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arXiv 1606.05856cond-mat.str-elcond-mat.mes-hall
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单层TaS $_2$的晶体结构和电子结构

Crystalline and electronic structure of single-layer TaS$_2$

Charlotte E. Sanders, Maciej Dendzik, Arlette S. Ngankeu, Andreas Eich, Albert Bruix, Marco Bianchi, Jill A. Miwa, Bjørk Hammer, Alexander A. Khajetoorians, Philip Hofmann

摘要:

在Au(111)衬底上外延生长单层TaS $_2$。所得的二维晶体采用1H多晶型物。电子结构由角分辨光电子能谱确定,并发现与密度泛函理论计算非常一致。发现单层TaS $_2$是强n型掺杂的,载流子浓度为每晶胞0.3(1)个额外电子。扫描隧道显微镜在4.7K以下没有观察到超导或电荷密度波态。

英文摘要:

Single-layer TaS$_2$ is epitaxially grown on Au(111) substrates. The resulting two-dimensional crystals adopt the 1H polymorph. The electronic structure is determined by angle-resolved photoemission spectroscopy and found to be in excellent agreement with density functional theory calculations. The single layer TaS$_2$ is found to be strongly n-doped, with a carrier concentration of 0.3(1) extra electrons per unit cell. No superconducting or charge density wave state is observed by scanning tunneling microscopy at temperatures down to 4.7 K.

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