We investigate the effects of stimulated scattering of optical lattice photons on atomic coherence times in a state-of-the art ${}^{87}\mathrm{Sr}$ optical lattice clock. Such scattering processes are found to limit the achievable coherence times to less than 12 s (corresponding to a quality factor of $1 \times 10^{16}$), significantly shorter than the predicted 145(40) s lifetime of ${}^{87}\mathrm{Sr}$'s excited clock state. We suggest that shallow, state-independent optical lattices with increased lattice constants can give rise to sufficiently small lattice photon scattering and motional dephasing rates as to enable coherence times on the order of the clock transition's natural lifetime. Not only should this scheme be compatible with the relatively high atomic density associated with Fermi-degenerate gases in three-dimensional optical lattices, but we anticipate that certain properties of various quantum states of matter can be used to suppress dephasing due to tunneling.
Laser cooling is a key ingredient for quantum control of atomic systems in a variety of settings. In divalent atoms, two-stage Doppler cooling is typically used to bring atoms to the uK regime. Here, we implement a pulsed radial cooling scheme using the ultranarrow 1S0-3P0 clock transition in ytterbium to realize sub-recoil temperatures, down to tens of nK. Together with sideband cooling along the one-dimensional lattice axis, we efficiently prepare atoms in shallow lattices at an energy of 6 lattice recoils. Under these conditions key limits on lattice clock accuracy and instability are reduc…
A Wannier-Stark optical lattice clock has demonstrated unprecedented measurement precision for optical atomic clocks. We present a systematic evaluation of the lattice light shift, a necessary next step for establishing this system as an accurate atomic clock. With precise control of the atomic motional states in the lattice, we report accurate measurements of the multipolar and the hyperpolar contributions and the operational lattice light shift with a fractional frequency uncertainty of 3.5$\times$10${}^{-19}$.
We study the trap depth requirement for the realization of an optical clock using atoms confined in a lattice. We show that site-to-site tunnelling leads to a residual sensitivity to the atom dynamics hence requiring large depths (50 to $100 E\_r$ for Sr) to avoid any frequency shift or line broadening of the atomic transition at the $10^{-17}-10^{-18}$ level. Such large depths and the corresponding laser power may, however, lead to difficulties (e.g. higher order light shifts, two-photon ionization, technical difficulties) and therefore one would like to operate the clock in much shallower tr…
Engineering a Hamiltonian system with tunable interactions provides opportunities to optimize performance for quantum sensing and explore emerging phenomena of many-body systems. An optical lattice clock based on partially delocalized Wannier-Stark states in a gravity-tilted shallow lattice supports superior quantum coherence and adjustable interactions via spin-orbit coupling, thus presenting a powerful spin model realization. The relative strength of the on-site and off-site interactions can be tuned to achieve a zero density shift at a `magic' lattice depth. This mechanism, together with a …
Quantum engineering of time-separated Raman laser pulses in three-level systems is presented to produce an ultra-narrow optical transition in bosonic alkali-earth clocks free from light shifts and with a significantly reduced sensitivity to laser parameter fluctuations. Based on a quantum artificial complex-wave-function analytical model, and supported by a full density matrix simulation including a possible residual effect of spontaneous emission from the intermediate state, atomic phase-shifts associated to Ramsey and Hyper-Ramsey two-photon spectroscopy in optical clocks are derived. Variou…
In 1949, Ramsey's method of separated oscillating fields was elaborated boosting over many decades metrological performances of atomic clocks and becoming the standard technique for very high precision spectroscopic measurements. A generalization of this interferometric method is presented replacing the two single coherent excitations by arbitrary composite laser pulses. The rotation of the state vector of a two-level system under the effect of a single pulse is described using the Pauli matrices basis of the SU(2) group. It is then generalized to multiple excitation pulses by a recursive Eule…
In quantum information science, the external control of qubits must be balanced with the extreme isolation of the qubits from the environment. Atomic qubit systems typically mitigate this balance through the use of gated laser fields that can create superpositions and entanglement between qubits. Here we propose the use of high-order optical Stark shifts from optical fields to manipulate the splitting of atomic qubits that are insensitive to other types of fields. We demonstrate a fourth-order AC Stark shift in a trapped atomic ion system that does not require extra laser power beyond that nee…
We investigate scattering of lattice laser radiation in a strontium optical lattice clock and its implications for operating clocks at interrogation times up to several tens of seconds. Rayleigh scattering does not cause significant decoherence of the atomic superposition state near a magic wavelength. Among the Raman scattering processes, lattice-induced decay of the excited state $(5s5p)\,{}^{3}\mathrm{P}_{0}$ to the ground state $(5s^2)\,{}^{1}\mathrm{S}_{0}$ via the state $(5s5p)\,{}^{3}\mathrm{P}_{1}$ is particularly relevant, as it reduces the effective lifetime of the excited state and …
The exquisite control exhibited over quantum states of individual particles has revolutionized the field of precision measurement, as exemplified by the most accurate atomic clock realized in single trapped ions. Whereas many-atom lattice clocks have shown advantages in measurement precision over trapped-ion clocks, their accuracy has remained 20 times worse. Here we demonstrate, for the first time, that a many-atom system achieves accuracy (6x10^{-18}) better than a single ion-based clock, with vastly reduced averaging times (3000 s). This is the first time a single clock has achieved the bes…
