Research on magnetic particles dispersed in a fluid medium, actuated by a rotating magnetic field, is becoming increasingly active for both lab-on-chip and bio-sensing applications. In this study, we experimentally investigate the behaviour of ferromagnetic filaments in a rotating field. Filaments are synthesized by linking micron-sized ferromagnetic particles with DNA strands. The experiments were conducted under different magnetic field strengths, frequencies and filament sizes, and deformation of the filaments was registered via microscope and camera. The results obtained showed that the body deformation is larger for longer filaments and higher frequencies and lower for larger magnetic field. The angle between the filament tangent at the centre and the magnetic field direction increases linearly with frequency at low-frequency regime. A further increase in the frequency will result in filament movement out of plane when the angle approaches 90 degrees. The experimental results were used to estimate magnetic moment and the bending elasticity of the filament.
Ferromagnetic filaments in a rotating magnetic field are studied both numerically and experimentally. The filaments are made from micron-sized ferromagnetic particles linked with DNA strands. It is found that at low frequencies of the rotating field a filament rotates synchronously with the field and beyond a critical frequency it undergoes a transition to a three dimensional regime. In this regime the tips of the filament rotate synchronously with the field on circular trajectories in the plane parallel to the plane of the rotating field. The characteristics of this motion found numerically m…
Extensive Langevin dynamics simulations are used to characterize the adsorption transition of a flexible magnetic filament grafted onto an attractive planar surface. Our results identify different structural transitions at different ratios of the thermal energy to the surface attraction strength: filament straightening, adsorption and the magnetic flux closure. The adsorption temperature of a magnetic filament is found to be higher in comparison to an equivalent nonmagnetic chain. The adsorption has been also investigated under the application of a static homogeneous external magnetic field. W…
We investigate the equilibrium morphologies of linear and ring-shaped magnetic filaments made from crosslinked ferromagnetic spherical or ellipsoidal colloidal particles. Using Langevin dynamics simulations, we calculate the radius of gyration and total magnetic moment of a single filament at zero field and different temperatures, analyzing the influence of the particles shape, the strength of their magnetic moment and the filament length. Our results show that, among such parameters, the shape of the particles has the strongest qualitative impact on the equilibrium behavior of the filaments.
External magnetic fields are known to attract and orient magnetically responsive colloidal particles. In the case of 2D microplatelets, rotating magnetic fields are typically used to orient them parallel to each other in a brick-and-mortar fashion. Thanks to this microstructure, the resulting composites achieve enhanced mechanical and functional properties. However, parts with complex geometry require their microstructure to be specifically tuned and controlled locally in 3D. Although the tunability of the microstructure along the vertical direction has already been demonstrated using magnetic…
We report the precessional rotation of magnetically isotropic ferromagnetic nanoparticles in a viscous liquid that are subjected to a rotating magnetic field. In contrast to magnetically anisotropic nanoparticles, the rotation of which occurs due to coupling between the magnetic and lattice subsystems through magnetocrystalline anisotropy, the rotation of isotropic nanoparticles is induced only by magnetic dissipation processes. We propose a theory of this phenomenon based on a set of equations describing the deterministic magnetic and rotational dynamics of such particles. Neglecting inertial…
A minimal system of equations is introduced and applied to study the drift motion of ferromagnetic particles suspended in a viscous fluid and subjected to a time-periodic driving force and a nonuniformly rotating magnetic field. It is demonstrated that the synchronized translational and rotational oscillations of these particles are accompanied by their drift in a preferred direction, which occurs under the action of the Magnus force. We calculate both analytically and numerically the drift velocity of particles characterized by single-domain cores and nonmagnetic shells and show that there ar…
Field-induced phase transitions in ferro-antiferromagnetic diblock copolymers
Dipartimento di Fisica e Astronomia and Sezione INFN, Università di Padova（帕多瓦大学物理与天文学系及INFN分部）；SUPA, School of Physics and Astronomy, University of Edinburgh（爱丁堡大学物理与天文学院）
