High Purcell factor generation of coherent on-chip single photons
F. Liu, A. J. Brash, J. O'Hara, L. M. P. P. Martins, C. L. Phillips, R. J. Coles, B. Royall, E. Clarke, C. Bentham, N. Prtljaga, I. E. Itskevich, L. R. Wilson, … 展开作者
F. Liu, A. J. Brash, J. O'Hara, L. M. P. P. Martins, C. L. Phillips, R. J. Coles, B. Royall, E. Clarke, C. Bentham, N. Prtljaga, I. E. Itskevich, L. R. Wilson, M. S. Skolnick, A. M. Fox
备注：
Manuscript with 9 pages and 5 figures plus supplementary materials comprising 12 pages and 11 figures
On-chip single-photon sources are key components for integrated photonic quantum technologies. Semiconductor quantum dots can exhibit near-ideal single-photon emission but this can be significantly degraded in on-chip geometries owing to nearby etched surfaces. A long-proposed solution to improve the indistinguishablility is by using the Purcell effect to reduce the radiative lifetime. However, until now only modest Purcell enhancements have been observed. Here we use pulsed resonant excitation to eliminate slow relaxation paths, revealing a highly Purcell-shortened radiative lifetime (22.7 ps) in a waveguide-coupled quantum dot-photonic crystal cavity system. This leads to near-lifetime-limited single-photon emission which retains high indistinguishablility (93.9%) on a timescale in which 20 photons may be emitted. Nearly background-free pulsed resonance fluorescence is achieved under $π$-pulse excitation, enabling demonstration of an on-chip, on-demand single-photon source with very high potential repetition rates.
A Compact Broadband Purcell Filter for Superconducting Quantum Circuits in a 3D Flip-Chip Architecture
Technical University of Munich（慕尼黑工业大学）；Walther-Meißner-Institut, Bayerische Akademie der Wissenschaften（瓦尔特·迈斯纳研究所，巴伐利亚科学院）；Fraunhofer EMFT Institute for Electronic Microsystems and Solid State Technologies（弗劳恩霍夫电子微系统和固态技术研究所）
Integrated photonic circuits provide a versatile toolbox of functionalities for advanced quantum optics applications. Here, we demonstrate an essential component of such a system in the form of a Purcell enhanced single-photon source based on a quantum dot coupled to a robust on-chip integrated resonator. For that, we develop GaAs monolithic ring cavities based on distributed Bragg reflector ridge waveguides. Under resonant excitation conditions, we observe an over twofold spontaneous emission rate enhancement using Purcell effect and gain a full coherent optical control of a QD-two-level syst…
We investigate the Smith-Purcell emission produced by electron- or ion-beam-driven coherent excitation of nuclei arranged in periodic crystal lattices. The excitation and subsequent radiative decay of the nuclei can leave the target in the initial ground state after $γ$-ray emission, thus generating a coherent superposition of the far-field photon amplitude emanating from different nuclei that results in sharp angular patterns at spectrally narrow nuclear transition energies. We focus on Fe-57 as an example of two-level nuclear lossy system giving rise to Smith-Purcell emission at 14.4\,keV wi…
The nitrogen-vacancy (NV) center in diamond has been established as a prime building block for quantum networks. However, scaling beyond a few network nodes is currently limited by low spin-photon entanglement rates, resulting from the NV center's low probability of coherent photon emission and collection. Integration into a cavity can boost both values via the Purcell effect, but poor optical coherence of near-surface NV centers has so far prevented their resonant optical control, as would be required for entanglement generation. Here, we overcome this challenge, and demonstrate resonant addr…
Several emission features mark semiconductor quantum dots as promising non-classical light sources for prospective quantum implementations. For long-distance transmission [1] and Si-based on-chip processing[2, 3], the possibility to match the telecom C-band [4] stands out, while source brightness and high single-photon purity are key features in virtually any quantum implementation [5, 6]. Here we present an InAs/InGaAs/GaAs quantum dot emitting in the telecom C-band coupled to a circular Bragg grating. The Purcell enhancement of the emission enables a simultaneously high brightness with a fib…
Cavity-embedded quantum emitters show strong modifications of free space radiation properties such as an enhanced decay known as the Purcell effect. The central parameter is the cooperativity $C$, the ratio of the square of the coherent cavity coupling strength over the product of cavity and emitter decay rates. For a single emitter, $C$ is independent of the transition dipole moment and dictated by geometric cavity properties such as finesse and mode waist. In a recent work [Phys. Rev. Lett. 119, 093601 (2017)] we have shown that collective excitations in ensembles of dipole-dipole coupled qu…
Silicon carbide has recently been developed as a platform for optically addressable spin defects. In particular, the neutral divacancy in the 4H polytype displays an optically addressable spin-1 ground state and near-infrared optical emission. Here, we present the Purcell enhancement of a single neutral divacancy coupled to a photonic crystal cavity. We utilize a combination of nanolithographic techniques and a dopant-selective photoelectrochemical etch to produce suspended cavities with quality factors exceeding 5,000. Subsequent coupling to a single divacancy leads to a Purcell factor of ~50…
