An experimental technique for the indirect manipulation and detection of electron spins entangled in two-dimensional magnetoexcitons has been developed. The kinetics of the spin relaxation has been investigated. Photoexcited spin-magnetoexcitons were found to exhibit extremely slow relaxation in specific quantum Hall systems, fabricated in high mobility GaAs/AlGaAs structures, namely, the relaxation time reaches values over one hundred microseconds. A qualitative explanation of this spin-relaxation kinetics is presented. Its temperature and magnetic field dependencies are discussed within the available theoretical framework.
Avoided crossing of the emission lines of a nearly free positive trion and a cyclotron replica of an exciton bound to an interface acceptor has been observed in the magneto-photoluminescence spectra of p-doped GaAs quantum wells. Identification of the localized state depended on the precise mapping of the anti-crossing pattern. The underlying coupling is caused by an exciton transfer combined with a resonant cyclotron excitation of an additional hole. The emission spectrum of the resulting magnetically tunable coherent state probes weak localization in the quantum well.
We report on a study of the zero-momentum cyclotron spin-flip excitation in the V=2 quantum Hall regime. Using the excitonic representation the excitation energy is calculated up to the second order Coulomb corrections. A considerable negative exchange shift relative to the cyclotron gap is established for cyclotron spin-flip excitations in the the spin-unpolarized electronic system. Under these conditions this type of states presents the {\it lowest-energy} excitations. For a fixed filling factor V=2 the energy shift is independent of the magnetic field which is in agreement with recent exper…
We report on the calculation of the cyclotron spin-flip excitation (CSFE) in a spin-polarized quantum Hall system at unit filling. This mode has a double-exciton component which contributes to the CSFE correlation energy but can not be found by means of a mean field approach. The result is compared with available experimental data.
The cyclotron spin-flip modes of spin unpolarized integer quantum Hall states ($ν=2,4$) have been studied with inelastic light scattering. The energy of these modes is significantly smaller compared to the bare cyclotron gap. Second order exchange corrections are held responsible for a negative energy contribution and render these modes the lowest energy excitations of unpolarized integer quantum Hall states.
I develop a theory of combined exciton-cyclotron resonance (ExCR) in a low-density two-dimensional electron gas in high magnetic fields. In the presence of excess electrons an incident photon creates an exciton and simultaneously excites one electron to higher-lying Landau levels. I derive exact ExCR selection rules that follow from the existing dynamical symmetries, magnetic translations and rotations about the magnetic field axis. The nature of the final states in the ExCR is elucidated. The relation between ExCR and shake-up processes is discussed. The double-peak ExCR structure for transit…
Time-resolved photoluminescence measurements show that the decay time for charged excitons in a GaAs two-dimensional electron gas increases by an order of magnitude at high magnetic fields. Unlike neutral excitons, the charged exciton center-of-mass is spatially confined in a ``magnetically-adjustable quantum dot'' by the cyclotron orbit and the quantum well. The inhibited recombination is explained by a reduced phase coherence volume of the magnetically-confined charged excitons.
We find unexpected low energy excitations of fully spin-polarized composite-fermion ferromagnets in the fractional quantum Hall liquid, resulting from a complex interplay between a topological order manifesting through new energy levels and a magnetic order due to spin polarization. The lowest energy modes, which involve spin reversal, are remarkable in displaying unconventional negative dispersion at small momenta followed by a deep roton minimum at larger momenta. This behavior results from a nontrivial mixing of spin-wave and spin-flip modes creating a spin-flip excitonic state of composite…
Motivated by experimental developments introducing the concept of spin-orbit separation, we study the real-space time evolution of an excitonic wave-packet using a two-orbital Hubbard model. The exciton is created by exciting an electron from a lower energy half-filled orbital to a higher energy empty orbital. We carry out the real-time dynamics of the resulting excitonic wave-packet, using the time-dependent density matrix renormalization group method. We find clear evidence of charge-spin and spin-orbit separation in real-space, by tracking the time evolution of local observables. We show th…
Transformation of Coulomb interaction terms to the pseudo-orbital basis constituted by $J=1/2$ and $3/2$ states arising from spin-orbit coupling provides a versatile tool. This formalism is applied to investigate magnetic anisotropy effects on low-energy spin-wave excitations as well as high-energy spin-orbit exciton modes in $\rm Sr_2 Ir O_4$. The Hund's coupling term explictly yields easy-plane anisotropy, resulting in gapless (in-plane) and gapped (out-of-plane) modes, in agreement with recent resonant inelastic x-ray scattering (RIXS) measurements. The collective mode of inter-orbital, spi…
Cyclotron spin-flip excitation in a nu=2 quantum Hall system, being separated from the ground state by a slightly smaller gap than the cyclotron energy and from upper magnetoplasma excitation by the Coulomb gap [S. Dickmann and I.V. Kukushkin, Phys. Rev. B 71, 241310(R) (2005) ; L.V. Kulik, I.V. Kukushkin, S. Dickmann, V.E. Kirpichev, A.B. Vankov, A.L. Parakhonsky, J.H. Smet, K. von Klitzing, and W. Wegscheider, Phys. Rev. B 72, 073304 (2005)] cannot relax in a purely electronic way except only with the emission of a shortwave acoustic phonon (k~3*10^7/cm). As a result, relaxation in a modern …
Spin-flip excitations in a quantum Hall electron system at fixed filling factor nu=2 are modelled and studied under conditions of a strong Coulomb interaction when the `Landau level mixing' is a dominant factor determining the excitation energy. The `one-exciton' approach used for the purely electronic excitations in question allows us to describe the Stoner transition from the unpolarized/paramgnet state to the polarized/ferromagnet one. The theoretical results are compared with the available experimental data.
Manipulation of localized excitons in CrPS$_4$ by temperature and magnetic field
National University of Singapore（新加坡国立大学）；National Laboratory of the Rockies（落基山国家实验室）；Laboratoire National des Champs Magnétiques Intenses, LNCMI-EMFL, CNRS UPR3228,Univ. Grenoble Alpes, Univ. Toulouse, Univ. Toulouse 3, INSA-T（强磁场国家实验室，LNCMI-EMFL，CNRS UPR3228，格勒诺布尔阿尔卑斯大学，图卢兹大学，图卢兹第三大学，法国国家高等理工学院）；University of Chemistry and Technology Prague（布拉格化工大学）；King’s College London（伦敦国王学院）
