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arXiv 1608.05709cond-mat.str-elcond-mat.supr-con
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$A$ Fe $_\mathbf{2}$ As $_\mathbf{2}$($A=\,$ Ca,Sr,and Ba)单晶的光学性质

Optical properties of $A$Fe$_\mathbf{2}$As$_\mathbf{2}$ ($A=\,$Ca, Sr, and Ba) single crystals

Y. M. Dai, A. Akrap, S. L. Bud'ko, P. C. Canfield, C. C. Homes

摘要:

详细的光学性质已被确定为铁基材料$A$ Fe $_2$作为$_2$,其中$A=\,$钙,锶,钡,在铁砷($a-b$)平面在一个很宽的频率范围内偏振的光,以上和以下的磁性和结构转变在$T_N =$ 172,195,和138 K,分别。复电导率的实部和虚部同时使用两个Drude项与一系列振荡器相结合来拟合。在$T_N$以上,自由载流子响应由弱的、窄的Drude项和强的、宽的Drude项组成,这两者仅显示出弱的温度依赖性。在$T_N$以下,等离子体频率略有降低,但窄德鲁德项的散射率急剧下降,而对于宽德鲁德项,等离子体频率显著降低,而散射率的降低虽然显著,但并不严重。对于$T\ll{T_N}$的窄Drude项,观察到的散射率的小值可能与电子带的狄拉克锥状色散有关。在$T_N$以下,出现了与重构费米面和在$Δ_1 \simeq$ 45 $-$ 80 meV和$Δ_2 \simeq$ 110 $-$ 210 meV处的带隙相关的光导性的新特征。与自由载流子相关联的光谱权重的减小被带隙结构捕获,具体地,来自窄Drude项的光谱权重似乎被转移到低能带隙特征中,而来自宽项的缺失权重转移到高能带隙。

英文摘要:

The detailed optical properties have been determined for the iron-based materials $A$Fe$_2$As$_2$, where $A=\,$Ca, Sr, and Ba, for light polarized in the iron-arsenic ($a-b$) planes over a wide frequency range, above and below the magnetic and structural transitions at $T_N =$ 172, 195, and 138 K, respectively. The real and imaginary parts of the complex conductivity are fit simultaneously using two Drude terms in combination with a series of oscillators. Above $T_N$, the free-carrier response consists of a weak, narrow Drude term, and a strong, broad Drude term, both of which show only a weak temperature dependence. Below $T_N$ there is a slight decrease of the plasma frequency but a dramatic drop in the scattering rate for the narrow Drude term, and for the broad Drude term there is a significant decrease in the plasma frequency, while the decrease in the scattering rate, albeit significant, is not as severe. The small values observed for the scattering rates for the narrow Drude term for $T\ll{T_N}$ may be related to the Dirac cone-like dispersion of the electronic bands. Below $T_N$ new features emerge in the optical conductivity that are associated with the reconstruction Fermi surface and the gapping of bands at $Δ_1 \simeq$ 45 $-$ 80 meV, and $Δ_2 \simeq$ 110 $-$ 210 meV. The reduction in the spectral weight associated with the free carriers is captured by the gap structure, specifically, the spectral weight from the narrow Drude term appears to be transferred into the low-energy gap feature, while the missing weight from the broad term shifts to the high-energy gap.

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