The stability and outstanding coherence of dopants and other atom-like defects in tailored host crystals make them a leading platform for the implementation of distributed quantum information processing and sensing in quantum networks. Albeit the required efficient light-matter coupling can be achieved via the integration into nanoscale resonators, in this approach the proximity of interfaces is detrimental to the coherence of even the least-sensitive emitters. Here, we establish an alternative: By integrating a 19 micrometer thin erbium-doped crystal into a cryogenic Fabry-Perot resonator wit…
Purcell-Engineered Hybrid Coupler for Leakage-Suppressed Robust CZ Gates
Zhejiang Qizhen Quantum Technology Co（浙江启真量子科技有限公司）；Institute of Quantum Sensing, Zhejiang University（浙江大学量子传感研究所）；Key Laboratory of Opto-electronic Technology, Ministry of Education, Beijing University of Technology（北京工业大学光电技术教育部重点实验室）；Hunan Normal University（湖南师范大学）
We report a numerical design procedure for pursuing a near-unity coupling efficiency in quantum dot-cavity ridge waveguide single-photon sources by performing simulations with the finite element method. Our optimum design which is based on a 1D nanobeam cavity, achieves a high source efficiency $ε_{xy}$ of 97.7$\%$ for an isotropic in-plane dipole, together with a remarkable Purcell factor of 38.6. Such a good performance is mainly attributed to the high index contrast of GaAs/SiO$_2$ and a careful cavity design achieving constructive interference and low scattering losses. Furthermore, we ana…
We report on cryogenic coupling of organic molecules to ring microresonators obtained by looping sub-wavelength waveguides (nanoguides). We discuss fabrication and characterization of the chip-based nanophotonic elements which yield resonator finesse in the order of 20 when covered by molecular crystals. Our observed extinction dips from single molecules reach 22%, consistent with the expected Purcell enhancements up to 11 folds. Future efforts will aim at efficient coupling of a handful of molecules via their interaction with a ring microresonator mode, setting the ground for the realization …
The limitations for the coherent manipulation of neutral atoms with fabricated solid state devices, so-called `atom chips', are addressed. Specifically, we examine the dominant decoherence mechanism, which is due to the magnetic noise originating from the surface of the atom chip. It is shown that the contribution of fluctuations in the chip wires at the shot noise level is not negligible. We estimate the coherence times and discuss ways to increase them. Our main conclusion is that future advances should allow for coherence times as long as one second, a few micrometers away from the surface.
The interaction of single quantum emitters with an optical cavity enables the realization of efficient spin-photon interfaces, an essential resource for quantum networks. The dynamical control of the spontaneous emission rate of quantum emitters in cavities has important implications in quantum technologies, e.g. for shaping the emitted photons waveform, for generating quantum entanglement, or for driving coherently the optical transition while preventing photon emission. Here we demonstrate the dynamical control of the Purcell enhanced emission of a small ensemble of erbium ions doped into na…
Realization of quantum optical circuits is at the heart of quantum photonic information processing. A long-standing obstacle however has been the absence of a platform of single photon sources (SPSs) that simultaneously satisfies the following required characteristics: spatially ordered SPS arrays that produce, on-demand, highly pure, and indistinguishable single photons with sufficiently uniform emission characteristics across the array, needed for controlled interference between photons from distinct sources to enable functional quantum optical networks. Here we report on such a platform of …
Entanglement-based technologies, such as quantum information processing, quantum simulations, and quantum-enhanced metrology, have the potential to revolutionise our way of computing and measuring and help clarifying the puzzling concept of entanglement itself. Ultracold atoms on atom chips are attractive for their implementation, as they provide control over quantum systems in compact, robust, and scalable setups. An important tool in this system is a potential depending on the internal atomic state. Coherent dynamics in this potential combined with collisional interactions allows entanglemen…
Realizing a controllable network with multiple degrees of interaction is a challenge to physics and engineering. Here, we experimentally report an on-chip reconfigurable network based on nanoelectromechanical resonators with nearest-neighbor (NN) and next-nearest-neighbor (NNN) strong couplings. By applying different parametric voltages on the same on-chip device, we carry out perfect coherent transfer in NN and NNN coupled array networks. Moreover, the low-loss resonators ensure the desired evolution to achieve perfect transfer and the demonstration of the parity-dependent phase relation at t…
We report the observation of nonclassical light generated via photon blockade in a photonic crystal cavity with a strongly coupled quantum dot. By tuning the frequency of the probe laser with respect to the cavity and quantum dot resonance we can probe the system in either photon blockade or photon-induced tunneling regime. The transition from one regime to the other is confirmed by the measurement of the second order correlation that changes from anti-bunching to bunching.
