Spectral manifestations of hybrid Tamm-microcavity modes in a 1D photonic crystal bounded with a silver layer and containing a nematic liquid crystal layer working as a microcavity have been studied using numerical simulation. It is demonstrated that the hybrid modes can be effectively tuned owing to the high sensitivity of the liquid crystal to the temperature and external electric field variations. It is established that the effect of temperature on the transmission spectrum of the investigated structure is most pronounced at the point of the phase transition of the liquid crystal to the isotropic state, where the refractive index jump is observed.
We propose a composite multilayer structure consist of graphene Tamm plasmon and Bragg reflector with defect layer to realize the low threshold and tunable optical bistability (OB) at the terahertz frequencies. This low-threshold OB originates from the couple of the Tamm plasmon (TP) and the defect mode (DM). We discuss the influence of graphene and the DM on the hysteretic response of the TM-polarized reflected light. It is found that the switch-up and switch-down threshold required to observe the optical bistable behavior are lowered markedly due to the excitation of the TP and DM. Besides, …
It was widely accepted that embedding of metallic layers into optoelectronic structures is detrimental to lasing due absorption in metal. However, recently macroscopic optical coherence and lasing was observed in microcavities with intra-cavity single metallic layer. Here we propose the design of the of microcavity-type structure with two intra-cavity metallic layers which could serve as contacts for electrical pumping. The design of optical modes based on utilizing peculiarities of Tamm plasmon provides vanishing absorption due to fixing of the node of electric field of optical mode to metall…
Optical Tamm States (OTS) are confined optical modes that can occur at the interface between two highly reflective structures. However, due to the strong reflectance required, their implemen-tation with highly processable and metal-free flexible materials has proven challenging. Herein, we develop the first structure supporting OTS based only on organic polymeric materials, demon-strating a photonic platform based on non-critical, widely available, and easily processable mate-rials. The structures fabricated present large areas and consist of a narrowband multi-layered polymeric Distributed Br…
We have developed a technique for realizing a two-dimensional quadrupolar microcavity with its deformation variable from 0% to 20% continuously. We employed a microjet ejected from a noncircular orifice in order to generate a stationary column with modulated quadrupolar deformation in its cross section. Wavelength red shifts of low-order cavity modes due to shape deformation were measured and were found to be in good agreement with the wave calculation for the same deformation, indicating the observed deformation is quadrupolar in nature.
We report controllable manipulation of slow and fast light in a whispering-gallery-mode (WGM) microtoroid resonator fabricated from Erbium (Er3+) doped silica. We observe continuous transition of the coupling between the fiber-taper waveguide and the microresonator from undercoupling to critical coupling and then to overcoupling regimes by increasing the pump power even though the spatial distance between the resonator and the waveguide was kept fixed. This, in turn, enables switching from fast to slow light and vice versa just by increasing the optical gain. An enhancement of delay of two-fol…
Photonic crystals and metamaterials have emerged as two classes of tailorable materials that enable precise control of light. Plasmonic crystals, which can be thought of as photonic crystals fabricated from plasmonic materials, Bragg scatter incident electromagnetic waves from a repeated unit cell. However, plasmonic crystals, like metamaterials, are composed of subwavelength unit cells. Here, we study terahertz plasmonic crystals of several periods in a two dimensional electron gas. This plasmonic medium is both extremely subwavelength ($\approx λ/100$) and reconfigurable through the applicat…
Ultralow noise, yet tunable lasers are a revolutionary tool in precision spectroscopy, displacement measurements at the standard quantum limit, and the development of advanced optical atomic clocks. Further applications include LIDAR, coherent communications, frequency synthesis, and precision sensors of strain, motion, and temperature. While all applications benefit from lower frequency noise, many also require a laser that is robust and compact. Here, we introduce a dual-microcavity laser that leverages one chip-integrable silica microresonator to generate tunable 1550 nm laser light via sti…
Complex optical systems such as high-quality microcavities enabled by advanced lithography and processing techniques paved the way to various light-matter interactions (LMI) studies. Without lattice-matching constraints in epitaxy, coating techniques or shaky open cavity constructions, sub-micrometer-precise lithographic development of a polymer photoresist paves the way to polymer microcavity structures for various spectral regions based on the material's transparency and the geometrical sizes. We introduce a new approach based on 3D nanowriting in photoresist, which can be employed to achiev…
