We show that the recently proposed cooling-by-doping mechanism allows to efficiently prepare interesting nonequilibrium states of the Hubbard model. Using nonequilibrium dynamical mean field theory and a particle-hole symmetric setup with dipolar excitations to full and empty bands we produce cold photo-doped Mott insulating states with a sharp Drude peak in the optical conductivity, a superconducting state in the repulsive Hubbard model with an inverted population, and $η$-paired states in systems with a large density of doublons and holons. The reshuffling of entropy into full and empty bands not only provides an efficient cooling mechanism, it also allows to overcome thermalization bottlenecks and slow dynamics that have been observed in systems cooled by the coupling to boson baths.
A theory is presented for a nonequilibrium phase transition in the two-dimensional Hubbard model coupled to electrodes. Nonequilibrium magnetic and superconducting phase diagram is determined by the Keldysh method, where the electron correlation is treated in the fluctuation exchange approximation. The nonequilibrium distribution function in the presence of electron correlation is evoked to capture a general feature in the phase diagram.
Resonant inelastic X-ray scattering (RIXS) detects various types of high- and low-energy elementary excitations in correlated solids, and this tool will play an increasingly important role in investigations of time-dependent phenomena in photo-excited systems. While theoretical frameworks for the computation of equilibrium RIXS spectra are well established, the development of appropriate methods for nonequilibrium simulations are an active research field. Here, we apply a recently developed nonequilibrium dynamical mean field theory (DMFT) based approach to compute the RIXS response of photo-e…
We study the single-band Hubbard model in the presence of a large spatially uniform electric field out of equilibrium. Using the Keldysh nonequilibrium formalism, we solve the problem using perturbation theory in the Coulomb interaction U. We present numerical results for the charge current, the total energy of the system and the double occupancy on an infinite-dimensional hypercubic lattice with nearest-neighbor hopping. The system is isolated from an external bath and is in the paramagnetic state. We show that an electric field pulse can drive the system to a steady nonequilibrium state, whi…
Nonlinear transport in the one dimensional Hubbard model at half-filling under a finite bias voltage is investigated by the adaptive time-dependent density matrix renormalization group method. For repulsive on-site interaction, dielectric breakdown of the Mott insulating ground state to a current-carrying nonequilibrium steady state is clearly observed when the voltage exceeds the charge gap. It is found that by increasing the voltage further the current-voltage characteristics are scaled only by the charge gap and the scaling curve exhibits almost linear dependence on the voltage whose slope …
We present a straightforward implementation scheme for solving the time dependent Schrödinger equation for systems described by the Hubbard Hamiltonian with time dependent hoppings. The computations can be performed for clusters of up to 14 sites with in principle general geometry. For the time evolution, we use the exponential midpoint rule, where the exponentials are computed via a Krylov subspace method, which only uses matrix-vector multiplication. The presented implementation uses standard libraries for constructing sparse matrices and for linear algebra therefore the approach is easy to …
A model for nonequilibrium dynamical mean-field theory is constructed for the infinite dimensional Hubbard lattice. We impose nonequilibrium by expressing the physical orbital as a superposition of a left-($L$) moving and right-($R$) moving electronic state with the respective chemical potential $μ_L$ and $μ_R$. Using the second-order iterative perturbation theory we calculate the quasi-particle properties as a function of the chemical potential bias between the $L$ and $R$ movers, i.e. $Φ= μ_L - μ_R$. The evolution of the nonequilibrium quasi-particle spectrum is mapped out as a function of t…
The nonequilibrium variational-cluster approach is applied to study the real-time dynamics of the double occupancy in the one-dimensional Fermi-Hubbard model after different fast changes of hopping parameters. A simple reference system, consisting of isolated Hubbard dimers, is used to discuss different aspects of the numerical implementation of the approach in the general framework of nonequilibrium self-energy functional theory. Opposed to a direct solution of the Euler equation, its time derivative is found to serve as numerically tractable and stable conditional equation to fix the time-de…
Dynamical correlations and nonequilibrium sum rules in photodoped Hubbard ladders
