We study experimentally and theoretically a coherently-driven strongly-coupled quantum dot-microcavity system. Our focus is on physics of the unexplored intermediate excitation regime where the resonant laser field dresses a strongly-coupled single exciton-photon (polariton) system resulting in a ladder of laser-dressed Jaynes-Cummings states. In that case both the coupling of the emitter to the confined light field of the microcavity and to the light field of the external laser are equally important, as proved by observation of injection pulling of the polariton branches by an external laser. This intermediate interaction regime is of particular interest since it connects the purely quantum mechanical Jaynes-Cummings ladder and the semi-classical Autler-Townes ladder. Exploring the driving strength-dependence of the mutually coupled system we establish the maximum in the resonance fluorescence signal to be a robust fingerprint of the intermediate regime and observe signatures indicating the laser-dressed Jaynes-Cummings ladder. In order to address the underlying physics we excite the coupled system via the matter component of fermionic nature undergoing saturation - in contrast to commonly used cavity-mediated excitation.
Fundamental and second-subharmonic Autler-Townes splitting in classical systems
Technical University of Munich（慕尼黑工业大学）；Ain Shams University（艾因夏姆斯大学）；Munich Center for Quantum Science and Technology (MCQST)（慕尼黑量子科学与技术中心）；TUM Center for Quantum Engineering (ZQE)（慕尼黑工业大学量子工程中心）
We present a proof-of-principle of how electronic transport measurements permits the observation of the Autler-Townes doublet, an optical property of nanodevices. The quantum physical system consists of one optically pumped quantum dot, a second auxiliary quantum dot, and a superconductor lead which provides an effective coupling between the dots via crossed Andreev reflection. Electrodes, working as source and drain, acts as nonequilibrium electronic reservoirs. Our calculations of the photocurrent at both, transient and stationary regimes, obtained using a density matrix formalism for open q…
Routers, switches, and repeaters are essential components of modern information-processing systems. Similar devices will be needed in future superconducting quantum computers. In this work we investigate experimentally the time evolution of Autler-Townes splitting in a superconducting phase qubit under the application of a control tone resonantly coupled to the second transition. A three-level model that includes independently determined parameters for relaxation and dephasing gives excellent agreement with the experiment. The results demonstrate that the qubit can be used as a ON/OFF switch w…
The Berry phase of Bloch states can have profound effects on electron dynamics lead to novel transport phenomena, such as the anomalous Hall effect and the valley Hall effect. Recently, it was predicted that the Berry phase effect can also modify the exciton states in transition metal dichalcogenide monolayers, and lift the energy degeneracy of exciton states with opposite angular momentum through an effective valley-orbital coupling. Here, we report the first observation and control of the Berry-phase induced splitting of the 2p-exciton states in monolayer molybdenum diselenide using the intr…
When a three-level quantum system is irradiated by an intense coupling field resonant with one of the three possible transitions, the absorption peak of an additional probe field involving the remaining level is split. This process is known in quantum optics as the Autler-Townes effect. We observe these phenomena in a superconducting Josephson phase qubit, which can be considered an "artificial atom" with a multilevel quantum structure. The spectroscopy peaks can be explained reasonably well by a simple three-level Hamiltonian model. Simulation of a more complete model (including dissipation, …
We present spectroscopic measurements of the Autler-Townes doublet and the sidebands of the Mollow triplet in a driven superconducting qubit. The ground to first excited state transition of the qubit is strongly pumped while the resulting dressed qubit spectrum is probed with a weak tone. The corresponding transitions are detected using dispersive read-out of the qubit coupled off-resonantly to a microwave transmission line resonator. The observed frequencies of the Autler-Townes and Mollow spectral lines are in good agreement with a dispersive Jaynes-Cummings model taking into account higher …
We propose a method to achieve significant optical signal delays exploiting the effect of Autler-Townes splitting in an inhomogeneously broadened quantum dot medium. The absorption and slow-down effects are compared for three schemes i.e. $Ξ$, V and $Λ$, corresponding to different excitation configurations. Qualitative differences of the V-scheme compared to the $Ξ$- and $Λ$-scheme are found, which show that features of Autler-Townes splitting are only revealed in the V-scheme. The underlying physical mechanisms causing this discrepancy are analyzed and discussed. Finally we compare field prop…
We have observed the Autler-Townes doublet in a superconducting Al/AlOx/Al transmon qubit that acts as an artificial atom embedded in a three-dimensional Cu microwave cavity at a temperature of 22 mK. Using pulsed microwave spectroscopy, the three lowest transmon levels are isolated, eliminating unwanted effects of higher qubit modes and cavity modes. The long coherence time (~40 us) of the transmon enables us to observe a clear Autler-Townes splitting at drive amplitudes much smaller than the transmon level anharmonicity (177 MHz). Three-level density matrix simulations with no free parameter…
We present a detailed theoretical analysis of a multi-level quantum system coupled to two radiation fields and subject to decoherence. We concentrate on an effect known from quantum optics as the Autler-Townes splitting, which has been recently demonstrated experimentally [M. A. Sillanpaa et al., Phys. Rev. Lett. 103, 193601 (2009)] in a superconducting phase qubit. In the three-level approximation, we derive analytical solutions and describe how they can be used to extract the decoherence rates and to account for the measurement data. Better agreement with the experiment can be obtained by ex…
