Entanglement between light and matter combines the advantage of long distance transmission of photonic qubits with the storage and processing capabilities of atomic qubits. To distribute photonic states efficiently over long distances several schemes to encode qubits have been investigated -- time-bin encoding being particularly promising due to its robustness against decoherence in optical fibers. Here, we demonstrate the generation of entanglement between a photonic time-bin qubit and a single collective atomic spin excitation (spin-wave) in a cold atomic ensemble, followed by the mapping of the atomic qubit onto another photonic qubit. A magnetic field that induces a periodic dephasing and rephasing of the atomic excitation ensures the temporal distinguishability of the two time-bins and plays a central role in the entanglement generation. To analyse the generated quantum state, we use largely imbalanced Mach-Zehnder interferometers to perform projective measurements in different qubit bases and verify the entanglement by violating a CHSH Bell inequality.
Superradiance, the enhanced collective emission of energy from a coherent ensemble of quantum systems, has been typically studied in atomic ensembles. In this work we study theoretically the enhanced emission of energy from coherent ensembles of harmonic oscillators. We show that it should be possible to observe harmonic oscillator superradiance for the first time in waveguide arrays in integrated photonics. Furthermore, we describe how pairwise correlations within the ensemble can be measured with this architecture. These pairwise correlations are an integral part of the phenomenon of superra…
Collective measurements on identically prepared quantum systems can extract more information than local measurements, thereby enhancing information-processing efficiency. Although this nonclassical phenomenon has been known for two decades, it has remained a challenging task to demonstrate the advantage of collective measurements in experiments. Here we introduce a general recipe for performing deterministic collective measurements on two identically prepared qubits based on quantum walks. Using photonic quantum walks, we realize experimentally an optimized collective measurement with fidelity…
Photonic condensates are complex systems exhibiting phase transitions due to the interaction with their molecular environment. Given the macroscopic number of molecules that form a reservoir of excitations, numerical simulations are expensive, even for systems with few cavity modes. We present a systematic construction of molecular excitation profiles with a clear hierarchical ordering, such that only modes in the lowest order in the hierarchy directly affect the cavity photon dynamics. In addition to a substantial gain in computational efficiency for simulations of photon dynamics, the explic…
We present a theoretical framework to describe the collective emission of light by entangled atomic states. Our theory applies to the low excitation regime, where most of the atoms are initially in the ground state, and relies on a bosonic description of the atomic excitations. In this way, the problem of light emission by an ensemble of atoms can be solved exactly, including dipole-dipole interactions and multiple light scattering. Explicit expressions for the emitted photonic states are obtained in several situations, such as those of atoms in regular lattices and atomic vapors. We determine…
In this paper, we employ theoretical and experimental efforts and realize a proof-of-principle verification of device-independent QKD based on the photonic setup. On the theoretical side, we enhance the loss tolerance for real device imperfections by combining different approaches, namely, random post-selection, noisy preprocessing, and developed numerical methods to estimate the key rate via the von Neumann entropy. On the experimental side, we develop a high-quality polarization-entangled photon source achieving a state-of-the-art (heralded) detection efficiency about 87.5%. This efficiency …
We demonstrate scattering of laser light from two InAs quantum dots coupled to a photonic crystal waveguide, which is achieved by strain-tuning the optical transitions of the dots into mutual resonance. By performing measurements of the intensity and photon statistics of transmitted laser light before and after tuning the dots into resonance, we show that the nonlinearity is enhanced by collective scattering. In addition to providing a means of manipulating few-photon optical nonlinearities, our approach establishes new opportunities for multi-emitter quantum optics in a solid-state platform.
