Collective super- and subradiant dynamics between distant optical quantum emitters
Alexey Tiranov, Vasiliki Angelopoulou, Cornelis Jacobus van Diepen, Björn Schrinski, Oliver August Dall'Alba Sandberg, Ying Wang, Leonardo Midolo, Sven Scholz, … 展开作者
Alexey Tiranov, Vasiliki Angelopoulou, Cornelis Jacobus van Diepen, Björn Schrinski, Oliver August Dall'Alba Sandberg, Ying Wang, Leonardo Midolo, Sven Scholz, Andreas Dirk Wieck, Arne Ludwig, Anders Søndberg Sørensen, Peter Lodahl
Photon emission is the hallmark of light-matter interaction and the foundation of photonic quantum science, enabling advanced sources for quantum communication and computing. Although single-emitter radiation can be tailored by the photonic environment, the introduction of multiple emitters extends this picture. A fundamental challenge, however, is that the radiative dipole-dipole coupling rapidly decays with spatial separation, typically within a fraction of the optical wavelength. We realize distant dipole-dipole radiative coupling with pairs of solid-state optical quantum emitters embedded in a nanophotonic waveguide. We dynamically probe the collective response and identify both super- and subradiant emission as well as means to control the dynamics by proper excitation techniques. Our work constitutes a foundational step toward multiemitter applications for scalable quantum-information processing.
This Letter shows that chains of optical or microwave emitters coupled to a 1D waveguide support subradiant states with close pairs of excited emitters, which have longer lifetimes than even the most subradiant states with only a single excitation. Exact, analytical expressions for non-radiative excitation dimer states are obtained in the limit of infinite chains. To understand the mechanism underlying these states, we present a formal equivalence between subradiant dimers and single localized excitations around a chain defect (unoccupied site). Our analytical mapping permits extension to emit…
An array of $N$ closely spaced dipole coupled quantum emitters exhibits super- and subradiance with characteristic tailorable spatial radiation patterns. Optimizing their geometry and distance with respect to the spatial profile of a near resonant optical cavity mode allows to increase the ratio between light scattering into the cavity mode and free space by several orders of magnitude. This leads to a distinct nonlinear particle number scaling of the relative strength of coherent light-matter interactions versus decay. In particular, for subradiant states the collective cooperativity increase…
We study collective `free-space' radiation properties of two distant single-layer arrays of quantum emitters as two-level atoms. We show that this system can support a long-lived Bell superposition state of atomic excitations exhibiting strong subradiance, which corresponds to a non-local excitation of the two arrays. We describe the preparation of these states and their application in quantum information as resource of non-local entanglement, including deterministic quantum state transfer with high fidelity between the arrays representing quantum memories. We discuss experimental realizations…
The properties of coupled emitters can differ dramatically from those of their individual constituents. Canonical examples include sub- and super-radiance, wherein the decay rate of a collective excitation is reduced or enhanced due to correlated interactions with the environment. Here, we systematically study the properties of collective excitations for regularly spaced arrays of quantum emitters coupled to a one-dimensional (1D) waveguide. We find that, for low excitation numbers, the modal properties are well-characterized by spin waves with a definite wavevector. Moreover, the decay rate o…
A ring of sub-wavelength spaced dipole-coupled quantum emitters possesses only few radiant but many extraordinarily subradiant collective modes. These exhibit a 3D-confined spatial radiation field pattern forming a nano-scale high-Q optical resonator. We show that tailoring the geometry, orientation and distance between two such rings allows for increasing the ratio of coherent ring-to-ring coupling versus free-space emission by several orders of magnitude. In particular we find that subradiant excitations, when delocalized over several ring sites, are effectively transported between the rings…
Cavity-embedded quantum emitters show strong modifications of free space radiation properties such as an enhanced decay known as the Purcell effect. The central parameter is the cooperativity $C$, the ratio of the square of the coherent cavity coupling strength over the product of cavity and emitter decay rates. For a single emitter, $C$ is independent of the transition dipole moment and dictated by geometric cavity properties such as finesse and mode waist. In a recent work [Phys. Rev. Lett. 119, 093601 (2017)] we have shown that collective excitations in ensembles of dipole-dipole coupled qu…
The Hermitian part of the dipole-dipole interaction in infinite periodic arrays of two-level atoms yields an energy band of singly excited states. In this Letter, we show that a dispersion relation, $ω_k-ω_{k_\ex} \propto (k-k_{\ex})^s$, near the band edge of the infinite system leads to the existence of subradiant states of finite one-dimensional arrays of $N$ atoms with decay rates scaling as $N^{-(s+1)}$. This explains the recently discovered $N^{-3}$ scaling and it leads to the prediction of power law scaling with higher power for special values of the lattice period. For the quantum optic…
We study a system of two distant quantum emitters coupled via a one-dimensional waveguide where the electromagnetic field has a direction-dependent velocity. As a consequence, the onset of collective emission is non-simultaneous and, for appropriate parameters, while one of the emitters exhibits superradiance the other can be subradiant. Interference effects enable the system to radiate in a preferential direction depending on the atomic state and the field propagation phases. We characterize such directional emission as a function of various parameters, delineating the conditions for optimal …
