Disordered systems provide paradigmatic instances of ergodicity breaking and localization phenomena. Here we explore the dynamics of excitations in a system of Rydberg atoms held in optical tweezers. The finite temperature produces an intrinsic uncertainty in the atomic positions, which translates into quenched correlated disorder in the interatomic interaction strengths. In a simple approach, the dynamics in the many-body Hilbert space can be understood in terms of a one-dimensional Anderson-like model with disorder on every other site, featuring both localized and delocalized states. We conduct an experiment on an eight-atom chain and observe a clear suppression of excitation transfer. Our experiment accesses a regime which is described by a two-dimensional Anderson model on a "trimmed" square lattice. Our results thus provide a concrete example in which the absence of excitation propagation in a many-body system is directly related to Anderson-like localization in the Hilbert space, which is believed to be the mechanism underlying many-body localization.
The emergent phases of strongly correlated spin-1/2 Fermi gases of Rydberg dressed atoms in a one dimensional optical lattice are theoretically investigated. At weak coupling a bosonization description is used to demonstrate the ability to drive alternating quantum phase transitions between distinct Luttinger liquids. At strong coupling the ground state develops non-trivial phase separation exhibiting Luttinger liquid ''puddles'' separated by magnetic domain walls due to the interplay of the incommensurate filling and the Rydberg core length scale. These phases can be detected in ultracold gas…
We study the non-equilibrium steady state arising from the interplay between coherent and dissipative dynamics in strongly interacting Rydberg gases using a recently introduced variational method [H. Weimer, Phys. Rev. Lett. 114, 040402 (2015)]. We give a detailed discussion of the properties of this novel approach, and we provide a comparison with methods related to the Bogoliubov-Born-Green-Kirkwood-Yvon hierarchy. We find that the variational approach offers some intrinsic advantages, and we also show that it is able to explain the experimental results obtained in an ultracold Rydberg gas o…
We have investigated formation of structures of Rydberg atoms excited from a disordered gas of ultracold atoms, using rate equations for two-photon Rydberg excitation in a single atom without eliminating the intermediate state. We have explored the validity range of these rate equations and defined a simple measure to determine, whether our model is applicable for a given set of laser parameters. We have applied these rate equations in Monte Carlo simulations of ultracold gases, for different laser beam profiles, and compared these simulations to experimental observations and find a general ag…
Dense Rydberg gases are out-of-equilibrium systems where strong density-density interactions give rise to effective kinetic constraints. They cause dynamic arrest associated with highly-constrained many-body configurations, leading to slow relaxation and glassy behavior. Multi-component Rydberg gases feature additional long-range interactions such as excitation-exchange. These are analogous to particle swaps used to artificially accelerate relaxation in simulations of atomistic models of classical glass formers. In Rydberg gases, however, swaps are real physical processes, which provide dynami…
We show that the excitation of long-range Rydberg molecules in a three-dimensional optical lattice can be used as a position- and time-sensitive probe of the site occupancy in the system. To this end, we detect the ions which are continuously generated by the decay of the formed Rydberg molecules. While a superfluid gas shows molecule formation for all parameters, a Mott insulator with $n=1$ filling reveals a strong suppression of the number of formed molecules. In the limit of weak probing, the technique can be used to probe the superfluid to Mott-insulator transition in real-time. Our method…
Atoms excited into high-lying Rydberg states and under strong dipole-dipole interactions exhibit phenomena associated with highly correlated and complex systems. We perform first principles numerical simulations on the dynamics of such systems. The emergence of a roton minimum in the excitation spectrum, as expected in strongly correlated gases and accurately described by Feynman's theory of liquid helium, is shown to significantly inhibit particle transport, with a strong suppression of the diffusion coefficient, due to the emerging spatial order. We also demonstrate how the ability to tempor…
We have studied the associative ionization of a Rydberg atom and a ground state atom in an ultracold Rydberg gas. The measured scattering cross section is three orders of magnitude larger than the geometrical size of the produced molecule. This giant enhancement of the reaction kinetics is due to an efficient directed mass transport which is mediated by the Rydberg electron. We also find that the total inelastic scattering cross section is given by the geometrical size of the Rydberg electron's wavefunction.
