arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 1409.0433cond-mat.str-elcond-mat.supr-con
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Ho $_2$ RhIn $_8$的富磁phase diagram的磁结构

Magnetic structures in the rich magnetic phase diagram of Ho$_2$RhIn$_8$

Petr Čermák, Karel Prokeš, Bachir Ouladdiaf, Martin Boehm, Marie Kratochvílová, Pavel Javorský

摘要:

四配位的Ho $_2$ RhIn $_8$化合物的磁相图具有与许多相关系统相似的特征,揭示了零磁场AF 1和场诱导AF 2相。对于任何相关化合物,尚未报道AF 2相中的磁序的详细信息。此外,只有Ho $_2$ RhIn $_8$相图包含一个小区域的无公度零场AF 3相。我们用几种衍射仪对Ho $_2$ RhIn $_8$单晶进行了大量的中子衍射实验,包括在水平和垂直磁场下的实验,最高可达4 T。我们提出的详细信息中的所有磁相的丰富的相图Ho $_2$ RhIn $_8$的磁结构。在每个相位中,Ho磁矩沿四元$c$轴指向。基态AF 1相位的特征在于传播矢量$\textbf{k}$ =(1/2,0,0)。更复杂的亚铁磁AF 2相由四个传播矢量$\textbf{k}_{0}$ =(0,0,0),$\textbf{k}_{1}$ =(1/2,0,0),$\textbf{k}_{2}$ =(0,1/2,1/2),$\textbf{k}_{3}$ =(1/2,1/2,1/2)描述。AF 3相中的磁结构与$\textbf{k}_{AF3}$ =(0.5,$δ$,0)不相称。我们的结果与基于晶体场理论的理论计算结果一致。

英文摘要:

The magnetic phase diagram of the tetragonal Ho$_2$RhIn$_8$ compound has similar features to many related systems, revealing a zero magnetic field AF1 and a field-induced AF2 phases. Details of the magnetic order in the AF2 phase were not reported yet for any of the related compounds. In addition, only the Ho$_2$RhIn$_8$ phase diagram contains a small region of the incommensurate zero-field AF3 phase. We have performed a number of neutron diffraction experiments on single crystals of Ho$_2$RhIn$_8$ using several diffractometers including experiments in both horizontal and vertical magnetic fields up to 4 T. We present details of the magnetic structures in all magnetic phases of the rich phase diagram of Ho$_2$RhIn$_8$. The Ho magnetic moments point along the tetragonal $c$ axis in every phase. The ground-state AF1 phase is characterized by propagation vector $\textbf{k}$ = (1/2, 0, 0). The more complex ferrimagnetic AF2 phase is described by four propagation vectors $\textbf{k}_{0}$ = (0, 0, 0), $\textbf{k}_{1}$ = (1/2, 0, 0), $\textbf{k}_{2}$ = (0, 1/2, 1/2), $\textbf{k}_{3}$ = (1/2, 1/2, 1/2). The magnetic structure in the AF3 phase is incommensurate with $\textbf{k}_{AF3}$ = (0.5, $δ$, 0). Our results are consistent with theoretical calculations based on crystal field theory.

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