School of Physical Sciences, The Open University（开放大学物理科学学院）；PASQAL SAS（帕斯卡尔公司）；Condensed matter physics and Material Science Division, Brookhaven National Laboratory（布鲁克海文国家实验室凝聚态物理与材料科学部）
We discuss the general formalism and validity of weak-coupling perturbation theory as an impurity solver for nonequilibrium dynamical mean-field theory. The method is implemented and tested in the Hubbard model, using expansions up to fourth order for the paramagnetic phase at half filling and third order for the antiferromagnetic and paramagnetic phase away from half filling. We explore various types of weak-coupling expansions and examine the accuracy and applicability of the methods for equilibrium and nonequilibrium problems. We find that in most cases an expansion of local self-energy dia…
We study dynamical phase transitions from antiferromagnetic to paramagnetic states driven by an interaction quench in the fermionic Hubbard model using the nonequilibrium dynamical mean-field theory. We identify two dynamical transition points where the relaxation behavior qualitatively changes: one corresponds to the thermal phase transition at which the order parameter decays critically slowly in a power law $\propto t^{-1/2}$, and the other is connected to the existence of nonthermal antiferromagnetic order in systems with effective temperature above the thermal critical temperature. The fr…
The nonequilibrium dynamics of strongly-correlated fermions in lattice systems have attracted considerable interest in the condensed matter and ultracold atomic-gas communities. While experiments have made remarkable progress in recent years, there remains a need for the further development of theoretical tools that can account for both the nonequilibrium conditions and strong correlations. For instance, time-dependent theoretical quantum approaches based on the density matrix renormalization group (DMRG) methods have been primarily applied to one-dimensional setups. Recently, two-dimensional …
We theoretically investigate the effects of the lattice geometry on the nonequilibrium dynamics of photo-excited carriers in a half-filled two-dimensional Hubbard model. Using a nonequilibrium generalization of the dynamical cluster approximation, we compare the relaxation dynamics in lattices which interpolate between the triangular lattice and square lattice configuration and thus reveal the role of the geometric frustration in these strongly correlated nonequilibrium systems. In particular, we show that the cooling effect resulting from the disordering of the spin background is less effecti…
We perform an ab-initio comparison between nonequilibrium dynamical mean-field theory and optical lattice experiments by studying the time evolution of double occupations in the periodically driven Fermi-Hubbard model. For off-resonant driving, the range of validity of a description in terms of an effective static Hamiltonian is determined and its breakdown due to energy absorption close to resonance is demonstrated. For near-resonant driving, we investigate the response to a change in driving amplitude and discover an asymmetric excitation spectrum with respect to the detuning. In general, we…
We review recent developments in the theory of interacting quantum many-particle systems that are not in equilibrium. We focus mainly on the nonequilibrium generalizations of the flow equation approach and of dynamical mean-field theory (DMFT). In the nonequilibrium flow equation approach one first diagonalizes the Hamiltonian iteratively, performs the time evolution in this diagonal basis, and then transforms back to the original basis, thereby avoiding a direct perturbation expansion with errors that grow linearly in time. In nonequilibrium DMFT, on the other hand, the Hubbard model can be m…
Motivated by recent experiments in ultracold atomic gases that explore the nonequilibrium dynamics of interacting quantum many-body systems, we investigate the opposite limit of Landau's Fermi liquid paradigm: We study a Hubbard model with a sudden interaction quench, that is the interaction is switched on at time t=0. Using the flow equation method, we are able to study the real time dynamics for weak interaction U in a systematic expansion and find three clearly separated time regimes: i) An initial buildup of correlations where the quasiparticles are formed. ii) An intermediate quasi-steady…
We discuss current carrying non-equilibrium steady state of an open fermionic Hubbard chain that is strongly driven by markovian incoherent processes localized at the chain ends. An explicit form of exact many-body density operator for any value of the coupling parameter is presented. The structure of a matrix product form of the solution is encoded in terms of a novel diagrammatic technique which should allow for generalization to other integrable non-equillibrium models.
