In this paper we study an archetypical scenario in which repulsive Casimir-Polder forces between an atom or molecule and two macroscopic bodies can be achieved. This is an extension of previous studies of the interaction between a polarizable atom and a wedge, in which repulsion occurs if the atom is sufficiently anisotropic and close enough to the symmetry plane of the wedge. A similar repulsion occurs if such an atom passes a thin cylinder or a wire. An obvious extension is to compute the interaction between such an atom and two facing wedges, which includes as a special case the interaction of an atom with a conducting screen possessing a slit, or between two parallel wires. To this end we further extend the electromagnetic multiple-scattering formalism for three-body interactions. To test this machinery we reinvestigate the interaction of a polarizable atom between two parallel conducting plates. In that case, three-body effects are shown to be small, and are dominated by three- and four-scattering terms. The atom-wedge calculation is illustrated by an analogous scalar situation, described in the Appendix. The wedge-wedge-atom geometry is difficult to analyze because this is a scale-free problem. But it is not so hard to investigate the three-body corrections to the interaction between an anisotropic atom or nanoparticle and a pair of parallel conducting cylinders, and show that the three-body effects are very small and do not affect the Casimir-Polder repulsion at large distances between the cylinders. Finally, we consider whether such highly anisotropic atoms needed for repulsion are practically realizable. Since this appears rather difficult to accomplish, it may be more feasible to observe such effects with highly anisotropic nano particles.
Various applications of the multiple scattering technique to calculating Casimir energy are described. These include the interaction between dilute bodies of various sizes and shapes, temperature dependence, interactions with multilayered and corrugated bodies, and new examples of exactly solvable separable bodies.
A novel formalism for the evaluation of the Casimir-Polder potential in an arbitrary gauge of vector potentials is introduced. The ground state energy of a neutral atom in the presence of an infinite two-dimensional plane with Chern-Simons interaction is derived at zero temperature. The essential feature of the result is its dependence on the antisymmetric part of a dipole moment correlation function.
It has been increasingly becoming clear that Casimir and Casimir-Polder entropies may be negative in certain regions of temperature and separation. In fact, the occurrence of negative entropy seems to be a nearly ubiquitous phenomenon. This is most highlighted in the quantum vacuum interaction of a nanoparticle with a conducting plate or between two nanoparticles. It has been argued that this phenomenon does not violate physical intuition, since the total entropy, including the self-entropies of the plate and the nanoparticle, should be positive. New calculations, in fact, seem to bear this ou…
Casimir-Polder interactions are considered in an inhomogeneous, dispersive background. We consider both the interaction between a polarizable atom and a perfectly conducting wall, and between such an atom and a plane interface between two different inhomogeneous dielectric media. Renormalization is achieved by subtracting the interaction with the local inhomogeneous medium by itself. The results are expressed in general form, and generalize the Dzyaloshinskii-Lifshitz-Pitaevskii interaction between a spatially homogeneous dielectric interface and a polarizable atom.
This Resource Letter provides a guide to the literature on van der Waals and Casimir-Polder forces. Journal articles, books, and other documents are cited on the following topics: van der Waals forces, retarded dispersion forces or Casimir-Polder forces between atoms or molecules, Casimir-Polder forces between a molecule and a dielectric or conducting body, the summation of Casimir-Polder forces as leading to the Casimir and Lifshitz forces between conducting and dielectric bodies, Casimir friction, applications to nanotechnology, the nature of the quantum vacuum, and experimental tests of the…
We derive the exact Casimir-Polder potential for a polarizable microparticle inside an ideal metal cylindrical shell using the Green function method. The exact Casimir-Polder potential for a particle outside a shell, obtained recently by using the Hamiltonian approach, is rederived and confirmed. The exact quantum field theoretical result is compared with that obtained using the proximity force approximation and a very good agreement is demonstrated at separations below 0.1$R$, where $R$ is the radius of the cylinder. The developed methods are applicable in the theory of topological defects.
