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arXiv 1812.00560cond-mat.mtrl-sci
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高Neel温度低维反铁磁体SrRu2O6的拉曼光谱

Raman spectroscopy of the low dimensional antiferromagnet with large Neel temperature SrRu2O6

Yu. S. Ponosov, E. V. Komleva, D. A. Zamyatin, R. I. Walton, S. V. Streltsov

摘要:

我们报告的SrRu $_2$ O $_6$具有非常高的N $\acute{\textrm{e}}$ el温度的层状材料的拉曼测量结果。没有额外的声子模式被检测到的温度下的磁转变,从而排除了降低的对称性的磁有序相。当温度接近$T_N$时,一些声子的软化和阻尼的不寻常增加表明在$T\geq300K$出现了连续的相互作用的电子激发。我们还观察到在2050 cm $^{-1}$处的强烈拉曼响应。极化依赖性的分析和与现有的理论数据的比较表明,这个峰可能起源于分子轨道之间的跃迁先前提出的SrRu $_2$ O $_6$的磁性。

英文摘要:

We report results of the Raman measurements for SrRu$_2$O$_6$ having extraordinary high N$\acute{\textrm{e}}$el temperature for a layered material. No additional phonon modes were detected at the temperature of magnetic transition thus excluding lowering of the symmetry in the magnetically ordered phase. An unusual increase in softening and damping of some phonons as the temperature approaches $T_N$ indicate the appearance of a continuum of interacting electronic excitations at $T\geq300K$. We also observe an intensive Raman response at 2050 cm$^{-1}$. Analysis of the polarization dependence and comparison with available theoretical data shows that this peak likely originates from the transitions between molecular orbitals previously proposed to explain the magnetic properties of SrRu$_2$O$_6$.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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