arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 1706.01262cond-mat.str-el
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弱耦合量子自旋链Sr $_{2}$ CuO $_{3}$和SrCuO $_{2}$中的杂质

Impurities in weakly coupled quantum spin chains Sr$_{2}$CuO$_{3}$ and SrCuO$_{2}$

Koushik Karmakar, Rabindranath Bag, Markos Skoulatos, Christian Rüegg, Surjeet Singh

摘要:

利用非弹性中子散射、比热和体磁化测量方法研究了非磁性Zn $^{2+}$(自旋$0$)和磁性Ni $^{2+}$(自旋$1$)杂质对准一维自旋$1/2$海森堡反铁磁体Sr $_{2}$ CuO $_{3}$基态和低激发态的影响.我们发现,1 \% Ni $^{2+}$掺杂在Sr $_2$ CuO $_3$的自旋子激发中的一个相当大的自旋间隙的结果,类似于Ni掺杂的SrCuO $_2$以前报道的情况[参考文献1]。然而,在此为了比较而研究的SrCuO $_2$中类似水平的Zn $^{2+}$掺杂没有揭示任何自旋能隙的迹象。发现在Zn $^{2+}$和Ni $^{2+}$杂质的存在下,磁有序温度被抑制,然而,发现由于Ni $^{2+}$的抑制率比Zn $^{2+}$显著得多。研究了磁场对有序化温度的影响。我们发现,随着磁场的增加,不仅磁有序温度逐渐升高,而且与磁有序相关的比热反常的大小也逐渐增大,这可以定性地理解为是由于场诱导的量子涨落的抑制。

英文摘要:

We study the effect of non-magnetic Zn$^{2+}$ (spin-$0$) and magnetic Ni$^{2+}$ (spin-$1$) impurities on the ground state and low-lying excitations of the quasi-one-dimensional spin-$1/2$ Heisenberg antiferromagnet Sr$_{2}$CuO$_{3}$ using inelastic neutron scattering, specific heat and bulk magnetization measurements. We show that 1 \% Ni$^{2+}$ doping in Sr$_2$CuO$_3$ results in a sizable spin gap in the spinon excitations, analogous to the case of Ni-doped SrCuO$_2$ previously reported [ref. 1]. However, a similar level of Zn$^{2+}$ doping in SrCuO$_2$, investigated here for comparison, did not reveal any signs of a spin gap. Magnetic ordering temperature was found to be suppressed in the presence of both Zn$^{2+}$ and Ni$^{2+}$ impurities, however, the rate of suppression due to Ni$^{2+}$ was found to be much more pronounced than for Zn$^{2+}$. Effect of magnetic field on the ordering temperature is investigated. We found that with increasing magnetic field, not only the magnetic ordering temperature gradually increases but the size of specific heat anomaly associated with the magnetic ordering also progressively enhances, which can be qualitatively understood as due to the field induced suppression of quantum fluctuations.

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