Casimir and Casimir-Polder repulsion have been known for more than 50 years. The general "Lifshitz" configuration of parallel semi-infinite dielectric slabs permits repulsion if they are separated by a dielectric fluid that has a value of permittivity that is intermediate between those of the dielectric slabs. This was indirectly confirmed in the 1970s, and more directly by Capasso's group recently. It has also been known for many years that electrically and magnetically polarizable bodies can experience a repulsive quantum vacuum force. More amenable to practical application are situations wh…
We propose a method to separate enantiomers using parity violation in the Casimir-Polder potential between chiral mirrors and chiral molecules. The proposed setup involves a molecular beam composed of chiral molecules passing through a planar cavity consisting of two chiral mirrors. Enantiomers of opposite handedness are deflected differently due to a chiral dependence of the Casimir-Polder potential resulting in the separation of the enantiomers. Our setup provides an alternative experimental tool for enantiomer separation, as well as shedding light on the fundamental properties of the Casimi…
As part of our program to develop the description of three-body effects in quantum vacuum phenomena, we study the three-body interaction of two anisotropically polarizable atoms with a perfect electrically conducting plate, a generalization of earlier work. Three- and four-scattering effects are important, and lead to nonmonotonic behavior.
We study the nonequilibrium Casimir-Polder force on an atom prepared in an incoherent superposition of internal energy-eigenstates, which is placed in a magnetoelectric environment of nonuniform temperature. After solving the coupled atom--field dynamics within the framework of macroscopic quantum electrodynamics, we derive a general expression for the thermal Casimir-Polder force.
The Casimir and Casimir-Polder interactions are investigated in a stack of equally spaced graphene layers. The optical response of the individual graphene is taken into account using gauge invariant components of the polarization tensor extended to the whole complex frequency plane. The planar symmetry for the electromagnetic boundary conditions is further used to obtain explicit forms for the Casimir energy stored in the stack and the Casimir-Polder energy between an atom above the stack. Our calculations show that these fluctuation induced interactions experience strong thermal effects due t…
Recently, the topic of Casimir repulsion has received a great deal of attention, largely because of the possibility of technological application. The general subject has a long history, going back to the self-repulsion of a conducting spherical shell and the repulsion between a perfect electric conductor and a perfect magnetic conductor. Recently it has been observed that repulsion can be achieved between ordinary conducting bodies, provided sufficient anisotropy is present. For example, an anisotropic polarizable atom can be repelled near an aperture in a conducting plate. Here we provide new…
It has always been conventionally understood that, in the dilute limit, the Casimir energy of interaction between bodies or the Casimir self-energy of a dielectric body could be identified with the sum of the van der Waals or Casimir-Polder energies of the constituents of the bodies. Recently, this proposition for self-energies has been challenged by Avni and Leonhardt [Ann.\ Phys.\ {\bf 395}, 326 (2018)], who find that the energy or self-stress of a homogeneous dielectric ball with permittivity $\varepsilon$ begins with a term of order $\varepsilon-1$. Here we demonstrate that this cannot be …
We discuss the scalar analogue of the Casimir-Polder force between a sphere and a uniaxially corrugated surface with Dirichlet boundary conditions. Presenting a formulation that is nonperturbative in the height profile of the surface, we give explicit numerical results for a sinuosoidal corrugation profile.
We propose a new method to measure Casimir-Polder force in an optical cavity by means of atomic excitations. We utilize a framework in which Unruh-DeWitt Hamiltonian mimics the full matter-field interaction and find a connection between the excitation rate of the two-level atom and the Casimir-Polder energy, allowing to map one onto the other. We argue that such a realization opens a route to study Casimir-Polder potentials through measurement of excited state's population in large, spatially compact ensembles of atoms.
We study the effect of two non-interacting impurity atoms near by a one-dimensional nanowire, which is modeled as a tight-binding hopping model. The virtual single-electron hopping between two impurities will induce an additional energy depending on the distance of two impurities, which gives a electronic Casimir-Polder effect. We find that the Casimir-Polder force between the two impurities decreases with the impurity-impurity distance exponentially. And the effects of nanowire and finite temperature on the Casimir-Polder force are also discussed in detail, respectively.
We consider the three-body Casimir-Polder interaction between three atoms during their dynamical self-dressing. We show that the time-dependent three-body Casimir-Polder interaction energy displays nonlocal features related to quantum properties of the electromagnetic field and to the nonlocality of spatial field correlations. We discuss the measurability of this intriguing phenomenon and its relation with the usual concept of stationary three-body forces.