Several recent experiments have established by measuring the Mandel Q parameter that the number of Rydberg excitations in ultracold gases exhibits sub-Poissonian statistics. This effect is attributed to the Rydberg blockade that occurs due to the strong interatomic interactions between highly-excited atoms. Because of this blockade effect, the system can end up in a state in which all particles are either excited or blocked: a jamming limit. We analyze appropriately constructed random-graph models that capture the blockade effect, and derive formulae for the mean and variance of the number of …
We present photo-excitation of ultra-long-range Rydberg molecules as a probe of spatial correlations in quantum gases. Rydberg molecules can be created with well-defined internuclear spacing, set by the radius of the outer lobe of the Rydberg electron wavefunction $R_n$. By varying the principal quantum number $n$ of the target Rydberg state, the molecular excitation rate can be used to map the pair-correlation function of the trapped gas $g^{(2)}(R_n)$. We demonstrate this with ultracold Sr gases and probe pair-separation length scales ranging from $R_n = 1400 - 3200$ $a_0$, which are on the …
We study a two-dimensional lattice gas of atoms that are photo-excited to high-lying Rydberg states in which they interact via the van-der-Waals interaction. We explore the regime of dominant nearest neighbor interaction where this system is intimately connected to a quantum version of Baxter's hard squares model. We show that the strongly correlated ground state of the Rydberg gas can be analytically described by a projected entangled pair state that constitutes the ground state of the quantum hard squares model. This correspondence allows us to identify a first order phase boundary where the…
We present an analytical theory for the nonlinear optical response of a strongly interacting Rydberg gas under conditions of electromagnetically induced transparency. Simple formulae for the third order optical susceptibility are derived and shown to be in excellent agreement with recent experiments. The obtained expressions reveal strong nonlinearities, which in addition are of highly nonlocal character. This property together with enormous strength of the Rydberg-induced nonlinearities is shown to yield a unique laboratory platform for nonlinear wave phenomena, such as collapse-arrested modu…
We propose a novel scheme to efficiently tune the scattering length of two colliding ground-state atoms by off-resonantly coupling the scattering-state to an excited Rydberg-molecular state using laser light. For the s-wave scattering of two colliding ${^{87}}\mathrm{Rb}$ atoms, we demonstrate that the effective optical length and pole strength of this Rydberg optical Feshbach resonance can be tuned over several orders of magnitude, while incoherent processes and losses are minimised. Given the ubiquity of Rydberg molecular states, this technique should be generally applicable to homo-nuclear …
The non-equilibrium dynamics of a gas of cold atoms in which Rydberg states are off-resonantly excited is studied in the presence of noise. The interplay between interaction and off-resonant excitation leads to an initial dynamics where aggregates of excited Rydberg atoms slowly nucleate and grow, eventually reaching long-lived meta-stable arrangements which then relax further on much longer timescales. This growth dynamics is governed by an effective Master equation which permits a transparent and largely analytical understanding of the underlying physics. By means of extensive numerical simu…
In the presence of strong dephasing noise the dynamics of Rydberg gases becomes effectively classical, due to the rapid decay of quantum superpositions between atomic levels. Recently a great deal of attention has been devoted to the stochastic dynamics that emerges in that limit, revealing several interesting features, including kinetically-constrained glassy behaviour, self-similarity and aggregation effects. However, the non-equilibrium physics of these systems, in particular in the regime where coherent and dissipative processes contribute on equal footing, is yet far from being understood…
Recent experiments with strongly interacting, driven Rydberg ensembles have introduced a promising setup for the study of self-organized criticality (SOC) in cold atom systems. Based on this setup, we theoretically propose a control mechanism for the paradigmatic avalanche dynamics of SOC in terms of a time-dependent drive amplitude. This gives access to a variety of avalanche dominated, self-organization scenarios, prominently including self-organized criticality, as well as sub- and supercritical dynamics. We analyze the dependence of the dynamics on external scales and spatial dimensionalit…
We show that the dynamics of a laser driven Rydberg gas in the limit of strong dephasing is described by a master equation with manifest kinetic constraints. The equilibrium state of the system is uncorrelated but the constraints in the dynamics lead to spatially correlated collective relaxation reminiscent of glasses. We study and quantify the evolution towards equilibrium in one and two dimensions, and analyze how the degree of glassiness and the relaxation time are controlled by the interaction strength between Rydberg atoms. We also find that spontaneous decay of Rydberg excitations leads …
