Dynamics of large complex systems, such as relaxation towards equilibrium in classical statistical mechanics, often obeys a master equation. The equation significantly simplifies the complexities but describes essential information of occupation probabilities. A related fundamental question is the thermalization, a coherent evolution of an isolated many-body quantum state into a state that seems to be in thermal equilibrium. It is valuable to find an effective equation describing this complex dynamics. Here, we experimentally investigate the question by observing sudden quench dynamics of quantum Ising-like models implemented in our quantum simulator, defect-free single-atom tweezers in conjunction with Rydberg atom interaction. We find that saturation of local observables, a thermalization signature, obeys a master equation experimentally constructed by time-resolved monitoring the occupation probabilities of prequench states and imposing the principle of the detailed balance. Our experiment agrees with theories, and demonstrates the detailed balance in a thermalization dynamics that does not require coupling to baths or postulated randomness.
To facilitate quantum simulation of open quantum systems at finite temperatures, an important ingredient is to achieve thermalization on a given time-scale. We consider a Rydberg aggregate (an arrangement of Rydberg atoms that interact via long-range interactions) embedded in a laser-driven atomic environment. For the smallest aggregate (two atoms), suitable laser parameters can be found by brute force scanning of the four tunable laser parameters. For more atoms, however, such parameter scans are too computationally costly. Here we apply Gaussian processes to predict the thermalization perfor…
We question the microcanonical hypothesis, often made to account for the thermalization of complex closed quantum systems, on the specific example of a chain of two-level atoms optically driven by a resonant laser beam and strongly interacting via Rydberg-Rydberg dipole-dipole interactions. Along its (necessarily unitary) evolution, this system is indeed expected to thermalize, i.e. observables, such as the number of excitations, stop oscillating and reach equilibrium-like expectation values. The latter are often calculated through assuming the system can be effectively described by a thermal-…
We show that the quantum dimer state on the Kagome lattice, which was recently realized with high fidelity in a Rydberg quantum simulator [Semeghini et al., Science 374, 6572 (2021)], offers a sufficient resource for universal measurement-based quantum computations. In particular, we provide an efficient encoding of logical qubits in this state, and give explicit measurement sequences that implement a universal set of gates on these qubits. Since the building blocks of the proposed measurements have already been experimentally implemented, our work highlights one possible path towards promotin…
We experimentally emulate interaction induced blockade and local spin freezing in two and three qubit Nuclear Magnetic Resonance (NMR) architecture. These phenomena are identical to the Rydberg blockade and Rydberg biased freezing. In Rydberg blockade, the simultaneous excitation of two or more atoms is blocked due to the level shift induced by the strong Van der Waal's interaction. In such a strong interaction regime, one can also observe Rydberg biased freezing, wherein the dynamics is confined to a subspace, with the help of multiple drives with unequal amplitudes. Here we drive NMR qubits …
Quantum scrambling measured by out-of-time-ordered correlator (OTOC) has an important role in understanding the physics of black holes and evaluating quantum chaos. It is known that Rydberg atom has been a general interest due to its extremely favourable properties for building a quantum simulator. Fast and efficient quantum simulators can be developed by studying quantum scrambling in related systems. Here we present a general quantum circuit to theoretically implement an interferometric protocol which is a technique proposed to measure OTOC functions. We apply this circuit to measure OTOC an…
Trapped ions are a versatile platform for the investigation of quantum many-body phenomena, in particular for the study of scenarios where long-range interactions are mediated by phonons. Recent experiments have shown that the trapped ion platform can be augmented by exciting high-lying Rydberg states. This introduces controllable state-dependent interactions that are independent from the phonon structure. However, the many-body physics in this newly accessible regime is largely unexplored. We show that this system grants access to generalized Dicke model physics, where dipolar interactions be…
The most recent manifestation of cold Rydberg atom quantum simulators that employs tailored optical tweezer arrays enables the study of many-body dynamics under so-called facilitation conditions. We show how the facilitation mechanism yields a Hilbert space structure in which the many-body states organize into synthetic lattices, which feature in general one or several flat bands and may support immobile localized states. We focus our discussion on the case of a ladder lattice geometry for which we analyze in particular the influence of disorder generated by the uncertainty of the atomic posit…
Recent realization of a kinetically-constrained chain of Rydberg atoms by Bernien et al. [Nature 551, 579 (2017)] resulted in the observation of unusual revivals in the many-body quantum dynamics. In our previous work [arXiv:1711.03528] such dynamics was attributed to the existence of "quantum scarred" eigenstates in the many-body spectrum of the experimentally realized model. Here we present a detailed study of the eigenstate properties of the same model. We find that the majority of the eigenstates exhibit anomalous thermalization: the observable expectation values converge to their Gibbs en…
We propose a setup of an open quantum system in which the environment can be tuned such that either Markovian or non-Markovian system dynamics can be achieved. The implementation uses ultracold Rydberg atoms, relying on their strong long-range interactions. Our suggestion extends the features available for quantum simulators of molecular systems employing Rydberg aggregates and presents a new test bench for fundamental studies of the classification of system-environment interactions and the resulting system dynamics in open quantum systems.