We study the mechanical stability of a tunable high-finesse microcavity under ambient conditions and investigate light-induced effects that can both suppress and excite mechanical fluctuations. As an enabling step, we demonstrate the ultra-precise electronic stabilization of a microcavity. We then show that photothermal mirror expansion can provide high-bandwidth feedback and improve cavity stability by almost two orders of magnitude. At high intracavity power, we observe self-oscillations of mechanical resonances of the cavity. We explain the observations by a dynamic photothermal instability…
An add-drop filter (ADF) fabricated using a whispering gallery mode resonator has different crosstalks for add and drop functions due to non-zero intrinsic losses of the resonator. Here, we show that introducing gain medium in the resonator and optically pumping it below the lasing threshold not only allows loss compensation to achieve similar and lower crosstalks but also tunability in bandwidth and add-drop efficiency. For an active ADF fabricated using an erbium-ytterbium co-doped microsphere, we achieved 24-fold enhancement in the intrinsic quality factor, 3.5-fold increase in drop efficie…
Spatial light modulators (SLMs) are central to numerous applications ranging from high-speed displays to adaptive optics, structured illumination microscopy, and holography. After decades of advances, SLM arrays based on liquid crystals can now reach large pixel counts exceeding 10^6 with phase-only modulation with a pixel pitch of less than 10 μm and reflectance around 75%. However, the rather slow modulation speed in such SLMs (below hundreds of Hz) presents limitations for many applications. Here we propose an SLM architecture that can achieve high pixel count with high-resolution phase-onl…
Raman lasers based on bulk diamond are a valuable resource for generating coherent light in wavelength regimes where no common laser diodes are available. Nevertheless, the widespread use of such lasers is limited by their high threshold power requirements on the order of several Watts. Using on-chip microresonators, a significant reduction of the lasing threshold by more than two orders of magnitude has been shown. However, these resonators lack a continuous tuning mechanism and, mainly due to fabrication limitations, their implementation in the visible remains elusive. Here, we propose a pla…
The spontaneous emission of atoms can be controlled by placing them between two mirrors that form an optical cavity. Rapid advances in material processing techniques in the last 10 years have made it possible to fabricate microscopic optical cavities that can be finely tuned into resonance with the emitter. This has enabled progress in single-photon sources, nano-lasers and spectroscopy of new nano-emitters such as semiconductor quantum dots and Nitrogen-vacancy centres in diamond. Here we introduce a step-by-step method for computing the Purcell factor of the latest generation of open tunable…
Whispering gallery mode (WGM) microcavities strongly enhance nonlinear optical processes like optical frequency comb, Raman scattering and optomechanics, which nowadays enable cutting-edge applications in microwave synthesis, optical sensing spectroscopy, and integrated photonics. Yet, tunability of their resonances, mostly via coarse and complicated mechanism through temperature, electrical or mechanical means, still poses a major challenge for precision applications as above. Here we introduce a new passive scheme to finely tune resonances of WGMs at MHz precision with an external probe. Suc…
Optical microcavities are a powerful tool to enhance spontaneous emission of individual quantum emitters. However, the broad emission spectra encountered in the solid state at room temperature limit the influence of a cavity, and call for ultra-small mode volume. We demonstrate Purcell-enhanced single photon emission from nitrogen-vacancy (NV) centers in nanodiamonds coupled to a tunable fiber-based microcavity with a mode volume down to $1.0\,λ^{3}$. We record cavity-enhanced fluorescence images and study several single emitters with one cavity. The Purcell effect is evidenced by enhanced flu…
Electrically reconfigurable dipolar polaritons with highly tunable nonlinearity in a homobilayer microcavity
Tsinghua University（清华大学）；University of Washington（华盛顿大学）；Beijing Academy of Quantum Information Sciences（北京量子信息科学研究院）；National Institute for Materials Science（国立材料研究所）；Nanyang Technological University（南洋理工大学）；Frontier Science Center for Quantum Information（量子信息前沿科学中心）
Light responsive devices employing molecular photo-switches are interesting for displays and dynamic light filtering. In this work, polymeric microcavities embedding a layer of photochromic compound have been studied by means of the transfer matrix method. Different polymers, such as poly vinyl carbazole, poly styrene and cellulose acetate, have been used. A microcavity that includes random one-dimensional photonic structures sandwiching the photochromic layer has also been studied. Propagation of light pulses through the microcavities has been analysed.
