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arXiv 1607.03381cond-mat.str-elcond-mat.mtrl-scicond-mat.supr-con
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三角结构PtBi2体相和表面电子结构的角分辨光电子能谱研究

Bulk and surface electronic structure of trigonal structured PtBi2 studied by angle-resolved photoemission spectroscopy

Q. Yao, Y. P. Du, X. J. Yang, Y. Zheng, D. F. Xu, X. H. Niu, H. F. Yang, P. Dudin, T. K. Kim, M. Hoesch, I. Vobornik, Z. -A. Xu, X. G. Wan, D. L. Feng, D. W. Shen

摘要:

具有层状三角晶体结构的PtBi2最近被报道表现出非常规的大线性磁电阻,但所涉及的机制仍然是难以捉摸的。利用高分辨角分辨光电子能谱,系统地研究了它的体相和表面电子结构。通过与第一性原理计算的仔细比较,我们的实验区分了低洼的体带纠缠表面状态,允许估计样品的真实化学计量。我们发现显着的电子掺杂PtBi 2,这意味着大量的Bi缺乏诱导的障碍。在布里渊区的边界上发现了一个类狄拉克锥表面态,它被认为是一个没有拓扑保护的偶然狄拉克带。我们的研究结果排除了量子极限引起的线性带色散的非常规的大线性磁阻的原因。

英文摘要:

PtBi2 with a layered trigonal crystal structure was recently reported to exhibit an unconventional large linear magnetoresistance, while the mechanism involved is still elusive. Using high resolution angle-resolved photoemission spectroscopy, we present a systematic study on its bulk and surface electronic structure. Through careful comparison with first-principle calculations, our experiment distinguishes the low-lying bulk bands from entangled surface states, allowing the estimation of the real stoichiometry of samples. We find significant electron doping in PtBi2, implying a substantial Bi deficiency induced disorder therein. We discover a Dirac-cone-like surface state on the boundary of the Brillouin zone, which is identified as an accidental Dirac band without topological protection. Our findings exclude quantum-limit-induced linear band dispersion as the cause of the unconventional large linear magnetoresistance.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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