We study the role of dipolar interactions in the standard protocol used to achieve dynamic nuclear polarization (DNP). In the so-called spin-temperature regime, where the interactions establish an effective thermodynamic behavior in the out-of-equilibrium stationary state, we provide numerical predictions for the level of hyperpolarization. We show that nuclear spins equilibrate to the effective spin-temperature established among the electron spins of radicals, as expected from the quantum theory of thermalization. Moreover, we present an analytical technique to estimate the spin temperature, and thus, the nuclear hyperpolarization in the steady state, as a function of interaction strength and quenched disorder. This reproduces both our numerical data and experimental results. Our central finding is that the nuclear hyperpolarization increases steadily upon reducing the interaction strength (by diluting the radical density). Interestingly, the highest polarization is reached at a point where the establishment of a spin temperature is just about to break down due to the incipient many-body localization transition in the electron spin system.
Dynamic Nuclear Polarization (DNP) is to date the most effective technique to increase the nuclear polarization up to a factor $100,000$ opening disruptive perspectives for medical applications. In DNP, the nuclear spins are driven to an - out of equilibrium - hyperpolarized state by microwave saturation of the electron spins in interaction with them. Here we show that the electron dipolar interactions compete with the local magnetic fields resulting in two distinct dynamical phases: for strong interactions the electron spins equilibrate to an extremely low effective temperature that boosts DN…
The many-body localization transition in quasiperiodic systems has been extensively studied in recent ultracold atom experiments. At intermediate quasiperiodic potential strength, a surprising Griffiths-like regime with slow dynamics appears in the absence of random disorder and mobility edges. In this work, we study the interacting Aubry-Andre model, a prototype quasiperiodic system, as a function of incommensurate potential strength using a novel dynamical measure, information scrambling, in a large system of 200 lattice sites. Between the thermal phase and the many-body localized phase, we …
Entanglement is usually quantified by von Neumann entropy, but its properties are much more complex than what can be expressed with a single number. We show that the three distinct dynamical phases known as thermalization, Anderson localization, and many-body localization are marked by different patterns of the spectrum of the reduced density matrix for a state evolved after a quantum quench. While the entanglement spectrum displays Poisson statistics for the case of Anderson localization, it displays universal Wigner-Dyson statistics for both the cases of many-body localization and thermaliza…
We study quantum information scrambling, specifically the growth of Heisenberg operators, in large disordered spin chains using matrix product operator dynamics to scan across the thermalization-localization quantum phase transition. We observe ballistic operator growth for weak disorder, and a sharp transition to a phase with sub-ballistic operator spreading. The critical disorder strength for the ballistic to sub-ballistic transition is well below the many body localization phase transition, as determined from finite size scaling of energy eigenstate entanglement entropy in small chains. In …
We study the thermalizing properties of the mass-deformed SYK model, in a regime of parameters where the eigenstates are ergodically extended over just portions of the full Fock space, as an all-to-all toy model of many-body localization. Our numerical results strongly support the hypothesis that, although considerably delayed, thermalization is still present in this regime. Our results add to recent studies indicating that many-body localization should be interpreted as a strict Fock-space localization.
