Multilayers of Co90Fe10/Pd with different bilayer thicknesses, have been deposited by dc-magnetron sputtering on thermally oxidized Si wafers. Transmission electron microscopy showed that the highly textured crystalline films had columnar structure, while scanning transmission electron microscopy and atomic force microscopy respectively indicated some layer waviness and surface roughness. The magnetic domain structure and perpendicular magnetic anisotropy (PMA) of the Co90Fe10/Pd multilayers were investigated by off-axis electron holography and magnetic force microscopy. The Co90Fe10 layer thickness was the primary factor determining the magnetic domain size and the perpendicular magnetization: both decreased as the thickness increased. The strongest PMA was observed in the sample with the thinnest magnetic layer of 0.45 nm.
We studied the dynamics of magnetization through an investigation of the magnetoimpedance effect in CoFeB/(Ta, Ag, Cu) multilayered thin films grown by magnetron sputtering. Impedance measurements were analyzed in terms of the mechanisms responsible for their variations at different frequency intervals and the magnetic and structural properties of the multilayers. Analysis of the mechanisms responsible for magnetoimpedance according to frequency and external magnetic field showed that for the CoFeB/Cu multilayer, ferromagnetic resonance (FMR) contributes significantly to the magnetoimpedance e…
The authors studied an effect of ferromagnetic (Co20Fe60B20 or Fe) layer insertion on tunnel magnetoresistance (TMR) properties of MgO-barrier magnetic tunnel junctions (MTJs) with CoFe/Pd multilayer electrodes. TMR ratio in MTJs with CoFeB/MgO/Fe stack reached 67% at an-nealing temperature (Ta) of 200 degree C and then decreased rapidly at Ta over 250 degree C. The degradation of the TMR ratio may be related to crystallization of CoFe(B) into fcc(111) or bcc(011) texture result-ing from diffusion of B into Pd layers. MTJs which were in-situ annealed at 350oC just after depo-siting bottom CoFe…
Magnetic and magnetostrictive hysteresis loops of TbCo/CoFe multilayers under field applied along the hard magnetization axis are studied using vectorial magnetization measurements, optical deflectometry and magneto optical Kerr microscopy. Even a very small angle misalignment between hard axis and magnetic field direction is shown to drastically change the shape of magnetization and magnetostrictive torsion hysteresis loops. Two kinds of magnetic domains are revealed during the magnetization: big regions with opposite rotation of spontaneous magnetization vector and spontaneous magnetic domai…
We study thin films and magnetic tunnel junction nanopillars based on Ta/Co$_{20}$Fe$_{60}$B$_{20}$/MgO multilayers by electrical transport and magnetometry measurements. These measurements suggest that an ultrathin magnetic oxide layer forms at the Co$_{20}$Fe$_{60}$B$_{20}$/MgO interface. At approximately 160 K, the oxide undergoes a phase transition from an insulating antiferromagnet at low temperatures to a conductive weak ferromagnet at high temperatures. This interfacial magnetic oxide is expected to have significant impact on the magnetic properties of CoFeB-based multilayers used in sp…
We report on a strong perpendicular magnetic anisotropy in [CoFe 0.4nm/Pd t]6 (t = 1.0-2.0 nm) multilayers fabricated by DC sputtering in a ultrahigh vacuum chamber. Saturation magnetization, $M_s$, and uniaxial anisotropy, $K_u$, of the multilayers decrease with increasing the spacing thickness, with a $M_s$ of 155 emu/cc and a $K_u$ of 1.14$\times 10^5$ J/m$^3$ at a spacing thickness of t = 2 nm. X-ray absorption spectroscopy and X-ray magnetic circular dichroism measurements reveal that spin and orbital magnetic moments of Co and Fe in CoFe film decrease as function of Pd thickness, indicat…
Perpendicular magnetic anisotropy (PMA) and dynamic magnetization reversal process in [CoFeB $t$ nm/Pd 1.0 nm]$_n$ ($t$ = 0.4, 0.6, 0.8, 1.0, and 1.2 nm; $n$ = 2 - 20) multilayer films have been studied by means of magnetic hysteresis and Kerr effect measurements. Strong and controllable PMA with an effective uniaxial anisotropy up to 7.7$\times$ 10$^6$ J.m$^{-3}$ and a saturation magnetization as low as 200 emu/cc are achieved. Surface/interfacial anisotropy of CoFeB/Pd interfaces, the main contribution to the PMA, is separated from the effective uniaxial anisotropy of the films, and appears …
We present results of the analysis of Brillouin Light Scattering (BLS) measurements of spin waves performed on ultrathin single and multirepeat CoFeB layers with adjacent heavy metal layers. From a detailed study of the spin-wave dispersion relation, we independently extract the Heisenberg exchange interaction (also referred to as symmetric exchange interaction), the Dzyaloshinskii-Moriya interaction (DMI, also referred to as antisymmetric exchange interaction), and the anisotropy field. We find a large DMI in CoFeB thin films adjacent to a Pt layer and nearly vanishing DMI for CoFeB films adj…
Current induced domain wall (DW) motion has been investigated in a 600-nm wide nanowire using multilayer film with a structure of Ta(5 nm)/Pd(5 nm)/[CoFe(0.4 nm)/Pd(1.2 nm)]$_{15}$/Ta(5 nm)in terms of anomalous Hall effect measurements. It is found that motion of DWs can be driven by a current density as low as 1.44$\times$10$^{11}$ A.m$^{-2}$. The effect of the Oersted field ($H_{Oe}$) and spin transfer torque field ($H_{ST}$), which are considered as effective fields for DW motion, has been quantitatively separated from the dependence of depinning fields on the current. The results show that…
Observation by SANS and PNR of pure Néel-type domain wall profiles and skyrmion suppression below room temperature in magnetic [Pt/CoFeB/Ru]$_{10}$ multilayers