The realization of robust strong coupling and entanglement between distant quantum emitters (QEs) is very important for scalable quantum information processes. However, it is hard to achieve it based on conventional systems. Here, we propose theoretically and demonstrate numerically a scheme to realize such strong coupling and entanglement. Our scheme is based on the photonic crystal platform with topologically protected edge state and zero-dimensional topological corner cavities. When the QEs are put into topological cavities, the strong coupling between them can be fulfilled with the assista…
Inspired by recent advances in the manipulation of atoms trapped near 1D waveguides and pro- posals to use surface acoustic waves on piezoelectric substrates for the same purpose, we show the potential of two-dimensional platforms. We exploit the directional emission of atoms near photonic crystal slabs with square symmetry to build perfect subradiant states of 2 distant atoms, possible in 2D only for finite lattices with reflecting boundaries. We also show how to design massively parallel 1D arrays of atoms above a single crystal, useful for multi-port output of nonclassical light, by ex- plo…
The control and manipulation of quantum-entangled non-local states is a crucial step for the development of quantum information processing. A promising route to achieve such states on a wide scale is to couple solid-state quantum emitters through their coherent dipole-dipole interactions. Entanglement in itself is challenging, as it requires both nanometric distances between emitters and nearly degenerate electronic transitions. Implementing hyperspectral imaging to identify pairs of coupled organic molecules trapped in a low temperature matrix, we reach distinctive spectral signatures of maxi…
We investigate a one-dimensional quantum emitter chain where transport of excitations and correlations takes place via nearest neighbor, dipole-dipole interactions. In the presence of collective radiative emission, we show that a phase imprinting wavepacket initialization procedure can lead to subradiant transport and can preserve quantum correlations. In the context of cavity mediated transport, where emitters are coupled to a common delocalized optical mode, we analyze the effect of frequency disorder and nonidentical photon-emitter couplings on excitation transport.
The interaction of quantum emitters with structured baths modifies both their individual and collective dynamics. In González-Tudela \emph{et al} we show how exotic quantum dynamics emerge when QEs are spectrally tuned around the middle of the band of a two-dimensional structured reservoir, where we predict the failure of perturbative treatments, anisotropic interactions and novel super and subradiant behaviour. In this work, we provide further analysis of that situation, together with a complete analysis for the quantum emitter dynamics in spectral regions different from the center of the ban…
Ordered lattices of emitters with subwavelength periodicities support unconventional forms of light-matter interactions arising from collective effects. Here, we propose the realization and control of subradiant optical states within the radiation continuum in two-dimensional lattices. We show how bound states in the continuum (BICs) which are completely decoupled from radiative states emerge in non-Bravais lattices of emitters. Symmetry breaking results in quasi-BICs with greatly extended lifetimes, which can be exploited for quantum information storage. The analytical derivation of a general…
We show how to generate and control the correlations in a set of two distant quantum emitters coupled to a one-dimensional dissipative plasmonic waveguide. An external laser field enhances the dimer's steady-state correlations and allows an active control (switching on/off) of nonclassical correlations. The plasmon-assisted dipolar-interacting qubits exhibit persistent correlations, which in turn can be decoupled and made to evolve independently from each other. The setup enables long-distance ($\sim 1\, μ$m) qubit control that works for both resonant and detuned emitters. For suitable emitter…
Inherent binary or collective interactions in ensembles of quantum emitters induce a spread in the energy and lifetime of their eigenstates. While this typically causes fast decay and dephasing, in many cases certain special entangled collective states with minimal decay can be found, which possess ideal properties for spectroscopy, precision measurements or information storage. We show that for a specific choice of laser frequency, power and geometry or a suitable configuration of control fields one can efficiently prepare these states. We demonstrate this by studying preparation schemes for …
We present a combined classical and quantum electrodynamics description of the coupling between two circularly-polarized quantum emitters held above a metal surface supporting surface plasmons. Depending on their position and their natural frequency, the emitter-emitter interactions evolve from being reciprocal to nonreciprocal, which makes the system a highly tunable platform for chiral coupling at the nanoscale. By relaxing the stringent material and geometrical constraints for chirality, we explore the interplay between coherent and dissipative coupling mechanisms in the system. Thus, we re…
Starting from the paradigmatic spin-boson model (SBM), we investigate the static and dynamical properties of a system of two distant two-level emitters coupled to a one-dimensional Ohmic waveguide beyond the rotating wave approximation. Employing static and dynamical polaron Ansätze we study the effects of finite separation distance on the behavior of the photon-mediated Ising-like interaction, qubit frequency renormalization, ground-state magnetization, and entanglement entropy of the two-qubit system. Based on previous works we derive an effective approximate Hamiltonian for the two-impurity…