Bright, entangled multiphoton sources based on atom photon interactions are an essential requirement in the realization of several quantum information and quantum computation schemes based on photonic quantum systems. Here, we experimentally demonstrate a four photon polarization entangled GHZ state obtained from Doppler broadened atomic ensembles of 87Rb atoms. Owing to collective two photon coherence in the Doppler broadened cascade-type atomic system, our setup enables the generation of robust four photon GHZ states with a fidelity of 0.82 and a measured four photon average coincidence rate…
We outline a proposal for a method of preparing an encoded two-state system (logical qubit) that is immune to collective noise acting on the Hilbert space of the states supporting it. The logical qubit is comprised of three photonic three-state systems (qutrits) and is generated by the process of spontaneous parametric down conversion. The states are constructed using linear optical elements along with three down-conversion sources, and are deemed successful by the simultaneous detection of six events. We also show how to select a maximally entangled state of two qutrits by similar methods. Fo…
A scheme for heralded generation of frequency-bin photonic qubits via spontaneous four-wave mixing in a system of coupled microring resonators (photonic molecule) is developed so that the qubit state is fully controlled by the frequency amplitude of the pump field. It is shown that coupling parameters of the photonic molecule can be optimized to provide generation of nearly pure heralded photons. The heralded qubit state does not depend on the microring resonator mode frequency, thereby allowing to take advantage of frequency multiplexing for improving efficiency of quantum information process…
We report on the realization and verification of quantum entanglement between an NV electron spin qubit and a telecom-band photonic qubit. First we generate entanglement between the spin qubit and a 637 nm photonic time-bin qubit, followed by photonic quantum frequency conversion that transfers the entanglement to a 1588 nm photon. We characterize the resulting state by correlation measurements in different bases and find a lower bound to the Bell state fidelity of F = 0.77 +/- 0.03. This result presents an important step towards extending quantum networks via optical fiber infrastructure.
Recent experimental advances enable the fabrication of photonic lattices in which the light propagates with non-trivial energy dispersions. When interfaced with quantum emitters, such systems yield strong collective spontaneous emission phenomena, such as perfect sub-radiance, in which the decay into the bath is completely suppressed, forming bound-states-in-the-continuum. Since such photonic lattices are generally lossy, an alternative way of probing them consists in coherently driving them to an steady-state from which photoluminescence can be extracted. Here, we formalize connections betwee…
The encoding of quantum information in photonic time-bin qubits is apt for long distance quantum communication schemes. In practice, due to technical constraints such as detector response time, or the speed with which co-polarized time-bins can be switched, other encodings, e.g. polarization, are often preferred for operations like state detection. Here, we present the conversion of qubits between polarization and time-bin encodings using a method that is based on an ultrafast optical Kerr shutter and attain efficiencies of 97% and an average fidelity of 0.827+/-0.003 with shutter speeds near …
The task of measuring in two mutually unbiased bases is central to many quantum information protocols, as well as being of fundamental interest. Increasingly, there is an experimental focus on generating and controlling high-dimensional photonic states. One approach is to use the arrival time of a photon, which can be split into discrete time bins. An important problem associated with such states is the difficulty in experimentally realizing a measurement that is mutually unbiased with respect to the time-of-arrival. We propose a simple and compact scheme to measure in both the time of arrival…
A novel method of preparing a single photon in temporally-delocalized entangled modes is proposed and analyzed. We show that two single-photon pulses propagating in a driven nonabsorbing medium with different group velocities are temporally split under parametric interaction into well-separated pulses. As a consequence, the single-photon "time-bin-entangled" states are generatedwith a programmable entanglement, which is easily controlled by driving field intensity. The experimental study of nonclassical features and nonlocality in generated states by means of balanced homodyne tomography is di…
The mapping of photonic states to collective excitations of atomic ensembles is a powerful tool which finds a useful application in the realization of quantum memories and quantum repeaters. In this work we show that cold atoms in optical lattices can be used to perform an entangling unitary operation on the transferred atomic excitations. After the release of the quantum atomic state, our protocol results in a deterministic two qubit gate for photons. The proposed scheme is feasible with current experimental techniques and robust against the dominant sources of noise.