We consider vacuum fluctuations of the quantum electromagnetic field in the presence of an infinite and perfectly conducting plate. We evaluate how the change of vacuum fluctuations due to the plate modifies the Casimir-Polder potential between two atoms placed near the plate. We use two different methods to evaluate the Casimir-Polder potential in the presence of the plate. They also give new insights on the role of boundary conditions in the Casimir-Polder interatomic potential, as well as indications for possible generalizations to more complicated boundary conditions.
We show that the Casimir-Polder interaction may induce coherent oscillations between degenerate atomic states. We illustrate this effect by computing the Casimir-Polder induced Rabi frequency on a $^{87}$Rb atom as it interacts with a reflecting surface. The atom oscillates between two Zeeman sublevels of its ground state undergoing a periodic exchange of angular momentum with the vacuum photons.
The three-body Casimir-Polder potential between one excited and two ground-state atoms is evaluated. A physical model based on the dressed field correlations of vacuum fluctuations is used, generalizing a model previously introduced for three ground-state atoms. Although the three-body potential with one excited atom is already known in the literature, our model gives new insights on the nature of non-additive Casimir-Polder forces with one or more excited atoms.
We investigate the Casimir-Polder force acting on a polarizable microparticle in the geometry of a straight cosmic string. In order to develop this analysis we evaluate the electromagnetic field Green tensor on the imaginary frequency axis. The expression for the Casimir-Polder force is derived in the general case of anisotropic polarizability. In dependence of the eigenvalues for the polarizability tensor and of the orientation of its principal axes, the Casimir-Polder force can be either repulsive or attractive. Moreover, there are situations where the force changes the sign with separation.…
Making use of the quantum correlators associated with the Maxwell field vacuum distorted by the presence of plane parallel material surfaces we derive the Casimir-Polder interaction in the presence of plane parallel conducting walls and in the presence of a conducting wall and a magnetically permeable one.
A time-dependent Casimir-Polder force is shown to arise during the time evolution of a partially dressed two-level atom. The partially dressed atom is obtained by a rapid change of an atomic parameter such as its transition frequency, due to the action of some external agent. The electromagnetic field fluctuations around the atom, averaged over the solid angle for simplicity, are calculated as a function of time, and it is shown that the interaction energy with a second atom yields a dynamical Casimir-Polder potential between the two atoms.
We develop a dynamical approach to study the Casimir-Polder force between a initially bare molecule and a magnetodielectric body at finite temperature. Switching on the interaction between the molecule and the field at a particular time, we study the resulting temporal evolution of the Casimir-Polder interaction. The dynamical self-dressing of the molecule and its population-induced dynamics are accounted for and discussed. In particular, we find that the Casimir-Polder force between a chiral molecule and a perfect mirror oscillates in time with a frequency related to the molecular transition …
We critically discuss the common belief that the thermal Casimir-Polder force can always be represented as a Matsubara sum, as it is true for the Casimir force. On the contrary, an exact treatment of the atom-field coupling reveals that for a ground-state atom, terms associated with virtual-photon absorption contribute to the force which are identified as a signature of non-equilibrium dynamics. Even the equilibrium force on a thermalized atom or molecule may be overestimated when using the ground-state polarizability instead of its thermal counterpart.
We consider the Casimir-Polder interaction between two atoms, one in the ground state and the other in its excited state. The interaction is time-dependent for this system, because of the dynamical self-dressing and the spontaneous decay of the excited atom. We calculate the dynamical Casimir-Polder potential between the two atoms using an effective Hamiltonian approach. The results obtained and their physical meaning are discussed and compared with previous results based on a time-independent approach which uses a non-normalizable dressed state for the excited atom.
We propose a method to probe dispersive atom-surface interactions by measuring via two-photon Bragg spectroscopy the dynamic structure factor of a Bose-Einstein condensate above corrugated surfaces. This method takes advantage of the condensate coherence to reveal the spatial Fourier components of the lateral Casimir-Polder interaction energy.
