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arXiv 1706.04296cond-mat.mtrl-sci
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电选通(Bi,Sb)_2Te_3薄膜中螺旋度相关的光电流

Helicity dependent photocurrent in electrically gated (Bi,Sb)_2Te_3 thin films

Yu Pan, Qing-Ze Wang, Andrew L. Yeats, Timothy Pillsbury, Thomas C. Flanagan, Anthony Richardella, Haijun Zhang, David D. Awschalom, Chao-Xing Liu, Nitin Samarth

摘要:

已知圆偏振光在室温下在三维拓扑绝缘体中产生依赖于螺旋度的定向光电流。令人惊讶的是,这种现象很容易在光子能量下观察到,这些光子能量将电子激发到远高于自旋动量锁定狄拉克锥的状态,并且螺旋度相关光电流的潜在机制仍然不清楚。我们通过对(Bi,Sb)_2Te_3薄膜中螺旋度相关光电流随光激发入射角、波长和门控化学势的函数关系的全面研究,解决了这个难题。我们的观察使我们能够明确地确定的螺旋度依赖的光电流的主导机制的圆形光电效应。此外,我们使用分析计算将光电流的方向性与拓扑表面态和体能带之间的不对称光学跃迁联系起来。我们获得的见解是重要的工程光自旋电子器件,依赖于自旋和电荷电流的光学转向。

英文摘要:

Circularly polarized photons are known to generate a directional helicity-dependent photocurrent in three-dimensional topological insulators at room temperature. Surprisingly, the phenomenon is readily observed at photon energies that excite electrons to states far above the spin-momentum locked Dirac cone and the underlying mechanism for the helicity-dependent photocurrent is still not understood. We resolve the puzzle through a comprehensive study of the helicity-dependent photocurrent in (Bi,Sb)_2Te_3 thin films as a function of the incidence angle of the optical excitation, its wavelength, and the gate-tuned chemical potential. Our observations allow us to unambiguously identify the circular photo-galvanic effect as the dominant mechanism for the helicity-dependent photocurrent. Additionally, we use an analytical calculation to relate the directional nature of the photocurrent to asymmetric optical transitions between the topological surface states and bulk bands. The insights we obtain are important for engineering opto-spintronic devices that rely on optical steering of spin and charge currents.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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