We show that a metastable $η$--pairing superconducting phase can be induced by photodoping doublons and holes into a strongly repulsive fermionic Hubbard model. The doublon-hole condensate originates from an intrinsic doublon-hole exchange interaction and does not rely on the symmetry of the half-filled Hubbard model. It extends over a wide range of doublon densities and effective temperatures. Different non-equilibrium protocols to realize this state are proposed and numerically tested. We also study the optical conductivity in the superconducting phase, which exhibits ideal metallic behavior, i.e., a delta function at zero-frequency in the conductivity, in conjunction with a negative conductivity at large frequencies. These characteristic optical properties can provide a fingerprint of the $η$-pairing phase in pump-probe experiments.
Ultrafast laser pulses can redistribute charges in Mott insulators on extremely short time scales, leading to the fast generation of photocarriers. It has recently been demonstrated that these photocarriers can form a novel $η$--paired condensate at low temperatures, featuring a staggered superconducting pairing field. In this conference paper, we discuss the origin of the $η$--paired hidden phase and its optical response which may be detected in a pump-probe experiment. The hidden phase may be relevant for possible light-induced superconductivity in Mott insulators.
Photodoped states are widely observed in laser-excited Mott insulators, in which charge excitations are quickly created and can exist beyond the duration of the external driving. Despite the fruitful experimental explorations, theoretical studies on the microscopic models face the challenge to simultaneously deal with exponentially separated time scales, especially in multi-band systems, where the long-time behaviors are often well beyond the reach of state-of-the-art numerical tools. Here, we address this difficulty by introducing a steady-state description of photodoped Mott insulators using…
Photoemission Signatures of Photoinduced Carriers and Excitons in One-Dimensional Mott Insulators
The University of Tokyo（东京大学）；Institute for Materials Research, Tohoku University（东北大学物质材料研究机构）；RIKEN Center for Emergent Matter Science (CEMS)（理化学研究所新兴物质科学中心）；Trans-Scale Quantum Science Institute, University of Tokyo（东京大学跨尺度量子科学研究所）
Dynamical correlations and nonequilibrium sum rules in photodoped Hubbard ladders
School of Physical Sciences, The Open University（开放大学物理科学学院）；PASQAL SAS（帕斯卡尔公司）；Condensed matter physics and Material Science Division, Brookhaven National Laboratory（布鲁克海文国家实验室凝聚态物理与材料科学部）
One of the most successful theories of a non-Fermi liquid metallic state is the composite Fermi liquid (CFL) theory of the half-filled Landau level. In this paper, we study continuous quantum phase transitions out of the CFL state and into a Landau Fermi liquid, in the limit of no disorder and fixed particle number. This transition can be induced by tuning the bandwidth of the Landau level relative to the interaction energy, for instance through an externally applied periodic potential. We find a transition to the Landau Fermi liquid through a gapless Mott insulator with a Fermi surface of neu…
We propose a novel quantum spin liquid state that can explain many of the intriguing experimental properties of the low-temperature phase of the organic spin liquid candidate materials. This state of paired fermionic spinons preserves all symmetries of the system, and it has a gapless excitation spectrum with quadratic bands that touch at momentum ~ k = 0. This quadratic band touching is protected by the symmetry of the system. Using variational Monte Carlo techniques, we show that this state has highly competitive energy in the triangular lattice Heisenberg model supplemented with a realistic…
We study the energetics of Gutzwiller projected BCS states of various symmetries for the triangular lattice antiferromagnet with a four particle ring exchange using variational Monte Carlo methods. In a range of parameters the energetically favored state is found to be a projected $d_{x^2-y^2}$ paired state which breaks lattice rotational symmetry. We show that the properties of this nematic or orientationally ordered paired spin liquid state as a function of temperature and pressure can account for many of the experiments on organic materials. We also study the ring-exchange model with ferrom…
We study the effects of doping a Mott insulator on the honeycomb lattice where spins interact via direction dependent Kitaev couplings J_K, and weak antiferromagnetic Heisenberg couplings J. This model is known to have a spin liquid ground state and may potentially be realized in correlated insulators with strong spin orbit coupling. The effect of hole doping is studied within a t-J-J_K model, treated using the SU(2) slave boson formulation, which correctly captures the parent spin liquid. We find superconductor ground states with spin triplet pairing that spontaneously break time reversal sym…
In this paper we explore possible phases arising from doping neutral excitons into a Mott insulator in the context of moiré bilayers. We consider two moiré layers coupled together only through inter-layer repulsion and there is a U(2)$\times$ U(2) symmetry. The densities of the two layers can be tuned to be $n_t=x,n_b=1-x$ with $n_t+n_b=1$. $x=0$ limit is a layer polarized Mott insulator and small $x$ regime can be reached by doping inter-layer excitons at density $x$. Charge gap can remain finite at small $x$, as is demonstrated experimentally in the WSe$_2$-hBN-WSe$_2$/WS$_2$ system. To capt…
Paired valence electrons forming covalent bonds in molecues are confined cooper pair correlations. High pressure dissociates molecules in solid H2S, SiH4, H2 etc. and form extended structures. However, valence electrons are resilient and continue to bond and sometimes resonate. It is suggested that some structures contain emergent Mott insulators (EMI) and support superconductivity and other phases, under special conditions. In pressurized solid H2S, we propose presence of a sublattice of relatively narrow, nearly half filled band of H atoms, trapped in ordered interstitials of colvalently bon…
We study the two-band Hubbard model in infinite dimensions by solving the dynamical mean-field equations with a strong coupling continuous-time quantum Monte Carlo method and show that an $s$-wave superconducting state can be stabilized in the repulsively interacting case. We discuss how this superconducting state competes with the metallic and paired Mott states. The effects of the Hund coupling and crystalline electric field are also addressed.