Open-access microcavities are a powerful tool to enhance light-matter interactions for solid-state quantum and nano systems and are key to advance applications in quantum technologies. For this purpose, the cavities should simultaneously meet two conflicting requirements - full tunability to cope with spatial and spectral inhomogeneities of a material, and highest stability under operation in a cryogenic environment to maintain resonance conditions. To tackle this challenge, we have developed a fully-tunable, open-access, fiber-based Fabry-Pérot microcavity platform which can be operated also …
Microcavities have long been recognized as indispensable elements in quantum photonic research due to their usefulness for enhanced light extraction and light-matter interaction. A conventional high-Q cavity structure typically allows only a single optical transition to be tuned into resonance with a specific mode. The transition to a more advanced double-cavity structure, however, introduces new and interesting possibilities such as enhancing two spectrally close optical transitions at the same time with two distinct cavity modes. Here, we investigate a cavity structure composed of a monolith…
Typical microresonators exhibit a large frequency spacing between resonances and a limited tunability. This impedes their use in a large class of applications which require a resonance of the microcavity to coincide with a predetermined frequency. Here, we experimentally overcome this limitation with highly prolate-shaped whispering-gallery-mode "bottle microresonators" fabricated from standard optical glass fibers. Our resonators combine an ultra-high quality factor of 360 million, a small mode volume, and near lossless fibre coupling, characteristic of whispering-gallery-mode resonators, wit…
High-finesse, open-geometry microcavities have recently emerged as a versatile tool for enhancing interactions between photons and material systems, with a range of applications in quantum optics and quantum information science. However, mechanical vibrations pose a considerable challenge to their operation within a closed-cycle cryostat, particularly when spatial tunability and free-space optical access are required. Here, we present the design and characterization of a system that can achieve $\sim$16 pm-rms passive mechanical stability between two high-finesse mirrors while permitting both …
Recent technological advancements have allowed to implement in solid-state cavity-based devices phenomena of quantum nature such as vacuum Rabi splitting, controllable single photon emission and quantum entanglement. For a sufficiently strong coupling between a quantum emitter and a cavity, large quality factors ($Q$) along with small modal volume ($V_{eff}$) are essential. Here we show that by applying a 5nm Al coating to the sidewalls of a submicrometer-sized Fabry-Pérot microcavity, the cavity $Q$ can be temperature-tuned from few hundreds at room temperatures to 2$\times$10$^5$ below 30~K.…
We report on the coupling of a single Nitrogen-vacancy (NV) center in a nanodiamond to a fiber-based microcavity at room temperature. Investigating the very same NV center inside the cavity and in free-space allows to systematically explore a new regime of phonon-assisted cavity feeding. Making use of the NV center's strongly broadened emission, we realize a widely tunable, narrowband single photon source. A master equation model well reproduces our experimental results and predicts a transition into a Purcell-enhanced emission regime at low temperatures.
We report controlled manipulation of mode splitting in an optical microresonator coupled to two nanoprobes. It is demonstrated that, by controlling the positions of the nanoprobes, the split modes can be tuned simultaneously or individually and experience crossing or anti-crossing in frequency and linewidth. A tunable transition between standing wave mode and travelling wave mode is also observed. Underlying physics is discussed by developing a two-scatterer model which can be extended to multiple scatterers. Observed rich dynamics and tunability of split modes in a single microresonator will …
The strong coupling of an IR-active molecular transition with an optical mode of the cavity results in vibrational polaritons, which opens a new way to control chemical reactivity via confined electromagnetic fields of the cavity. In this study, we design a voltage-tunable open microcavity and we show the formation of multiple vibrational polaritons in methyl salicylate. A Rabi splitting and polariton anticrossing behaviour is observed when the cavity mode hybridizes with the C=O stretching vibration of methyl salicylate. As this vibration contributes to the reaction coordinate of the photoind…
We demonstrate experimentally a new form of induced transparency, i.e., chaos-induced transparency, in a slightly deformed microcavity which support both continuous chaotic modes and discrete regular modes with Q factors exceeding 3X?10^7. When excited by a focused laser beam, the induced transparency in the transmission spectrum originates from the destructive interference of two parallel optical pathways: (i) directly refractive excitation of the chaotic modes, and (ii) excitation of the ultra-high-Q regular mode via chaos-assisted dynamical tunneling mechanism coupling back to the chaotic m…