We develop a new approach to understanding intrinsic mechanisms that cause the $T_1$-decay rate of a multi-level superconducting qubit to depend on the photonic population of a coupled, detuned cavity. Our method yields simple analytic expressions for both the coherently driven or thermally excited cases which are in good agreement with full master equation numerics, and also facilitates direct physical intuition. It also predicts several new phenomena. In particular, we find that in a wide range of settings, the cavity-qubit detuning controls whether a non-zero photonic population increases o…
Quantum memory is the core device for the construction of large-scale quantum networks. For scalable and convenient practical applications, integrated optical memories, especially on-chip optical memories, are crucial requirements because they can be easily integrated with other on-chip devices. Here, we report the coherent optical memory based on a type-IV waveguide fabricated on the surface of a rare-earth ion-doped crystal (i.e. $\mathrm{Eu^{3+}}$:$\mathrm{Y_2SiO_5}$). The properties of the optical transition ($\mathrm{{^7}F{_0}\rightarrow{^5}D{_0}}$) of the $\mathrm{Eu^{3+}}$ ions inside t…
Optically-active spin systems coupled to photonic cavities with high cooperativity can generate strong light-matter interactions, a key ingredient in quantum networks. But obtaining high cooperativities for quantum information processing often involves the use of photonic crystal cavities that feature a poor optical access from the free space, especially to circularly polarized light required for the coherent control of the spin. Here, we demonstrate coupling with cooperativity as high as $8$ of an InAs/GaAs quantum dot to a fabricated bullseye cavity that provides nearly degenerate and Gaussi…
We propose a method to decouple the nanomechanical resonator in optomechanical systems from the environmental noise by introducing a chaotic coherent feedback loop. We find that the chaotic controller in the feedback loop can modulate the dynamics of the controlled optomechanical system and induce a broadband response of the mechanical mode. This broadband response of the mechanical mode will cut off the coupling between the mechanical mode and the environment and thus suppress the environmental noise of the mechanical modes. As an application, we use the protected optomechanical system to act…
In the control of classical mechanical systems, the feedback has been successfully applied to the production of the desired nonlinear dynamics. However, how much this can be done is still an open problem in quantum mechanical systems. This paper proposes a scheme of generating strong nonlinear quantum effects via the recently developed coherent feedback techniques, which can be shown to outperform the measurement-based quantum feedback scheme that can only generate pseudo-nonlinear quantum effects. Such advancement is demonstrated by two application examples in quantum optics on chip. In the f…
The scaleup of quantum computers operating in the microwave domain requires advanced control electronics, and the use of integrated components that operate at the temperature of the quantum devices is potentially beneficial. However, such an approach requires ultra-low power dissipation and high signal quality in order to ensure quantum-coherent operations. Here, we report an on-chip device that is based on a Josephson junction coupled to a spiral resonator and is capable of coherent continuous-wave microwave emission. We show that characteristics of the device accurately follow a theory based…
Integrated photonic circuits are an integral part of all-optical and on-chip quantum information processing and quantum computer. Deterministically integrated single-photon sources in nanoplasmonic circuits lead to densely packed scalable quantum logic circuits operating beyond the diffraction limit. Here, we report the coupling efficiency of single-photon sources to the plasmonic waveguide, characteristic transmission spectrum, propagation length, decay length, and plasmonic Purcell factor. We simulated the transmission spectrum to find the appropriate wavelength for various width of the diel…
WaveguideQEDoffers the possibility of generating strong coherent atomic interactions either through appropriate atomic configurations in the dissipative regime or in the bandgap regime. In this work, we show how to harness these interactions in order to herald the generation of highly entangled atomic states, which afterwards can be mapped to generate single mode multi-photonic states with high fidelities.Weintroduce two protocols for the preparation of the atomic states, we discuss their performance and compare them to previous proposals. In particular, we show that one of them reaches high p…
We predict and study the quantum-electrodynamical effect of parametric self-induced excitation of a molecule moving above the dielectric or conducting medium with periodic grating. In this case the radiation reaction force modulates the molecular transition frequency which results in a parametric instability of dipole oscillations even from the level of quantum or thermal fluctuations. The present mechanism of instability of electrically neutral molecules is different from that of the well-known Smith-Purcell and transition radiation in which a moving charge and its oscillating image create an…
