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arXiv 1802.02536cond-mat.mes-hallcond-mat.mtrl-scicond-mat.str-el
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二维材料中电荷密度波的低频噪声和滑移

Low-Frequency Noise and Sliding of the Charge Density Waves in Two-Dimensional Materials

Guanxiong Liu, Sergey Rumyantsev, Matthew. A. Bloodgood, Tina T. Salguero, Alexander A. Balandin

摘要:

最近,人们对电荷密度波(CDW)现象重新产生了兴趣,这主要是由二维(2D)层状CDW材料(例如1 T-TaS 2)的出现驱动的,其特征在于非常高的向CDW相的转变温度。在广泛研究的具有准一维晶体结构的经典块体CDW材料中,载流子输运表现出有趣的滑动行为,在频域中表现为“窄带”和“宽带”噪声。尽管人们对二维CDW的物理特性越来越关注,但关于CDW滑动的报道很少,特别是在准二维稀土碲化物中,并且没有任何二维CDW系统中的噪声。在这里,我们报告的结果低频噪声(LFN)测量1 T-TaS 2薄膜原型二维CDW系统,因为它们是驱动从近相称(NC)到不相称(IC)CDW阶段的电压和温度刺激。我们发现,在1 T-TaS 2器件的噪声有两个明显的最大值在偏置电压,这对应于CDW滑动和NC到IC相变的开始。我们观察到不寻常的洛伦兹噪声特性和非常强的噪声依赖于电偏压和温度。我们认为,LFN在二维CDW系统有独特的物理起源,不同于已知的基本噪声类型。二维CDW材料中LFN的特性可以通过调用NC-CDW相中相互作用的离散波动子的概念来解释。噪声光谱可以作为一个有用的工具来理解电子输运现象的二维CDW材料的特点是共存的不同的阶段和强CDW钉扎。

英文摘要:

There has been a recent renewal of interest in charge-density-wave (CDW) phenomena, primarily driven by the emergence of two-dimensional (2D) layered CDW materials, such as 1T-TaS2, characterized by very high transition temperatures to CDW phases. In the extensively studied classical bulk CDW materials with quasi-1D crystal structure, the charge carrier transport exhibits intriguing sliding behavior, which reveals itself in the frequency domain as "narrowband" and "broadband" noise. Despite the increasing attention on physics of 2D CDWs, there have been few reports of CDW sliding, specifically in quasi-2D rare-earth tritellurides and none on the noise in any of 2D CDW systems. Here we report the results of low-frequency noise (LFN) measurements on 1T-TaS2 thin films - archetypal 2D CDW systems, as they are driven from the nearly commensurate (NC) to incommensurate (IC) CDW phases by voltage and temperature stimuli. We have found that noise in 1T-TaS2 devices has two pronounced maxima at the bias voltages, which correspond to the onset of CDW sliding and the NC-to-IC phase transition. We observed unusual Lorentzian noise features and exceptionally strong noise dependence on electric bias and temperature. We argue that LFN in 2D CDW systems has unique physical origin, different from known fundamental noise types. The specifics of LFN in 2D CDW materials can be explained by invoking the concept of interacting discrete fluctuators in the NC-CDW phase. Noise spectroscopy can serve as a useful tool for understanding electronic transport phenomena in 2D CDW materials characterized by coexistence of different phases and strong CDW pinning.

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