An ultracold atom above a horizontal mirror experiences quantum reflection from the attractive Casimir-Polder interaction, which holds it against gravity and leads to quantum levitation states. We analyze this system by using a Liouville transformation of the Schrödinger equation and a Langer coordinate adapted to problems with a classical turning point. Reflection on the Casimir-Polder attractive well is replaced by reflection on a repulsive wall and the problem is then viewed as an ultracold atom trapped inside a cavity with gravity and Casimir-Polder potentials acting respectively as top an…
We use a derivative expansion for gently curved surfaces to compute the leading and the next-to-leading curvature corrections to the Casimir-Polder interaction between a polarizable small particle and a non-planar surface. While our methods apply to any homogeneous and isotropic surface, explicit results are presented here for perfect conductors. We show that the derivative expansion of the Casimir-Polder potential follows from a resummation of its perturbative series, for small in-plane momenta. We consider the retarded, non-retarded and classical high temperature limits.
Using a recently developed theory of the Casimir force (Raabe C and Welsch D-G 2005 Phys. Rev. A 71 013814), we calculate the force that acts on a plate in front of a planar wall and the force that acts on the plate in the case where the plate is part of matter that fills the space in front of the wall. We show that in the limit of a dielectric plate whose permittivity is close to unity, the force obtained in the former case reduces to the ordinary, i.e., unscreened Casimir-Polder force acting on isolated atoms. In the latter case, the theory yields the Casimir-Polder force that is screened by…
Within leading-order perturbation theory, the Casimir-Polder potential of a ground-state atom placed within an arbitrary arrangement of dispersing and absorbing linear bodies can be expressed in terms of the polarizability of the atom and the scattering Green tensor of the body-assisted electromagnetic field. Based on a Born series of the Green tensor, a systematic expansion of the Casimir-Polder potential in powers of the susceptibilities of the bodies is presented. The Born expansion is used to show how and under which conditions the Casimir-Polder force can be related to microscopic many-at…
Casimir-Polder potential is investigated for a polarizable microparticle in the geometry of a straight cosmic string with a metallic cylindrical shell. The electromagnetic field Green tensor is evaluated on the imaginary frequency axis. The expressions for the Casimir-Polder potential is derived in the general case of anisotropic polarizability for the both interior and exterior regions of the shell. The potential is decomposed into pure string and shell-induced parts. The latter dominates for points near the shell, whereas the pure string part is dominant near the string and at large distance…
We develop a new theory for Casimir-Lifshitz and Casimir-Polder interactions with semiconductor surfaces that takes into account charge drift in the bulk material. The corresponding frequency-dependent dispersion relations describe a crossover between Lifshitz results for dielectrics and for good conductors. In the quasi-static limit, our calculated reflection amplitudes coincide with those recently computed to account for Debye screening in the thermal Lifshitz force with conducting surfaces with small density of carriers.
We find the low-temperature behavior of the Casimir-Polder free energy for a polarizable and magnetizable atom interacting with a plate made of ferromagnetic dielectric material. It is shown that the corresponding Casimir-Polder entropy goes to zero with vanishing temperature, i.e., the Nernst heat theorem is satisfied, if the dc conductivity of the plate material is disregarded in calculations. If the dc conductivity is taken into account, the Nernst theorem is violated. These results are discussed in light of recent experiments.
We review different aspects of the atom-atom and atom-wall Casimir-Polder forces. We first discuss the role of a boundary condition on the interatomic Casimir-Polder potential between two ground-state atoms, and give a physically transparent interpretation of the results in terms of vacuum fluctuations and image atomic dipoles. We then discuss the known atom-wall Casimir-Polder force for ground- and excited-state atoms, using a different method which is also suited for extension to time-dependent situations. Finally, we consider the fluctuation of the Casimir-Polder force between a ground-stat…
We investigate the magnetic dipole coupling between a metallic surface and an atom in a thermal state, ground state and excited hyperine state. This interaction results in a repulsive correction and - unlike the electrical dipole contribution - depends sensitively on the Ohmic dissipation in the material.
We investigate how the combination of nonequilibrium effects and material properties impacts on the Casimir-Polder interaction between an atom and a surface. By addressing systems with temperature inhomogeneities and laser interactions, we show that nonmonotonous energetic landscapes can be produced where barriers and minima appear. Our treatment provides a self-consistent quantum theoretical framework for investigating the properties of a class of nonequilibrium atom-surface interactions.