We report a fully fibered source emitting cross time-bin entangled photons at 1540 nm from type-II spontaneous parametric down conversion. Compared to standard time-bin entanglement realizations, the preparation interferometer requires no phase stabilization, simplifying its implementation in quantum key distribution experiments. Franson/Bell-type tests of such a cross time-bin state are performed and lead to two-photon interference raw visibilities greater than 95%, which are only limited by the dark-counts in the detectors and imperfections in the analysis system. Just by trusting the random…
We demonstrate two approaches for unbalanced interferometers as time-bin qubit analyzers for quantum communication, robust against mode distortions and polarization effects as expected from free-space quantum communication systems including wavefront deformations, path fluctuations, pointing errors, and optical elements. Despite strong spatial and temporal distortions of the optical mode of a time-bin qubit, entangled with a separate polarization qubit, we verify entanglement using the Negative Partial Transpose, with the measured visibility of up to 0.85$\pm$0.01. The robustness of the analyz…
Photonic chip based time-bin entanglement has attracted significant attention because of its potential for quantum communication and computation. Useful time-bin entanglement systems must be able to generate, manipulate and analyze entangled photons on a photonic chip for stable, scalable and reconfigurable operation. Here we report the first time-bin entanglement photonic chip that integrates time-bin generation, wavelength demultiplexing and entanglement analysis. A two-photon interference fringe with an 88.4% visibility is measured (without subtracting any noise), indicating the high perfor…
Phase transitions, being the ultimate manifestation of collective behaviour, are typically features of many-particle systems only. Here, we describe the experimental observation of collective behaviour in small photonic condensates made up of only a few photons. Moreover, a wide range of both equilibrium and non-equilibrium regimes, including Bose-Einstein condensation or laser-like emission are identified. However, the small photon number and the presence of large relative fluctuations places major difficulties in identifying different phases and phase transitions. We overcome this limitation…
We investigate the steady state photon transport in a nonequilibrium collective-qubit model. By adopting the noninteracting blip approximation, which is applicable in the strong photon-qubit coupling regime, we describe the essential contribution of indirect qubit-qubit interaction to the population distribution, mediated by the photonic baths. The linear relations of both the optimal flux and noise power with the qubits system size are obtained. Moreover, the inversed power-law style for the finite-size scaling of the optimal photon-qubit coupling strength is exhibited, which is proposed to b…
We study light scattering off a two-dimensional (2D) array of atoms driven to Rydberg levels. We show that the problem can be mapped to a generalized model of waveguide QED, consisting of multiple 1D photonic channels (transverse modes), each of which directionally coupled to a corresponding Rydberg surface mode of the array. In the Rydberg blockade regime, collective excitations of different surface modes block each other, leading to multi-channel correlated photonic states. Using an analytical approach, we characterize inter-channel quantum correlations, and elucidate the role of collective …
Faithfully storing an unknown quantum light state is essential to advanced quantum communication and distributed quantum computation applications. The required quantum memory must have high fidelity to improve the performance of a quantum network. Here we report the reversible transfer of photonic polarization states into collective atomic excitation in a compact solid-state device. The quantum memory is based on an atomic frequency comb (AFC) in rare-earth ion doped crystals. We obtain up to 0.998 process fidelity for the storage and retrieval process of single-photon-level coherent pulse. Th…
Quantum optical microcombs in integrated ring resonators generate entangled photon pairs over many spectral modes, and allow the preparation of high dimensional qudit states. Ideally, those sources should be programmable and have a high generation rate, with comb lines tightly spaced for the implementation of efficient qudit gates based on electro-optic frequency mixing. While these requirements cannot all be satisfied by a single resonator device, for which there is a trade-off between high generation rate and tight bin spacing, a promising strategy is the use of multiple resonators, each gen…
We have proposed a scheme of multi-qubit \textit{quantum random access memory} (qRAM) based on the impedance matched photon echo quantum memory incorporated together with the control three-level atom in two coupled QED cavities. A set of matching conditions for basic physical parameters of the qRAM scheme that provides an efficient quantum control of the fast single photon storage and read-out has been found. In particular, it was found that the qRAM operation is determined by the properties of the photonic molecular realized in the qRAM dynamics. Herein, the maximal efficiency of the qRAM is …
Quantum interfaces between photons and ensembles of atoms have emerged as powerful tools for quantum technologies. A major objective for such interfaces is high fidelity storage and retrieval of a photon in a collective quantum state of many atoms. This requires long-lived collective superposition states, which is typically achieved with immobilized atoms. Thermal atomic vapors, which present a simple and scalable resource, have, so far, only been used for continuous variable processing or for discrete variable processing on short time scales where atomic motion is negligible. We develop a the…
Long-duration quantum memories for photonic qubits are essential components for achieving long-distance quantum networks and repeaters. The mapping of optical states onto coherent spin-waves in rare earth ensembles is a particularly promising approach to quantum storage. However, it remains challenging to achieve long-duration storage at the quantum level due to read-out noise caused by the required spin-wave manipulation. In this work, we apply dynamical decoupling techniques and a small magnetic field to achieve the storage of six temporal modes for 20, 50 and 100 ms in a $^{151}$Eu$^{3+}$:Y…
Photonic quantum information with time-bins: Principles and applications
University of Calgary（卡尔加里大学）；California Institute of Technology（加州理工学院）；John A. Paulson School of Engineering and Applied Sciences, Harvard University（哈佛大学约翰·A·保尔森工程与应用科学学院）
We describe a technique for manipulating quantum information stored in collective states of mesoscopic ensembles. Quantum processing is accomplished by optical excitation into states with strong dipole-dipole interactions. The resulting ``dipole blockade'' can be used to inhibit transitions into all but singly excited collective states. This can be employed for a controlled generation of collective atomic spin states as well as non-classical photonic states and for scalable quantum logic gates. An example involving a cold Rydberg gas is analyzed.