A theoretical spectroscopic analysis of a microwave driven superconducting charge qubit (Cooper-pair box coupled) to an RLC oscillator model is performed. By treating the oscillator as a probe through the backreaction effect of the qubit on the oscillator circuit, we extract frequency splitting features analogous to the Autler-Townes effect from quantum optics, thereby extending the analogies between superconducting and quantum optical phenomenology. These features are found in a frequency band that avoids the need for high frequency measurement systems and therefore may be of use in qubit cha…
We report on the observation of spin dependent optically dressed states and optical Stark effect on an individual Mn spin in a semiconductor quantum dot. The vacuum-to-exciton or the exciton-to-biexciton transitions in a Mn-doped quantum dot are optically dressed by a strong laser field and the resulting spectral signature is measured in photoluminescence. We demonstrate that the energy of any spin state of a Mn atom can be independently tuned using the optical Stark effect induced by a control laser. High resolution spectroscopy reveals a power, polarization and detuning dependent Autler-Town…
We show theoretically that a quantum-dot circuit quantum electrodynamics (CQED) device can be used as a probe of the Overhauser field in quantum dots. By coupling a transmission line to the interdot tunneling gate, an electromagnetically-induced-transparency (EIT) scheme can be established, whose Fano-type interference leads to a sharp curvature in the reflection spectrum around resonance. This sharp feature persists even in the presence of the fluctuating spin bath, rendering a high-resolution method to extract the bath's statistical information. For strong nuclear spin fields, the reflection…
We discuss the optical response of a quantum molecule under the action of two lasers fields. Using a realistic model and parameters, we map the physical conditions to find three different phenomena reported in the literature: the tunneling induced transparency, the formation of Autler-Townes doublets, and the creation of a Mollow-like triplet. We found that the electron tunneling between quantum dots is the responsible for the different optical regime. Our results not only explain the experimental results in the literature but also give insights for future experiments and applications in optic…
We investigate the near infrared interband absorption of semiconductor quantum wells driven by intense terahertz radiation in the regime of ultrastrong coupling, where the Rabi frequency is a significant fraction of the frequency of the strongly driven transition. With the driving frequency tuned just below the lowest frequency transition between valence subbands, a particularly interesting phenomenon is observed. As the THz power increases, a new peak emerges above the frequency of the undriven exciton peak which grows and eventually becomes the larger of the two. This reversal of relative pe…
We present an experimental investigation on the spectral characteristics of an artificial atom "transmon qubit" constituting a three-level cascade system (Ξ-system) in the presence of a pair of external driving fields. We observe two different types of Autler-Townes (AT) splitting: type I, where the phenomenon of two-photon resonance tends to diminish as the coupling field strength increases, and type II, where this phenomenon mostly stays constant. We find that the types are determined by the cooperative effect of the decay rates and the field strengths. Theoretically analyzing the density-ma…
We explore routing of propagating phonons in analogy with previous experiments on photons. Surface acoustic waves (SAWs) in the microwave regime are scattered by a superconducting transmon qubit. The transmon can be tuned on or off resonance with the incident SAW field using an external magnetic field or the Autler-Townes effect, and thus the reflection and transmission of the SAW field can be controlled in time. We observe 80% extinction in the transmission of the low power continuous signal and a 40 ns rise time of the router. The slow propagation speed of SAWs on solid surfaces allows for i…
We propose a scheme to realize a highly efficient solid state source of photon pairs using cavity-assisted stimulated Raman adiabatic passage (STIRAP) in a single quantum dot, where a single photon from pump pulse and two stokes photons from cavity mode drives the Raman transition. The Autler-Townes doublet, generated by using a resonant continuous wave laser between biexciton and exciton states, and two-photon-resonant transition through strongly coupled cavity mode are utilized to facilitate (1+2)type Raman transition in the quantum dot. We show in the case of weak pump although the probabil…
We report on the investigation of a superconducting anharmonic multi-level circuit that is coupled to a harmonic readout resonator. We observe multi-photon transitions via virtual energy levels of our system up to the fifth excited state. The back-action of these higher-order excitations on our readout device is analyzed quantitatively and demonstrated to be in accordance with theoretical expectation. By applying a strong microwave drive we achieve multi-photon dressing within our anharmonic circuit which is dynamically coupled by a weak probe tone. The emerging higher-order Rabi sidebands and…
While the advanced coherent control of qubits is now routinely carried out in low frequency (GHz) systems like single spins, it is far more challenging to achieve for two-level systems in the optical domain. This is because the latter evolve typically in the THz range, calling for tools of ultrafast, coherent, nonlinear optics. Using four-wave mixing micro-spectroscopy, we here measure the optically driven dynamics of a single exciton quantum state confined in a semiconductor quantum dot. In a combined experimental and theoretical approach, we reveal the intrinsic Rabi oscillation dynamics by …
We propose to use molecular picocavity ensembles as macroscopic coherent nonlinear optical devices enabled by nanoscale strong coupling. For a generic picocavity model that includes molecular and photonic disorder, we derive theoretical performance bounds for coherent cross-phase modulation signals using weak classical fields of different frequencies. We show that strong coupling of the picocavity {\it vacua} with a specific vibronic sideband in the molecular emission spectrum results in a significant variation of the effective refractive index of the metamaterial relative to a molecule-free s…