Quantum many-body scars have attracted much interest as a violation of the eigenstate thermalization hypothesis (ETH) due to recent experimental observation in Rydberg atoms and related theoretical studies. In this paper, we construct a model hosting exact Floquet quantum many-body scars, which violate the Floquet version of ETH. We consider two uniformly-driven static Hamiltonians prohibiting neighboring up spins (Rydberg blockade) like the PXP model, and construct a binary drive composed of them. We show that there exists a four-dimensional subspace which completely avoids thermalization to …
Following Feynman and as elaborated on by Lloyd, a universal quantum simulator (QS) is a controlled quantum device which reproduces the dynamics of any other many particle quantum system with short range interactions. This dynamics can refer to both coherent Hamiltonian and dissipative open system evolution. We investigate how laser excited Rydberg atoms in large spacing optical or magnetic lattices can provide an efficient implementation of a universal QS for spin models involving (high order) n-body interactions. This includes the simulation of Hamiltonians of exotic spin models involving n-…
Recently the Rydberg blockade effect has been utilized to realize quantum spin liquid on the kagome lattice. Evidence of quantum spin liquid has been obtained experimentally by directly measuring non-local string order. In this letter, we report a BCS-type variational wave function study of the spin liquid state in this model. This wave function is motivated by mapping the Rydberg blockade model to a lattice gauge theory, where the local gauge conservations replace the role of constraints from the Rydberg blockade. We determine the variational parameter from the experimental measurement of the…
The eigenstate thermalization hypothesis (ETH) offers a universal mechanism for the approach to equilibrium of closed quantum many-body systems. So far, however, experimental studies have focused on the relaxation dynamics of observables as described by the diagonal part of ETH, whose verification requires substantial numerical input. This leaves many of the general assumptions of ETH untested. Here, we propose a theory-independent route to probe the full ETH in quantum simulators by observing the emergence of fluctuation-dissipation relations, which directly probe the off-diagonal part of ETH…
Quantum phase transitions (QPTs) involve transformations between different states of matter that are driven by quantum fluctuations. These fluctuations play a dominant role in the quantum critical region surrounding the transition point, where the dynamics are governed by the universal properties associated with the QPT. While time-dependent phenomena associated with classical, thermally driven phase transitions have been extensively studied in systems ranging from the early universe to Bose Einstein Condensates, understanding critical real-time dynamics in isolated, non-equilibrium quantum sy…
Gauge theories form the foundation of modern physics, with applications ranging from elementary particle physics and early-universe cosmology to condensed matter systems. We perform quantum simulations of the unitary dynamics of a U(1) symmetric gauge field theory and demonstrate emergent irreversible behavior. The highly constrained gauge theory dynamics is encoded in a one-dimensional Bose--Hubbard simulator, which couples fermionic matter fields through dynamical gauge fields. We investigate global quantum quenches and the equilibration to a steady state well approximated by a thermal ensem…
We show how to implement a Rydberg-atom quantum simulator to study the non-equilibrium dynamics of an Abelian (1+1)-D lattice gauge theory. The implementation locally codifies the degrees of freedom of a $\mathbf{Z}_3$ gauge field, once the matter field is integrated out by means of the Gauss' local symmetries. The quantum simulator scheme is based on current available technology and scalable to considerable lattice sizes. It allows, within experimentally reachable regimes, to explore different string dynamics and to infer information about the Schwinger $U(1)$ model.