The many-body localized (MBL) phase is characterized by a complete set of quasi-local integrals of motion and area-law entanglement of excited eigenstates. We study the effect of non-Abelian continuous symmetries on MBL, considering the case of $SU(2)$ symmetric disordered spin chains. The $SU(2)$ symmetry imposes strong constraints on the entanglement structure of the eigenstates, precluding conventional MBL. We construct a fixed-point Hamiltonian, which realizes a non-ergodic (but non-MBL) phase characterized by eigenstates having logarithmic scaling of entanglement with the system size, as …
Many-body localization (MBL) is a phase of matter that is characterized by the absence of thermalization. Dynamical generation of a large number of local quantum numbers has been identified as one key characteristic of this phase, quite possibly the microscopic mechanism of breakdown of thermalization and the phase transition itself. We formulate a robust algorithm, based on Wegner Wilson flow (WWF) renormalization, for computing these conserved quantities and their interactions. We present evidence for the existence of distinct fixed point distributions of the latter: a flat "white noise" dis…
Thermalization in many-body systems can be inhibited by the application of a linearly increasing potential, which is known as Stark many-body localization. Here we investigate the fate of this phenomenon on a two-dimensional disorder-free lattice with up to $24 \times 6$ sites. Similar to the one-dimensional case, "density-polarized" regions can act as bottlenecks for transport and thermalization on laboratory timescales. However, compared to the one-dimensional case, a substantially stronger potential gradient is needed to prevent thermalization when an extra spatial dimension is involved. Th…
We study the quantum thermalization and information scrambling dynamics of an experimentally realizable quantum spin model with homogeneous XX-type all-to-all interactions and random local potentials. We identify the thermalization-localization transition by changing the disorder strength, under a proper all-to-all interaction strength. The scrambling dynamics in the localization phase shows novel behaviors distinct from that of local models. The operator scrambling grows almost equally fast in both phases. In the thermal phase, we show there exhibits fast scrambling without appealing to the s…
Polarization selectivity of light-field-induced charge localization was investigated in an organic metal alpha-(BEDT-TTF)2I3 with a triangular lattice. Dependences of transient reflectivity spectra on polarizations of the 7-fs pump and probe lights indicate that a short-range charge order (CO) is efficiently induced from the metallic phase for the pump polarization perpendicular to the 1010-type CO axis. Numerical solution of a time-dependent Schrodinger equation clarified that the 1010-CO is induced by field-induced re-distribution of charges cooperating with competing inter-site Coulomb repu…
Localization due to the presence of disorder has proven crucial for our current understanding of relaxation in isolated quantum systems. The many-body localized phase constitutes a robust alternative to the thermalization of complex interacting systems, but recently the importance of disorder has been brought into question. Starting from translationally invariant $(1 + 1)$-dimensional quantum electrodynamics, we modify the dynamics of the gauge field and reveal a mechanism of disorder-free localization. We consider two different discretizations of the continuum model resulting in a free-fermio…
We review the physics of many-body localization in models with incommensurate potentials. In particular, we consider one-dimensional quasiperiodic models with single-particle mobility edges. Although a conventional perspective suggests that delocalized states act as a thermalizing bath for the localized states in the presence of of interactions, there is evidence that such systems can display non-ergodicity. This is in part due to the fact that the delocalized states do not have any kind of protection due to symmetry or topology and are thus susceptible to localization. A study of non-interact…
We numerically explore the many body localization (MBL) transition through the lens of the {\it entanglement spectrum}. While a direct transition from localization to thermalization is believed to obtain in the thermodynamic limit (the exact details of which remain an open problem), in finite system sizes there exists an intermediate `quantum critical' regime. Previous numerical investigations have explored the crossover from thermalization to criticality, and have used this to place a numerical {\it lower} bound on the critical disorder strength for MBL. A careful analysis of the {\it high en…
In two spatial dimensions, topological order is robust for static deformations at zero temperature, while it is fragile at any finite temperature. How robust is topological order after a quantum quench? In this paper we show that topological order thermalizes under the unitary evolution after a quantum quench. If the quench preserves gauge symmetry, there is a residual topological entropy exactly like in the finite temperature case. We obtain this result by studying the time evolution of the topological 2-Rényi entropy in a fully analytical, exact way. These techniques can be then applied to s…
This paper describes experiments utilizing a unique property of electron-glasses to gain information on the fundamental nature of the interacting Anderson-localized phase. The methodology is based on measuring the energy absorbed by the electronic system from alternating electromagnetic fields as function of their frequency. Experiments on three-dimensional (3D) amorphous indium-oxide films suggest that, in the strongly localized regime, the energy spectrum is discrete and inelastic electron-electron events are strongly suppressed. These results imply that, at low temperatures, electron therma…
Many-body localization (MBL) is currently a hot issue of interacting systems, in which quantum mechanics overcomes thermalization of statistical mechanics. Like Anderson localization of non-interacting electrons, disorders are usually crucial in engineering the quantum interference in MBL. For translation invariant systems, however, the breakdown of eigenstate thermalization hypothesis due to a \emph{pure} many-body quantum effect is still unclear. Here we demonstrate a possible MBL phenomenon without disorder, which emerges in a lightly doped Hubbard model with very strong interaction. By mea…
Thermalization of random-field Heisenberg spin chain is probed by time evolution of density correlation functions. Studying the impacts of average energies of initial product states on dynamics of the system, we provide arguments in favor of the existence of a mobility edge in the large system-size limit.
