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arXiv 1812.04076physics.optics
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作为高折射率介质Mie纳米谐振器的过渡金属二硫属化物纳米盘

Transition metal dichalcogenide nanodisks as high-index dielectric Mie nanoresonators

Ruggero Verre, Denis G. Baranov, Battulga Munkhbat, Jorge Cuadra, Mikael Käll, Timur Shegai

摘要:

单层过渡金属二硫属化物(TMDC)最近被提出作为一个独特的激子平台,先进的光学和电子功能。然而,尽管进行了大量的研究工作,但人们在很大程度上忽视了,除了显示出丰富的激子物理特性外,TMDC还具有非常高的折射率。这为利用这些材料构建基于亚波长几何模式的谐振纳米天线提供了可能性。在这里,我们表明,从剥离的多层WS $_2$制造的纳米盘支持不同的米氏共振和所谓的anapole状态,可以很容易地调谐在可见光和近红外光谱范围内的波长通过改变纳米盘的大小和纵横比。我们认为,TMDC材料的各向异性和激子的存在,大大丰富了纳米光子学的基础上等离子体和众所周知的高折射率材料,如硅的传统方法的补充。作为一个概念验证,我们展示了一种新的制度的光-物质相互作用,anapole激子极化激元,我们实现在一个单一的WS $_2$纳米盘。因此,我们的研究结果表明,纳米图案的TMDC是有前途的高折射率纳米光子学应用的材料,具有丰富的功能和优越的前景。

英文摘要:

Monolayer transition metal dichalcogenides (TMDCs) have recently been proposed as a unique excitonic platform for advanced optical and electronic functionalities. However, in spite of intense research efforts, it has been largely overlooked that, in addition to displaying rich exciton physics, TMDCs also possess a very high refractive index. This opens a possibility to utilize these materials for constructing resonant nanoantennas based on subwavelength geometrical modes. Here we show that nanodisks fabricated from exfoliated multilayer WS$_2$ support distinct Mie resonances and so-called anapole states that can be easily tuned in wavelength over the visible and near-infrared spectral range by varying the nanodisks' size and aspect ratio. We argue that the TMDC material anisotropy and the presence of excitons substantially enrich nanophotonics by complementing traditional approaches based on plasmonics and well-known high-index materials such as silicon. As a proof-of-concept, we demonstrate a novel regime of light-matter interaction, anapole-exciton polaritons, which we realize within a single WS$_2$ nanodisk. Our results thus suggest that nanopatterned TMDCs are promising materials for high-index nanophotonics applications with enriched functionalities and superior prospects.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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