We derive a general procedure for evaluating the ${\rm n}$th derivative of a time-dependent operator in the Heisenberg representation and employ this approach to calculate the zeroth to third spectral moment sum rules of the retarded electronic Green's function and self-energy for a system described by the Holstein-Hubbard model allowing for arbitrary spatial and time variation of all parameters (including spatially homogeneous electric fields and parameter quenches). For a translationally invariant (but time-dependent) Hamiltonian, we also provide sum rules in momentum space. The sum rules ca…
The nonequilibrium dynamics of correlated charge transfer along a one-dimensional chain in presence of a phonon environment is investigated within a dissipative Hubbard model. For this generalization of the ubiquitous spin-boson model the crucial role of symmetries is analysed in detail and corresponding invariant subspaces are identified. It is shown that the time evolution typically occurs in each of the disjunct subspaces independently leading e.g. asymptotically to a non-Boltzmann equilibrium state. Based on these findings explicit results are obtained for two interacting electrons by mean…
We present a framework of semiclassical superconductivity (SC) dynamics that properly includes effects of spatial fluctuations for the attractive Hubbard model. We consider both coherent and adiabatic limits. To model the coherent SC dynamics, we develop a real-space von~Neumann equation based on the time-dependent Hartree-Fock-Bogoliubov theory. Applying our method to interaction quenches in the negative-$U$ Hubbard model, we show that the relaxation of SC order at weak coupling is dominated by Landau-damping. At strong coupling, we find a two-stage relaxation of the pairing field: a collapse…
We solve the impurity problem which arises within nonequilibrium dynamical mean-field theory for the Hubbard model by means of a self-consistent perturbation expansion around the atomic limit. While the lowest order, known as the non-crossing approximation (NCA), is reliable only when the interaction U is much larger than the bandwidth, low-order corrections to the NCA turn out to be sufficient to reproduce numerically exact Monte Carlo results in a wide parameter range that covers the insulating phase and the metal-insulator crossover regime at not too low temperatures. As an application of t…
Using the Lindblad equation approach, we derive the range of the parameters of an interacting one-dimensional electronic chain connected to two reservoirs in the large bias limit in which an optimal working point (corresponding to a change in the monotonicity of the stationary current as a function of the applied bias) emerges in the nonequilibrium stationary state. In the specific case of the one-dimensional spinless fermionic Hubbard chain, we prove that an optimal working point emerges in the dependence of the stationary current on the coupling between the chain and the reservoirs, both in …
We derive expressions for the zeroth and the first three spectral moment sum rules for the retarded Green's function and for the zeroth and the first spectral moment sum rules for the retarded self-energy of the inhomogeneous Bose-Hubbard model in nonequilibrium, when the local on-site repulsion and the chemical potential are time-dependent, and in the presence of an external time-dependent electromagnetic field. We also evaluate these moments for equilibrium, where all time dependence and external fields vanish. Unlike similar sum rules for the Fermi-Hubbard model, in the Bose-Hubbard model c…
Using nonequilibrium dynamical mean-field theory, we study the isolated Hubbard model in a static electric field in the limit of weak interactions. Linear response behavior is established at long times, but only if the interaction exceeds a critical value, below which the system exhibits an AC-type response with Bloch oscillations. The transition from AC to DC response is defined in terms of the universal long-time behavior of the system, which does not depend on the initial condition.