Simulating neural network criticality and resource dynamics with Rydberg gases
RPTU University Kaiserslautern-Landau（莱茵兰-普法尔茨技术大学凯泽斯劳滕-兰道分校）；State Research Center OPTIMAS（OPTIMAS州立研究中心）；Max Planck Graduate Center with Johannes Gutenberg University Mainz (MPGC)（美因茨约翰内斯·古腾堡大学马克斯·普朗克研究生院）
In this paper, we study Bose-Einstein condensation of Rydberg-dressed atoms considering finite range interactions. We use Hartree-Fock-Bogoliubov approximation based on Mean-Field approach. Moreover, within this approximation modified by the finite-range character of the two-body interaction we shall obtain analytical expressions for thermodynamic quantities of Rydberg-dressed Bose gas. The imaginary part of the quasiparticle spectrum of a BEC signals the instability of the roton mode with respect to the formation of supersolid state. Our theory predicts a second-order quantum phase transition…
We study the out-of-equilibrium dynamics of dissipative gases of atoms excited to two or more high-lying Rydberg states. This situation bears interesting similarities to classical binary (in general $p$-ary) mixtures of particles. The effective forces between the components are determined by the inter-level and intra-level interactions of Rydberg atoms. These systems permit to explore new parameter regimes which are physically inaccessible in a classical setting, for example one in which the mixtures exhibit non-additive interactions. In this situation the out-of-equilibrium evolution is chara…
We present optimal control protocols to prepare different many-body quantum states of Rydberg atoms in optical lattices. Specifically, we show how to prepare highly ordered many-body ground states, GHZ states as well as some superposition of symmetric excitation number Fock states, that inherit the translational symmetry from the Hamiltonian, within sufficiently short excitation times minimizing detrimental decoherence effects. For the GHZ states, we propose a two-step detection protocol to experimentally verify the optimal preparation of the target state based only on standard measurement tec…
Two-dimensional (2D) spectroscopy uses multiple electromagnetic pulses to infer the properties of a complex system. A paradigmatic class of target systems are molecular aggregates, for which one can obtain information on the eigenstates, various types of static and dynamic disorder and on relaxation processes. However, two-dimensional spectra can be difficult to interpret without precise knowledge of how the signal components relate to microscopic Hamiltonian parameters and system-bath interactions. Here we show that two-dimensional spectroscopy can be mapped in the microwave domain to highly …
We discuss techniques to generate long-range interactions in a gas of groundstate alkali atoms, by weakly admixing excited Rydberg states with laser light. This provides a tool to engineer strongly correlated phases with reduced decoherence from inelastic collisions and spontaneous emission. As an illustration, we discuss the quantum phases of dressed atoms with dipole-dipole interactions confined in a harmonic potential, as relevant to experiments. We show that residual spontaneous emission from the Rydberg state acts as a heating mechanism, leading to a quantum-classical crossover.
We observe the shift of Rydberg levels of rubidium close to a copper surface when atomic clouds are repeatedly deposited on it. We measure transition frequencies of rubidium to S and D Rydberg states with principal quantum numbers n between 31 and 48 using the technique of electromagnetically induced transparency. The spectroscopic measurement shows a strong increase of electric fields towards the surface that evolves with the deposition of atoms. Starting with a clean surface, we measure the evolution of electrostatic fields in the range between 30 and 300 \mum from the surface. We find that …
As was recently shown in Ref. 1, many eigenstates of a random Rydberg gas with resonant dipole-dipole interactions are highly delocalized. Although the high degree of delocalization is generic to various types of power-law interactions and to both two and three-dimensional systems, in their detailed aspects the coherence distributions are sensitive to these parameters and vary dramatically between different systems. We calculate the eigenstates of both two and three-dimensional gases and quantify their delocalization throughout the atoms in the gas using a coherence measure. By contrasting the…
We investigate the possibility of realizing supersolid quantum phases in bosonic Rydberg-excited quantum lattice gases in the presence of non-unitary processes, by simulating the dynamical evolution starting from initial preparation in non-dissipative equilibrium states. Within Gutzwiller theory, we first analyze the many-body ground-state of a bosonic Rydberg-excited quantum gas in a two dimensional optical lattice for variable atomic hopping rates and Rabi detunings. Furthermore, we perform time evolution of different supersolid phases using the Lindblad-master equation. With the inclusion o…