We study the dynamics of an interacting quantum spin chain under the application of a linearly increasing field. This model exhibits a type of localization known as Stark many-body localization. The dynamics shows a strong dependence on the initial conditions, indicating that the system violates the conventional ("strong") eigenstate thermalization hypothesis at any finite gradient of the field. This is contrary to reports of a numerically observed ergodic phase. Therefore, the localization is crucially distinct from disorder-driven many-body localization, in agreement with recent predictions …
We study the statistical and dynamical aspects of a translation-invariant Hamiltonian, without quench disorder, as an example of the manifestation of the phenomenon of many-body localization. This is characterized by the breakdown of thermalization and by information preservation of initial preparations at long times. To realize this, we use quasi-periodic long-range interactions, which are now achievable in high-finesse cavity experiments, to find evidence suggestive of a divergent time-scale in which charge inhomogeneities in the initial state survive asymptotically. This is reminiscent of a…
The concept of geometrical frustration has led to rich insights into condensed matter physics, especially as a mechansim to produce exotic low energy states of matter. Here we show that frustration provides a natural vehicle to generate models exhibiting anomalous thermalization of various types within high energy states. We consider three classes of non-integrable frustrated spin models: (I) systems with local conserved quantities where the number of symmetry sectors grows exponentially with the system size but more slowly than the Hilbert space dimension, (II) systems with exact eigenstates …
Probing many-body localization crossover in quasiperiodic Floquet circuits on a quantum processor
RIKEN Center for Computational Science（理化学研究所计算科学中心）；RIKEN Center for Quantum Computing（理化学研究所量子计算中心）；RIKEN Center for Interdisciplinary Theoretical and Mathematical Sciences（理化学研究所交叉理论与数学科学中心）；RIKEN Pioneering Research Institute（理化学研究所先驱研究所）；Jožef Stefan Institute（约热·斯特凡研究所）；University of Ljubljana（卢布尔雅那大学）
Many-body localization (MBL) addresses the absence of thermalization in interacting quantum systems, with non-ergodic high-energy eigenstates behaving as ground states, only area-law entangled. However, computing highly excited many-body eigenstates using exact methods is very challenging. Instead, we show that one can address high-energy MBL physics using ground-state methods, which are much more amenable to many efficient algorithms. We find that a localized many-body ground state of a given interacting disordered Hamiltonian $\mathcal{H}_0$ is a very good approximation for a high-energy eig…
The random field S=1/2 Heisenberg chain exhibits a dynamical many body localization transition at a critical disorder strength, which depends on the energy density. At weak disorder, the eigenstate thermalization hypothesis (ETH) is fulfilled on average, making local observables smooth functions of energy, whose eigenstate-to-eigenstate fluctuations decrease exponentially with system size. We demonstrate the validity of ETH in the thermal phase as well as its breakdown in the localized phase and show that rare states exist which do not strictly follow ETH, becoming more frequent closer to the …
We introduce a solvable model of driven fermions that elucidates the role of the localization transition in driven disordered magnets, as used in the context of dynamic nuclear polarization. Instead of spins, we study a set of non-interacting fermions that are coupled locally to nuclear spins and tend to hyperpolarize them. The induced hyperpolarization is a fingerprint of the driven steady state of the fermions, which undergo an Anderson Localization (AL) transition upon increasing the disorder. Our central result is that the maximal hyperpolarization level is always found close to the locali…
We study the real-time dynamics of local occupation numbers in a one-dimensional model of spinless fermions with a random on-site potential for a certain class of initial states. The latter are thermal (mixed or pure) states of the model in the presence of an additional static force, but become non-equilibrium states after a sudden removal of this static force. For this class and high temperatures, we show that the induced dynamics is given by a single correlation function at equilibrium, independent of the initial expectation values being prepared close to equilibrium (by a weak static force)…
In quantum statistical mechanics, closed many-body systems that do not exhibit thermalization after an arbitrarily long time in spite of the presence of interactions are called as many-body localized systems, and recently have been vigorously investigated. After a brief review of this topic, we consider a many-body interacting quantum system in one dimension, which has conformal symmetry and integrability. We exactly solve the system and discuss its thermal or non-thermal behavior.
