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arXiv 1606.01773cond-mat.mes-hall
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衬底表面极性声子对石墨烯中电子的拖曳

Drag of electrons in graphene by substrate surface polar phonons

S. V. Koniakhin, A. V. Nalitov

摘要:

已知通过基底的表面极性声子(SPP)的电子散射降低了它们在支撑的石墨烯中的迁移率。然而,没有实验证据表明SPP对石墨烯中热电现象的电子拖曳的贡献:石墨烯热电性与莫特定律表现出良好的一致性,这意味着扩散对热电性的贡献在宽范围的载流子密度和温度中占主导地位。在这里,我们发展了一个完整的理论,电子在石墨烯的牵引SPP。通过求解电子被表面等离子体散射的玻尔兹曼输运方程,推导出表面等离子体阻力对石墨烯热电势的贡献。相比,扩散热电势,得到的值似乎是一个数量级较低的各种基板。这可以解释为低占有数的SPP和短的平均自由程的声子源于他们的小群速度。我们的结论是,石墨烯的热电实验可以在莫特定律的框架内处理。

英文摘要:

It is known that electron scattering by surface polar phonons (SPPs) of the substrate reduces their mobility in supported graphene. However, there is no experimental evidence for contribution of drag of electrons by SPP to thermoelectric phenomena in graphene: graphene thermopower exhibits good agreement with Mott's law, which means that the diffusion contribution to the thermopower is dominant in a wide range of carrier densities and temperatures. Here we develop a complete theory of drag of electrons in graphene by SPP. By solving Boltzmann transport equation for electrons scattered by SPPs we derive SPP drag contribution to the thermopower in graphene. Compared to diffusion thermopower, obtained values appear to be one order of magnitude lower for various substrates. This can be explained by low occupation number of the SPPs and short mean free path of such phonons stemming from their small group velocity. We conclude that experiments on thermopower in graphene can be treated within the framework of Mott's law.

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