We present an original self-error-rejecting photonic qubit transmission scheme for both the polarization and spatial states of photon systems transmitted over collective noise channels. In our scheme, we use simple linear-optical elements, including half-wave plates, 50:50 beam splitters, and polarization beam splitters, to convert spatial-polarization modes into different time bins. By using postselection in different time bins, the success probability of obtaining the uncorrupted states approaches 1/4 for single-photon transmission, which is not influenced by the coefficients of noisy channe…
Higher dimensional quantum systems are an important avenue for new explorations in quantum computing as well as quantum communications. One of the ubiquitous resources in quantum technologies is entanglement. However, so far, entanglement has been certified in higher dimensional systems through suitable bounds on known entanglement measures. In this work, we have, for the first time, quantified the amount of entanglement in bi-partite pure qutrit states by analytically relating statistical correlation measures and known measures of entanglement, and have determined the amount of entanglement i…
Time reversal is one of the most intriguing yet elusive wave phenomenon of major interest in different areas of classical and quantum physics. Time reversal requires in principle to flip the sign of the Hamiltonian of the system, leading to a revival of the initial state (Loschmidt echo). Here it is shown that Loschmidt echo of photons can be observed in an optical setting without resorting to reversal of the Hamiltonian. We consider photonic propagation in a binary waveguide lattice and show that, by exchanging the two sublattices after some propagation distance, a Loschmidt echo can be obser…
We demonstrate theoretically that photon-photon attraction can be engineered in the continuum of scattering states for pairs of photons propagating in a hollow-core photonic crystal fiber filled with cold atoms. The atoms are regularly spaced in an optical lattice configuration and the photons are resonantly tuned to an internal atomic transition. We show that the hard-core repulsion resulting from saturation of the atomic transitions induces bunching in the photonic component of the collective atom-photon modes (polaritons). Bunching is obtained in a frequency range as large as tens of GHz, a…
Photon emission is the hallmark of light-matter interaction and the foundation of photonic quantum science, enabling advanced sources for quantum communication and computing. Although single-emitter radiation can be tailored by the photonic environment, the introduction of multiple emitters extends this picture. A fundamental challenge, however, is that the radiative dipole-dipole coupling rapidly decays with spatial separation, typically within a fraction of the optical wavelength. We realize distant dipole-dipole radiative coupling with pairs of solid-state optical quantum emitters embedded …
The future challenge of quantum communication are scalable quantum networks, which require coherent and reversible mapping of photonic qubits onto stationary atomic systems (quantum memories). A crucial requirement for realistic networks is the ability to efficiently store multiple qubits in one quantum memory. Here we demonstrate coherent and reversible mapping of 64 optical modes at the single photon level in the time domain onto one solid-state ensemble of rare-earth ions. Our light-matter interface is based on a high-bandwidth (100 MHz) atomic frequency comb, with a pre-determined storage …
Photonic time bin qubits are well suited to transmission via optical fibres and waveguide circuits. The states take the form $\frac{1}{\sqrt{2}}(α\ket{0} + e^{iϕ}β\ket{1})$, with $\ket{0}$ and $\ket{1}$ referring to the early and late time bin respectively. By controlling the phase of a laser driving a spin-flip Raman transition in a single-hole-charged InAs quantum dot we demonstrate complete control over the phase, $ϕ$. We show that this photon generation process can be performed deterministically, with only a moderate loss in coherence. Finally, we encode different qubits in different energ…
A comparative study of a qutrit (three-level atomic system) coupled to a classical field in a typical Markovian reservoir (free space) and in a photonic band-gap (PBG) crystal is carried out. The aim of the study is to assess the collective impact of structured environment and classical control of the system on the dynamics of quantum coherence, non-Markovianity, and estimation of parameters which are initially encoded in the atomic state. We show that the constructive interplay of PBG material as a medium and classical driving field as a part of system results in a significant enhancement of …
We show that the damping rate of elementary excitations of hybrid systems close to a phase transition can undergo a remarkable resonance like enhancement before mode softening takes place. In particular, we consider the friction of a collective density wave in a homogeneous superfluid of weakly interacting bosonic atoms coupled to the electromagnetic field of a single mode optical resonator. Here the Beliaev damping can thus be controlled by an external laser drive and be enhanced by several orders of magnitude.
