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arXiv 1802.09437cond-mat.supr-conquant-ph
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腔量子电动力学极化激元增强的电子-声子耦合及其对超导电性的影响

Cavity quantum-electrodynamical polaritonically enhanced electron-phonon coupling and its influence on superconductivity

Michael A. Sentef, Michael Ruggenthaler, Angel Rubio

摘要:

迄今为止,激光对固体的控制主要是在泵浦-探测框架中的强经典非线性光-物质耦合的背景下讨论的。在这里,我们提出了一个量子电动力学的设置,以解决耦合的低维量子材料量子腔中的量子化电磁场。利用一个描述FeSe/SrTiO $_3$电子-声子长程前向散射的原型模型系统,我们研究了在材料的二维界面处声子极化激元的形成如何改变Migdal-Eliashberg模拟中的有效耦合和超导性质。我们发现,通过高度极化的偶极声子,大的腔增强的电子-声子耦合是可能的,但超导性没有增强的前向散射配对机制,由于耦合增强和模式软化之间的相互作用。耦合和模式频率的临界温度的依赖关系的分析表明,腔增强超导性是可能的更传统的短程配对机制。我们的研究结果表明,量子腔使工程的基本耦合在固体铺平了道路,以前所未有的控制材料的性能。

英文摘要:

Laser control of solids was so far mainly discussed in the context of strong classical nonlinear light-matter coupling in a pump-probe framework. Here we propose a quantum-electrodynamical setting to address the coupling of a low-dimensional quantum material to quantized electromagnetic fields in quantum cavities. Using a protoypical model system describing FeSe/SrTiO$_3$ with electron-phonon long-range forward scattering, we study how the formation of phonon polaritons at the 2D interface of the material modifies effective couplings and superconducting properties in a Migdal-Eliashberg simulation. We find that through highly polarizable dipolar phonons, large cavity-enhanced electron-phonon couplings are possible but superconductivity is not enhanced for the forward-scattering pairing mechanism due to the interplay between coupling enhancement and mode softening. An analysis of critical temperature dependencies on couplings and mode frequencies suggests that that cavity-enhanced superconductivity is possible for more conventional short-range pairing mechanisms. Our results demonstrate that quantum cavities enable the engineering of fundamental couplings in solids paving the way to unprecedented control of material properties.

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