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arXiv 1904.04656cond-mat.mes-hall
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非中心对称金属费米面拓扑变化的热电和光学探测

Thermoelectric and optical probes for a Fermi surface topology change in noncentrosymmetric metals

Sonu Verma, Tutul Biswas, Tarun Kanti Ghosh

摘要:

非中心对称金属如Li $_2$(Pd $_{1-x}$ Pt $_x$)$_3$ B在带接触点的下方和上方具有不同的费米表面拓扑,在带接触点处自旋简并不被自旋-轨道耦合提升。我们研究热电和光学响应作为探针,这种费米表面拓扑结构的变化。我们发现,当费米能级下降穿过能带接触点时,化学势表现出从三维到一维的维度交叉特征。这种维度交叉是由于带接触点上下存在不同的费米面拓扑。通过自洽求解玻尔兹曼输运方程,得到了短程散射体弛豫时间的精确表达式。由于非中心对称块状金属的一维性质,当费米能级低于能带接触点时,热电功率和品质因数显著提高。当费米能级接近范霍夫奇点时,热电优值超过2。同样,零动量极限下的零频率和有限频率光学电导率的研究反映了费米面拓扑变化的本质。霍尔系数和光吸收宽度表现出不同的签名响应费米表面拓扑结构的变化。

英文摘要:

Noncentrosymmetric metals such as Li$_2$(Pd$_{1-x}$Pt$_x$)$_3$B have different Fermi surface topology below and above the band touching point where spin-degeneracy is not lifted by the spin-orbit coupling. We investigate thermoelectric and optical response as probes for this Fermi surface topology change. We show that the chemical potential displays a dimensional crossover from a three-dimensional to one-dimensional characteristics as the descending Fermi energy crosses the band touching point. This dimensional crossover is due to the existence of different Fermi surface topology above and below the band touching point. We obtain an exact expression of relaxation time due to short-range scatterer by solving Boltzmann transport equations self-consistently. The thermoelctric power and figure of merit are significantly enhanced as the Fermi energy goes below the band touching point owing to the underlying one-dimensional-like nature of noncentrosymmteric bulk metals. The value of thermoelectric figure of merit goes beyond two as the Fermi energy approaches to the van Hove singularity for lower spin-orbit coupling. Similarly, the studies of the zero-frequency and finite-frequency optical conductivities in the zero-momentum limit reflect the nature of topological change of the Fermi surface. The Hall coefficient and optical absorption width exhibit distinct signatures in response to the changes in Fermi surface topology.

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