We study ultracold Rydberg-dressed Bose gases subject to artificial gauge fields in the fractional quantum Hall (FQH) regime. The characteristics of the Rydberg interaction gives rise to interesting many-body ground states different from standard FQH physics in the lowest Landau level (LLL). The non-local but rapidly decreasing interaction potential favors crystalline ground states for very dilute systems. While a simple Wigner crystal becomes energetically favorable compared to the Laughlin liquid for filling fractions $ν<1/12$, a correlated crystal of composite particles emerges already for …
We systematically investigate the topological properties of spin polarized Rydberg-dressed fermionic atoms loaded in a bilayer optical lattice. Through tuning the Rydberg coupling strength and the inter-layer tunneling amplitude, we identify different types of topological superfluid states generated from the inter-layer pairing and relative gauge phase modulation of the couples 2D $p$-wave superfluids. These phases includes gapped/gapless with/without time reversal symmetry. One of the most interesting states is a gapless paired topological superfluid with both the time-reversal symmetry and p…
One of the major challenges in realizing a strongly interacting lattice gas using Rydberg states is the occurrence of avalanche loss processes. As these are directly proportional to the total Rydberg fraction, the commonly suggested solution is using far off-resonantly excited Rydberg states. We instead propose the realization of a correlated bosonic lattice gas at near-resonant excitation, where the total Rydberg fraction in the bulk is low due to the strong, interaction-driven effective detuning. Using real-space dynamical mean-field theory we show that its reduced effect at the boundary of …
The statistics of strongly interacting, ultracold Rydberg gases are governed by the interplay of two factors: geometrical restrictions induced by blockade effects, and quantum mechanical effects. To shed light on their relative roles in the statistics of Rydberg gases, we compare three models in this paper: a quantum mechanical model describing the excitation dynamics within a Rydberg gas, a Random Sequential Adsorption (RSA) process on a Random Geometric Graph (RGG), and a RSA process on a Decomposed Random Intersection Graph (DRIG). The latter model is new, and refers to choosing a particula…
We numerically investigate the quantum crystallographic phases of a Rydberg-dressed Bose gas loaded on a square lattice by using the mean-field Gross--Pitaevskii model. For a relatively weak lattice confinement, the phases of ground state undergo amorphism, polycrystal, and polymorphism following the increase of the blockade radius, and if the confinement is stronger, a single crystal with a specific filling factor will be formed. In order to distinctively characterize these phases, the structure function is also studied. In such an anisotropic system, we report that the first diagonal element…
We identify a relation between the dynamics of ultracold Rydberg gases in which atoms experience a strong dipole blockade and spontaneous emission, and a stochastic process that models certain wireless random-access networks. We then transfer insights and techniques initially developed for these wireless networks to the realm of Rydberg gases, and explain how the Rydberg gas can be driven into crystal formations using our understanding of wireless networks. Finally, we propose a method to determine Rabi frequencies (laser intensities) such that particles in the Rydberg gas are excited with spe…
Engineering quantum phases with spontaneously broken symmetries is a major goal of research in different fields. Trapped ultracold Rydberg-excited atoms in optical lattices are a promising platform for realizing quantum phases with broken lattice translational symmetry since they are interacting over distances larger than the lattice constant. Although numerous theoretical works on trapped Rydberg-excited gases have predicted such phases, in particular density wave or supersolid phases, their experimental observation proves to be difficult due to challenges such as scattering processes and the…
The physics of highly excited Rydberg atoms is governed by blockade or exclusion interactions that hinder the excitation of atoms in the proximity of a previously excited one. This leads to cooperative effects and a relaxation dynamics displaying space-time heterogeneity similar to what is observed in the relaxation of glass-forming systems. Here we establish theoretically the existence of a glassy dynamical regime in an open Rydberg gas, associated with phase coexistence at a first-order transition in dynamical large deviation functions. This transition occurs between an active phase of low d…
We examine possible low-temperature phases of a repulsively Rydberg-dressed Fermi gas in a three-dimensional free space. It is shown that the collective density excitations develop a roton minimum, which is softened at a wavevector smaller than the Fermi wavevector when the particle density is above a critical value. The mean field calculation shows that unlike the insulating charge density waves states often observed in conventional condensed matters, a self-assembled metallic density wave state emerges at low temperatures. In particular, the density wave state supports a Fermi surface and a …