We find exponentially many exact quantum many-body scar states in a two-dimensional PXP model -- an effective model for a two-dimensional Rydberg atom array in the nearest-neighbor blockade regime. Such scar states are remarkably simple valence bond solids despite being at effectively infinite temperature, and thus strongly violate the eigenstate thermalization hypothesis. Given a particular boundary condition, such eigenstates have integer-valued energies. Moreover, certain charge-density-wave initial states give rise to strong oscillations in the Rydberg excitation density after a quantum qu…
The lattice compact Abelian Higgs model is a non-perturbative regularized formulation of low-energy scalar quantum electrodynamics. In 1+1 dimensions, this model can be quantum simulated using a ladder-shaped optical lattice with Rydberg-dressed atoms (Zhang et al., Phys. Rev. Lett. 121, 223201). In this setup, one spatial dimension is used to carry the angular momentum of the quantum rotors. One can use truncations corresponding to spin-2 and spin-1 to build local Hilbert spaces associated with the links of the lattice. We argue that ladder-shaped configurable arrays of Rydberg atoms can be u…
We discuss laser dressed dipolar and Van der Waals interactions between atoms and polar molecules, so that a cold atomic gas with laser admixed Rydberg levels acts as a designed reservoir for both elastic and inelastic collisional processes. The elastic scattering channel is characterized by large elastic scattering cross sections and repulsive shields to protect from close encounter collisions. In addition, we discuss a dissipative (inelastic) collision where a spontaneously emitted photon carries away (kinetic) energy of the collision partners, thus providing a significant energy loss in a s…
Collège de France, PSL University（法兰西公学院，巴黎文理研究大学）；CPHT, CNRS, École Polytechnique, IP Paris（法国国家科学研究中心，巴黎综合理工学院，巴黎理工学院）；Center for Computational Quantum Physics, Flatiron Institute（平顿研究所计算量子物理中心）；Leiden Institute of Advanced Computer Science & Leiden Institute of Physics, Universiteit Leiden（莱顿大学高级计算机科学研究所与物理研究所）；Center for Computational Mathematics, Flatiron Institute（平顿研究所计算数学中心）；Department of Physics and Astronomy, Rutgers University（罗格斯大学物理与天文学系）；DQMP, Université de Genève（日内瓦大学物质结构与凝聚态物理系）
Gauge theories are the cornerstone of our understanding of fundamental interactions among particles. Their properties are often probed in dynamical experiments, such as those performed at ion colliders and high-intensity laser facilities. Describing the evolution of these strongly coupled systems is a formidable challenge for classical computers, and represents one of the key open quests for quantum simulation approaches to particle physics phenomena. Here, we show how recent experiments done on Rydberg atom chains naturally realize the real-time dynamics of a lattice gauge theory at system si…
Dirac Spin Liquid Candidate in a Rydberg Quantum Simulator
Université Paris-Saclay, Institut d’Optique Graduate School, CNRS, Laboratoire Charles Fabry（巴黎萨克雷大学、高等光学学院、法国国家科学研究中心、夏尔·法布里实验室）；Princeton University（普林斯顿大学）；Harvard University（哈佛大学）；Institute of Physics, Chinese Academy of Sciences（中国科学院物理研究所）；Max-Born-Institut（马克斯·玻恩研究所）；Nanomaterials and Nanotechnology Research Center (CINN-CSIC), Universidad de Oviedo (UO)（纳米材料与纳米技术研究中心（CINN-CSIC）、阿斯图里亚斯大学）；Carnegie Mellon University（卡内基梅隆大学）
Rydberg atoms are remarkable tools for quantum simulation and computation. They are the focus of an intense experimental activity mainly based on low-angular-momentum Rydberg states. Unfortunately, atomic motion and levels lifetime limit the experimental time-scale to about 100$μ$s. Here, we demonstrate laser trapping of long-lived circular Rydberg states for up to 10ms. Our method is very general and opens many opportunities for quantum simulation. The 10ms trapping time corresponds to thousands of interaction cycles in a circular-state-based quantum simulator. It is also promising for quantu…
Quantum spin systems with kinetic constraints have become paradigmatic for exploring collective dynamical behaviour in many-body systems. Here we discuss a facilitated spin system which is inspired by recent progress in the realization of Rydberg quantum simulators. This platform allows to control and investigate the interplay between facilitation dynamics and the coupling of spin degrees of freedom to lattice vibrations. Developing a minimal model, we show that this leads to the formation of polaronic quasiparticle excitations which are formed by many-body spin states dressed by phonons. We i…
Rydberg atom arrays are programmable quantum simulators capable of preparing interacting qubit systems in a variety of quantum states. Due to long experimental preparation times, obtaining projective measurement data can be relatively slow for large arrays, which poses a challenge for state reconstruction methods such as tomography. Today, novel groundstate wavefunction ansätze like recurrent neural networks (RNNs) can be efficiently trained not only from projective measurement data, but also through Hamiltonian-guided variational Monte Carlo (VMC). In this paper, we demonstrate how pretrainin…
