（魏茨曼科学研究所）；Chemnitz University of Technology（开姆尼茨工业大学）；Heidelberg University（海德堡大学）；Merck Electronics KGaA（默克电子股份公司）；University of Freiburg（弗赖堡大学）
This paper reports the development of a methodology combining microstrip ferromagnetic resonance (MS-FMR) and digital image correlation (DIC) in order to silmuteanously measure the voltage-induced strains and the magnetic resonance in artificial magnetoelectric heterostructures (magnetic films/piezoelectric substrate? or magnetic films/flexible substrate/piezoelectric actuator ?). The overall principle of the technique and the related analytical modelling are described. It is powerful to estimate the magnetostriction coefficient of ferromagnetic thin films and can be used to determine the effe…
Strong ferromagnetic interlayer exchange couplings $J$ in perpendicularly magnetized systems are becoming increasingly desirable for applications. We study whether ferromagnetic interlayer exchange couplings can be measured by a combination of broadband ferromagnetic resonance methods and magnetometry hysteresis loops. For this we model the switching and the eigenexcitations in bilayer systems comprising a soft layer coupled to a thicker harder layer that possesses higher perpendicular magnetic anisotropy. For large $J >0$ the switching fields are essentially independent of $J$ but the frequen…
Imaging the magnetic configuration of thin-films has been a long-standing area of research. Since a few years, the emergence of two-dimensional ferromagnetic materials calls for innovation in the field of magnetic imaging. As the magnetic moments are extremely small, standard techniques like SQUID, torque magnetometry, magnetic force microscopy and Kerr effect microscopy are challenging and often lead to the detection of parasitic magnetic contributions or spurious effects. In this work, we report a new magnetic microscopy technique based on the combination of magnetic circular dichroism and S…
The influence of a transverse static magnetic field on the magnetic hyperthermia properties is studied on a system of large-losses ferromagnetic FeCo nanoparticles. The simultaneous measurement of the high-frequency hysteresis loops and of the temperature rise provides an interesting insight into the losses and heating mechanisms. A static magnetic field of only 40 mT is enough to cancel the heating properties of the nanoparticles, a result reproduced using numerical simulations of hysteresis loops. These results cast doubt on the possibility to perform someday magnetic hyperthermia inside a m…
Spinel oxides are an ideal setting to explore the interplay between configurational entropy, site selectivity, and magnetism in high entropy oxides. In this work we characterize the magnetic properties of the spinel (Cr,Mn,Fe,Co,Ni)$_3$O$_4$ and study the evolution of its magnetism as a function of non-magnetic gallium substitution. Across the range of compositions studied here, from 0% to 40% Ga, magnetic susceptibility and powder neutron diffraction measurements show that ferrimagnetic order is robust in the spinel HEO. However, we also find that the ferrimagnetic order is highly tunable, wi…
We report the results of micromagnetic simulations of domain wall (DW) nucleation and pinning/depinning processes in ferromagnetic planar structure consisting of nanowire (NW) with perpendicular anisotropy and special V-shaped nanoparticle (NP) with in-plane anisotropy located on top of NW. The magnetization reversal features of this system in an external magnetic field are investigated depending on the direction of particle magnetic moment. Possible variants of magnetic logic cells (LCs) based on such system are discussed.
Planar macroscopic magnetic tunnel junctions exhibit well defined zero bias anomalies when a thin layer of ferromagnetic CoFe(B) nanodots is inserted within a MgO based tunnel barrier. The conductance curves exhibit a single and a double peak, respectively, for anti-parallel and parallel alignment of the magnetizations of the electrodes which sandwich the tunnel barrier. This leads to a suppression of the tunneling magnetoresistance near zero bias. We show that the double peak structure indicates that the zero-bias anomaly is spin-split due to a magnetic exchange interaction between the magnet…