Ultracold atomic gases have been used extensively in recent years to realize textbook examples of condensed matter phenomena. Recently, phase transitions to ordered structures have been predicted for gases of highly excited, 'frozen' Rydberg atoms. Such Rydberg crystals are a model for dilute metallic solids with tunable lattice parameters, and provide access to a wide variety of fundamental phenomena. We investigate theoretically how such structures can be created in four distinct cold atomic systems, by using tailored laser-excitation in the presence of strong Rydberg-Rydberg interactions. W…
We study excitation transport in a two-dimensional system of randomly assembled spins with power-law hopping in two dimensions. This model can be realized in cold atom quantum simulators with Rydberg atoms. In these experiments, due to the Rydberg blockade effect, the degree of disorder in the system is effectively tunable by varying the spin density. We study dynamics and eigenstate properties of the model as a function of disorder strength and system size and discuss potential limitations for experiments. At strong disorder we predominantly observe localized eigenstates with power-law tails.…
Quantum information scrambling in strongly disordered Rydberg spin systems
Centre Européen des Sciences Quantiques (CESQ-ISIS, UMR7006), Université de Strasbourg et CNRS（斯特拉斯堡大学与法国国家科学研究中心）；Physikalisches Institut, Universität Heidelberg（海德堡大学物理研究所）；Institut für Festkörpertheorie und -optik, Friedrich-Schiller-Universität Jena（耶拿大学凝聚态理论与光学研究所）
Ultra-cold gases excited to strongly interacting Rydberg states are a promising system for quantum simulations of many-body systems. For off-resonant excitation of such systems in the dissipative regime, highly correlated many-body states exhibiting, among other characteristics, intermittency and multi-modal counting distributions are expected to be created. So far, experiments with Rydberg atoms have been carried out in the resonant, non-dissipative regime. Here we realize a dissipative gas of rubidium Rydberg atoms and measure its full counting statistics for both resonant and off-resonant e…
The devil's staircase is a fractal structure that characterizes the ground state of one-dimensional classical lattice gases with long-range repulsive convex interactions. Its plateaus mark regions of stability for specific filling fractions which are controlled by a chemical potential. Typically such staircase has an explicit particle-hole symmetry, i.e., the staircase at more than half-filling can be trivially extracted from the one at less than half filling by exchanging the roles of holes and particles. Here we introduce a quantum spin chain with competing short-range attractive and long-ra…
Recent theoretical studies predict that structural disorder, serving as a bridge connecting a crystalline material to an amorphous material, can induce a topological insulator from a trivial phase. However, to experimentally observe such a topological phase transition is very challenging due to the difficulty in controlling structural disorder in a quantum material. Given experimental realization of randomly positioned Rydberg atoms, such a system is naturally suited to studying structural disorder induced topological phase transitions and topological amorphous phases. Motivated by the develop…
Controllable Rydberg atom arrays have provided new insights into fundamental properties of quantum matter both in and out of equilibrium. In this work, we study the effect of experimentally relevant positional disorder on Rydberg atoms trapped in a 2D square lattice under anti-blockade (facilitation) conditions. We show that the facilitation conditions lead the connectivity graph of a particular subspace of the full Hilbert space to form a 2D Lieb lattice, which features a singular flat band. Remarkably, we find three distinct regimes as the disorder strength is varied: a critical regime, a de…
We investigate the ground-state properties and excitations of Rydberg-dressed bosons in both three and two dimensions, using the hypernetted-chain Euler-Lagrange approximation, which accounts for correlations and thus goes beyond the mean field approximation. The short-range behavior of the pair distribution function signals the instability of the homogeneous system towards the formation of droplet crystals at strong couplings and large soft-core radius. This tendency to spatial density modulation coexists with off-diagonal long-range order. The contribution of the correlation energy to the gr…
The ability to control and tune interactions in ultracold atomic gases has paved the way towards the realization of new phases of matter. Whereas experiments have so far achieved a high degree of control over short-ranged interactions, the realization of long-range interactions would open up a whole new realm of many-body physics and has become a central focus of research. Rydberg atoms are very well-suited to achieve this goal, as the van der Waals forces between them are many orders of magnitude larger than for ground state atoms. Consequently, the mere laser excitation of ultracold gases ca…