State-of-the-art atomic clocks are based on the precise detection of the energy difference between two atomic levels, measured as a quantum phase accumulated in a given time interval. Optical-lattice clocks (OLCs) now operate at or near the standard quantum limit (SQL) that arises from the quantum noise associated with discrete measurement outcomes. While performance beyond the SQL has been achieved in microwave clocks and other atomic sensors by engineering quantum correlations (entanglement) between the atoms, the generation of entanglement on an optical-clock transition and operation of suc…
We present a novel method for engineering an optical clock transition that is robust against external field fluctuations and is able to overcome limits resulting from field inhomogeneities. The technique is based on the application of continuous driving fields to form a pair of dressed states essentially free of all relevant shifts. Specifically, the clock transition is robust to magnetic shifts, quadrupole and other tensor shifts, and amplitude fluctuations of the driving fields. The scheme is applicable to either a single ion or an ensemble of ions, and is relevant for several types of ions,…
Building scalable quantum systems that demonstrate genuine performance enhancement based on entanglement is a major scientific goal for fields including computing, networking, simulations, and metrology. The tremendous challenge arises from the fragility of entanglement in increasingly larger sized quantum systems. Optical atomic clocks utilizing a large number of atoms have pushed the frontier of measurement science, building on precise engineering of quantum states and control of atomic interactions. However, today's state-of-the-art optical atomic clocks are limited by the quantum projectio…
Improved systematic uncertainty evaluation of the $^{171}$Yb optical lattice clock NMIJ-Yb1 with uncertainty of $2.6\times10^{-17}$
National Metrology Institute of Japan (NMIJ), National Institute of Advanced Industrial Science and Technology (AIST)（日本国家计量院（NMIJ），产业技术综合研究所（AIST））；Department of Physics, Graduate School of Engineering Science, Yokohama National University（横滨国立大学工学研究科物理系）
A new class of atomic interferences using ultra-narrow optical transitions are pushing quantum engineering control to a very high level of precision for a next generation of sensors and quantum gate operations. In such context, we propose a new quantum engineering approach to Ramsey-Bordé interferometry introducing multiple composite laser pulses with tailored pulse duration, Rabi field amplitude, frequency detuning and laser phase-step. We explore quantum metrology with hyper-Ramsey and hyper-Hahn-Ramsey clocks below the $10^-18$ level of fractional accuracy by a fine tuning control of light …
The use of ultra-precise optical clocks in space ("master clocks") will allow for a range of new applications in the fields of fundamental physics (tests of Einstein's theory of General Relativity, time and frequency metrology by means of the comparison of distant terrestrial clocks), geophysics (mapping of the gravitational potential of Earth), and astronomy (providing local oscillators for radio ranging and interferometry in space). Within the ELIPS-3 program of ESA, the "Space Optical Clocks" (SOC) project aims to install and to operate an optical lattice clock on the ISS towards the end of…
Precision metrology and quantum measurement often demand matter be prepared in well defined quantum states for both internal and external degrees of freedom. Laser-cooled neutral atoms localized in a deeply confining optical potential satisfy this requirement. With an appropriate choice of wavelength and polarization for the optical trap, two electronic states of an atom can experience the same trapping potential, permitting coherent control of electronic transitions independent of the atomic center-of-mass motion. We review a number of recent experiments that use this approach to investigate …
Trapped atomic ions are a proven and powerful tool for the fundamental research of quantum physics. They have emerged in recent years as one of the most promising candidates for several practical technologies including quantum computers, quantum simulators, atomic clocks, mass spectrometers and quantum sensors. Advanced fabrication techniques, taken from established and nascent disciplines, are being deployed to create novel, reliable devices with a view to large scale integration and commercial compatibility. This review will cover the fundamentals of ion trapping before proceeding with a dis…
A new generation of atomic sensors using ultra-narrow optical clock transitions and composite pulses are pushing quantum engineering control to a very high level of precision for applied and fundamental physics. Here, we propose a new version of Ramsey-Bordé interferometry introducing arbitrary composite laser pulses with tailored pulse duration, Rabi field, detuning and phase-steps. We explore quantum metrology below the $10^{-18}$ level of fractional accuracy by a fine tuning control of light excitation parameters protecting ultra-narrow optical clock transitions against residual light-shift…
Solid-state electronic spins are extensively studied in quantum information science, as their large magnetic moments offer fast operations for computing and communication, and high sensitivity for sensing. However, electronic spins are more sensitive to magnetic noise, but engineering of their spectroscopic properties, e.g. using clock transitions and isotopic engineering, can yield remarkable spin coherence times, as for electronic spins in GaAs, donors in silicon and vacancy centres in diamond. Here we demonstrate simultaneously induced clock transitions for both microwave and optical domain…
Exact and asymptotic lineshape expressions are derived from the semi-classical density matrix representation describing a set of closed three-level atomic or molecular states including decoherences, relaxation rates and light-shifts. An accurate analysis of the exact steady-state Dark Resonance profile describing the Autler-Townes doublet, the Electromagnetically Induced Transparency or Coherent Population Trapping resonance and the Fano-Feshbach lineshape, leads to the linewidth expression of the two-photon Raman transition and frequency-shifts associated to the clock transition. From an adia…