We study the optomechanical coupling of a single-layer graphene with a high-Q Fabry-Perot microcavity in the membrane-in-the-middle configuration. In ordinary dissipative coupling systems, mechanical oscillators modulate the loss associated with the input coupling of the cavity mode; while in our system, the graphene oscillator couples dissipatively with the cavity mode through modulating its absorption loss. By analyzing the effects of the interband transition of a graphene suspended near the node of the cavity field, we obtain strong and tunable dissipative coupling without excessively reduc…
The field of spinoptronics is underpinned by good control over photonic spin-orbit coupling in devices that possess strong optical nonlinearities. Such devices might hold the key to a new era of optoelectronics where momentum and polarization degrees-of-freedom of light are interwoven and interfaced with electronics. However, manipulating photons through electrical means is a daunting task given their charge neutrality and requires complex electro-optic modulation of their medium. In this work, we present electrically tunable microcavity exciton-polariton resonances in a Rashba-Dresselhaus spi…
Photonic crystals based on graphene plasmons (GPs) are highly tunable and can accurately control photonic transmission at the nanoscales. In this work, the transfer matrix method (TMM) is introduced to study graphene plasmonic crystal (GPC) with periodic surface conductivity in the case of normal incidence. The introduction of TMM after considering the abnormal phase scattering of the abrupt interface gives an idea to accurately manipulate plasmonic crystal structures, and can reduce the calculation workload to a certain extent. The effectiveness of the proposed method is verified with the pla…
Second-harmonic and sum-frequency mixing phenomena associated with 3D-localized photonic modes are studied in InP-based planar photonic crystal microcavities excited by short-pulse radiation near 1550 nm. Three-missing-hole microcavities that support two closely-spaced modes exhibit rich second-order scattering spectra that reflect intra- and inter-mode mixing via the bulk InP chi(2) during ring-down after excitation by the broadband, resonant pulse. Simultaneous excitation with a non-resonant source results in tunable second-order radiation from the microcavity.
A method for the electrically controlled synchronous mode tuning in the transmittance and reflectance spectra of a photonic structure consisting of an asymmetric dielectric Fabry-Perot microcavity and an ultrathin metallic film has been proposed. The excitation of a broadband Tamm plasmon-polariton at the metal-Bragg mirror interface is accompanied by the two phenomena opposing one another. Due to the strong absorption induced by the metal, a sufficient rejection level in reflection of the off-resonant radiation has been obtained in a wide spectral range, which almost coincides with the photon…
We report on the development of on-chip microcavities and show their potential as a platform for cavity quantum electrodynamics experiments. Microcavity arrays were formed by the controlled buckling of SiO2/Ta2O5 Bragg mirrors, and exhibit a reflectance-limited finesse of 3500 and mode volumes as small as 35lambda^3. We show that the cavity resonance can be thermally tuned into alignment with the D2 transition of 87Rb, and outline two methods for providing atom access to the cavity. Owing to their small mode volume and high finesse, these cavities exhibit single-atom cooperativities as high as…
In this dissertation novel resonant propulsion of dielectric microspheres is studied with the goal of sorting spheres with identical resonances, which are critical for developing microspherical photonics. First, evanescent field couplers were developed by fixing tapered microfibers in mechanically robust platforms. The tapers were obtained by chemical etching techniques. Using these platforms, WGMs modal numbers, coupling regimes and quality factors were determined for various spheres and compared with theory. Second, the spectroscopic properties of photonic molecules formed by spheres with be…
Liquid crystals (LCs) form an extremely rich range of self-assembled topological structures with artificially or naturally created topological defects. Some of the main applications of LCs are various optical and photonic devices, where compared to their solid state counterparts soft photonic systems are fundamentally different in terms of unique properties such as self-assembly, self-healing, large tunability, sensitivity to external stimuli and biocompatibility. Here we show that complex tunable microlasers emitting structured light can be generated from self-assembled topological LC superst…
Room-temperature polariton condensate in a two-dimensional hybrid perovskite
Carl von Ossietzky Universität Oldenburg（奥格斯堡卡尔冯奥西茨基大学）；University of Valencia（瓦伦西亚大学）；University of Exeter（埃克塞特大学）；Fraunhofer-Institute for Applied Optics and Precision Engineering IOF（弗劳恩霍夫应用光学和精密工程研究所IOF）；Friedrich Schiller University（弗里德里希·席勒大学）；Bar-Ilan Univ.（巴伊兰大学）；Weizmann Institute of Science（魏茨曼科学研究所）