Sufficient disorder is believed to localize static and periodically-driven interacting chains. With quasiperiodic driving by $D$ incommensurate tones, the fate of this many-body localization (MBL) is unknown. We argue that randomly disordered MBL exists for $D=2$, but not for $D\geq 3$. Specifically, a putative two-tone driven MBL chain is neither destabilized by thermal avalanches seeded by rare thermal regions, nor by the proliferation of long-range many-body resonances. For $D\geq 3$, however, sufficiently large thermal regions have continuous local spectra and slowly thermalize the entire …
Thermal and many-body localized phases are separated by a dynamical phase transition of a new kind. We analyze the distribution of off-diagonal matrix elements of local operators across the many-body localization transition (MBLT) in a disordered spin chain, and use it to characterize the breakdown of the eigenstate thermalization hypothesis and to extract the many-body Thouless energy. We find a wide critical region around the MBLT, where Thouless energy becomes smaller than the level spacing, while matrix elements show critical dependence on the energy difference. In the same region, matrix …
Stark many-body localized (SMBL) systems have been shown both numerically and experimentally to have Bloch many-body oscillations, quantum many-body scars, and fragmentation in the large field tilt limit. Likewise, they are believed to show localization similar to disordered MBL. We explain and analytically prove all these observations by rigorously showing the existence of novel algebraic structures that are exponentially stable in time, which we call dynamical l-bits. Moreover, we show that many-body Bloch oscillations persist even at infinite temperature for exponentially long-times. We num…
Many-body localization (MBL) describes a quantum phase where an isolated interacting system subject to sufficient disorder displays non-ergodic behavior, evading thermal equilibrium that occurs under its own dynamics. Previously, the thermalization-MBL transition has been largely characterized with the growth of disorder. Here, we explore a new axis, reporting on an energy resolved MBL transition using a 19-qubit programmable superconducting processor, which enables precise control and flexibility of both disorder strength and initial state preparations. We observe that the onset of localizati…
Stark many-body localization (SMBL) is a phenomenon observed in interacting systems with a nearly uniform spatial gradient applied field. Contrasting to the traditional many-body localization phenomenon, SMBL does not require disorder. Here we investigate SMBL in a spin-$1/2$ described by a Heisenberg model including a next-nearest-neighbor exchange coupling. By employing an exact diagonalization approach and time evolution calculation we analyze both level spacing ratio (LSR) statistics of the Hamiltonian model as well as the dynamics of the system from a given initial state. Our results reve…
Many-body localization (MBL), characterized by the absence of thermalization and the violation of conventional thermodynamics, has elicited much interest both as a fundamental physical phenomenon and for practical applications in quantum information. A phenomenological model, which describes the system using a complete set of local integrals of motion (LIOMs), provides a powerful tool to understand MBL, but can be usually only computed approximately. Here we explicitly compute a complete set of LIOMs with a non-perturbative approach, by maximizing the overlap between LIOMs and physical spin op…
We consider a random time evolution operator composed of a circuit of random unitaries coupling even and odd neighboring spins on a chain in turn. In spirit of Floquet evolution, the circuit is time-periodic; each timestep is repeated with the same random instances. We obtain analytical results for arbitrary local Hilbert space dimension d: On a single site, average time evolution acts as a depolarising channel. In the spin 1/2 (d=2) case, this is further quantified numerically. For that, we develop a new numerical method that reduces complexity by an exponential factor. Haar-distributed unita…