We study the phase diagram of two weakly coupled one-dimensional dipolar boson chains at half-odd-integer fillings. We find that the system contains a rich phase diagram. Four different phases are found. They are the Mott insulators, the single-particle resonant superfluid, the paired superfluid, and the bond- or inter-chain density waves. Moreover, the Mott insulating phase can be further classified according to a hidden string order parameter, which is analogous to the one investigated recently in the one-dimensional boson Mott insulator at integer fillings.
To analyze the ground-state phase diagram of Bose-Bose mixtures loaded into $d$-dimensional hypercubic optical lattices, we perform a strong-coupling power-series expansion in the kinetic energy term (plus a scaling analysis) for the two-species Bose-Hubbard model with onsite boson-boson interactions. We consider both repulsive and attractive interspecies interaction, and obtain an analytical expression for the phase boundary between the incompressible Mott insulator and the compressible superfluid phase up to third order in the hoppings. In particular, we find a re-entrant quantum phase trans…
We study two-component (or pseudospin-1/2) bosons with pair hopping interactions in synthetic dimension, for which a feasible experimental scheme on a square optical lattice is also presented. Previous studies have shown that two-component bosons with on-site interspecies interaction can only generate nontrivial interspecies paired superfluid (super-counter-fluidity or pair-superfluid) state. In contrast, apart from interspecies paired superfluid, we reveal two new phases by considering this additional pair hopping interaction. These novel phases are intraspecies paired superfluid (molecular s…
We study the conditions under which, using a canonical transformation, the phases sought after for the repulsive Hubbard model, namely a Mott insulator in the paramagnetic and anti-ferromagnetic phases, and a putative d-wave superfluid can be deduced from observations in an optical lattice loaded with a spin-imbalanced ultra-cold Fermi gas with attractive interactions, thus realizing the attractive Hubbard model. We show that the Mott insulator and antiferromagnetic phase of the repulsive Hubbard model are in fact more easy to observe as a paired, and superfluid phase respectively, in the attr…
There is a growing interest in the $U(1)$ Coulomb liquid in both quantum materials in pyrochlore ice and cluster Mott insulators and cold atom systems. We explore a paired hardcore boson model on a pyrochlore lattice. This model is equivalent to the XYZ spin model that was proposed for rare-earth pyrochlores with "dipole-octupole" doublets. Since this model has no sign problem for quantum Monte Carlo (QMC) simulations in a large parameter regime, we carry out both analytical and QMC calculations. We find that the $U(1)$ Coulomb liquid is quite stable and spans a rather large portion of the pha…
Based on first-principles calculations, we explored the interplay between stacking effect and electron-electron correlation in the layered vdW material of bulk 1T-NbS2 with a 2D charge density wave (CDW) order. Without considering the Coulomb correlation, two energetically favorable out-of-plane stacking configurations are identified: one is a metallic phase with a single-layer stacking pattern, another is a band insulator with a paired-bilayer stacking configuration. Even though the Coulomb correlation is taken into account, the two energetic favorable stacking orders are still far more stabl…
How the ground state nature can be dramatically changed by the distinct underlying spin correlation is a central issue of doped Mott insulators. The two-leg XXZ ladder provides a prototypical spin background, which can be tuned from a long-range Néel order to a short-range ``spin liquid'' via the superexchange anisotropy, giving rise to a complex phase diagram at finite doping. By density matrix renormalization group method, we show that although the charge is always self-localized in the Néel ordered phase, a second insulating phase emerges, in which the doped holes become paired but remain l…
We consider two species of hard-core bosons with density dependent hopping in a one-dimensional optical lattice, for which we propose experimental realizations using time-periodic driving. The quantum phase diagram for half-integer filling is determined by combining different advanced numerical simulations with analytic calculations. We find that a reduction of the density-dependent hopping induces a Mott-insulator to superfluid transition. For negative hopping a previously unknown state is found, where one species induces a gauge phase of the other species, which leads to a superfluid phase o…
The ground state phase diagram of the 1D Hubbard chain with pair-hopping interaction is studied. The analysis of the model is performed using the continuum-limit field theory approach and exact diagonalization studies. At half-filling the phase diagram is shown to consist of two superconducting states with Cooper pair center-of-mass momentum Q=0 (BCS-η_0 phase) and Q=π(η_π-phase) and four insulating phases corresponding to the Mott antiferromagnet, the Peierls dimerized phase, the charge-density-wave (CDW) insulator as well as an unconventional insulating phase characterized by the coexistence…