Waveguides allow for direct coupling of emitters separated by large distances, offering a path to connect remote quantum systems. However, when facing the distances needed for practical applications, retardation effects due to the finite speed of light are often overlooked. Previous works studied the non-Markovian dynamics of emitters with retardation, but the properties of the radiated field remain mostly unexplored. By considering a toy model of two distant two-level atoms coupled through a waveguide, we observe that the spectrum of the radiated field exhibits non-Markovian features such as …
Efficient and versatile interfaces for the interaction of light with matter are an essential cornerstone for quantum science. A fundamentally new avenue of controlling light-matter interactions has been recently proposed based on the rich interplay of photon-mediated dipole-dipole interactions in structured subwavelength arrays of quantum emitters. Here we report on the direct observation of the cooperative subradiant response of a two-dimensional (2d) square array of atoms in an optical lattice. We observe a spectral narrowing of the collective atomic response well below the quantum-limited d…
We study cooperative phenomena in the fluctuation-induced forces between a surface and a system of neutral two-level quantum emitters prepared in a coherent collective state, showing that the total Casimir-Polder force on the emitters can be modified via their mutual correlations. Particularly, we find that a collection of emitters prepared in a super- or subradiant state experiences an enhanced or suppressed collective vacuum-induced force, respectively. The collective nature of dispersion forces can be understood as resulting from the interference between the different processes contributing…
We analyze the dynamics of quantum beats in a system of two V-type three-level atoms coupled to a waveguide. We show that quantum beats can be collectively enhanced or suppressed, akin to Dicke super- and sub-radiance, depending on the interatomic separation and the initial correlations between the atoms. In particular, the interference properties of the collective beats are determined by the distance between the atoms modulo the beat wavelength. We study the collective atomic and field dynamics, illustrating a crossover from a Markovian to a non-Markovian regime as the atomic separation becom…
A ring of sub-wavelength spaced dipole-coupled quantum emitters features extraordinary optical properties when compared to a one-dimensional chain or a random collection of emitters. One finds the emergence of extremely subradiant collective eigenmodes similar to an optical resonator, which feature strong 3D sub-wavelength field confinement. Motivated by structures commonly appearing in natural light harvesting complexes, we extend these studies to stacked concentric multi-ring geometries. We predict that double rings allow to engineer significantly darker and better confined collective excita…
Dipole-coupled subwavelength quantum emitter arrays respond cooperatively to external light fields as they may host collective delocalized excitations (a form of excitons) with super- or subradiant character. Deeply subwavelength separations typically occur in molecular ensembles, where in addition to photon-electron interactions, electron-vibron couplings and vibrational relaxation processes play an important role. We provide analytical and numerical results on the modification of super- and subradiance in molecular rings of dipoles including excitations of the vibrational degrees of freedom.…
We consider the radiative properties of a system of two identical correlated atoms interacting with the electromagnetic field in its vacuum state in the presence of a generic dielectric environment. We suppose that the two emitters are prepared in a symmetric or antisymmetric superposition of one ground state and one excited state and we evaluate the transition rate to the collective ground state, showing distinctive cooperative radiative features. Using a macroscopic quantum electrodynamics approach to describe the electromagnetic field, we first obtain an analytical expression for the decay …
A scheme to utilize atom-like emitters coupled to nanophotonic waveguides is proposed for the generation of many-body entangled states and for the reversible mapping of these states of matter to photonic states of an optical pulse in the waveguide. Our protocol makes use of decoherence-free subspaces (DFS) for the atomic emitters with coherent evolution within the DFS enforced by strong dissipative coupling to the waveguide. By switching from subradiant to superradiant states, entangled atomic states are mapped to photonic states with high fidelity. An implementation using ultracold atoms coup…
We investigate Dicke subradiance of distant quantum sources in free space, i.e., the spatial emission pattern of spontaneously radiating non-interacting multi-level atoms or multi-photon sources, prepared in totally antisymmetric states. We find that the radiated intensity is marked by a strong suppression of spontaneous emission in particular directions. In resemblance to the analogous, yet inverted, superradiant emission profiles of $N$ distant two-level atoms prepared in symmetric Dicke states, we call the corresponding emission pattern $\textit{directional Dicke subradiance}$. We also show…
Photon-mediated interactions between quantum systems are essential for realizing quantum networks and scalable quantum information processing. We demonstrate such interactions between pairs of silicon-vacancy (SiV) color centers strongly coupled to a diamond nanophotonic cavity. When the optical transitions of the two color centers are tuned into resonance, the coupling to the common cavity mode results in a coherent interaction between them, leading to spectrally-resolved superradiant and subradiant states. We use the electronic spin degrees of freedom of the SiV centers to control these opti…