We investigate theoretically the Casimir-Polder potential of an atom which is driven by a laser field close to a surface. This problem is addressed in the framework of macroscopic quantum electrodynamics using the Green's tensor formalism and we distinguish between two different approaches, a perturbative ansatz and a method based on Bloch equations. We apply our results to a concrete example, namely an atom close to a perfectly conducting mirror, and create a scenario where the tunable Casimir-Polder potential becomes similar to the respective potential of an undriven atom due to fluctuating …
We study the resonant Casimir--Polder potential of an excited atom near a half space containing magneto-electric meta-material of various kinds on the basis of macroscopic quantum electrodynamics. Analytical results are obtained in the nonretarded and retarded distance regimes and numerical examples are given. We compare our findings with the potential of an excited atom near a left-handed superlens.
The problem of nonlocality in the dynamical three-body Casimir-Polder interaction between an initially excited and two ground-state atoms is considered. It is shown that the nonlocal spatial correlations of the field emitted by the excited atom during the initial part of its spontaneous decay may become manifest in the three-body interaction. The observability of this new phenomenon is discussed.
Atom-surface forces using excited states have a host of compelling applications, including repulsive and lateral forces. However, such states can be fragile and difficult to prepare. Here we report an explicit normal-mode based calculation of the Casimir-Polder potential between a ground-state atom and a non-dispersive surface in the presence of an external quantised field. The potential we derive shares some features with that of excited-state Casimir-Polder forces even though we consider a ground-state atom. Our work provides a physically transparent and intuitive picture of driven Casimir-P…
The low temperature expansion of the free energy of atom/plane system is considered for general symmetric form of tensor conductivity of the plane. It is shown that the first correction is proportional to second order of the temperature $\sim T^2$ and comes from TM mode. The agreement of the expansion and exact expressions for different models of conductivity is numerically demonstrated.
We consider the quantum fluctuations of the Casimir-Polder force between a neutral atom and a perfectly conducting wall in the ground state of the system. In order to obtain the atom-wall force fluctuation we first define an operator directly associated to the force experienced by the atom considered as a polarizable body in an electromagnetic field, and we use a time-averaged force operator in order to avoid ultraviolet divergences appearing in the fluctuation of the force. This time-averaged force operator takes into account that any measurement involves a finite time. We also calculate the …
In this paper we calculate the Casimir-Polder force density (force per unit area acting on the elements of the surface) on a metallic plate placed in front of a neutral atom. To obtain the force density we use the quantum operator associated to the electromagnetic stress tensor. We explicitly show that the integral of this force density over the plate reproduces the total force acting on the plate. This result shows that, although the force is obtained as a sum of surface element-atom contributions, the stress-tensor method includes also nonadditive components of Casimir-Polder forces in the e…
We develop the scattering approach to calculate the exact dispersive Casimir-Polder potential between a ground-state atom and a rectangular grating. Our formalism allows, in principle, for arbitrary values of the grating amplitude and period, and of the atom-grating distance. We compute numerically the potential for a Rb atom on top of a Si grating and compare the results with the potential for a flat surface taken at the local atom-surface distance (proximity force approximation). Except for very short separation distances, the potential is nearly sinusoidal along the direction transverse to …
We study the Casimir-Polder interaction at finite temperatures between a polarizable small, anisotropic particle and a non-planar surface using a derivative expansion. We obtain the leading and the next-to-leading curvature corrections to the interaction for low and high temperatures. Explicit results are provided for the retarded limit in the presence of a perfectly conducting surface.
We consider the out-of-thermal-equilibrium Casimir-Polder interaction between atoms of He$^*$, Na, Cs, and Rb and a cavity wall made of sapphire coated with a vanadium dioxide film which undergoes the dielectric-to-metal phase transition with increasing wall temperature. Numerical computations of the Casimir-Polder force and its gradient as the functions of atom-wall separation and wall temperature are made when the latter exceeds the temperature of the environment. The obtained results are compared with those in experiment on measuring the gradient of the Casimir-Polder force between $^{87}$R…
We predict a repulsive Casimir-Polder-type dispersion interaction between a single neutron and a metal or dielectric surface. We consider a scenario where a single neutron is subject to an external magnetic field. Due to its intrinsic magnetic moment, the neutron then forms a magnetisable two-level system which can exchange virtual photons with a nearby surface. The resulting dispersion interaction between a purely magnetic object (neutron) and a purely electric one (surface) is found to be repulsive, in contrast to the typical attractive interaction between electric objects. Its magnitude is …
We show that the claims expressed in the Comment arXiv:0810.3244v1 by R.S. Decca et al against our paper, D.A.R. Dalvit and S.K. Lamoreaux, Phys. Rev. Lett. {\bf 101}, 163203 (2008), are wrong and manifestly inconsistent with basic principles of statistical physics.