Spin current generated by spin Hall effect in the heavy metal would diffuse up and down to adjacent ferromagnetic layers and exert torque on their magnetization, called spin-orbit torque. Antiferromagnetically coupled trilayers, namely the so-called synthetic antiferromagnets (SAF), are usually employed to serve as the pinned layer of spintronic devices based on spin valves and magnetic tunnel junctions to reduce the stray field and/or increase the pinning field. Here we investigate the spin-orbit torque in MgO/CoFeB/Ta/CoFeB/MgO perpendicularly magnetized multilayer with interlayer antiferrom…
We report that strong perpendicular magnetic anisotropy of the ferromagnetic layer in a W/CoFeB/MgO multilayer structure can be established by inserting a Hf layer as thin as 0.25 nm between the W and CoFeB layers. The Hf spacer also allows transmission of spin currents generated by an in-plane charge current in the W layer to apply strong spin torque on the CoFeB, thereby enabling current-driven magnetic switching. The antidamping-like and field-like components of the spin torque exerted on a 1 nm CoFeB layer are of comparable magnitudes in this geometry. Both components originate from the sp…
Studies of magnetization dynamics have incessantly facilitated the discovery of fundamentally novel physical phenomena, making steady headway in the development of magnetic and spintronics devices. The dynamics can be induced and detected electrically, offering new functionalities in advanced electronics at the nanoscale. However, its scattering mechanism is still disputed. Understanding the mechanism in thin films is especially important, because most spintronics devices are made from stacks of multilayers with nanometer thickness. The stacks are known to possess interfacial magnetic anisotro…
We report on the magnetization depth profile of a hybrid exchange spring system in which a Co/Pd multilayer with perpendicular anisotropy is coupled to a CoFeB thin film with in-plane anisotropy. The competition between these two orthogonal anisotropies promotes a strong depth dependence of the magnetization orientation. The angle of the magnetization vector is sensitive both to the strength of the individual anisotropies and to the local exchange constant, and is thus tunable by changing the thickness of the CoFeB layer and by substituting Ni for Pd in one layer of the Co/Pd stack. The result…
A chiral bobber is a localized three-dimensional magnetization configuration, terminated by a singularity. Chiral bobbers coexist with magnetic skyrmions in chiral magnets, lending themselves to new types of skyrmion-complementary bits of information. However, the on-demand creation of bobbers, as well as their direct observation remained elusive. Here, we introduce a new mechanism for creating a stable chiral bobber lattice state via the proximity of two skyrmion species with comparable size. This effect is experimentally demonstrated in a Cu$_2$OSeO$_3$/[Ta/CoFeB/MgO]$_4$ heterostructure in …
Deterministic current-induced spin-orbit torque (SOT) switching of magnetization in a heavy transition metal/ferromagnetic metal/oxide magnetic heterostructure with the ferromagnetic layer being perpendicularly-magnetized typically requires an externally-applied in-plane field to break the switching symmetry. We show that by inserting an in-plane magnetized ferromagnetic layer CoFeB underneath the conventional W/CoFeB/MgO SOT heterostructure, deterministic SOT switching of the perpendicularly-magnetized top CoFeB layer can be realized without the need of in-plane bias field. Kerr imaging study…
Discontinuous magnetic multilayers [CoFe/Al2O3] are studied by use of magnetometry, susceptometry and numeric simulations. Soft ferromagnetic Co80Fe20 nanoparticles are embedded in a diamagnetic insulating a-Al2O3 matrix and can be considered as homogeneously magnetized superspins exhibiting randomness of size (viz. moment), position and anisotropy. Lacking intra-particle core-surface ordering, generic freezing processes into collective states rather than individual particle blocking are encountered. With increasing particle density one observes first superspin glass and then superferromagneti…
Beyond conventional skyrmions in synthetic antiferromagnets
University of Glasgow（格拉斯哥大学）；Swiss Federal Laboratories for Material Science and Technology (Empa)（瑞士联邦材料科学与技术研究所）；National Physical Laboratory（英国国家物理实验室）；University of California, Santa Cruz（加州大学圣克鲁兹分校）；Politecnico di Bari（巴里理工大学）；University of Leeds（利兹大学）；Lawrence Berkeley National Laboratory（劳伦斯伯克利国家实验室）
The magnetic skyrmion is a nanoscale topological object characterized by the winding of the magnetic moments, appearing in magnetic materials with broken inversion symmetry. Because of its low current threshold for driving, the skyrmions have been intensely studied toward novel storage applications by using electron-beam, X-ray, and visible light microscopies. Here, we show that the skyrmions can be imaged via thermoelectric signals of spin-caloritronic phenomena in combination with focused heating. We applied a local temperature gradient to a CoFeB/Ta/W multilayer film with scanning a heating…
3D tomographic imaging of skyrmionic cocoons using HERALDO
Laboratoire Albert Fert, CNRS, Thales, Université Paris-Saclay（阿尔贝·费尔实验室，法国国家科学研究中心，泰雷兹集团，巴黎萨克雷大学）；Spin-ion Technologies（Spin-ion 科技公司）；Helmholtz-Zentrum Berlin（亥姆霍兹柏林中心）；University of Augsburg（奥格斯堡大学）；Max Planck Institute for Chemical Physics of Solids（马克斯·普朗克固体化学物理研究所）；International Institute for Sustainability with Knotted Chiral Meta Matter (WPI-SKCM2), Hiroshima University（广岛大学打结手性超物质可持续发展国际研究所（WPI-SKCM2））