The recent experimental implementation of condensed matter models in optical lattices has motivated research on their nonequilibrium behavior. Predictions on the dynamics of superconductors following a sudden quench of the pairing interaction have been made based on the effective BCS Hamiltonian; however, their experimental verification requires the preparation of a suitable excited state of the Hubbard model along a twofold constraint: (i) a sufficiently nonadiabatic ramping scheme is essential to excite the nonequilibrium dynamics, and (ii) overheating beyond the critical temperature of supe…
We address the steady-state behavior of a system consisting of several correlated monoatomic layers sandwiched between two metallic leads under the influence of a bias voltage. In particular, we investigate the effect of the local Hubbard and of the long-range Coulomb interactions on the charge redistribution at the interface. We provide a detailed study of the importance of the various system parameters, like Hubbard $U$, lead-correlated region coupling strength, and the applied voltage on the charge distribution in the correlated region and in the adjacent parts of the leads. Our results are…
Relaxation of electrons in a Hubbard model coupled to a dissipative bosonic bath is studied to simulate the pump-probe photoemission measurement. From this insight, we propose an experimental method of eliciting unoccupied part of the single-particle spectra at the equilibrium of doped-Mott insulators. We reveal first that effective temperatures of distribution functions and electronic spectra are different during the relaxation, which makes the frequently employed thermalization picture inappropriate. Contrary to the conventional analysis, we show that the unoccupied spectra at equilibrium ca…
An elusive goal in the field of driven quantum matter is the induction of long-range order. Here, we demonstrate a mechanism based on light-induced evaporative cooling of holes in a correlated electron system. Since the entropy of a filled narrow band grows rapidly with hole doping, the isentropic transfer of holes from a doped Mott insulator to such a band results in a drop of temperature. Strongly correlated Fermi liquids and symmetry-broken states could thus be produced by dipolar excitations. Using nonequilibrium dynamical mean field theory, we show that suitably designed chirped pulses al…
Strongly interacting fermionic atoms are shown to develop $η$-pairing superfluid correlations in a nonequilibrium steady state in the presence of spontaneous emission of light from atoms. On the basis of the Hubbard model subject to spontaneous decay between internal spin states, we show that prohibition of radiative decay due to the Pauli exclusion principle and destructive interference between doublon-decay processes lead to nonequilibrium $η$ pairing. Because of the non-thermal nature of the steady state, pair correlations arise even from a completely uncorrelated infinite-temperature initi…
We investigate features in the single-particle spectral function beyond the Hubbard bands in the strongly correlated normal phase of the Bose-Hubbard model. There are two distinct classes of additional peaks generated by the bosonic statistics. The first type is thermally activated Hubbard "sidebands", with the same physical origin as the zero-temperature Hubbard bands, but generated by excitations from thermally activated local occupation number states. The second class are two-particle fluctuation resonances driven by the lattice dynamics. In the unity filling Mott insulator, this takes the …
By employing unbiased numerical methods, we show that pulse irradiation can induce unconventional superconductivity even in the Mott insulator of the Hubbard model. The superconductivity found here in the photoexcited state is due to the $η$-pairing mechanism, characterized by staggered pair-density-wave oscillations in the off-diagonal long-range correlation, and is absent in the ground-state phase diagram; i.e., it is induced neither by a change of the effective interaction of the Hubbard model nor by simple photocarrier doping. Because of the selection rule, we show that the nonlinear optic…
A numerical approach is presented that allows to compute nonequilibrium steady state properties of strongly correlated quantum many-body systems. The method is imbedded in the Keldysh Green's function formalism and is based upon the idea of the variational cluster approach as far as the treatment of strong correlations is concerned. It appears that the variational aspect is crucial as it allows for a suitable optimization of a "reference" system to the nonequilibrium target state. The approach is neither perturbative in the many-body interaction nor in the field, that drives the system out of …
We show theoretically that the sudden application of an appropriate ac field to correlated lattice fermions flips the band structure and effectively switches the interaction from repulsive to attractive. The nonadiabatically driven system is characterized by a negative temperature with a population inversion. We numerically demonstrate the converted interaction in an ac-driven Hubbard model with the nonequilibrium dynamical mean-field theory solved by the continuous-time quantum Monte Carlo method. Based on this, we propose an efficient ramp-up protocol for ac fields that can suppress heating,…