We have considered the interaction of a pair of spatially separated two-level atoms with the electromagnetic field in its vacuum state and we have analyzed the amount of entanglement induced between the two atoms by the non local field fluctuations. This has allowed us to characterize the quantum nature of the non local correlations of the electromagnetic field vacuum state as well as to link the induced quantum entanglement with Casimir-Polder potentials.
We study the influence of thermal Casimir-Polder forces on the near-surface trapping of cold polar molecules, with emphasis on LiH and YbF near an Au surface at room temperature. We show that for a molecule initially prepared in its electronic and rovibrational ground state, the Casimir-Polder force oscillates with the molecule-wall separation. The non-resonant force contribution and the evanescent part of the resonant force contribution almost exactly cancel at high temperature which results in a saturation of the (attractive) force in this limit. A dynamical calculation reveals how the spati…
We evaluate the Casimir-Polder potential between two atoms in the presence of an infinite perfectly conducting plate and at nonzero temperature. In order to calculate the potential, we use a method based on equal-time spatial correlations of the electric field, already used to evaluate the effect of boundary conditions on interatomic potentials. This method gives also a transparent physical picture of the role of a finite temperature and boundary conditions on the Casimir-Polder potential. We obtain an analytical expression of the potential both in the near and far zones, and consider several …
We investigate the possibility to trap ultracold atoms near the outside of a metallic carbon nanotube (CN) which we imagine to use as a miniaturized current-carrying wire. We calculate atomic spin flip lifetimes and compare the strength of the Casimir-Polder potential with the magnetic trapping potential. Our analysis indicates that the Casimir-Polder force is the dominant loss mechanism and we compute the minimum distance to the carbon nanotube at which an atom can be trapped.
In this paper we review different aspects of the dynamical Casimir- Polder potential between a neutral atom and a perfectly conducting plate under nonequilibrium conditions. In order to calculate the time evolution of the atom-wall Casimir-Polder potential, we solve the Heisenberg equations describing the dynamics of the coupled system using an iterative technique. Different nonequilibrium initial states are considered, such as bare and partially dressed states. The partially dressed states considered are obtained by a sudden change of a physical parameter of the atom or of its position relati…
The time-dependent Casimir-Polder force arising during the time evolution of an initially bare two-level atom, interacting with the radiation field and placed near a perfectly conducting wall, is considered. Initially the electromagnetic field is supposed to be in the vacuum state and the atom in its ground state. The analytical expression of the force as a function of time and atom-wall distance, is evaluated from the the time-dependent atom-field interaction energy. Physical features and limits of validity of the results are discussed in detail.
Recently D. A. R. Dalvit and S. K. Lamoreaux arXiv:0805.1676 [Phys. Rev. Lett. v.101, 163203 (2008)] suggested the modification of the reflection coefficients in the Lifshitz theory taking into account the screening effects and diffusion currents. We demonstrate that the suggested modification is thermodynamically and experimentally inconsistent.
The thermal correction to the energy of Casimir-Polder interaction of atoms with a suspended graphene membrane described by the Dirac model is investigated. We show that a major impact on the thermal correction is made by the size of the gap in the energy spectrum of graphene quasiparticles. Specifically, if the temperature is much smaller than the gap parameter (alternatively, larger or of the order of the gap parameter), the thermal correction is shown to be relatively small (alternatively, large). We have calculated the free energy of the thermal Casimir-Polder interaction of atoms of He, N…
An atom irradiated by an off-resonant laser field near a surface is expected to experience the sum of two fundamental potentials, the optical potential of the laser field and the Casimir--Polder potential of the surface. Here, we report a new non-additive potential, namely the laser-induced Casimir--Polder potential, which arises from a correlated coupling of the atom with both the laser and the quantum vacuum. We apply this result to an experimentally realizable scenario of an atomic mirror with an evanescent laser beam leaking out of a surface. We show that the non-additive term is significa…