Slow swift electrons with low self-inertia interact differently with matter and light in comparison with their relativistic counterparts: they are easily recoiled, reflected, and also diffracted form optical gratings and nanostructures. As a consequence, they can be also better manipulated into the desired shape. For example, they get bunched quite fast in interaction with acceleration gratings in presence of an external electromagnetic radiation, a phenomenon which can be desirable in development of superradiant coherent light sources. Here, I examine the spatiotemporal behavior of pulsed ele…
Nano-mechanical oscillators as well as Rydberg-atomic waveguides hosted on micro-fabricated chip surfaces hold promise to become pillars of future quantum technologies. In a hybrid platform with both, we show that beams of Rydberg atoms in waveguides can quantum-coherently interrogate and manipulate nanomechanical elements, allowing full quantum state tomography. Central to the tomography are quantum non-demolition measurements using the Rydberg atoms as probes. Quantum coherent displacement of the oscillator is also made possible, by driving the atoms with external fields while they interact …
The nitrogen-vacancy (NV) center in diamond has an optically addressable, highly coherent spin. However, an NV center even in high quality single-crystalline material is a very poor source of single photons: extraction out of the high-index diamond is inefficient, the emission of coherent photons represents just a few per cent of the total emission, and the decay time is large. In principle, all three problems can be addressed with a resonant microcavity. In practice, it has proved difficult to implement this concept: photonic engineering hinges on nano-fabrication yet it is notoriously diffic…
Quantum key distribution (QKD) can distribute symmetric key bits between remote legitimate users with the guarantee of quantum mechanics principles. For practical applications, the compact and robust photonic components for QKD are essential, and there are increasing attention to integrate the source, detector and modulators on a photonic chip. However, the massive and parallel QKD based on wavelength multiplexing are still challenge, due to the limited coherent light sources on the chip. Here, we introduce the Kerr dissipative soliton in a microresonator, which provides the locked coherent fr…
We report on the observation of bright emission of single photons under pulsed resonance fluorescence conditions from a single quantum dot (QD) in a micropillar cavity. The brightness of the QD fluorescence is greatly enhanced via the coupling to the fundamental mode of a micropillar, allowing us to determine a single photon extraction efficiency of $(20.7\pm0.8)~\%$ per linear polarization basis. This yields an overall extraction efficiency of $(41.4\pm1.5)~\%$ in our device. We observe the first Rabi-oscillation in a weakly coupled quantum dot-micropillar system under coherent pulsed optical…
Integrated photonics has enabled much progress towards quantum technologies. Many applications, including quantum communication, sensing, and distributed and cloud quantum computing, will require coherent photonic interconnection between separate chip-based sub-systems. Large-scale quantum computing systems and architectures may ultimately require quantum interconnects to enable scaling beyond the limits of a single wafer and towards "multi-chip" systems. However, coherently interconnecting separate chips is challenging due to the fragility of these quantum states and the demanding challenges …
Advances in quantum photonics have shown that chip-scale quantum devices are translating from the realm of basic research to applied technologies. Recent developments in integrated photonic circuits and single photon detectors indicate that the bottleneck for fidelity in quantum photonic processes will ultimately lie with the photon sources. We present and demonstrate a silicon nanophotonic chip capable of emitting telecommunication band photon pairs that exhibit the highest raw degree of time-energy entanglement from a micro/nanoscale source, to date. Biphotons are generated through cavity-en…
Tailored photonic cavities allow enhancing light-matter interaction ultimately to create a fully coherent quantum interface. Here, we report on an integrated microdisk cavity containing self-assembled quantum dots to coherently route photons between different access waveguides. We measure a Purcell factor of $F_{exp}=6.9\pm0.9$ for a cavity quality factor of about 10,000, allowing us to observe clear signatures of coherent scattering of photons by the quantum dots. We show how this integrated system can coherently re-route photons between the drop and bus ports, and how this routing is control…
Deterministic single-photon source with on-chip 5.6 GHz acoustic clock
Paul-Drude-Institut für Festkörperelektronik, Leibniz-Institut im Forschungsverbund Berlin e.V.（柏林莱布尼茨固体电子学保罗·德鲁德研究所）；Department of Physics, University of Colorado, Boulder（科罗拉多大学博尔德分校物理系）；National Institute of Standards and Technology（美国国家标准与技术研究院）
Above-Unity Coherent Cooperativity of Tin-Vacancy Centers in Diamond Photonic Crystal Cavities
QuTech, Delft University of Technology（代尔夫特理工大学 QuTech）；Kavli Institute of Nanoscience Delft, Delft University of Technology（代尔夫特理工大学卡弗里纳米科学研究所）；ICFO—Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology（巴塞罗那科技大学 ICFO-光子科学研究所）
Yangtze Delta Industrial Innovation Center of Quantum Science and Technology（量子科学与技术长三角产业创新中心）；China Academy of Electronics and Information Technology（中国电子科技集团公司）
